--- _id: '51339' author: - first_name: Jonas full_name: Babai-Hemati, Jonas last_name: Babai-Hemati - first_name: Felix full_name: vom Bruch, Felix id: '71245' last_name: vom Bruch - first_name: Harald full_name: Herrmann, Harald id: '216' last_name: Herrmann - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn citation: ama: Babai-Hemati J, vom Bruch F, Herrmann H, Silberhorn C. Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters. Optics Express. Published online 2024. doi:10.1364/oe.510319 apa: Babai-Hemati, J., vom Bruch, F., Herrmann, H., & Silberhorn, C. (2024). Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters. Optics Express. https://doi.org/10.1364/oe.510319 bibtex: '@article{Babai-Hemati_vom Bruch_Herrmann_Silberhorn_2024, title={Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters}, DOI={10.1364/oe.510319}, journal={Optics Express}, publisher={Optica Publishing Group}, author={Babai-Hemati, Jonas and vom Bruch, Felix and Herrmann, Harald and Silberhorn, Christine}, year={2024} }' chicago: Babai-Hemati, Jonas, Felix vom Bruch, Harald Herrmann, and Christine Silberhorn. “Tailored Second Harmonic Generation InTi-Diffused PPLN Waveguides Usingmicro-Heaters.” Optics Express, 2024. https://doi.org/10.1364/oe.510319. ieee: 'J. Babai-Hemati, F. vom Bruch, H. Herrmann, and C. Silberhorn, “Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters,” Optics Express, 2024, doi: 10.1364/oe.510319.' mla: Babai-Hemati, Jonas, et al. “Tailored Second Harmonic Generation InTi-Diffused PPLN Waveguides Usingmicro-Heaters.” Optics Express, Optica Publishing Group, 2024, doi:10.1364/oe.510319. short: J. Babai-Hemati, F. vom Bruch, H. Herrmann, C. Silberhorn, Optics Express (2024). date_created: 2024-02-13T13:03:01Z date_updated: 2024-02-13T13:09:51Z department: - _id: '15' - _id: '623' - _id: '288' doi: 10.1364/oe.510319 keyword: - Atomic and Molecular Physics - and Optics language: - iso: eng project: - _id: '266' grant_number: PROFILNRW-2020-067 name: 'PhoQC: PhoQC: Photonisches Quantencomputing' publication: Optics Express publication_identifier: issn: - 1094-4087 publication_status: published publisher: Optica Publishing Group status: public title: Tailored second harmonic generation inTi-diffused PPLN waveguides usingmicro-heaters type: journal_article user_id: '216' year: '2024' ... --- _id: '54544' abstract: - lang: eng text: The biphoton correlation time, a measure for the conditional uncertainty in the temporal arrival of two photons from a photon pair source, is a key performance identifier for many quantum spectroscopy applications, with shorter correlation times typically yielding better performance. Furthermore, it provides fundamental insight into the effects of dispersion on the biphoton state. Here, we show that a characteristic dependence of the width of the temporal interferogram can be exploited to obtain insights into the amount of second-order dispersion inside the interferometer and to retrieve actual and Fourier-limited ultrashort biphoton correlation times of around 100 fs. In the presented scheme, we simultaneously measure spectral and temporal interferograms at the output of an SU(1,1) interferometer based on an integrated broadband parametric down conversion source in a Ti:LiNbO3 waveguide. article_number: '020350' author: - first_name: Franz full_name: Roeder, Franz id: '88149' last_name: Roeder - first_name: René full_name: Pollmann, René id: '78890' last_name: Pollmann - first_name: Michael full_name: Stefszky, Michael id: '42777' last_name: Stefszky - first_name: Matteo full_name: Santandrea, Matteo id: '55095' last_name: Santandrea orcid: 0000-0001-5718-358X - first_name: Kai Hong full_name: Luo, Kai Hong id: '36389' last_name: Luo orcid: 0000-0003-1008-4976 - first_name: V. full_name: Quiring, V. last_name: Quiring - first_name: Raimund full_name: Ricken, Raimund last_name: Ricken - first_name: Christof full_name: Eigner, Christof id: '13244' last_name: Eigner orcid: https://orcid.org/0000-0002-5693-3083 - first_name: Benjamin full_name: Brecht, Benjamin id: '27150' last_name: Brecht orcid: '0000-0003-4140-0556 ' - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn citation: ama: Roeder F, Pollmann R, Stefszky M, et al. Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer. PRX Quantum. 2024;5(2). doi:10.1103/prxquantum.5.020350 apa: Roeder, F., Pollmann, R., Stefszky, M., Santandrea, M., Luo, K. H., Quiring, V., Ricken, R., Eigner, C., Brecht, B., & Silberhorn, C. (2024). Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer. PRX Quantum, 5(2), Article 020350. https://doi.org/10.1103/prxquantum.5.020350 bibtex: '@article{Roeder_Pollmann_Stefszky_Santandrea_Luo_Quiring_Ricken_Eigner_Brecht_Silberhorn_2024, title={Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer}, volume={5}, DOI={10.1103/prxquantum.5.020350}, number={2020350}, journal={PRX Quantum}, publisher={American Physical Society (APS)}, author={Roeder, Franz and Pollmann, René and Stefszky, Michael and Santandrea, Matteo and Luo, Kai Hong and Quiring, V. and Ricken, Raimund and Eigner, Christof and Brecht, Benjamin and Silberhorn, Christine}, year={2024} }' chicago: Roeder, Franz, René Pollmann, Michael Stefszky, Matteo Santandrea, Kai Hong Luo, V. Quiring, Raimund Ricken, Christof Eigner, Benjamin Brecht, and Christine Silberhorn. “Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer.” PRX Quantum 5, no. 2 (2024). https://doi.org/10.1103/prxquantum.5.020350. ieee: 'F. Roeder et al., “Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer,” PRX Quantum, vol. 5, no. 2, Art. no. 020350, 2024, doi: 10.1103/prxquantum.5.020350.' mla: Roeder, Franz, et al. “Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer.” PRX Quantum, vol. 5, no. 2, 020350, American Physical Society (APS), 2024, doi:10.1103/prxquantum.5.020350. short: F. Roeder, R. Pollmann, M. Stefszky, M. Santandrea, K.H. Luo, V. Quiring, R. Ricken, C. Eigner, B. Brecht, C. Silberhorn, PRX Quantum 5 (2024). date_created: 2024-06-01T12:48:51Z date_updated: 