[{"project":[{"name":"PhoQC: PhoQC: Photonisches Quantencomputing","_id":"266","grant_number":"PROFILNRW-2020-067"}],"_id":"51339","user_id":"216","department":[{"_id":"15"},{"_id":"623"},{"_id":"288"}],"keyword":["Atomic and Molecular Physics","and Optics"],"language":[{"iso":"eng"}],"type":"journal_article","publication":"Optics Express","status":"public","date_updated":"2024-02-13T13:09:51Z","publisher":"Optica Publishing Group","date_created":"2024-02-13T13:03:01Z","author":[{"first_name":"Jonas","full_name":"Babai-Hemati, Jonas","last_name":"Babai-Hemati"},{"full_name":"vom Bruch, Felix","id":"71245","last_name":"vom Bruch","first_name":"Felix"},{"last_name":"Herrmann","id":"216","full_name":"Herrmann, Harald","first_name":"Harald"},{"first_name":"Christine","id":"26263","full_name":"Silberhorn, Christine","last_name":"Silberhorn"}],"title":"Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters","doi":"10.1364/oe.510319","publication_status":"published","publication_identifier":{"issn":["1094-4087"]},"year":"2024","citation":{"bibtex":"@article{Babai-Hemati_vom Bruch_Herrmann_Silberhorn_2024, title={Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters}, DOI={10.1364/oe.510319}, journal={Optics Express}, publisher={Optica Publishing Group}, author={Babai-Hemati, Jonas and vom Bruch, Felix and Herrmann, Harald and Silberhorn, Christine}, year={2024} }","mla":"Babai-Hemati, Jonas, et al. “Tailored Second Harmonic Generation InTi-Diffused PPLN Waveguides Usingmicro-Heaters.” Optics Express, Optica Publishing Group, 2024, doi:10.1364/oe.510319.","short":"J. Babai-Hemati, F. vom Bruch, H. Herrmann, C. Silberhorn, Optics Express (2024).","apa":"Babai-Hemati, J., vom Bruch, F., Herrmann, H., & Silberhorn, C. (2024). Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters. Optics Express. https://doi.org/10.1364/oe.510319","ama":"Babai-Hemati J, vom Bruch F, Herrmann H, Silberhorn C. Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters. Optics Express. Published online 2024. doi:10.1364/oe.510319","ieee":"J. Babai-Hemati, F. vom Bruch, H. Herrmann, and C. Silberhorn, “Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters,” Optics Express, 2024, doi: 10.1364/oe.510319.","chicago":"Babai-Hemati, Jonas, Felix vom Bruch, Harald Herrmann, and Christine Silberhorn. “Tailored Second Harmonic Generation InTi-Diffused PPLN Waveguides Usingmicro-Heaters.” Optics Express, 2024. https://doi.org/10.1364/oe.510319."}},{"status":"public","abstract":[{"text":"The biphoton correlation time, a measure for the conditional uncertainty in the temporal arrival of two photons from a photon pair source, is a key performance identifier for many quantum spectroscopy applications, with shorter correlation times typically yielding better performance. Furthermore, it provides fundamental insight into the effects of dispersion on the biphoton state. Here, we show that a characteristic dependence of the width of the temporal interferogram can be exploited to obtain insights into the amount of second-order dispersion inside the interferometer and to retrieve actual and Fourier-limited ultrashort biphoton correlation times of around 100 fs. In the presented scheme, we simultaneously measure spectral and temporal interferograms at the output of an SU(1,1) interferometer based on an integrated broadband parametric down conversion source in a Ti:LiNbO3 waveguide.","lang":"eng"}],"type":"journal_article","publication":"PRX Quantum","language":[{"iso":"eng"}],"article_number":"020350","user_id":"88149","department":[{"_id":"288"},{"_id":"623"}],"project":[{"name":"MiLiQuant: Miniaturisierte Lichtquellen für den industriellen Einsatz in Quantensensoren und Quanten-Imaging-Systemen (MiLiQuant) - Teilvorhaben: Technologie und Theorie für MIR Quanten-Imaging Systeme","_id":"207","grant_number":"13N15065"},{"grant_number":"101070700","_id":"571","name":"MIRAQLS: MIRAQLS: Mid-infrared Quantum Technology for Sensing"},{"name":"E2TPA: Exploiting Entangled Two-Photon Absorption","_id":"190"}],"_id":"54544","citation":{"apa":"Roeder, F., Pollmann, R., Stefszky, M., Santandrea, M., Luo, K. H., Quiring, V., Ricken, R., Eigner, C., Brecht, B., & Silberhorn, C. (2024). Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer. PRX Quantum, 5(2), Article 020350. https://doi.org/10.1103/prxquantum.5.020350","mla":"Roeder, Franz, et al. “Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer.” PRX Quantum, vol. 5, no. 2, 020350, American Physical Society (APS), 2024, doi:10.1103/prxquantum.5.020350.","short":"F. Roeder, R. Pollmann, M. Stefszky, M. Santandrea, K.H. Luo, V. Quiring, R. Ricken, C. Eigner, B. Brecht, C. Silberhorn, PRX Quantum 5 (2024).","bibtex":"@article{Roeder_Pollmann_Stefszky_Santandrea_Luo_Quiring_Ricken_Eigner_Brecht_Silberhorn_2024, title={Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer}, volume={5}, DOI={10.1103/prxquantum.5.020350}, number={2020350}, journal={PRX Quantum}, publisher={American Physical Society (APS)}, author={Roeder, Franz and Pollmann, René and Stefszky, Michael and Santandrea, Matteo and Luo, Kai Hong and Quiring, V. and Ricken, Raimund and Eigner, Christof and Brecht, Benjamin and Silberhorn, Christine}, year={2024} }","ama":"Roeder F, Pollmann R, Stefszky M, et al. Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer. PRX Quantum. 2024;5(2). doi:10.1103/prxquantum.5.020350","ieee":"F. Roeder et al., “Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer,” PRX Quantum, vol. 5, no. 2, Art. no. 020350, 2024, doi: 10.1103/prxquantum.5.020350.","chicago":"Roeder, Franz, René Pollmann, Michael Stefszky, Matteo Santandrea, Kai Hong Luo, V. Quiring, Raimund Ricken, Christof Eigner, Benjamin Brecht, and Christine Silberhorn. “Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer.” PRX Quantum 5, no. 2 (2024). https://doi.org/10.1103/prxquantum.5.020350."},"intvolume":" 5","year":"2024","issue":"2","publication_status":"published","publication_identifier":{"issn":["2691-3399"]},"doi":"10.1103/prxquantum.5.020350","title":"Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer","date_created":"2024-06-01T12:48:51Z","author":[{"first_name":"Franz","full_name":"Roeder, Franz","id":"88149","last_name":"Roeder"},{"first_name":"René","last_name":"Pollmann","full_name":"Pollmann, René","id":"78890"},{"full_name":"Stefszky, Michael","id":"42777","last_name":"Stefszky","first_name":"Michael"},{"last_name":"Santandrea","orcid":"0000-0001-5718-358X","id":"55095","full_name":"Santandrea, Matteo","first_name":"Matteo"},{"orcid":"0000-0003-1008-4976","last_name":"Luo","id":"36389","full_name":"Luo, Kai Hong","first_name":"Kai Hong"},{"first_name":"V.","last_name":"Quiring","full_name":"Quiring, V."},{"full_name":"Ricken, Raimund","last_name":"Ricken","first_name":"Raimund"},{"orcid":"https://orcid.org/0000-0002-5693-3083","last_name":"Eigner","full_name":"Eigner, Christof","id":"13244","first_name":"Christof"},{"orcid":"0000-0003-4140-0556 ","last_name":"Brecht","full_name":"Brecht, Benjamin","id":"27150","first_name":"Benjamin"},{"id":"26263","full_name":"Silberhorn, Christine","last_name":"Silberhorn","first_name":"Christine"}],"volume":5,"publisher":"American Physical Society (APS)","date_updated":"2024-06-01T13:00:53Z"},{"publication":"Physical Review Letters","type":"journal_article","status":"public","_id":"54812","department":[{"_id":"15"},{"_id":"623"},{"_id":"288"}],"user_id":"27150","article_number":"240802","language":[{"iso":"eng"}],"publication_identifier":{"issn":["0031-9007","1079-7114"]},"publication_status":"published","issue":"24","year":"2024","intvolume":" 132","citation":{"chicago":"Weinbrenner, Lisa T., Nidhin Prasannan, Kiara Hansenne, Sophia Denker, Jan Sperling, Benjamin Brecht, Christine Silberhorn, and Otfried Gühne. “Certifying the Topology of Quantum Networks: Theory and Experiment.” Physical Review Letters 132, no. 24 (2024). https://doi.org/10.1103/physrevlett.132.240802.","ieee":"L. T. Weinbrenner et al., “Certifying the Topology of Quantum Networks: Theory and Experiment,” Physical Review Letters, vol. 132, no. 24, Art. no. 240802, 2024, doi: 10.1103/physrevlett.132.240802.","ama":"Weinbrenner LT, Prasannan N, Hansenne K, et al. Certifying the Topology of Quantum Networks: Theory and Experiment. Physical Review Letters. 2024;132(24). doi:10.1103/physrevlett.132.240802","short":"L.T. Weinbrenner, N. Prasannan, K. Hansenne, S. Denker, J. Sperling, B. Brecht, C. Silberhorn, O. Gühne, Physical Review Letters 132 (2024).","bibtex":"@article{Weinbrenner_Prasannan_Hansenne_Denker_Sperling_Brecht_Silberhorn_Gühne_2024, title={Certifying the Topology of Quantum Networks: Theory and Experiment}, volume={132}, DOI={10.1103/physrevlett.132.240802}, number={24240802}, journal={Physical Review Letters}, publisher={American Physical Society (APS)}, author={Weinbrenner, Lisa T. and Prasannan, Nidhin and Hansenne, Kiara and Denker, Sophia and Sperling, Jan and Brecht, Benjamin and Silberhorn, Christine and Gühne, Otfried}, year={2024} }","mla":"Weinbrenner, Lisa T., et al. “Certifying the Topology of Quantum Networks: Theory and Experiment.” Physical Review Letters, vol. 132, no. 24, 240802, American Physical Society (APS), 2024, doi:10.1103/physrevlett.132.240802.","apa":"Weinbrenner, L. T., Prasannan, N., Hansenne, K., Denker, S., Sperling, J., Brecht, B., Silberhorn, C., & Gühne, O. (2024). Certifying the Topology of Quantum Networks: Theory and Experiment. Physical Review Letters, 132(24), Article 240802. https://doi.org/10.1103/physrevlett.132.240802"},"date_updated":"2024-06-19T06:59:45Z","publisher":"American Physical Society (APS)","volume":132,"date_created":"2024-06-19T06:36:54Z","author":[{"last_name":"Weinbrenner","full_name":"Weinbrenner, Lisa T.","first_name":"Lisa T."