2024-06-01T13:00:53Z department: - _id: '288' - _id: '623' doi: 10.1103/prxquantum.5.020350 intvolume: ' 5' issue: '2' language: - iso: eng project: - _id: '207' grant_number: 13N15065 name: 'MiLiQuant: Miniaturisierte Lichtquellen für den industriellen Einsatz in Quantensensoren und Quanten-Imaging-Systemen (MiLiQuant) - Teilvorhaben: Technologie und Theorie für MIR Quanten-Imaging Systeme' - _id: '571' grant_number: '101070700' name: 'MIRAQLS: MIRAQLS: Mid-infrared Quantum Technology for Sensing' - _id: '190' name: 'E2TPA: Exploiting Entangled Two-Photon Absorption' publication: PRX Quantum publication_identifier: issn: - 2691-3399 publication_status: published publisher: American Physical Society (APS) status: public title: Measurement of Ultrashort Biphoton Correlation Times with an Integrated Two-Color Broadband SU(1,1)-Interferometer type: journal_article user_id: '88149' volume: 5 year: '2024' ... --- _id: '54812' article_number: '240802' author: - first_name: Lisa T. full_name: Weinbrenner, Lisa T. last_name: Weinbrenner - first_name: Nidhin full_name: Prasannan, Nidhin id: '71403' last_name: Prasannan - first_name: Kiara full_name: Hansenne, Kiara last_name: Hansenne - first_name: Sophia full_name: Denker, Sophia last_name: Denker - first_name: Jan full_name: Sperling, Jan id: '75127' last_name: Sperling orcid: 0000-0002-5844-3205 - first_name: Benjamin full_name: Brecht, Benjamin id: '27150' last_name: Brecht orcid: '0000-0003-4140-0556 ' - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn - first_name: Otfried full_name: Gühne, Otfried last_name: Gühne citation: ama: 'Weinbrenner LT, Prasannan N, Hansenne K, et al. Certifying the Topology of Quantum Networks: Theory and Experiment. Physical Review Letters. 2024;132(24). doi:10.1103/physrevlett.132.240802' apa: 'Weinbrenner, L. T., Prasannan, N., Hansenne, K., Denker, S., Sperling, J., Brecht, B., Silberhorn, C., & Gühne, O. (2024). Certifying the Topology of Quantum Networks: Theory and Experiment. Physical Review Letters, 132(24), Article 240802. https://doi.org/10.1103/physrevlett.132.240802' bibtex: '@article{Weinbrenner_Prasannan_Hansenne_Denker_Sperling_Brecht_Silberhorn_Gühne_2024, title={Certifying the Topology of Quantum Networks: Theory and Experiment}, volume={132}, DOI={10.1103/physrevlett.132.240802}, number={24240802}, journal={Physical Review Letters}, publisher={American Physical Society (APS)}, author={Weinbrenner, Lisa T. and Prasannan, Nidhin and Hansenne, Kiara and Denker, Sophia and Sperling, Jan and Brecht, Benjamin and Silberhorn, Christine and Gühne, Otfried}, year={2024} }' chicago: 'Weinbrenner, Lisa T., Nidhin Prasannan, Kiara Hansenne, Sophia Denker, Jan Sperling, Benjamin Brecht, Christine Silberhorn, and Otfried Gühne. “Certifying the Topology of Quantum Networks: Theory and Experiment.” Physical Review Letters 132, no. 24 (2024). https://doi.org/10.1103/physrevlett.132.240802.' ieee: 'L. T. Weinbrenner et al., “Certifying the Topology of Quantum Networks: Theory and Experiment,” Physical Review Letters, vol. 132, no. 24, Art. no. 240802, 2024, doi: 10.1103/physrevlett.132.240802.' mla: 'Weinbrenner, Lisa T., et al. “Certifying the Topology of Quantum Networks: Theory and Experiment.” Physical Review Letters, vol. 132, no. 24, 240802, American Physical Society (APS), 2024, doi:10.1103/physrevlett.132.240802.' short: L.T. Weinbrenner, N. Prasannan, K. Hansenne, S. Denker, J. Sperling, B. Brecht, C. Silberhorn, O. Gühne, Physical Review Letters 132 (2024). date_created: 2024-06-19T06:36:54Z date_updated: 2024-06-19T06:59:45Z department: - _id: '15' - _id: '623' - _id: '288' doi: 10.1103/physrevlett.132.240802 intvolume: ' 132' issue: '24' language: - iso: eng publication: Physical Review Letters publication_identifier: issn: - 0031-9007 - 1079-7114 publication_status: published publisher: American Physical Society (APS) status: public title: 'Certifying the Topology of Quantum Networks: Theory and Experiment' type: journal_article user_id: '27150' volume: 132 year: '2024' ... --- _id: '54668' abstract: - lang: eng text: Samples of dielectric optical waveguides of rib or strip type in thin-film lithium niobate (TFLN) technology are characterized with respect to their optical loss using the Fabry-Pérot method. Attributing the losses mainly to sidewall roughness, we employ a simple perturbational procedure, based on rigorously computed mode profiles of idealized channels, to estimate the attenuation for waveguides with different cross sections. A single fit parameter suffices for an adequate modelling of the effect of the waveguide geometry on the loss levels. author: - first_name: Manfred full_name: Hammer, Manfred id: '48077' last_name: Hammer orcid: 0000-0002-6331-9348 - first_name: Silia full_name: Babel, Silia id: '63231' last_name: Babel orcid: https://orcid.org/0000-0002-1568-2580 - first_name: Henna full_name: Farheen, Henna id: '53444' last_name: Farheen orcid: 0000-0001-7730-3489 - first_name: Laura full_name: Padberg, Laura id: '40300' last_name: Padberg - first_name: J. Christoph full_name: Scheytt, J. Christoph id: '37144' last_name: Scheytt orcid: '0000-0002-5950-6618 ' - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn - first_name: Jens full_name: Förstner, Jens id: '158' last_name: Förstner orcid: 0000-0001-7059-9862 citation: ama: Hammer M, Babel S, Farheen H, et al. Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides. Optics Express. 2024;32(13):22878. doi:10.1364/oe.521766 apa: Hammer, M., Babel, S., Farheen, H., Padberg, L., Scheytt, J. C., Silberhorn, C., & Förstner, J. (2024). Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides. Optics Express, 32(13), 22878. https://doi.org/10.1364/oe.521766 bibtex: '@article{Hammer_Babel_Farheen_Padberg_Scheytt_Silberhorn_Förstner_2024, title={Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides}, volume={32}, DOI={10.1364/oe.521766}, number={13}, journal={Optics Express}, publisher={Optica Publishing Group}, author={Hammer, Manfred and Babel, Silia and Farheen, Henna and Padberg, Laura and Scheytt, J. Christoph and Silberhorn, Christine and Förstner, Jens}, year={2024}, pages={22878} }' chicago: 'Hammer, Manfred, Silia Babel, Henna Farheen, Laura Padberg, J. Christoph Scheytt, Christine Silberhorn, and Jens Förstner. “Estimation of Losses Caused by Sidewall Roughness in Thin-Film Lithium Niobate Rib and Strip Waveguides.” Optics Express 32, no. 13 (2024): 22878. https://doi.org/10.1364/oe.521766.' ieee: 'M. Hammer et al., “Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides,” Optics Express, vol. 32, no. 13, p. 22878, 2024, doi: 10.1364/oe.521766.' mla: Hammer, Manfred, et al. “Estimation of Losses Caused by Sidewall Roughness in Thin-Film Lithium Niobate Rib and Strip Waveguides.” Optics Express, vol. 32, no. 13, Optica Publishing Group, 2024, p. 22878, doi:10.1364/oe.521766. short: M. Hammer, S. Babel, H. Farheen, L. Padberg, J.C. Scheytt, C. Silberhorn, J. Förstner, Optics Express 32 (2024) 22878. date_created: 2024-06-10T11:18:06Z date_updated: 2024-07-22T07:43:02Z ddc: - '530' department: - _id: '61' - _id: '429' - _id: '623' - _id: '263' - _id: '288' doi: 10.1364/oe.521766 file: - access_level: open_access content_type: application/pdf creator: fossie date_created: 2024-06-10T11:25:00Z date_updated: 2024-06-10T11:25:00Z file_id: '54669' file_name: 2024-06 Hammer - Optics Express - Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides.pdf file_size: 4004782 relation: main_file file_date_updated: 2024-06-10T11:25:00Z has_accepted_license: '1' intvolume: ' 32' issue: '13' keyword: - tet_topic_waveguide language: - iso: eng oa: '1' page: '22878' project: - _id: '53' grant_number: '231447078' name: 'TRR 142: TRR 142 - Maßgeschneiderte nichtlineare Photonik: Von grundlegenden Konzepten zu funktionellen Strukturen' - _id: '175' grant_number: '231447078' name: 'TRR 142 - C11: TRR 142 - Kompakte Photonenpaar-Quelle mit ultraschnellen Modulatoren auf Basis von CMOS und LNOI (C11*)' - _id: '167' grant_number: '231447078' name: 'TRR 142 - B06: TRR 142 - Ultraschnelle kohärente opto-elektronische Kontrolle eines photonischen Quantensystems (B06*)' - _id: '266' grant_number: PROFILNRW-2020-067 name: 'PhoQC: PhoQC: Photonisches Quantencomputing' publication: Optics Express publication_identifier: issn: - 1094-4087 publication_status: published publisher: Optica Publishing Group status: public title: Estimation of losses caused by sidewall roughness in thin-film lithium niobate rib and strip waveguides type: journal_article user_id: '158' volume: 32 year: '2024' ... --- _id: '49652' abstract: - lang: eng text: Broadband coherent anti-Stokes Raman scattering (BCARS) is a powerful spectroscopy method combining high signal intensity with spectral sensitivity, enabling rapid imaging of heterogeneous samples in biomedical research and, more recently, in crystalline materials. However, BCARS encounters spectral distortion due to a setup-dependent non-resonant background (NRB). This study assesses BCARS reproducibility through a round robin experiment using two distinct BCARS setups and crystalline materials with varying structural complexity, including diamond, 6H-SiC, KDP, and KTP. The analysis compares setup-specific NRB correction procedures, detected and NRB-removed spectra, and mode assignment. We determine the influence of BCARS setup parameters like pump wavelength, pulse width, and detection geometry and provide a practical guide for optimizing BCARS setups for solid-state applications. article_number: '112' article_type: original author: - first_name: Franz full_name: Hempel, Franz last_name: Hempel - first_name: Federico full_name: Vernuccio, Federico last_name: Vernuccio - first_name: Lukas full_name: König, Lukas last_name: König - first_name: Robin full_name: Buschbeck, Robin last_name: Buschbeck - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Giulio full_name: Cerullo, Giulio last_name: Cerullo - first_name: Dario full_name: Polli, Dario last_name: Polli - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng citation: ama: 'Hempel F, Vernuccio F, König L, et al. Comparing transmission- and epi-BCARS: a round robin on solid-state materials. Applied Optics. 2024;63(1). doi:10.1364/ao.505374' apa: 'Hempel, F., Vernuccio, F., König, L., Buschbeck, R., Rüsing, M., Cerullo, G., Polli, D., & Eng, L. M. (2024). Comparing transmission- and epi-BCARS: a round robin on solid-state materials. Applied Optics, 63(1), Article 112. https://doi.org/10.1364/ao.505374' bibtex: '@article{Hempel_Vernuccio_König_Buschbeck_Rüsing_Cerullo_Polli_Eng_2024, title={Comparing transmission- and epi-BCARS: a round robin on solid-state materials}, volume={63}, DOI={10.1364/ao.505374}, number={1112}, journal={Applied Optics}, publisher={Optica Publishing Group}, author={Hempel, Franz and Vernuccio, Federico and König, Lukas and Buschbeck, Robin and Rüsing, Michael and Cerullo, Giulio and Polli, Dario and Eng, Lukas M.}, year={2024} }' chicago: 'Hempel, Franz, Federico Vernuccio, Lukas König, Robin Buschbeck, Michael Rüsing, Giulio Cerullo, Dario Polli, and Lukas M. Eng. “Comparing Transmission- and Epi-BCARS: A Round Robin on Solid-State Materials.” Applied Optics 63, no. 1 (2024). https://doi.org/10.1364/ao.505374.' ieee: 'F. Hempel et al., “Comparing transmission- and epi-BCARS: a round robin on solid-state materials,” Applied Optics, vol. 63, no. 1, Art. no. 112, 2024, doi: 10.1364/ao.505374.' mla: 'Hempel, Franz, et al. “Comparing Transmission- and Epi-BCARS: A Round Robin on Solid-State Materials.” Applied Optics, vol. 63, no. 1, 112, Optica Publishing Group, 2024, doi:10.1364/ao.505374.' short: F. Hempel, F. Vernuccio, L. König, R. Buschbeck, M. Rüsing, G. Cerullo, D. Polli, L.M. Eng, Applied Optics 63 (2024). date_created: 2023-12-15T07:32:38Z date_updated: 2025-04-03T12:36:01Z department: - _id: '15' - _id: '288' - _id: '623' doi: 10.1364/ao.505374 intvolume: ' 63' issue: '1' keyword: - Atomic and Molecular Physics - and Optics - Engineering (miscellaneous) - Electrical and Electronic Engineering language: - iso: eng main_file_link: - open_access: '1' url: https://arxiv.org/pdf/2306.09701.pdf oa: '1' publication: Applied Optics publication_identifier: issn: - 1559-128X - 2155-3165 publication_status: published publisher: Optica Publishing Group quality_controlled: '1' related_material: link: - relation: confirmation url: https://arxiv.org/abs/2306.09701 status: public title: 'Comparing transmission- and epi-BCARS: a round robin on solid-state materials' type: journal_article user_id: '22501' volume: 63 year: '2024' ... --- _id: '57028' abstract: - lang: eng text: Lithium niobate and lithium tantalate are among the most widespread materials for nonlinear, integrated photonics. Mixed crystals with arbitrary Nb–Ta ratios provide an additional degree of freedom to not only tune materials properties, such as the birefringence but also leverage the advantages of the singular compounds, for example, by combining the thermal stability of lithium tantalate with the larger nonlinear or piezoelectric constants of lithium niobate. Periodic poling allows to achieve phase-matching independent of waveguide geometry and is, therefore, one of the commonly used methods in integrated nonlinear optics. For mixed crystals, periodic poling has been challenging so far due to the lack of homogeneous, mono-domain crystals, which severely inhibit domain growth and nucleation. In this work, we investigate surface-near (<1μm depth) domain inversion on x-cut lithium niobate tantalate mixed crystals via electric field poling and lithographically structured electrodes. We find that naturally occurring head-to-head or tail-to-tail domain walls in the as-grown crystal inhibit domain inversion at a larger scale. However, periodic poling is possible if the gap size between the poling electrodes is of the same order of magnitude or smaller than the average size of naturally occurring domains. This work provides the basis for the nonlinear optical application of lithium niobate tantalate mixed crystals. author: - first_name: Laura full_name: Bollmers, Laura id: '61375' last_name: Bollmers - first_name: Tobias full_name: Babai-Hemati, Tobias last_name: Babai-Hemati - first_name: Boris full_name: Koppitz, Boris last_name: Koppitz - first_name: Christof full_name: Eigner, Christof id: '13244' last_name: Eigner orcid: https://orcid.org/0000-0002-5693-3083 - first_name: Laura full_name: Padberg, Laura id: '40300' last_name: Padberg - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn citation: ama: Bollmers L, Babai-Hemati T, Koppitz B, et al. Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals. Applied Physics Letters. 2024;125(15). doi:10.1063/5.0210972 apa: Bollmers, L., Babai-Hemati, T., Koppitz, B., Eigner, C., Padberg, L., Rüsing, M., Eng, L. M., & Silberhorn, C. (2024). Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals. Applied Physics Letters, 125(15). https://doi.org/10.1063/5.0210972 bibtex: '@article{Bollmers_Babai-Hemati_Koppitz_Eigner_Padberg_Rüsing_Eng_Silberhorn_2024, title={Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals}, volume={125}, DOI={10.1063/5.0210972}, number={15}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Bollmers, Laura and Babai-Hemati, Tobias and Koppitz, Boris and Eigner, Christof and Padberg, Laura and Rüsing, Michael and Eng, Lukas M. and Silberhorn, Christine}, year={2024} }' chicago: Bollmers, Laura, Tobias Babai-Hemati, Boris Koppitz, Christof Eigner, Laura Padberg, Michael Rüsing, Lukas M. Eng, and Christine Silberhorn. “Surface-near Domain Engineering in Multi-Domain x-Cut Lithium Niobate Tantalate Mixed Crystals.” Applied Physics Letters 125, no. 15 (2024). https://doi.org/10.1063/5.0210972. ieee: 'L. Bollmers et al., “Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals,” Applied Physics Letters, vol. 125, no. 15, 2024, doi: 10.1063/5.0210972.' mla: Bollmers, Laura, et al. “Surface-near Domain Engineering in Multi-Domain x-Cut Lithium Niobate Tantalate Mixed Crystals.” Applied Physics Letters, vol. 125, no. 15, AIP Publishing, 2024, doi:10.1063/5.0210972. short: L. Bollmers, T. Babai-Hemati, B. Koppitz, C. Eigner, L. Padberg, M. Rüsing, L.M. Eng, C. Silberhorn, Applied Physics Letters 125 (2024). date_created: 2024-11-13T08:06:59Z date_updated: 2024-11-15T09:15:08Z department: - _id: '15' - _id: '623' - _id: '230' - _id: '288' doi: 10.1063/5.0210972 intvolume: ' 125' issue: '15' language: - iso: eng project: - _id: '168' grant_number: '231447078' name: 'TRR 142 - B07: TRR 142 - Polaronen-Einfluss auf die optischen Eigenschaften von Lithiumniobat (B07*)' publication: Applied Physics Letters publication_identifier: issn: - 0003-6951 - 1077-3118 publication_status: published publisher: AIP Publishing status: public title: Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals type: journal_article user_id: '61375' volume: 125 year: '2024' ... --- _id: '59269' abstract: - lang: eng text: Ferroelectric materials play a crucial role in a broad range of technologies due to their unique properties that are deeply connected to the pattern and behavior of their ferroelectric (FE) domains. Chief among them, barium titanate (BaTiO3; BTO) sees widespread applications such as in electronics but equally is a ferroelectric model system for fundamental research, e.g., to study the interplay of such FE domains, the domain walls (DWs), and their macroscopic properties, owed to BTO’s multiple and experimentally accessible phase transitions. Here, we employ Second Harmonic Generation Microscopy (SHGM) to in situ investigate the cubic-to-tetragonal (at ∼126°C) and the tetragonal-to-orthorhombic (at ∼5°C) phase transition in single-crystalline BTO via three-dimensional (3D) DW mapping. We demonstrate that SHGM imaging provides the direct visualization of FE domain switching as well as the domain dynamics in 3D, shedding light on the interplay of the domain structure and phase transition. These results allow us to extract the different transition temperatures locally, to unveil the hysteresis behavior, and to determine the type of phase transition at play (first/second order) from the recorded SHGM data. The capabilities of SHGM in uncovering these crucial phenomena can easily be applied to other ferroelectrics to provide new possibilities for in situ engineering of advanced ferroic devices. article_number: '154102' article_type: original author: - first_name: Benjamin full_name: Kirbus, Benjamin last_name: Kirbus - first_name: Samuel D. full_name: Seddon, Samuel D. last_name: Seddon - first_name: Iuliia full_name: Kiseleva, Iuliia last_name: Kiseleva - first_name: Elke full_name: Beyreuther, Elke last_name: Beyreuther - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng citation: ama: Kirbus B, Seddon SD, Kiseleva I, Beyreuther E, Rüsing M, Eng LM. Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy. Journal of Applied Physics. 2024;136(15). doi:10.1063/5.0237769 apa: Kirbus, B., Seddon, S. D., Kiseleva, I., Beyreuther, E., Rüsing, M., & Eng, L. M. (2024). Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy. Journal of Applied Physics, 136(15), Article 154102. https://doi.org/10.1063/5.0237769 bibtex: '@article{Kirbus_Seddon_Kiseleva_Beyreuther_Rüsing_Eng_2024, title={Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy}, volume={136}, DOI={10.1063/5.0237769}, number={15154102}, journal={Journal of Applied Physics}, publisher={AIP Publishing}, author={Kirbus, Benjamin and Seddon, Samuel D. and Kiseleva, Iuliia and Beyreuther, Elke and Rüsing, Michael and Eng, Lukas M.}, year={2024} }' chicago: Kirbus, Benjamin, Samuel D. Seddon, Iuliia Kiseleva, Elke Beyreuther, Michael Rüsing, and Lukas M. Eng. “Probing Ferroelectric Phase Transitions in Barium Titanate Single Crystals via In-Situ Second Harmonic Generation Microscopy.” Journal of Applied Physics 136, no. 15 (2024). https://doi.org/10.1063/5.0237769. ieee: 'B. Kirbus, S. D. Seddon, I. Kiseleva, E. Beyreuther, M. Rüsing, and L. M. Eng, “Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy,” Journal of Applied Physics, vol. 136, no. 15, Art. no. 154102, 2024, doi: 10.1063/5.0237769.' mla: Kirbus, Benjamin, et al. “Probing Ferroelectric Phase Transitions in Barium Titanate Single Crystals via In-Situ Second Harmonic Generation Microscopy.” Journal of Applied Physics, vol. 136, no. 15, 154102, AIP Publishing, 2024, doi:10.1063/5.0237769. short: B. Kirbus, S.D. Seddon, I. Kiseleva, E. Beyreuther, M. Rüsing, L.M. Eng, Journal of Applied Physics 136 (2024). date_created: 2025-04-02T15:57:11Z date_updated: 2025-04-02T15:59:55Z department: - _id: '15' - _id: '623' - _id: '288' doi: 10.1063/5.0237769 intvolume: ' 136' issue: '15' language: - iso: eng main_file_link: - open_access: '1' url: ' https://doi.org/10.1063/5.0237769' oa: '1' publication: Journal of Applied Physics publication_identifier: issn: - 0021-8979 - 1089-7550 publication_status: published publisher: AIP Publishing quality_controlled: '1' status: public title: Probing ferroelectric phase transitions in barium titanate single crystals via in-situ second harmonic generation microscopy type: journal_article user_id: '22501' volume: 136 year: '2024' ... --- _id: '59271' abstract: - lang: eng text: Lithium niobate (LNO) and lithium tantalate (LTO) see widespread use in fundamental research and commercial technologies reaching from electronics over classical optics to integrated quantum communication. The mixed crystal system lithium niobate tantalate (LNT) allows for the dedicate engineering of material properties by combining the advantages of the two parental materials LNO and LTO. Vibrational spectroscopies such as Raman spectroscopy or (Fourier transform) infrared (IR) spectroscopy are vital techniques to provide detailed insight into the material properties, which is central to the analysis and optimization of devices. This work presents a joint experimental–theoretical approach allowing to unambiguously assign the spectral features in the LNT material family through both Raman and IR spectroscopy, as well as providing an in‐depth explanation for the observed scattering efficiencies based on first‐principles calculations. The phononic contribution to the static dielectric tensor is calculated from the experimental and theoretical data using the generalized Lyddane–Sachs–Teller relation and compared with the results of the first‐principles calculations. author: - first_name: Felix full_name: Bernhardt, Felix last_name: Bernhardt - first_name: Soham full_name: Gharat, Soham last_name: Gharat - first_name: Alexander full_name: Kapp, Alexander last_name: Kapp - first_name: Florian full_name: Pfeiffer, Florian last_name: Pfeiffer - first_name: Robin full_name: Buschbeck, Robin last_name: Buschbeck - first_name: Franz full_name: Hempel, Franz last_name: Hempel - first_name: Oleksiy full_name: Pashkin, Oleksiy last_name: Pashkin - first_name: Susanne C. full_name: Kehr, Susanne C. last_name: Kehr - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Simone full_name: Sanna, Simone last_name: Sanna - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng citation: ama: 'Bernhardt F, Gharat S, Kapp A, et al. Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment. physica status solidi (a). 2024;222(1):2300968. doi:10.1002/pssa.202300968' apa: 'Bernhardt, F., Gharat, S., Kapp, A., Pfeiffer, F., Buschbeck, R., Hempel, F., Pashkin, O., Kehr, S. C., Rüsing, M., Sanna, S., & Eng, L. M. (2024). Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment. Physica Status Solidi (a), 222(1), 2300968. https://doi.org/10.1002/pssa.202300968' bibtex: '@article{Bernhardt_Gharat_Kapp_Pfeiffer_Buschbeck_Hempel_Pashkin_Kehr_Rüsing_Sanna_et al._2024, title={Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment}, volume={222}, DOI={10.1002/pssa.202300968}, number={1}, journal={physica status solidi (a)}, publisher={Wiley}, author={Bernhardt, Felix and Gharat, Soham and Kapp, Alexander and Pfeiffer, Florian and Buschbeck, Robin and Hempel, Franz and Pashkin, Oleksiy and Kehr, Susanne C. and Rüsing, Michael and Sanna, Simone and et al.