},{"last_name":"Prasannan","full_name":"Prasannan, Nidhin","id":"71403","first_name":"Nidhin"},{"full_name":"Hansenne, Kiara","last_name":"Hansenne","first_name":"Kiara"},{"last_name":"Denker","full_name":"Denker, Sophia","first_name":"Sophia"},{"first_name":"Jan","full_name":"Sperling, Jan","id":"75127","last_name":"Sperling","orcid":"0000-0002-5844-3205"},{"first_name":"Benjamin","id":"27150","full_name":"Brecht, Benjamin","orcid":"0000-0003-4140-0556 ","last_name":"Brecht"},{"last_name":"Silberhorn","full_name":"Silberhorn, Christine","id":"26263","first_name":"Christine"},{"full_name":"Gühne, Otfried","last_name":"Gühne","first_name":"Otfried"}],"title":"Certifying the Topology of Quantum Networks: Theory and Experiment","doi":"10.1103/physrevlett.132.240802"},{"issue":"13","year":"2024","date_created":"2024-06-10T11:18:06Z","publisher":"Optica Publishing Group","title":"Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides","publication":"Optics Express","file":[{"content_type":"application/pdf","relation":"main_file","creator":"fossie","date_created":"2024-06-10T11:25:00Z","date_updated":"2024-06-10T11:25:00Z","access_level":"open_access","file_id":"54669","file_name":"2024-06 Hammer - Optics Express - Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides.pdf","file_size":4004782}],"abstract":[{"text":"Samples of dielectric optical waveguides of rib or strip type in thin-film lithium niobate (TFLN) technology are characterized with respect to their optical loss using the Fabry-Pérot method. Attributing the losses mainly to sidewall roughness, we employ a simple perturbational procedure, based on rigorously computed mode profiles of idealized channels, to estimate the attenuation for waveguides with different cross sections. A single fit parameter suffices for an adequate modelling of the effect of the waveguide geometry on the loss levels.","lang":"eng"}],"language":[{"iso":"eng"}],"ddc":["530"],"keyword":["tet_topic_waveguide"],"publication_status":"published","publication_identifier":{"issn":["1094-4087"]},"has_accepted_license":"1","citation":{"ama":"Hammer M, Babel S, Farheen H, et al. Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides. Optics Express. 2024;32(13):22878. doi:10.1364/oe.521766","ieee":"M. Hammer et al., “Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides,” Optics Express, vol. 32, no. 13, p. 22878, 2024, doi: 10.1364/oe.521766.","chicago":"Hammer, Manfred, Silia Babel, Henna Farheen, Laura Padberg, J. Christoph Scheytt, Christine Silberhorn, and Jens Förstner. “Estimation of Losses Caused by Sidewall Roughness in Thin-Film Lithium Niobate Rib and Strip Waveguides.” Optics Express 32, no. 13 (2024): 22878. https://doi.org/10.1364/oe.521766.","apa":"Hammer, M., Babel, S., Farheen, H., Padberg, L., Scheytt, J. C., Silberhorn, C., & Förstner, J. (2024). Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides. Optics Express, 32(13), 22878. https://doi.org/10.1364/oe.521766","bibtex":"@article{Hammer_Babel_Farheen_Padberg_Scheytt_Silberhorn_Förstner_2024, title={Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides}, volume={32}, DOI={10.1364/oe.521766}, number={13}, journal={Optics Express}, publisher={Optica Publishing Group}, author={Hammer, Manfred and Babel, Silia and Farheen, Henna and Padberg, Laura and Scheytt, J. Christoph and Silberhorn, Christine and Förstner, Jens}, year={2024}, pages={22878} }","mla":"Hammer, Manfred, et al. “Estimation of Losses Caused by Sidewall Roughness in Thin-Film Lithium Niobate Rib and Strip Waveguides.” Optics Express, vol. 32, no. 13, Optica Publishing Group, 2024, p. 22878, doi:10.1364/oe.521766.","short":"M. Hammer, S. Babel, H. Farheen, L. Padberg, J.C. Scheytt, C. Silberhorn, J. Förstner, Optics Express 32 (2024) 22878."},"intvolume":" 32","page":"22878","author":[{"last_name":"Hammer","orcid":"0000-0002-6331-9348","id":"48077","full_name":"Hammer, Manfred","first_name":"Manfred"},{"first_name":"Silia","full_name":"Babel, Silia","id":"63231","last_name":"Babel","orcid":"https://orcid.org/0000-0002-1568-2580"},{"last_name":"Farheen","orcid":"0000-0001-7730-3489","full_name":"Farheen, Henna","id":"53444","first_name":"Henna"},{"first_name":"Laura","full_name":"Padberg, Laura","id":"40300","last_name":"Padberg"},{"last_name":"Scheytt","orcid":"0000-0002-5950-6618 ","full_name":"Scheytt, J. Christoph","id":"37144","first_name":"J. Christoph"},{"last_name":"Silberhorn","id":"26263","full_name":"Silberhorn, Christine","first_name":"Christine"},{"first_name":"Jens","orcid":"0000-0001-7059-9862","last_name":"Förstner","id":"158","full_name":"Förstner, Jens"}],"volume":32,"date_updated":"2024-07-22T07:43:02Z","oa":"1","doi":"10.1364/oe.521766","type":"journal_article","status":"public","user_id":"158","department":[{"_id":"61"},{"_id":"429"},{"_id":"623"},{"_id":"263"},{"_id":"288"}],"project":[{"_id":"53","name":"TRR 142: TRR 142 - Maßgeschneiderte nichtlineare Photonik: Von grundlegenden Konzepten zu funktionellen Strukturen","grant_number":"231447078"},{"_id":"175","name":"TRR 142 - C11: TRR 142 - Kompakte Photonenpaar-Quelle mit ultraschnellen Modulatoren auf Basis von CMOS und LNOI (C11*)","grant_number":"231447078"},{"grant_number":"231447078","_id":"167","name":"TRR 142 - B06: TRR 142 - Ultraschnelle kohärente opto-elektronische Kontrolle eines photonischen Quantensystems (B06*)"},{"_id":"266","name":"PhoQC: PhoQC: Photonisches Quantencomputing","grant_number":"PROFILNRW-2020-067"}],"_id":"54668","file_date_updated":"2024-06-10T11:25:00Z"},{"article_number":"112","article_type":"original","_id":"49652","user_id":"22501","department":[{"_id":"15"},{"_id":"288"},{"_id":"623"}],"status":"public","type":"journal_article","main_file_link":[{"url":"https://arxiv.org/pdf/2306.09701.pdf","open_access":"1"}],"doi":"10.1364/ao.505374","oa":"1","date_updated":"2025-04-03T12:36:01Z","author":[{"full_name":"Hempel, Franz","last_name":"Hempel","first_name":"Franz"},{"first_name":"Federico","full_name":"Vernuccio, Federico","last_name":"Vernuccio"},{"last_name":"König","full_name":"König, Lukas","first_name":"Lukas"},{"full_name":"Buschbeck, Robin","last_name":"Buschbeck","first_name":"Robin"},{"full_name":"Rüsing, Michael","id":"22501","orcid":"0000-0003-4682-4577","last_name":"Rüsing","first_name":"Michael"},{"first_name":"Giulio","full_name":"Cerullo, Giulio","last_name":"Cerullo"},{"first_name":"Dario","full_name":"Polli, Dario","last_name":"Polli"},{"first_name":"Lukas M.","last_name":"Eng","full_name":"Eng, Lukas M."}],"volume":63,"citation":{"bibtex":"@article{Hempel_Vernuccio_König_Buschbeck_Rüsing_Cerullo_Polli_Eng_2024, title={Comparing transmission- and epi-BCARS: a round robin on solid-state materials}, volume={63}, DOI={10.1364/ao.505374}, number={1112}, journal={Applied Optics}, publisher={Optica Publishing Group}, author={Hempel, Franz and Vernuccio, Federico and König, Lukas and Buschbeck, Robin and Rüsing, Michael and Cerullo, Giulio and Polli, Dario and Eng, Lukas M.}, year={2024} }","short":"F. Hempel, F. Vernuccio, L. König, R. Buschbeck, M. Rüsing, G. Cerullo, D. Polli, L.M. Eng, Applied Optics 63 (2024).","mla":"Hempel, Franz, et al. “Comparing Transmission- and Epi-BCARS: A Round Robin on Solid-State Materials.” Applied Optics, vol. 63, no. 1, 112, Optica Publishing Group, 2024, doi:10.1364/ao.505374.","apa":"Hempel, F., Vernuccio, F., König, L., Buschbeck, R., Rüsing, M., Cerullo, G., Polli, D., & Eng, L. M. (2024). Comparing transmission- and epi-BCARS: a round robin on solid-state materials. Applied Optics, 63(1), Article 112. https://doi.org/10.1364/ao.505374","ama":"Hempel F, Vernuccio F, König L, et al. Comparing transmission- and epi-BCARS: a round robin on solid-state materials. Applied Optics. 2024;63(1). doi:10.1364/ao.505374","ieee":"F. Hempel et al., “Comparing transmission- and epi-BCARS: a round robin on solid-state materials,” Applied Optics, vol. 63, no. 1, Art. no. 112, 2024, doi: 10.1364/ao.505374.","chicago":"Hempel, Franz, Federico Vernuccio, Lukas König, Robin Buschbeck, Michael Rüsing, Giulio Cerullo, Dario Polli, and Lukas M. Eng. “Comparing Transmission- and Epi-BCARS: A Round Robin on Solid-State Materials.” Applied Optics 63, no. 1 (2024). https://doi.org/10.1364/ao.505374."},"intvolume":" 63","publication_status":"published","publication_identifier":{"issn":["1559-128X","2155-3165"]},"related_material":{"link":[{"url":"https://arxiv.org/abs/2306.09701","relation":"confirmation"}]},"keyword":["Atomic and Molecular Physics","and Optics","Engineering (miscellaneous)","Electrical and Electronic Engineering"],"language":[{"iso":"eng"}],"abstract":[{"text":"Broadband coherent anti-Stokes Raman scattering (BCARS) is a powerful spectroscopy method combining high signal intensity with spectral sensitivity, enabling rapid imaging of heterogeneous samples in biomedical research and, more recently, in crystalline materials. However, BCARS encounters spectral distortion due to a setup-dependent non-resonant background (NRB). This study assesses BCARS reproducibility through a round robin experiment using two distinct BCARS setups and crystalline materials with varying structural complexity, including diamond, 6H-SiC, KDP, and KTP. The analysis compares setup-specific NRB correction procedures, detected and NRB-removed spectra, and mode assignment. We determine the influence of BCARS setup parameters like pump wavelength, pulse width, and detection geometry and provide a practical guide for optimizing BCARS setups for solid-state applications.","lang":"eng"}],"publication":"Applied Optics","title":"Comparing transmission- and epi-BCARS: a round robin on solid-state materials","publisher":"Optica Publishing Group","date_created":"2023-12-15T07:32:38Z","year":"2024","quality_controlled":"1","issue":"1"},{"type":"journal_article","publication":"Applied Physics Letters","status":"public","abstract":[{"lang":"eng","text":"Lithium niobate and lithium tantalate are among the most widespread materials for nonlinear, integrated photonics. Mixed crystals with arbitrary Nb–Ta ratios provide an additional degree of freedom to not only tune materials properties, such as the birefringence but also leverage the advantages of the singular compounds, for example, by combining the thermal stability of lithium tantalate with the larger nonlinear or piezoelectric constants of lithium niobate. Periodic poling allows to achieve phase-matching independent of waveguide geometry and is, therefore, one of the commonly used methods in integrated nonlinear optics. For mixed crystals, periodic poling has been challenging so far due to the lack of homogeneous, mono-domain crystals, which severely inhibit domain growth and nucleation. In this work, we investigate surface-near (<1μm depth) domain inversion on x-cut lithium niobate tantalate mixed crystals via electric field poling and lithographically structured electrodes. We find that naturally occurring head-to-head or tail-to-tail domain walls in the as-grown crystal inhibit domain inversion at a larger scale. However, periodic poling is possible if the gap size between the poling electrodes is of the same order of magnitude or smaller than the average size of naturally occurring domains. This work provides the basis for the nonlinear optical application of lithium niobate tantalate mixed crystals."}],"user_id":"61375","department":[{"_id":"15"},{"_id":"623"},{"_id":"230"},{"_id":"288"}],"project":[{"grant_number":"231447078","name":"TRR 142 - B07: TRR 142 - Polaronen-Einfluss auf die optischen Eigenschaften von Lithiumniobat (B07*)","_id":"168"}],"_id":"57028","language":[{"iso":"eng"}],"issue":"15","publication_status":"published","publication_identifier":{"issn":["0003-6951","1077-3118"]},"citation":{"ama":"Bollmers L, Babai-Hemati T, Koppitz B, et al. Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals. Applied Physics Letters. 2024;125(15). doi:10.1063/5.0210972","chicago":"Bollmers, Laura, Tobias Babai-Hemati, Boris Koppitz, Christof Eigner, Laura Padberg, Michael Rüsing, Lukas M. Eng, and Christine Silberhorn. “Surface-near Domain Engineering in Multi-Domain x-Cut Lithium Niobate Tantalate Mixed Crystals.” Applied Physics Letters 125, no. 15 (2024). https://doi.org/10.1063/5.0210972.","ieee":"L. Bollmers et al., “Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals,” Applied Physics Letters, vol. 125, no. 15, 2024, doi: 10.1063/5.0210972.","mla":"Bollmers, Laura, et al. “Surface-near Domain Engineering in Multi-Domain x-Cut Lithium Niobate Tantalate Mixed Crystals.” Applied Physics Letters, vol. 125, no. 15, AIP Publishing, 2024, doi:10.1063/5.0210972.","bibtex":"@article{Bollmers_Babai-Hemati_Koppitz_Eigner_Padberg_Rüsing_Eng_Silberhorn_2024, title={Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals}, volume={125}, DOI={10.1063/5.0210972}, number={15}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Bollmers, Laura and Babai-Hemati, Tobias and Koppitz, Boris and Eigner, Christof and Padberg, Laura and Rüsing, Michael and Eng, Lukas M. and Silberhorn, Christine}, year={2024} }","short":"L. Bollmers, T. Babai-Hemati, B. Koppitz, C. Eigner, L. Padberg, M. Rüsing, L.M. Eng, C. Silberhorn, Applied Physics Letters 125 (2024).","apa":"Bollmers, L., Babai-Hemati, T., Koppitz, B., Eigner, C., Padberg, L., Rüsing, M., Eng, L. M., & Silberhorn, C. (2024). Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals. Applied Physics Letters, 125(15). https://doi.org/10.1063/5.0210972"},"intvolume":" 125","year":"2024","date_created":"2024-11-13T08:06:59Z","author":[{"last_name":"Bollmers","id":"61375","full_name":"Bollmers, Laura","first_name":"Laura"},{"first_name":"Tobias","full_name":"Babai-Hemati, Tobias","last_name":"Babai-Hemati"},{"first_name":"Boris","full_name":"Koppitz, Boris","last_name":"Koppitz"},{"first_name":"Christof","full_name":"Eigner, Christof","id":"13244","orcid":"https://orcid.org/0000-0002-5693-3083","last_name":"Eigner"},{"first_name":"Laura","last_name":"Padberg","id":"40300","full_name":"Padberg, Laura"},{"first_name":"Michael","full_name":"Rüsing, Michael","id":"22501","last_name":"Rüsing","orcid":"0000-0003-4682-4577"},{"first_name":"Lukas M.","full_name":"Eng, Lukas M.","last_name":"Eng"},{"first_name":"Christine","full_name":"Silberhorn, Christine","id":"26263","last_name":"Silberhorn"}],"volume":125,"publisher":"AIP Publishing","date_updated":"2024-11-15T09:15:08Z","doi":"10.1063/5.0210972","title":"Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals"},{"year":"2024","quality_controlled":"1","issue":"15","title":"Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy","publisher":"AIP Publishing","date_created":"2025-04-02T15:57:11Z","abstract":[{"lang":"eng","text":"Ferroelectric materials play a crucial role in a broad range of technologies due to their unique properties that are deeply connected to the pattern and behavior of their ferroelectric (FE) domains. Chief among them, barium titanate (BaTiO3; BTO) sees widespread applications such as in electronics but equally is a ferroelectric model system for fundamental research, e.g., to study the interplay of such FE domains, the domain walls (DWs), and their macroscopic properties, owed to BTO’s multiple and experimentally accessible phase transitions. Here, we employ Second Harmonic Generation Microscopy (SHGM) to in situ investigate the cubic-to-tetragonal (at ∼126°C) and the tetragonal-to-orthorhombic (at ∼5°C) phase transition in single-crystalline BTO via three-dimensional (3D) DW mapping. We demonstrate that SHGM imaging provides the direct visualization of FE domain switching as well as the domain dynamics in 3D, shedding light on the interplay of the domain structure and phase transition. These results allow us to extract the different transition temperatures locally, to unveil the hysteresis behavior, and to determine the type of phase transition at play (first/second order) from the recorded SHGM data. The capabilities of SHGM in uncovering these crucial phenomena can easily be applied to other ferroelectrics to provide new possibilities for in situ engineering of advanced ferroic devices."}],"publication":"Journal of Applied Physics","language":[{"iso":"eng"}],"intvolume":" 136","citation":{"ama":"Kirbus B, Seddon SD, Kiseleva I, Beyreuther E, Rüsing M, Eng LM. Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy. Journal of Applied Physics. 2024;136(15). doi:10.1063/5.0237769","ieee":"B. Kirbus, S. D. Seddon, I. Kiseleva, E. Beyreuther, M. Rüsing, and L. M. Eng, “Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy,” Journal of Applied Physics, vol. 136, no. 15, Art. no. 154102, 2024, doi: 10.1063/5.0237769.","chicago":"Kirbus, Benjamin, Samuel D. Seddon, Iuliia Kiseleva, Elke Beyreuther, Michael Rüsing, and Lukas M. Eng. “Probing Ferroelectric Phase Transitions in Barium Titanate Single Crystals via In-Situ Second Harmonic Generation Microscopy.” Journal of Applied Physics 136, no. 15 (2024). https://doi.org/10.1063/5.0237769.","bibtex":"@article{Kirbus_Seddon_Kiseleva_Beyreuther_Rüsing_Eng_2024, title={Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy}, volume={136}, DOI={10.1063/5.0237769}, number={15154102}, journal={Journal of Applied Physics}, publisher={AIP Publishing}, author={Kirbus, Benjamin and Seddon, Samuel D. and Kiseleva, Iuliia and Beyreuther, Elke and Rüsing, Michael and Eng, Lukas M.}, year={2024} }","short":"B. Kirbus, S.D. Seddon, I. Kiseleva, E. Beyreuther, M. Rüsing, L.M. Eng, Journal of Applied Physics 136 (2024).","mla":"Kirbus, Benjamin, et al. “Probing Ferroelectric Phase Transitions in Barium Titanate Single Crystals via In-Situ Second Harmonic Generation Microscopy.” Journal of Applied Physics, vol. 136, no. 15, 154102, AIP Publishing, 2024, doi:10.1063/5.0237769.","apa":"Kirbus, B., Seddon, S. D., Kiseleva, I., Beyreuther, E., Rüsing, M., & Eng, L. M. (2024). Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy. Journal of Applied Physics, 136(15), Article 154102. https://doi.org/10.1063/5.0237769"},"publication_identifier":{"issn":["0021-8979","1089-7550"]},"publication_status":"published","doi":"10.1063/5.0237769","main_file_link":[{"open_access":"1","url":" https://doi.org/10.1063/5.0237769"}],"date_updated":"2025-04-02T15:59:55Z","oa":"1","volume":136,"author":[{"first_name":"Benjamin","full_name":"Kirbus, Benjamin","last_name":"Kirbus"},{"last_name":"Seddon","full_name":"Seddon, Samuel D.","first_name":"Samuel D."},{"full_name":"Kiseleva, Iuliia","last_name":"Kiseleva","first_name":"Iuliia"},{"full_name":"Beyreuther, Elke","last_name":"Beyreuther","first_name":"Elke"},{"orcid":"0000-0003-4682-4577","last_name":"Rüsing","full_name":"Rüsing, Michael","id":"22501","first_name":"Michael"},{"first_name":"Lukas M.","last_name":"Eng","full_name":"Eng, Lukas M."}],"status":"public","type":"journal_article","article_type":"original","article_number":"154102","_id":"59269","department":[{"_id":"15"},{"_id":"623"},{"_id":"288"}],"user_id":"22501"},{"department":[{"_id":"15"},{"_id":"623"},{"_id":"288"}],"user_id":"22501","_id":"59271","type":"journal_article","status":"public","volume":222,"author":[{"first_name":"Felix","last_name":"Bernhardt","full_name":"Bernhardt, Felix"},{"first_name":"Soham","full_name":"Gharat, Soham","last_name":"Gharat"},{"last_name":"Kapp","full_name":"Kapp, Alexander","first_name":"Alexander"},{"first_name":"Florian","full_name":"Pfeiffer, Florian","last_name":"Pfeiffer"},{"full_name":"Buschbeck, Robin","last_name":"Buschbeck","first_name":"Robin"},{"last_name":"Hempel","full_name":"Hempel, Franz","first_name":"Franz"},{"full_name":"Pashkin, Oleksiy","last_name":"Pashkin","first_name":"Oleksiy"},{"first_name":"Susanne C.","full_name":"Kehr, Susanne C.","last_name":"Kehr"},{"first_name":"Michael","orcid":"0000-0003-4682-4577","last_name":"Rüsing","full_name":"Rüsing, Michael","id":"22501"},{"first_name":"Simone","last_name":"Sanna","full_name":"Sanna, Simone"},{"full_name":"Eng, Lukas M.","last_name":"Eng","first_name":"Lukas M."}],"oa":"1","date_updated":"2025-04-02T16:07:19Z","doi":"10.1002/pssa.202300968","main_file_link":[{"url":"https://doi.org/10.1002/pssa.202300968","open_access":"1"}],"publication_identifier":{"issn":["1862-6300","1862-6319"]},"publication_status":"published","page":"2300968","intvolume":" 222","citation":{"ieee":"F. Bernhardt et al., “Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment,” physica status solidi (a), vol. 222, no. 1, p. 2300968, 2024, doi: 10.1002/pssa.202300968.","chicago":"Bernhardt, Felix, Soham Gharat, Alexander Kapp, Florian Pfeiffer, Robin Buschbeck, Franz Hempel, Oleksiy Pashkin, et al. “Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment.” Physica Status Solidi (a) 222, no. 1 (2024): 2300968. https://doi.org/10.1002/pssa.202300968.","ama":"Bernhardt F, Gharat S, Kapp A, et al. Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment. physica status solidi (a). 2024;222(1):2300968. doi:10.1002/pssa.202300968","apa":"Bernhardt, F., Gharat, S., Kapp, A., Pfeiffer, F., Buschbeck, R., Hempel, F., Pashkin, O., Kehr, S. C., Rüsing, M., Sanna, S., & Eng, L. M. (2024). Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment. Physica Status Solidi (a), 222(1), 2300968. https://doi.org/10.1002/pssa.202300968","mla":"Bernhardt, Felix, et al. “Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment.” Physica Status Solidi (a), vol. 222, no. 1, Wiley, 2024, p. 2300968, doi:10.1002/pssa.202300968.","bibtex":"@article{Bernhardt_Gharat_Kapp_Pfeiffer_Buschbeck_Hempel_Pashkin_Kehr_Rüsing_Sanna_et al._2024, title={Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment}, volume={222}, DOI={10.1002/pssa.202300968}, number={1}, journal={physica status solidi (a)}, publisher={Wiley}, author={Bernhardt, Felix and Gharat, Soham and Kapp, Alexander and Pfeiffer, Florian and Buschbeck, Robin and Hempel, Franz and Pashkin, Oleksiy and Kehr, Susanne C. and Rüsing, Michael and Sanna, Simone and et al.}, year={2024}, pages={2300968} }","short":"F. Bernhardt, S. Gharat, A. Kapp, F. Pfeiffer, R. Buschbeck, F. Hempel, O. Pashkin, S.C. Kehr, M. Rüsing, S. Sanna, L.M. Eng, Physica Status Solidi (a) 222 (2024) 2300968."},"language":[{"iso":"eng"}],"publication":"physica status solidi (a)","abstract":[{"text":"Lithium niobate (LNO) and lithium tantalate (LTO) see widespread use in fundamental research and commercial technologies reaching from electronics over classical optics to integrated quantum communication. The mixed crystal system lithium niobate tantalate (LNT) allows for the dedicate engineering of material properties by combining the advantages of the two parental materials LNO and LTO. Vibrational spectroscopies such as Raman spectroscopy or (Fourier transform) infrared (IR) spectroscopy are vital techniques to provide detailed insight into the material properties, which is central to the analysis and optimization of devices. This work presents a joint experimental–theoretical approach allowing to unambiguously assign the spectral features in the LNT material family through both Raman and IR spectroscopy, as well as providing an in‐depth explanation for the observed scattering efficiencies based on first‐principles calculations. The phononic contribution to the static dielectric tensor is calculated from the experimental and theoretical data using the generalized Lyddane–Sachs–Teller relation and compared with the results of the first‐principles calculations.","lang":"eng"}],"date_created":"2025-04-02T16:04:58Z","publisher":"Wiley","title":"Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment","issue":"1","year":"2024"},{"language":[{"iso":"eng"}],"abstract":[{"text":"Lithium niobate tantalate (LiNb1−xTaxO3, LNT) solid solutions offer exciting new possibilities for applications ranging from optics, piezotronics, and electronics beyond the capabilities of the widely used singular compounds of lithium niobate (LiNbO3, LN) or lithium tantalate (LiTaO3, LT). Crystal growth of homogeneous LNT single crystals by the Czochralski method is still challenging. One key aspect of homogeneous growth is the accurate knowledge of thermal conductivity through the crystal boule during the growth, which is central to control the crystal growth. Therefore, the temperature dependent thermal conductivity of pure LN, LT, and LNT solid solutions, as well as of selected doped LN and LT crystals (Mg, Zn) was investigated across the temperature range from 300 to 1300 K. The results that span across the whole composition range can directly be applied for optimizing growth conditions of both LNT solid solutions as well as doped and undoped LN and LT crystals.","lang":"eng"}],"publication":"Journal of Alloys and Compounds","title":"Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K","date_created":"2025-04-02T16:00:56Z","publisher":"Elsevier BV","year":"2024","quality_controlled":"1","article_type":"original","article_number":"176549","department":[{"_id":"15"},{"_id":"288"},{"_id":"623"}],"user_id":"22501","_id":"59270","status":"public","type":"journal_article","doi":"10.1016/j.jallcom.2024.176549","volume":1008,"author":[{"first_name":"Umar","full_name":"Bashir, Umar","last_name":"Bashir"},{"first_name":"Michael","id":"22501","full_name":"Rüsing, Michael","orcid":"0000-0003-4682-4577","last_name":"Rüsing"},{"full_name":"Klimm, Detlef","last_name":"Klimm","first_name":"Detlef"},{"last_name":"Blukis","full_name":"Blukis, Roberts","first_name":"Roberts"},{"first_name":"Boris","full_name":"Koppitz, Boris","last_name":"Koppitz"},{"full_name":"Eng, Lukas M.","last_name":"Eng","first_name":"Lukas M."},{"first_name":"Matthias","full_name":"Bickermann, Matthias","last_name":"Bickermann"},{"first_name":"Steffen","last_name":"Ganschow","full_name":"Ganschow, Steffen"}],"date_updated":"2025-04-02T16:02:26Z","intvolume":" 1008","citation":{"mla":"Bashir, Umar, et al. “Thermal Conductivity in Solid Solutions of Lithium Niobate Tantalate Single Crystals from 300 K up to 1300 K.” Journal of Alloys and Compounds, vol. 1008, 176549, Elsevier BV, 2024, doi:10.1016/j.jallcom.2024.176549.","short":"U. Bashir, M. Rüsing, D. Klimm, R. Blukis, B. Koppitz, L.M. Eng, M. Bickermann, S. Ganschow, Journal of Alloys and Compounds 1008 (2024).","bibtex":"@article{Bashir_Rüsing_Klimm_Blukis_Koppitz_Eng_Bickermann_Ganschow_2024, title={Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K}, volume={1008}, DOI={10.1016/j.jallcom.2024.176549}, number={176549}, journal={Journal of Alloys and Compounds}, publisher={Elsevier BV}, author={Bashir, Umar and Rüsing, Michael and Klimm, Detlef and Blukis, Roberts and Koppitz, Boris and Eng, Lukas M. and Bickermann, Matthias and Ganschow, Steffen}, year={2024} }","apa":"Bashir, U., Rüsing, M., Klimm, D., Blukis, R., Koppitz, B., Eng, L. M., Bickermann, M., & Ganschow, S. (2024). Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K. Journal of Alloys and Compounds, 1008, Article 176549. https://doi.org/10.1016/j.jallcom.2024.176549","chicago":"Bashir, Umar, Michael Rüsing, Detlef Klimm, Roberts Blukis, Boris Koppitz, Lukas M. Eng, Matthias Bickermann, and Steffen Ganschow. “Thermal Conductivity in Solid Solutions of Lithium Niobate Tantalate Single Crystals from 300 K up to 1300 K.” Journal of Alloys and Compounds 1008 (2024). https://doi.org/10.1016/j.jallcom.2024.176549.","ieee":"U. Bashir et al., “Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K,” Journal of Alloys and Compounds, vol. 1008, Art. no. 176549, 2024, doi: 10.1016/j.jallcom.2024.176549.","ama":"Bashir U, Rüsing M, Klimm D, et al. Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K. Journal of Alloys and Compounds. 2024;1008. doi:10.1016/j.jallcom.2024.176549"},"publication_identifier":{"issn":["0925-8388"]},"publication_status":"published"},{"main_file_link":[{"url":"https://jlupub.ub.uni-giessen.de/server/api/core/bitstreams/fb2b09e6-c0f8-4209-99a1-79fc81d9b1f9/content"}],"doi":"10.1103/physrevresearch.6.l042015","title":"Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls","date_created":"2025-04-02T16:08:55Z","author":[{"full_name":"Verhoff, Leonard M.","last_name":"Verhoff","first_name":"Leonard M."},{"last_name":"Pionteck","full_name":"Pionteck, Mike N.","first_name":"Mike N."},{"first_name":"Michael","full_name":"Rüsing, Michael","id":"22501","last_name":"Rüsing","orcid":"0000-0003-4682-4577"},{"first_name":"Holger","last_name":"Fritze","full_name":"Fritze, Holger"},{"first_name":"Lukas M.","full_name":"Eng, Lukas M.","last_name":"Eng"},{"last_name":"Sanna","full_name":"Sanna, Simone","first_name":"Simone"}],"volume":6,"date_updated":"2025-04-02T16:10:59Z","publisher":"American Physical Society (APS)","citation":{"ama":"Verhoff LM, Pionteck MN, Rüsing M, Fritze H, Eng LM, Sanna S. Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls. Physical Review Research. 2024;6(4). doi:10.1103/physrevresearch.6.l042015","chicago":"Verhoff, Leonard M., Mike N. Pionteck, Michael Rüsing, Holger Fritze, Lukas M. Eng, and Simone Sanna. “Two-Dimensional Electronic Conductivity in Insulating Ferroelectrics: Peculiar Properties of Domain Walls.” Physical Review Research 6, no. 4 (2024). https://doi.org/10.1103/physrevresearch.6.l042015.","ieee":"L. M. Verhoff, M. N. Pionteck, M. Rüsing, H. Fritze, L. M. Eng, and S. Sanna, “Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls,” Physical Review Research, vol. 6, no. 4, Art. no. L042015, 2024, doi: 10.1103/physrevresearch.6.l042015.","apa":"Verhoff, L. M., Pionteck, M. N., Rüsing, M., Fritze, H., Eng, L. M., & Sanna, S. (2024). Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls. Physical Review Research, 6(4), Article L042015. https://doi.org/10.1103/physrevresearch.6.l042015","mla":"Verhoff, Leonard M., et al. “Two-Dimensional Electronic Conductivity in Insulating Ferroelectrics: Peculiar Properties of Domain Walls.” Physical Review Research, vol. 6, no. 4, L042015, American Physical Society (APS), 2024, doi:10.1103/physrevresearch.6.l042015.","bibtex":"@article{Verhoff_Pionteck_Rüsing_Fritze_Eng_Sanna_2024, title={Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls}, volume={6}, DOI={10.1103/physrevresearch.6.l042015}, number={4L042015}, journal={Physical Review Research}, publisher={American Physical Society (APS)}, author={Verhoff, Leonard M. and Pionteck, Mike N. and Rüsing, Michael and Fritze, Holger and Eng, Lukas M. and Sanna, Simone}, year={2024} }","short":"L.M. Verhoff, M.N. Pionteck, M. Rüsing, H. Fritze, L.M. Eng, S. Sanna, Physical Review Research 6 (2024)."},"intvolume":" 6","year":"2024","issue":"4","publication_status":"published","publication_identifier":{"issn":["2643-1564"]},"language":[{"iso":"eng"}],"article_number":"L042015","user_id":"22501","department":[{"_id":"623"},{"_id":"288"},{"_id":"15"}],"_id":"59272","status":"public","abstract":[{"lang":"eng","text":"Ferroelectrics such as LiNbO3 (LN) are wide-band-gap insulators that may show a high local electric conductivity at the domain walls (DWs). The latter are interfaces separating regions of noncollinear polarization, which can be manipulated to build integrated nanoelectronic elements. In the present work, we model different DW types in LN from first principles. Our models reveal the DW morphology and shed light on their electronic properties: A strong band bending is predicted for charged DWs, leading to local metallicity. Defect trapping at the DW may further enhance the electric conductivity."