}, year={2024}, pages={2300968} }' chicago: 'Bernhardt, Felix, Soham Gharat, Alexander Kapp, Florian Pfeiffer, Robin Buschbeck, Franz Hempel, Oleksiy Pashkin, et al. “Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment.” Physica Status Solidi (a) 222, no. 1 (2024): 2300968. https://doi.org/10.1002/pssa.202300968.' ieee: 'F. Bernhardt et al., “Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment,” physica status solidi (a), vol. 222, no. 1, p. 2300968, 2024, doi: 10.1002/pssa.202300968.' mla: 'Bernhardt, Felix, et al. “Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment.” Physica Status Solidi (a), vol. 222, no. 1, Wiley, 2024, p. 2300968, doi:10.1002/pssa.202300968.' short: F. Bernhardt, S. Gharat, A. Kapp, F. Pfeiffer, R. Buschbeck, F. Hempel, O. Pashkin, S.C. Kehr, M. Rüsing, S. Sanna, L.M. Eng, Physica Status Solidi (a) 222 (2024) 2300968. date_created: 2025-04-02T16:04:58Z date_updated: 2025-04-02T16:07:19Z department: - _id: '15' - _id: '623' - _id: '288' doi: 10.1002/pssa.202300968 intvolume: ' 222' issue: '1' language: - iso: eng main_file_link: - open_access: '1' url: https://doi.org/10.1002/pssa.202300968 oa: '1' page: '2300968' publication: physica status solidi (a) publication_identifier: issn: - 1862-6300 - 1862-6319 publication_status: published publisher: Wiley status: public title: 'Lattice Dynamics of LiNb(1–x)Ta(x)O3 Solid Solutions: Theory and Experiment' type: journal_article user_id: '22501' volume: 222 year: '2024' ... --- _id: '59270' abstract: - lang: eng text: Lithium niobate tantalate (LiNb1−xTaxO3, LNT) solid solutions offer exciting new possibilities for applications ranging from optics, piezotronics, and electronics beyond the capabilities of the widely used singular compounds of lithium niobate (LiNbO3, LN) or lithium tantalate (LiTaO3, LT). Crystal growth of homogeneous LNT single crystals by the Czochralski method is still challenging. One key aspect of homogeneous growth is the accurate knowledge of thermal conductivity through the crystal boule during the growth, which is central to control the crystal growth. Therefore, the temperature dependent thermal conductivity of pure LN, LT, and LNT solid solutions, as well as of selected doped LN and LT crystals (Mg, Zn) was investigated across the temperature range from 300 to 1300 K. The results that span across the whole composition range can directly be applied for optimizing growth conditions of both LNT solid solutions as well as doped and undoped LN and LT crystals. article_number: '176549' article_type: original author: - first_name: Umar full_name: Bashir, Umar last_name: Bashir - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Detlef full_name: Klimm, Detlef last_name: Klimm - first_name: Roberts full_name: Blukis, Roberts last_name: Blukis - first_name: Boris full_name: Koppitz, Boris last_name: Koppitz - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng - first_name: Matthias full_name: Bickermann, Matthias last_name: Bickermann - first_name: Steffen full_name: Ganschow, Steffen last_name: Ganschow citation: ama: Bashir U, Rüsing M, Klimm D, et al. Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K. Journal of Alloys and Compounds. 2024;1008. doi:10.1016/j.jallcom.2024.176549 apa: Bashir, U., Rüsing, M., Klimm, D., Blukis, R., Koppitz, B., Eng, L. M., Bickermann, M., & Ganschow, S. (2024). Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K. Journal of Alloys and Compounds, 1008, Article 176549. https://doi.org/10.1016/j.jallcom.2024.176549 bibtex: '@article{Bashir_Rüsing_Klimm_Blukis_Koppitz_Eng_Bickermann_Ganschow_2024, title={Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K}, volume={1008}, DOI={10.1016/j.jallcom.2024.176549}, number={176549}, journal={Journal of Alloys and Compounds}, publisher={Elsevier BV}, author={Bashir, Umar and Rüsing, Michael and Klimm, Detlef and Blukis, Roberts and Koppitz, Boris and Eng, Lukas M. and Bickermann, Matthias and Ganschow, Steffen}, year={2024} }' chicago: Bashir, Umar, Michael Rüsing, Detlef Klimm, Roberts Blukis, Boris Koppitz, Lukas M. Eng, Matthias Bickermann, and Steffen Ganschow. “Thermal Conductivity in Solid Solutions of Lithium Niobate Tantalate Single Crystals from 300 K up to 1300 K.” Journal of Alloys and Compounds 1008 (2024). https://doi.org/10.1016/j.jallcom.2024.176549. ieee: 'U. Bashir et al., “Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K,” Journal of Alloys and Compounds, vol. 1008, Art. no. 176549, 2024, doi: 10.1016/j.jallcom.2024.176549.' mla: Bashir, Umar, et al. “Thermal Conductivity in Solid Solutions of Lithium Niobate Tantalate Single Crystals from 300 K up to 1300 K.” Journal of Alloys and Compounds, vol. 1008, 176549, Elsevier BV, 2024, doi:10.1016/j.jallcom.2024.176549. short: U. Bashir, M. Rüsing, D. Klimm, R. Blukis, B. Koppitz, L.M. Eng, M. Bickermann, S. Ganschow, Journal of Alloys and Compounds 1008 (2024). date_created: 2025-04-02T16:00:56Z date_updated: 2025-04-02T16:02:26Z department: - _id: '15' - _id: '288' - _id: '623' doi: 10.1016/j.jallcom.2024.176549 intvolume: ' 1008' language: - iso: eng publication: Journal of Alloys and Compounds publication_identifier: issn: - 0925-8388 publication_status: published publisher: Elsevier BV quality_controlled: '1' status: public title: Thermal conductivity in solid solutions of lithium niobate tantalate single crystals from 300 K up to 1300 K type: journal_article user_id: '22501' volume: 1008 year: '2024' ... --- _id: '59272' abstract: - lang: eng text: 'Ferroelectrics such as LiNbO3 (LN) are wide-band-gap insulators that may show a high local electric conductivity at the domain walls (DWs). The latter are interfaces separating regions of noncollinear polarization, which can be manipulated to build integrated nanoelectronic elements. In the present work, we model different DW types in LN from first principles. Our models reveal the DW morphology and shed light on their electronic properties: A strong band bending is predicted for charged DWs, leading to local metallicity. Defect trapping at the DW may further enhance the electric conductivity.' article_number: L042015 author: - first_name: Leonard M. full_name: Verhoff, Leonard M. last_name: Verhoff - first_name: Mike N. full_name: Pionteck, Mike N. last_name: Pionteck - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Holger full_name: Fritze, Holger last_name: Fritze - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng - first_name: Simone full_name: Sanna, Simone last_name: Sanna citation: ama: 'Verhoff LM, Pionteck MN, Rüsing M, Fritze H, Eng LM, Sanna S. Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls. Physical Review Research. 2024;6(4). doi:10.1103/physrevresearch.6.l042015' apa: 'Verhoff, L. M., Pionteck, M. N., Rüsing, M., Fritze, H., Eng, L. M., & Sanna, S. (2024). Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls. Physical Review Research, 6(4), Article L042015. https://doi.org/10.1103/physrevresearch.6.l042015' bibtex: '@article{Verhoff_Pionteck_Rüsing_Fritze_Eng_Sanna_2024, title={Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls}, volume={6}, DOI={10.1103/physrevresearch.6.l042015}, number={4L042015}, journal={Physical Review Research}, publisher={American Physical Society (APS)}, author={Verhoff, Leonard M. and Pionteck, Mike N. and Rüsing, Michael and Fritze, Holger and Eng, Lukas M. and Sanna, Simone}, year={2024} }' chicago: 'Verhoff, Leonard M., Mike N. Pionteck, Michael Rüsing, Holger Fritze, Lukas M. Eng, and Simone Sanna. “Two-Dimensional Electronic Conductivity in Insulating Ferroelectrics: Peculiar Properties of Domain Walls.” Physical Review Research 6, no. 4 (2024). https://doi.org/10.1103/physrevresearch.6.l042015.' ieee: 'L. M. Verhoff, M. N. Pionteck, M. Rüsing, H. Fritze, L. M. Eng, and S. Sanna, “Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls,” Physical Review Research, vol. 6, no. 4, Art. no. L042015, 2024, doi: 10.1103/physrevresearch.6.l042015.' mla: 'Verhoff, Leonard M., et al. “Two-Dimensional Electronic Conductivity in Insulating Ferroelectrics: Peculiar Properties of Domain Walls.” Physical Review Research, vol. 6, no. 4, L042015, American Physical Society (APS), 2024, doi:10.1103/physrevresearch.6.l042015.' short: L.M. Verhoff, M.N. Pionteck, M. Rüsing, H. Fritze, L.M. Eng, S. Sanna, Physical Review Research 6 (2024). date_created: 2025-04-02T16:08:55Z date_updated: 2025-04-02T16:10:59Z department: - _id: '623' - _id: '288' - _id: '15' doi: 10.1103/physrevresearch.6.l042015 intvolume: ' 6' issue: '4' language: - iso: eng main_file_link: - url: https://jlupub.ub.uni-giessen.de/server/api/core/bitstreams/fb2b09e6-c0f8-4209-99a1-79fc81d9b1f9/content publication: Physical Review Research publication_identifier: issn: - 2643-1564 publication_status: published publisher: American Physical Society (APS) status: public title: 'Two-dimensional electronic conductivity in insulating ferroelectrics: Peculiar properties of domain walls' type: journal_article user_id: '22501' volume: 6 year: '2024' ... --- _id: '59273' abstract: - lang: eng text: Ferroelectric domain walls (DWs) are promising structures for assembling future nano-electronic circuit elements on a larger scale since reporting domain wall currents of up to 1 mA per single DW. One key requirement hereto is their reproducible manufacturing by gaining preparative control over domain size and domain wall conductivity (DWC). To date, most works on DWC have focused on exploring the fundamental electrical properties of individual DWs within single-shot experiments, with an emphasis on quantifying the origins of DWC. Very few reports exist when it comes to comparing the DWC properties between two separate DWs, and literally nothing exists where issues of reproducibility in DWC devices have been addressed. To fill this gap while facing the challenge of finding guidelines for achieving predictable DWC performance, we report on a procedure that allows us to reproducibly prepare single hexagonal domains of a predefined diameter into uniaxial ferroelectric lithium niobate single crystals of 200 and 300 μm thickness, respectively. We show that the domain diameter can be controlled with an uncertainty of a few percent. As-grown DWs are then subjected to a standard procedure of current-limited high-voltage DWC enhancement, and they repetitively reach a DWC increase of six orders of magnitude. While all resulting DWs show significantly enhanced DWC values, their individual current–voltage (I–V) characteristics exhibit different shapes, which can be explained by variations in their 3D real structure reflecting local heterogeneities by defects, DW pinning, and surface-near DW inclination. article_type: original author: - first_name: Julius full_name: Ratzenberger, Julius last_name: Ratzenberger - first_name: Iuliia full_name: Kiseleva, Iuliia last_name: Kiseleva - first_name: Boris full_name: Koppitz, Boris last_name: Koppitz - first_name: Elke full_name: Beyreuther, Elke last_name: Beyreuther - first_name: Manuel full_name: Zahn, Manuel last_name: Zahn - first_name: Joshua full_name: Gössel, Joshua last_name: Gössel - first_name: Peter A. full_name: Hegarty, Peter A. last_name: Hegarty - first_name: Zeeshan H. full_name: Amber, Zeeshan H. last_name: Amber - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng citation: ama: Ratzenberger J, Kiseleva I, Koppitz B, et al. Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals. Journal of Applied Physics. 2024;136(10):104302. doi:10.1063/5.0219300 apa: Ratzenberger, J., Kiseleva, I., Koppitz, B., Beyreuther, E., Zahn, M., Gössel, J., Hegarty, P. A., Amber, Z. H., Rüsing, M., & Eng, L. M. (2024). Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals. Journal of Applied Physics, 136(10), 104302. https://doi.org/10.1063/5.0219300 bibtex: '@article{Ratzenberger_Kiseleva_Koppitz_Beyreuther_Zahn_Gössel_Hegarty_Amber_Rüsing_Eng_2024, title={Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals}, volume={136}, DOI={10.1063/5.0219300}, number={10}, journal={Journal of Applied Physics}, publisher={AIP Publishing}, author={Ratzenberger, Julius and Kiseleva, Iuliia and Koppitz, Boris and Beyreuther, Elke and Zahn, Manuel and Gössel, Joshua and Hegarty, Peter A. and Amber, Zeeshan H. and Rüsing, Michael and Eng, Lukas M.