}],"type":"journal_article","publication":"Physical Review Research"},{"publisher":"AIP Publishing","date_created":"2025-04-02T16:12:29Z","title":"Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals","quality_controlled":"1","issue":"10","year":"2024","language":[{"iso":"eng"}],"publication":"Journal of Applied Physics","abstract":[{"text":"Ferroelectric domain walls (DWs) are promising structures for assembling future nano-electronic circuit elements on a larger scale since reporting domain wall currents of up to 1 mA per single DW. One key requirement hereto is their reproducible manufacturing by gaining preparative control over domain size and domain wall conductivity (DWC). To date, most works on DWC have focused on exploring the fundamental electrical properties of individual DWs within single-shot experiments, with an emphasis on quantifying the origins of DWC. Very few reports exist when it comes to comparing the DWC properties between two separate DWs, and literally nothing exists where issues of reproducibility in DWC devices have been addressed. To fill this gap while facing the challenge of finding guidelines for achieving predictable DWC performance, we report on a procedure that allows us to reproducibly prepare single hexagonal domains of a predefined diameter into uniaxial ferroelectric lithium niobate single crystals of 200 and 300 μm thickness, respectively. We show that the domain diameter can be controlled with an uncertainty of a few percent. As-grown DWs are then subjected to a standard procedure of current-limited high-voltage DWC enhancement, and they repetitively reach a DWC increase of six orders of magnitude. While all resulting DWs show significantly enhanced DWC values, their individual current–voltage (I–V) characteristics exhibit different shapes, which can be explained by variations in their 3D real structure reflecting local heterogeneities by defects, DW pinning, and surface-near DW inclination.","lang":"eng"}],"date_updated":"2025-04-02T16:14:31Z","oa":"1","volume":136,"author":[{"first_name":"Julius","last_name":"Ratzenberger","full_name":"Ratzenberger, Julius"},{"last_name":"Kiseleva","full_name":"Kiseleva, Iuliia","first_name":"Iuliia"},{"first_name":"Boris","full_name":"Koppitz, Boris","last_name":"Koppitz"},{"full_name":"Beyreuther, Elke","last_name":"Beyreuther","first_name":"Elke"},{"full_name":"Zahn, Manuel","last_name":"Zahn","first_name":"Manuel"},{"first_name":"Joshua","full_name":"Gössel, Joshua","last_name":"Gössel"},{"last_name":"Hegarty","full_name":"Hegarty, Peter A.","first_name":"Peter A."},{"full_name":"Amber, Zeeshan H.","last_name":"Amber","first_name":"Zeeshan H."},{"first_name":"Michael","full_name":"Rüsing, Michael","id":"22501","orcid":"0000-0003-4682-4577","last_name":"Rüsing"},{"full_name":"Eng, Lukas M.","last_name":"Eng","first_name":"Lukas M."}],"doi":"10.1063/5.0219300","main_file_link":[{"url":" https://doi.org/10.1063/5.0219300","open_access":"1"}],"publication_identifier":{"issn":["0021-8979","1089-7550"]},"publication_status":"published","page":"104302","intvolume":" 136","citation":{"ama":"Ratzenberger J, Kiseleva I, Koppitz B, et al. Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals. Journal of Applied Physics. 2024;136(10):104302. doi:10.1063/5.0219300","chicago":"Ratzenberger, Julius, Iuliia Kiseleva, Boris Koppitz, Elke Beyreuther, Manuel Zahn, Joshua Gössel, Peter A. Hegarty, Zeeshan H. Amber, Michael Rüsing, and Lukas M. Eng. “Toward the Reproducible Fabrication of Conductive Ferroelectric Domain Walls into Lithium Niobate Bulk Single Crystals.” Journal of Applied Physics 136, no. 10 (2024): 104302. https://doi.org/10.1063/5.0219300.","ieee":"J. Ratzenberger et al., “Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals,” Journal of Applied Physics, vol. 136, no. 10, p. 104302, 2024, doi: 10.1063/5.0219300.","apa":"Ratzenberger, J., Kiseleva, I., Koppitz, B., Beyreuther, E., Zahn, M., Gössel, J., Hegarty, P. A., Amber, Z. H., Rüsing, M., & Eng, L. M. (2024). Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals. Journal of Applied Physics, 136(10), 104302. https://doi.org/10.1063/5.0219300","short":"J. Ratzenberger, I. Kiseleva, B. Koppitz, E. Beyreuther, M. Zahn, J. Gössel, P.A. Hegarty, Z.H. Amber, M. Rüsing, L.M. Eng, Journal of Applied Physics 136 (2024) 104302.","mla":"Ratzenberger, Julius, et al. “Toward the Reproducible Fabrication of Conductive Ferroelectric Domain Walls into Lithium Niobate Bulk Single Crystals.” Journal of Applied Physics, vol. 136, no. 10, AIP Publishing, 2024, p. 104302, doi:10.1063/5.0219300.","bibtex":"@article{Ratzenberger_Kiseleva_Koppitz_Beyreuther_Zahn_Gössel_Hegarty_Amber_Rüsing_Eng_2024, title={Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals}, volume={136}, DOI={10.1063/5.0219300}, number={10}, journal={Journal of Applied Physics}, publisher={AIP Publishing}, author={Ratzenberger, Julius and Kiseleva, Iuliia and Koppitz, Boris and Beyreuther, Elke and Zahn, Manuel and Gössel, Joshua and Hegarty, Peter A. and Amber, Zeeshan H. and Rüsing, Michael and Eng, Lukas M.}, year={2024}, pages={104302} }"},"_id":"59273","department":[{"_id":"288"},{"_id":"15"},{"_id":"623"}],"user_id":"22501","article_type":"original","type":"journal_article","status":"public"},{"publication":"Physical Review B","abstract":[{"lang":"eng","text":"Recently, ion exchange (IE) has been used to periodically modify the coercive field (Ec) of the crystal prior to periodic poling, to fabricate fine-pitch domain structures in Rb-doped KTiOPO4 (RKTP). Here, we use micro-Raman spectroscopy to understand the impact of IE on the vibrational modes related to the Rb/K lattice sites, TiO octahedra, and PO4 tetrahedra, which all form the basis of the RKTP crystal structure. We analyze the Raman spectra of three different RKTP samples: (1) a RKTP sample that shows a poled domain grating only, (2) a RKTP sample that has an Ec grating only, and (3) a RKTP sample that has both an Ec and a domain grating of the nominally same spacing. This allows us to determine the impact of IE on the vibrational modes of RKTP. We characterize the changes in the lower Raman peaks related to the alkali-metal ions, as well as observe lattice modifications induced by the incorporation of Rb+ that extend further into the crystal bulk than the expected IE depth. Moreover, the influence of IE on the domain walls is also manifested in their Raman peak shift. We discuss our results in terms of the deformation of the PO4and TiO groups. Our results highlight the intricate impact of IE on the crystal structure and how it facilitates periodic poling, paving the way for further development of the Ec-engineering technique."}],"language":[{"iso":"eng"}],"issue":"21","year":"2024","publisher":"American Physical Society (APS)","date_created":"2025-04-02T16:14:44Z","title":"Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching","type":"journal_article","status":"public","_id":"59274","user_id":"22501","department":[{"_id":"288"},{"_id":"15"},{"_id":"623"}],"article_type":"original","article_number":"214115","publication_status":"published","publication_identifier":{"issn":["2469-9950","2469-9969"]},"citation":{"apa":"Lee, C. S. J., Canalias, C., Buschbeck, R., Koppitz, B., Hempel, F., Amber, Z., Eng, L. M., & Rüsing, M. (2024). Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching. Physical Review B, 110(21), Article 214115. https://doi.org/10.1103/physrevb.110.214115","bibtex":"@article{Lee_Canalias_Buschbeck_Koppitz_Hempel_Amber_Eng_Rüsing_2024, title={Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching}, volume={110}, DOI={10.1103/physrevb.110.214115}, number={21214115}, journal={Physical Review B}, publisher={American Physical Society (APS)}, author={Lee, Cherrie S. J. and Canalias, Carlota and Buschbeck, Robin and Koppitz, Boris and Hempel, Franz and Amber, Zeeshan and Eng, Lukas M. and Rüsing, Michael}, year={2024} }","short":"C.S.J. Lee, C. Canalias, R. Buschbeck, B. Koppitz, F. Hempel, Z. Amber, L.M. Eng, M. Rüsing, Physical Review B 110 (2024).","mla":"Lee, Cherrie S. J., et al. “Impact of Ion Exchange on Vibrational Modes in Rb-Doped KTiOPO4: A Raman Spectroscopy Study on the Interplay between Ion Exchange and Polarization Switching.” Physical Review B, vol. 110, no. 21, 214115, American Physical Society (APS), 2024, doi:10.1103/physrevb.110.214115.","ama":"Lee CSJ, Canalias C, Buschbeck R, et al. Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching. Physical Review B. 2024;110(21). doi:10.1103/physrevb.110.214115","chicago":"Lee, Cherrie S. J., Carlota Canalias, Robin Buschbeck, Boris Koppitz, Franz Hempel, Zeeshan Amber, Lukas M. Eng, and Michael Rüsing. “Impact of Ion Exchange on Vibrational Modes in Rb-Doped KTiOPO4: A Raman Spectroscopy Study on the Interplay between Ion Exchange and Polarization Switching.” Physical Review B 110, no. 21 (2024). https://doi.org/10.1103/physrevb.110.214115.","ieee":"C. S. J. Lee et al., “Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching,” Physical Review B, vol. 110, no. 21, Art. no. 214115, 2024, doi: 10.1103/physrevb.110.214115."},"intvolume":" 110","date_updated":"2025-04-02T16:18:34Z","author":[{"full_name":"Lee, Cherrie S. J.","last_name":"Lee","first_name":"Cherrie S. J."},{"first_name":"Carlota","full_name":"Canalias, Carlota","last_name":"Canalias"},{"first_name":"Robin","last_name":"Buschbeck","full_name":"Buschbeck, Robin"},{"full_name":"Koppitz, Boris","last_name":"Koppitz","first_name":"Boris"},{"first_name":"Franz","last_name":"Hempel","full_name":"Hempel, Franz"},{"first_name":"Zeeshan","last_name":"Amber","full_name":"Amber, Zeeshan"},{"full_name":"Eng, Lukas M.","last_name":"Eng","first_name":"Lukas M."},{"last_name":"Rüsing","orcid":"0000-0003-4682-4577","full_name":"Rüsing, Michael","id":"22501","first_name":"Michael"}],"volume":110,"doi":"10.1103/physrevb.110.214115"},{"user_id":"22501","department":[{"_id":"288"},{"_id":"623"},{"_id":"15"}],"_id":"59275","language":[{"iso":"eng"}],"type":"journal_article","publication":"Advanced Physics Research","status":"public","abstract":[{"lang":"eng","text":"Studying and understanding many‐body interactions, particularly electron‐boson interactions, is essential for a deeper elucidation of fundamental physical phenomena and the development of novel material functionalities. Here, this aspect is explored in the weak itinerant ferromagnet LaCo2P2 by means of momentum‐resolved photoelectron spectroscopy (ARPES) and first‐principles calculations. The detailed ARPES patterns enable to unveil bulk and surface bands, spin splittings due to Rashba and exchange interactions, as well as the evolution of bands with temperature, which altogether creates a solid foundation for theoretical studies. The latter has allowed to establish the impact of electron‐boson interactions on the electronic structure, that are reflected in its strong renormalization driven by electron‐magnon interaction and the emergence of distinctive kinks of surface and bulk electron bands due to significant electron‐phonon coupling. Our results highlight the distinct impact of electron‐boson interactions on the electronic structure, particularly on the itinerant d states. Similar electronic states are observed in the isostructural iron pnictides, where electron‐boson interactions play a crucial role in the emergence of superconductivity. It is believed that further studies of material systems involving both magnetically active d‐ and f‐sublattices will reveal more advanced phenomena in the bulk and at distinct surfaces, driven by a combination of factors including Rashba and Kondo effects, exchange magnetism, and electron‐boson interactions."}],"date_created":"2025-04-02T16:18:56Z","author":[{"last_name":"Usachov","full_name":"Usachov, D. Yu.","first_name":"D. Yu."},{"first_name":"K.","last_name":"Ali","full_name":"Ali, K."},{"first_name":"G.","last_name":"Poelchen","full_name":"Poelchen, G."},{"full_name":"Mende, M.","last_name":"Mende","first_name":"M."},{"last_name":"Schulz","full_name":"Schulz, S.","first_name":"S."},{"full_name":"Peters, M.","last_name":"Peters","first_name":"M."},{"last_name":"Bokai","full_name":"Bokai, K.","first_name":"K."},{"full_name":"Sklyadneva, I. Yu.","last_name":"Sklyadneva","first_name":"I. Yu."},{"last_name":"Stolyarov","full_name":"Stolyarov, V.","first_name":"V."},{"full_name":"Chulkov, E. V.","last_name":"Chulkov","first_name":"E. V."},{"first_name":"K.","last_name":"Kliemt","full_name":"Kliemt, K."},{"full_name":"Paischer, S.","last_name":"Paischer","first_name":"S."},{"last_name":"Buczek","full_name":"Buczek, P. A.","first_name":"P. A."},{"last_name":"Heid","full_name":"Heid, R.","first_name":"R."},{"last_name":"Hempel","full_name":"Hempel, F.","first_name":"F."},{"id":"22501","full_name":"Rüsing, Michael","last_name":"Rüsing","orcid":"0000-0003-4682-4577","first_name":"Michael"},{"first_name":"A.","full_name":"Ernst, A.","last_name":"Ernst"},{"first_name":"C.","full_name":"Krellner, C.","last_name":"Krellner"},{"first_name":"S. V.","full_name":"Eremeev, S. V.","last_name":"Eremeev"},{"last_name":"Vyalikh","full_name":"Vyalikh, D. V.","first_name":"D. V."}],"publisher":"Wiley","date_updated":"2025-04-02T16:20:41Z","doi":"10.1002/apxr.202400137","title":"Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2","publication_status":"published","publication_identifier":{"issn":["2751-1200","2751-1200"]},"quality_controlled":"1","citation":{"ama":"Usachov DYu, Ali K, Poelchen G, et al. Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2. Advanced Physics Research. Published online 2024. doi:10.1002/apxr.202400137","ieee":"D. Yu. Usachov et al., “Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2,” Advanced Physics Research, 2024, doi: 10.1002/apxr.202400137.","chicago":"Usachov, D. Yu., K. Ali, G. Poelchen, M. Mende, S. Schulz, M. Peters, K. Bokai, et al. “Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2.” Advanced Physics Research, 2024. https://doi.org/10.1002/apxr.202400137.","bibtex":"@article{Usachov_Ali_Poelchen_Mende_Schulz_Peters_Bokai_Sklyadneva_Stolyarov_Chulkov_et al._2024, title={Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2}, DOI={10.1002/apxr.202400137}, journal={Advanced Physics Research}, publisher={Wiley}, author={Usachov, D. Yu. and Ali, K. and Poelchen, G. and Mende, M. and Schulz, S. and Peters, M. and Bokai, K. and Sklyadneva, I. Yu. and Stolyarov, V. and Chulkov, E. V. and et al.}, year={2024} }","mla":"Usachov, D. Yu., et al. “Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2.” Advanced Physics Research, Wiley, 2024, doi:10.1002/apxr.202400137.","short":"D.Yu. Usachov, K. Ali, G. Poelchen, M. Mende, S. Schulz, M. Peters, K. Bokai, I.Yu. Sklyadneva, V. Stolyarov, E.V. Chulkov, K. Kliemt, S. Paischer, P.A. Buczek, R. Heid, F. Hempel, M. Rüsing, A. Ernst, C. Krellner, S.V. Eremeev, D.V. Vyalikh, Advanced Physics Research (2024).","apa":"Usachov, D. Yu., Ali, K., Poelchen, G., Mende, M., Schulz, S., Peters, M., Bokai, K., Sklyadneva, I. Yu., Stolyarov, V., Chulkov, E. V., Kliemt, K., Paischer, S., Buczek, P. A., Heid, R., Hempel, F., Rüsing, M., Ernst, A., Krellner, C., Eremeev, S. V., & Vyalikh, D. V. (2024). Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2. Advanced Physics Research. https://doi.org/10.1002/apxr.202400137"},"year":"2024"},{"language":[{"iso":"eng"}],"keyword":["Ferroelectrics","lithium niobate","piezoresponse force microscopy"],"publication":"Journal of Applied Physics","abstract":[{"lang":"eng","text":"Piezoresponse force microscopy (PFM) is one of the most widespread methods for investigating and visualizing ferroelectric domain structures down to the nanometer length scale. PFM makes use of the direct coupling of the piezoelectric response to the crystal lattice, and hence, it is most often applied to spatially map the three-dimensional (3D) near-surface domain distribution of any polar or ferroic sample. Nonetheless, since most samples investigated by PFM are at least semiconducting or fully insulating, the electric ac field emerging from the conductive scanning force microscopy (SFM) tip penetrates the sample and, hence, may also couple to polar features that are deeply buried into the bulk of the sample under investigation. Thus, in the work presented here, we experimentally and theoretically explore the contrast and depth resolution capabilities of PFM, by analyzing the dependence of several key parameters. These key parameters include the depth of the buried feature, i.e., here a domain wall (DW), as well as PFM-relevant technical parameters such as the tip radius, the PFM drive voltage and frequency, and the signal-to-noise ratio. The theoretical predictions are experimentally verified using x-cut periodically poled lithium niobate single crystals that are specially prepared into wedge-shaped samples, in order to allow the buried feature, here the DW, to be “positioned” at any depth into the bulk. This inspection essentially contributes to the fundamental understanding in PFM contrast analysis and to the reconstruction of 3D domain structures down to a 1 μm-penetration depth into the sample."}],"date_created":"2024-07-01T21:00:43Z","publisher":"AIP Publishing","title":"Depth resolution in piezoresponse force microscopy","issue":"22","quality_controlled":"1","year":"2024","user_id":"22501","department":[{"_id":"15"},{"_id":"169"},{"_id":"288"},{"_id":"623"}],"_id":"54966","article_type":"original","type":"journal_article","status":"public","author":[{"full_name":"Roeper, Matthias","last_name":"Roeper","first_name":"Matthias"},{"first_name":"Samuel D.","full_name":"Seddon, Samuel D.","last_name":"Seddon"},{"first_name":"Zeeshan H.","full_name":"Amber, Zeeshan H.","last_name":"Amber"},{"full_name":"Rüsing, Michael","id":"22501","orcid":"0000-0003-4682-4577","last_name":"Rüsing","first_name":"Michael"},{"first_name":"Lukas M.","full_name":"Eng, Lukas M.","last_name":"Eng"}],"volume":135,"date_updated":"2025-04-03T12:35:34Z","oa":"1","main_file_link":[{"url":"https://doi.org/10.1063/5.0206784","open_access":"1"}],"doi":"10.1063/5.0206784","publication_status":"published","publication_identifier":{"issn":["0021-8979","1089-7550"]},"citation":{"short":"M. Roeper, S.D. Seddon, Z.H. Amber, M. Rüsing, L.M. Eng, Journal of Applied Physics 135 (2024).","bibtex":"@article{Roeper_Seddon_Amber_Rüsing_Eng_2024, title={Depth resolution in piezoresponse force microscopy}, volume={135}, DOI={10.1063/5.0206784}, number={22}, journal={Journal of Applied Physics}, publisher={AIP Publishing}, author={Roeper, Matthias and Seddon, Samuel D. and Amber, Zeeshan H. and Rüsing, Michael and Eng, Lukas M.}, year={2024} }","mla":"Roeper, Matthias, et al. “Depth Resolution in Piezoresponse Force Microscopy.” Journal of Applied Physics, vol. 135, no. 22, AIP Publishing, 2024, doi:10.1063/5.0206784.","apa":"Roeper, M., Seddon, S. D., Amber, Z. H., Rüsing, M., & Eng, L. M. (2024). Depth resolution in piezoresponse force microscopy. Journal of Applied Physics, 135(22). https://doi.org/10.1063/5.0206784","ama":"Roeper M, Seddon SD, Amber ZH, Rüsing M, Eng LM. Depth resolution in piezoresponse force microscopy. Journal of Applied Physics. 2024;135(22). doi:10.1063/5.0206784","chicago":"Roeper, Matthias, Samuel D. Seddon, Zeeshan H. Amber, Michael Rüsing, and Lukas M. Eng. “Depth Resolution in Piezoresponse Force Microscopy.” Journal of Applied Physics 135, no. 22 (2024). https://doi.org/10.1063/5.0206784.","ieee":"M. Roeper, S. D. Seddon, Z. H. Amber, M. Rüsing, and L. M. Eng, “Depth resolution in piezoresponse force microscopy,” Journal of Applied Physics, vol. 135, no. 22, 2024, doi: 10.1063/5.0206784."},"intvolume":" 135"},{"type":"misc","status":"public","user_id":"22501","department":[{"_id":"288"},{"_id":"15"},{"_id":"623"}],"_id":"59259","language":[{"iso":"eng"}],"citation":{"mla":"Schwabe, Tobias, et al. Quantum Photonic Systems in CMOS Compatible Silicon Nitride Technology . Zenodo, 2024, doi:10.5281/zenodo.15124929.","bibtex":"@book{Schwabe_Rüsing_Staal_Schwengelbeck_Bollmers_Padberg_Eigner_Silberhorn_Scheytt_2024, title={Quantum photonic systems in CMOS compatible silicon nitride technology }, DOI={10.5281/zenodo.15124929}, publisher={Zenodo}, author={Schwabe, Tobias and Rüsing, Michael and Staal, Niels and Schwengelbeck, Max and Bollmers, Laura and Padberg, Laura and Eigner, Christof and Silberhorn, Christine and Scheytt, J. Christoph}, year={2024} }","short":"T. Schwabe, M. Rüsing, N. Staal, M. Schwengelbeck, L. Bollmers, L. Padberg, C. Eigner, C. Silberhorn, J.C. Scheytt, Quantum Photonic Systems in CMOS Compatible Silicon Nitride Technology , Zenodo, 2024.","apa":"Schwabe, T., Rüsing, M., Staal, N., Schwengelbeck, M., Bollmers, L., Padberg, L., Eigner, C., Silberhorn, C., & Scheytt, J. C. (2024). Quantum photonic systems in CMOS compatible silicon nitride technology . Zenodo. https://doi.org/10.5281/zenodo.15124929","ama":"Schwabe T, Rüsing M, Staal N, et al. Quantum Photonic Systems in CMOS Compatible Silicon Nitride Technology . Zenodo; 2024. doi:10.5281/zenodo.15124929","chicago":"Schwabe, Tobias, Michael Rüsing, Niels Staal, Max Schwengelbeck, Laura Bollmers, Laura Padberg, Christof Eigner, Christine Silberhorn, and J. Christoph Scheytt. Quantum Photonic Systems in CMOS Compatible Silicon Nitride Technology . Zenodo, 2024. https://doi.org/10.5281/zenodo.15124929.","ieee":"T. Schwabe et al., Quantum photonic systems in CMOS compatible silicon nitride technology . Zenodo, 2024."},"year":"2024","date_created":"2025-04-02T11:24:23Z","author":[{"id":"39217","full_name":"Schwabe, Tobias","last_name":"Schwabe","first_name":"Tobias"},{"first_name":"Michael","orcid":"0000-0003-4682-4577","last_name":"Rüsing","id":"22501","full_name":"Rüsing, Michael"},{"full_name":"Staal, Niels","last_name":"Staal","first_name":"Niels"},{"last_name":"Schwengelbeck","full_name":"Schwengelbeck, Max","first_name":"Max"},{"first_name":"Laura","last_name":"Bollmers","id":"61375","full_name":"Bollmers, Laura"},{"first_name":"Laura","last_name":"Padberg","id":"40300","full_name":"Padberg, Laura"},{"first_name":"Christof","orcid":"https://orcid.org/0000-0002-5693-3083","last_name":"Eigner","id":"13244","full_name":"Eigner, Christof"},{"first_name":"Christine","last_name":"Silberhorn","full_name":"Silberhorn, Christine","id":"26263"},{"first_name":"J. Christoph","last_name":"Scheytt","orcid":"0000-0002-5950-6618 ","id":"37144","full_name":"Scheytt, J. Christoph"}],"publisher":"Zenodo","date_updated":"2025-04-03T12:34:56Z","doi":"10.5281/zenodo.15124929","title":"Quantum photonic systems in CMOS compatible silicon nitride technology "},{"doi":"10.1364/opticaq.532334","title":"Orchestrating time and color: a programmable source of high-dimensional entanglement","date_created":"2024-09-27T11:46:59Z","author":[{"first_name":"Laura","last_name":"Serino","id":"88242","full_name":"Serino, Laura"},{"full_name":"Ridder, Werner","id":"63574","last_name":"Ridder","first_name":"Werner"},{"first_name":"Abhinandan","last_name":"Bhattacharjee","id":"95902","full_name":"Bhattacharjee, Abhinandan"},{"last_name":"Gil López","full_name":"Gil López, Jano","id":"51223","first_name":"Jano"},{"orcid":"0000-0003-4140-0556 ","last_name":"Brecht","full_name":"Brecht, Benjamin","id":"27150","first_name":"Benjamin"},{"first_name":"Christine","full_name":"Silberhorn, Christine","id":"26263","last_name":"Silberhorn"}],"publisher":"Optica Publishing Group","date_updated":"2025-12-01T08:49:46Z","citation":{"mla":"Serino, Laura, et al. “Orchestrating Time and Color: A Programmable Source of High-Dimensional Entanglement.” Optica Quantum, Optica Publishing Group, 2024, doi:10.1364/opticaq.532334.","bibtex":"@article{Serino_Ridder_Bhattacharjee_Gil López_Brecht_Silberhorn_2024, title={Orchestrating time and color: a programmable source of high-dimensional entanglement}, DOI={10.1364/opticaq.532334}, journal={Optica Quantum}, publisher={Optica Publishing Group}, author={Serino, Laura and Ridder, Werner and Bhattacharjee, Abhinandan and Gil López, Jano and Brecht, Benjamin and Silberhorn, Christine}, year={2024} }","short":"L. Serino, W. Ridder, A. Bhattacharjee, J. Gil López, B. Brecht, C. Silberhorn, Optica Quantum (2024).","apa":"Serino, L., Ridder, W., Bhattacharjee, A., Gil López, J., Brecht, B., & Silberhorn, C. (2024). Orchestrating time and color: a programmable source of high-dimensional entanglement. Optica Quantum. https://doi.org/10.1364/opticaq.532334","ama":"Serino L, Ridder W, Bhattacharjee A, Gil López J, Brecht B, Silberhorn C. Orchestrating time and color: a programmable source of high-dimensional entanglement. Optica Quantum. Published online 2024. doi:10.1364/opticaq.532334","ieee":"L. Serino, W. Ridder, A. Bhattacharjee, J. Gil López, B. Brecht, and C. Silberhorn, “Orchestrating time and color: a programmable source of high-dimensional entanglement,” Optica Quantum, 2024, doi: 10.1364/opticaq.532334.","chicago":"Serino, Laura, Werner Ridder, Abhinandan Bhattacharjee, Jano Gil López, Benjamin Brecht, and Christine Silberhorn. “Orchestrating Time and Color: A Programmable Source of High-Dimensional Entanglement.” Optica Quantum, 2024. https://doi.org/10.1364/opticaq.532334."},"year":"2024","publication_status":"published","publication_identifier":{"issn":["2837-6714"]},"language":[{"iso":"eng"}],"user_id":"63574","department":[{"_id":"288"},{"_id":"623"},{"_id":"288"}],"project":[{"_id":"211","name":"QuICHE: Quanteninformation und Quantenkommunikation mit hochdimensionaler Informationskodierung (QuICHE)"}],"_id":"56267","status":"public","type":"journal_article","publication":"Optica Quantum"},{"date_created":"2024-05-14T12:40:48Z","publisher":"American Physical Society (APS)","title":"Realization of high-fidelity unitary operations on up to 64 frequency bins","issue":"2","year":"2024","language":[{"iso":"eng"}],"publication":"Physical Review Research","abstract":[{"lang":"eng","text":"The ability to apply user-chosen large-scale unitary operations with high fidelity to a quantum state is key to realizing future photonic quantum technologies. Here, we realize the implementation of programmable unitary operations on up to 64 frequency-bin modes. To benchmark the performance of our system, we probe different quantum walk unitary operations, in particular, Grover walks on four-dimensional hypercubes with similarities exceeding 95% and quantum walks with 400 steps on circles and finite lines with similarities of 98%. Our results open a path toward implementing high-quality unitary operations, which can form the basis for applications in complex tasks, such as Gaussian boson sampling.\r\n \r\n \r\n \r\n \r\n Published by the American Physical Society\r\n 2024\r\n \r\n \r\n "}],"author":[{"last_name":"De","full_name":"De, Syamsundar","first_name":"Syamsundar"},{"full_name":"Ansari, Vahid","last_name":"Ansari","first_name":"Vahid"},{"id":"75127","full_name":"Sperling, Jan","orcid":"0000-0002-5844-3205","last_name":"Sperling","first_name":"Jan"},{"first_name":"Sonja","id":"48188","full_name":"Barkhofen, Sonja","last_name":"Barkhofen"},{"full_name":"Brecht, Benjamin","id":"27150","orcid":"0000-0003-4140-0556 ","last_name":"Brecht","first_name":"Benjamin"},{"first_name":"Christine","id":"26263","full_name":"Silberhorn, Christine","last_name":"Silberhorn"}],"volume":6,"date_updated":"2025-12-18T16:14:39Z","doi":"10.1103/physrevresearch.6.l022040","publication_status":"published","publication_identifier":{"issn":["2643-1564"]},"citation":{"mla":"De, Syamsundar, et al. “Realization of High-Fidelity Unitary Operations on up to 64 Frequency Bins.” Physical Review Research, vol. 6, no. 2, L022040, American Physical Society (APS), 2024, doi:10.1103/physrevresearch.6.l022040.","short":"S. De, V. Ansari, J. Sperling, S. Barkhofen, B. Brecht, C. Silberhorn, Physical Review Research 6 (2024).","bibtex":"@article{De_Ansari_Sperling_Barkhofen_Brecht_Silberhorn_2024, title={Realization of high-fidelity unitary operations on up to 64 frequency bins}, volume={6}, DOI={10.1103/physrevresearch.6.l022040}, number={2L022040}, journal={Physical Review Research}, publisher={American Physical Society (APS)}, author={De, Syamsundar and Ansari, Vahid and Sperling, Jan and Barkhofen, Sonja and Brecht, Benjamin and Silberhorn, Christine}, year={2024} }","apa":"De, S., Ansari, V., Sperling, J., Barkhofen, S., Brecht, B., & Silberhorn, C. (2024). Realization of high-fidelity unitary operations on up to 64 frequency bins. Physical Review Research, 6(2), Article L022040. https://doi.org/10.1103/physrevresearch.6.l022040","ama":"De S, Ansari V, Sperling J, Barkhofen S, Brecht B, Silberhorn C. Realization of high-fidelity unitary operations on up to 64 frequency bins. Physical Review Research. 2024;6(2). doi:10.1103/physrevresearch.6.l022040","ieee":"S. De, V. Ansari, J. Sperling, S. Barkhofen, B. Brecht, and C. Silberhorn, “Realization of high-fidelity unitary operations on up to 64 frequency bins,” Physical Review Research, vol. 6, no. 2, Art. no. L022040, 2024, doi: 10.1103/physrevresearch.6.l022040.","chicago":"De, Syamsundar, Vahid Ansari, Jan Sperling, Sonja Barkhofen, Benjamin Brecht, and Christine Silberhorn. “Realization of High-Fidelity Unitary Operations on up to 64 Frequency Bins.” Physical Review Research 6, no. 2 (2024). https://doi.org/10.1103/physrevresearch.6.l022040."},"intvolume":" 6","user_id":"27150","department":[{"_id":"623"},{"_id":"288"},{"_id":"15"}],"project":[{"name":"QuPoPCoRN: QUPOPCORN: Quantum Particles on Programmable Complex Reconfigurable Networks","_id":"216"}],"_id":"54288","article_number":"L022040","type":"journal_article","status":"public"},{"date_created":"2024-06-19T06:58:17Z","publisher":"Optica Publishing Group","title":"Integrated, bright broadband, two-colour parametric down-conversion source","issue":"14","year":"2024","language":[{"iso":"eng"}],"publication":"Optics Express","abstract":[{"text":"Broadband quantum light is a vital resource for quantum metrology and spectroscopy applications such as quantum optical coherence tomography or entangled two photon absorption. For entangled two photon absorption in particular, very high photon flux combined with high time-frequency entanglement is crucial for observing a signal. So far these conditions could be met by using high power lasers driving degenerate, type 0 bulk-crystal spontaneous parametric down conversion (SPDC) sources. This naturally limits the available wavelength ranges and precludes deterministic splitting of the generated output photons. In this work we demonstrate an integrated two-colour SPDC source utilising a group-velocity matched lithium niobate waveguide, reaching both exceptional brightness 1.52⋅106pairssmWGHz and large bandwidth (7.8 THz FWHM) while pumped with a few mW of continuous wave (CW) laser light. By converting a narrow band pump to broadband pulses the created photon pairs show correlation times of Δτ ≈ 120 fs while maintaining the narrow bandwidth Δω\r\n p\r\n ≪ 1 MHz of the CW pump light, yielding strong time-frequency entanglement. Furthermore our process can be adapted to a wide range of central wavelengths.","lang":"eng"}],"volume":32,"author":[{"first_name":"René","last_name":"Pollmann","full_name":"Pollmann, René","id":"78890"},{"full_name":"Roeder, Franz","id":"88149","last_name":"Roeder","first_name":"Franz"},{"last_name":"Quiring","full_name":"Quiring, Victor","first_name":"Victor"},{"last_name":"Ricken","full_name":"Ricken, Raimund","first_name":"Raimund"},{"first_name":"Christof","orcid":"https://orcid.org/0000-0002-5693-3083","last_name":"Eigner","full_name":"Eigner, Christof","id":"13244"},{"id":"27150","full_name":"Brecht, Benjamin","last_name":"Brecht","orcid":"0000-0003-4140-0556 ","first_name":"Benjamin"},{"first_name":"Christine","last_name":"Silberhorn","id":"26263","full_name":"Silberhorn, Christine"}],"date_updated":"2025-12-19T11:37:41Z","doi":"10.1364/oe.522549","publication_identifier":{"issn":["1094-4087"]},"publication_status":"published","intvolume":" 32","citation":{"short":"R. Pollmann, F. Roeder, V. Quiring, R. Ricken, C. Eigner, B. Brecht, C. Silberhorn, Optics Express 32 (2024).","mla":"Pollmann, René, et al. “Integrated, Bright Broadband, Two-Colour Parametric down-Conversion Source.” Optics Express, vol. 32, no. 14, 23945, Optica Publishing Group, 2024, doi:10.1364/oe.522549.","bibtex":"@article{Pollmann_Roeder_Quiring_Ricken_Eigner_Brecht_Silberhorn_2024, title={Integrated, bright broadband, two-colour parametric down-conversion source}, volume={32}, DOI={10.1364/oe.522549}, number={1423945}, journal={Optics Express}, publisher={Optica Publishing Group}, author={Pollmann, René and Roeder, Franz and Quiring, Victor and Ricken, Raimund and Eigner, Christof and Brecht, Benjamin and Silberhorn, Christine}, year={2024} }","apa":"Pollmann, R., Roeder, F., Quiring, V., Ricken, R., Eigner, C., Brecht, B., & Silberhorn, C. (2024). Integrated, bright broadband, two-colour parametric down-conversion source. Optics Express, 32(14), Article 23945. https://doi.org/10.1364/oe.522549","ama":"Pollmann R, Roeder F, Quiring V, et al. Integrated, bright broadband, two-colour parametric down-conversion source. Optics Express. 2024;32(14). doi:10.1364/oe.522549","chicago":"Pollmann, René, Franz Roeder, Victor Quiring, Raimund Ricken, Christof Eigner, Benjamin Brecht, and Christine Silberhorn. “Integrated, Bright Broadband, Two-Colour Parametric down-Conversion Source.” Optics Express 32, no. 14 (2024). https://doi.org/10.1364/oe.522549.","ieee":"R. Pollmann et al., “Integrated, bright broadband, two-colour parametric down-conversion source,” Optics Express, vol. 32, no. 14, Art. no. 23945, 2024, doi: 10.1364/oe.522549."},"department":[{"_id":"15"},{"_id":"623"},{"_id":"288"}],"user_id":"78890","_id":"54815","article_type":"original","article_number":"23945","type":"journal_article","status":"public"},{"publication_status":"published","publication_identifier":{"issn":["1367-2630"]},"issue":"12","year":"2024","citation":{"apa":"Roeder, F., Gnanavel, A., Pollmann, R., Brecht, O., Stefszky, M., Padberg, L., Eigner, C., Silberhorn, C., & Brecht, B. (2024). Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared. New Journal of Physics, 26(12), Article 123025. https://doi.org/10.1088/1367-2630/ad9f98","short":"F. Roeder, A. Gnanavel, R. Pollmann, O. Brecht, M. Stefszky, L. Padberg, C. Eigner, C. Silberhorn, B. Brecht, New Journal of Physics 26 (2024).","bibtex":"@article{Roeder_Gnanavel_Pollmann_Brecht_Stefszky_Padberg_Eigner_Silberhorn_Brecht_2024, title={Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared}, volume={26}, DOI={10.1088/1367-2630/ad9f98}, number={12123025}, journal={New Journal of Physics}, publisher={IOP Publishing}, author={Roeder, Franz and Gnanavel, Abira and Pollmann, René and Brecht, Olga and Stefszky, Michael and Padberg, Laura and Eigner, Christof and Silberhorn, Christine and Brecht, Benjamin}, year={2024} }","mla":"Roeder, Franz, et al. “Ultra-Broadband Non-Degenerate Guided-Wave Bi-Photon Source in the near and Mid-Infrared.” New Journal of Physics, vol. 26, no. 12, 123025, IOP Publishing, 2024, doi:10.1088/1367-2630/ad9f98.","ieee":"F. Roeder et al., “Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared,” New Journal of Physics, vol. 26, no. 12, Art. no. 123025, 2024, doi: 10.1088/1367-2630/ad9f98.","chicago":"Roeder, Franz, Abira Gnanavel, René Pollmann, Olga Brecht, Michael Stefszky, Laura Padberg, Christof Eigner, Christine Silberhorn, and Benjamin Brecht. “Ultra-Broadband Non-Degenerate Guided-Wave Bi-Photon Source in the near and Mid-Infrared.” New Journal of Physics 26, no. 12 (2024). https://doi.org/10.1088/1367-2630/ad9f98.","ama":"Roeder F, Gnanavel A, Pollmann R, et al. Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared. New Journal of Physics. 2024;26(12). doi:10.1088/1367-2630/ad9f98"},"intvolume":" 26","date_updated":"2025-12-19T11:36:36Z","publisher":"IOP Publishing","date_created":"2024-12-27T19:01:14Z","author":[{"first_name":"Franz","last_name":"Roeder","full_name":"Roeder, Franz","id":"88149"},{"last_name":"Gnanavel","full_name":"Gnanavel, Abira","first_name":"Abira"},{"last_name":"Pollmann","id":"78890","full_name":"Pollmann, René","first_name":"René"},{"last_name":"Brecht","full_name":"Brecht, Olga","first_name":"Olga"},{"first_name":"Michael","last_name":"Stefszky","full_name":"Stefszky, Michael","id":"42777"},{"first_name":"Laura","id":"40300","full_name":"Padberg, Laura","last_name":"Padberg"},{"orcid":"https://orcid.org/0000-0002-5693-3083","last_name":"Eigner","full_name":"Eigner, Christof","id":"13244","first_name":"Christof"},{"first_name":"Christine","id":"26263","full_name":"Silberhorn, Christine","last_name":"Silberhorn"},{"last_name":"Brecht","orcid":"0000-0003-4140-0556 ","id":"27150","full_name":"Brecht, Benjamin","first_name":"Benjamin"}],"volume":26,"title":"Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared","doi":"10.1088/1367-2630/ad9f98","type":"journal_article","publication":"New Journal of Physics","abstract":[{"lang":"eng","text":"The latest applications in ultrafast quantum metrology require bright, broadband bi-photon sources with one of the photons in the mid-infrared and the other in the visible to near infrared. However, existing sources based on bulk crystals are limited in brightness due to the short interaction length and only allow for limited dispersion engineering. Here, we present an integrated PDC source based on a Ti:LiNbO3 waveguide that generates broadband bi-photons with central wavelengths at 860 nm and 2800 nm. Their spectral bandwidth exceeds 25 THz and is achieved by simultaneous matching of the group velocities (GVs) and cancellation of GV dispersion for the signal and idler field. We provide an intuitive understanding of the process by studying our source’s behavior at different temperatures and pump wavelengths, which agrees well with simulations."}],"status":"public","project":[{"name":"MIRAQLS: MIRAQLS: Mid-infrared Quantum Technology for Sensing","_id":"571"},{"_id":"190","name":"E2TPA: Exploiting Entangled Two-Photon Absorption"}],"_id":"57862","user_id":"78890","department":[{"_id":"288"},{"_id":"623"},{"_id":"15"}],"article_number":"123025","article_type":"original","language":[{"iso":"eng"}]},{"issue":"21","year":"2023","date_created":"2023-10-19T14:22:59Z","publisher":"Optica Publishing Group","title":"Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications","publication":"Optics Express","abstract":[{"text":"We report a titanium indiffused waveguide resonator featuring an integrated electro-optic modulator for cavity length stabilisation that produces close to 5 dB of squeezed light at 1550 nm (2.4 dB directly measured). The resonator is locked on resonance for tens of minutes with 70 mW of SH light incident on the cavity, demonstrating that photorefraction can be mitigated. Squeezed light production concurrent with cavity length stabilisation utilising the integrated EOM is demonstrated. The device demonstrates the suitability of this platform for squeezed light generation in network applications, where stabilisation to the reference field is typically necessary.","lang":"eng"}],"language":[{"iso":"eng"}],"keyword":["Atomic and Molecular Physics","and Optics"],"publication_identifier":{"issn":["1094-4087"]},"publication_status":"published","intvolume":" 31","citation":{"apa":"Stefszky, M., vom Bruch, F., Santandrea, M., Ricken, R., Quiring, V., Eigner, C., Herrmann, H., & Silberhorn, C. (2023). Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications. Optics Express, 31(21), Article 34903. https://doi.org/10.1364/oe.498423","mla":"Stefszky, M., et al. “Lithium Niobate Waveguide Squeezer with Integrated Cavity Length Stabilisation for Network Applications.” Optics Express, vol. 31, no. 21, 34903, Optica Publishing Group, 2023, doi:10.1364/oe.498423.","short":"M. Stefszky, F. vom Bruch, M. Santandrea, R. Ricken, V. Quiring, C. Eigner, H. Herrmann, C. Silberhorn, Optics Express 31 (2023).","bibtex":"@article{Stefszky_vom Bruch_Santandrea_Ricken_Quiring_Eigner_Herrmann_Silberhorn_2023, title={Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications}, volume={31}, DOI={10.1364/oe.498423}, number={2134903}, journal={Optics Express}, publisher={Optica Publishing Group}, author={Stefszky, M. and vom Bruch, F. and Santandrea, M. and Ricken, R. and Quiring, V. and Eigner, C. and Herrmann, H and Silberhorn, C}, year={2023} }","ieee":"M. Stefszky et al., “Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications,” Optics Express, vol. 31, no. 21, Art. no. 34903, 2023, doi: 10.1364/oe.498423.","chicago":"Stefszky, M., F. vom Bruch, M. Santandrea, R. Ricken, V. Quiring, C. Eigner, H Herrmann, and C Silberhorn. “Lithium Niobate Waveguide Squeezer with Integrated Cavity Length Stabilisation for Network Applications.” Optics Express 31, no. 21 (2023). https://doi.org/10.1364/oe.498423.","ama":"Stefszky M, vom Bruch F, Santandrea M, et al. Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications. Optics Express. 2023;31(21). doi:10.1364/oe.498423"},"volume":31,"author":[{"first_name":"M.","full_name":"Stefszky, M.","last_name":"Stefszky"},{"first_name":"F.","full_name":"vom Bruch, F.","last_name":"vom Bruch"},{"full_name":"Santandrea, M.","last_name":"Santandrea","first_name":"M."},{"first_name":"R.","last_name":"Ricken","full_name":"Ricken, R."},{"full_name":"Quiring, V.","last_name":"Quiring","first_name":"V."},{"last_name":"Eigner","full_name":"Eigner, C.","first_name":"C."},{"first_name":"H","last_name":"Herrmann","full_name":"Herrmann, H"},{"last_name":"Silberhorn","full_name":"Silberhorn, C","first_name":"C"}],"date_updated":"2023-11-02T09:26:42Z","doi":"10.1364/oe.498423","type":"journal_article","status":"public","department":[{"_id":"288"},{"_id":"623"}],"user_id":"42777","_id":"48349","article_number":"34903"}]