}, year={2024}, pages={104302} }' chicago: 'Ratzenberger, Julius, Iuliia Kiseleva, Boris Koppitz, Elke Beyreuther, Manuel Zahn, Joshua Gössel, Peter A. Hegarty, Zeeshan H. Amber, Michael Rüsing, and Lukas M. Eng. “Toward the Reproducible Fabrication of Conductive Ferroelectric Domain Walls into Lithium Niobate Bulk Single Crystals.” Journal of Applied Physics 136, no. 10 (2024): 104302. https://doi.org/10.1063/5.0219300.' ieee: 'J. Ratzenberger et al., “Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals,” Journal of Applied Physics, vol. 136, no. 10, p. 104302, 2024, doi: 10.1063/5.0219300.' mla: Ratzenberger, Julius, et al. “Toward the Reproducible Fabrication of Conductive Ferroelectric Domain Walls into Lithium Niobate Bulk Single Crystals.” Journal of Applied Physics, vol. 136, no. 10, AIP Publishing, 2024, p. 104302, doi:10.1063/5.0219300. short: J. Ratzenberger, I. Kiseleva, B. Koppitz, E. Beyreuther, M. Zahn, J. Gössel, P.A. Hegarty, Z.H. Amber, M. Rüsing, L.M. Eng, Journal of Applied Physics 136 (2024) 104302. date_created: 2025-04-02T16:12:29Z date_updated: 2025-04-02T16:14:31Z department: - _id: '288' - _id: '15' - _id: '623' doi: 10.1063/5.0219300 intvolume: ' 136' issue: '10' language: - iso: eng main_file_link: - open_access: '1' url: ' https://doi.org/10.1063/5.0219300' oa: '1' page: '104302' publication: Journal of Applied Physics publication_identifier: issn: - 0021-8979 - 1089-7550 publication_status: published publisher: AIP Publishing quality_controlled: '1' status: public title: Toward the reproducible fabrication of conductive ferroelectric domain walls into lithium niobate bulk single crystals type: journal_article user_id: '22501' volume: 136 year: '2024' ... --- _id: '59274' abstract: - lang: eng text: 'Recently, ion exchange (IE) has been used to periodically modify the coercive field (Ec) of the crystal prior to periodic poling, to fabricate fine-pitch domain structures in Rb-doped KTiOPO4 (RKTP). Here, we use micro-Raman spectroscopy to understand the impact of IE on the vibrational modes related to the Rb/K lattice sites, TiO octahedra, and PO4 tetrahedra, which all form the basis of the RKTP crystal structure. We analyze the Raman spectra of three different RKTP samples: (1) a RKTP sample that shows a poled domain grating only, (2) a RKTP sample that has an Ec grating only, and (3) a RKTP sample that has both an Ec and a domain grating of the nominally same spacing. This allows us to determine the impact of IE on the vibrational modes of RKTP. We characterize the changes in the lower Raman peaks related to the alkali-metal ions, as well as observe lattice modifications induced by the incorporation of Rb+ that extend further into the crystal bulk than the expected IE depth. Moreover, the influence of IE on the domain walls is also manifested in their Raman peak shift. We discuss our results in terms of the deformation of the PO4and TiO groups. Our results highlight the intricate impact of IE on the crystal structure and how it facilitates periodic poling, paving the way for further development of the Ec-engineering technique.' article_number: '214115' article_type: original author: - first_name: Cherrie S. J. full_name: Lee, Cherrie S. J. last_name: Lee - first_name: Carlota full_name: Canalias, Carlota last_name: Canalias - first_name: Robin full_name: Buschbeck, Robin last_name: Buschbeck - first_name: Boris full_name: Koppitz, Boris last_name: Koppitz - first_name: Franz full_name: Hempel, Franz last_name: Hempel - first_name: Zeeshan full_name: Amber, Zeeshan last_name: Amber - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 citation: ama: 'Lee CSJ, Canalias C, Buschbeck R, et al. Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching. Physical Review B. 2024;110(21). doi:10.1103/physrevb.110.214115' apa: 'Lee, C. S. J., Canalias, C., Buschbeck, R., Koppitz, B., Hempel, F., Amber, Z., Eng, L. M., & Rüsing, M. (2024). Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching. Physical Review B, 110(21), Article 214115. https://doi.org/10.1103/physrevb.110.214115' bibtex: '@article{Lee_Canalias_Buschbeck_Koppitz_Hempel_Amber_Eng_Rüsing_2024, title={Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching}, volume={110}, DOI={10.1103/physrevb.110.214115}, number={21214115}, journal={Physical Review B}, publisher={American Physical Society (APS)}, author={Lee, Cherrie S. J. and Canalias, Carlota and Buschbeck, Robin and Koppitz, Boris and Hempel, Franz and Amber, Zeeshan and Eng, Lukas M. and Rüsing, Michael}, year={2024} }' chicago: 'Lee, Cherrie S. J., Carlota Canalias, Robin Buschbeck, Boris Koppitz, Franz Hempel, Zeeshan Amber, Lukas M. Eng, and Michael Rüsing. “Impact of Ion Exchange on Vibrational Modes in Rb-Doped KTiOPO4: A Raman Spectroscopy Study on the Interplay between Ion Exchange and Polarization Switching.” Physical Review B 110, no. 21 (2024). https://doi.org/10.1103/physrevb.110.214115.' ieee: 'C. S. J. Lee et al., “Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching,” Physical Review B, vol. 110, no. 21, Art. no. 214115, 2024, doi: 10.1103/physrevb.110.214115.' mla: 'Lee, Cherrie S. J., et al. “Impact of Ion Exchange on Vibrational Modes in Rb-Doped KTiOPO4: A Raman Spectroscopy Study on the Interplay between Ion Exchange and Polarization Switching.” Physical Review B, vol. 110, no. 21, 214115, American Physical Society (APS), 2024, doi:10.1103/physrevb.110.214115.' short: C.S.J. Lee, C. Canalias, R. Buschbeck, B. Koppitz, F. Hempel, Z. Amber, L.M. Eng, M. Rüsing, Physical Review B 110 (2024). date_created: 2025-04-02T16:14:44Z date_updated: 2025-04-02T16:18:34Z department: - _id: '288' - _id: '15' - _id: '623' doi: 10.1103/physrevb.110.214115 intvolume: ' 110' issue: '21' language: - iso: eng publication: Physical Review B publication_identifier: issn: - 2469-9950 - 2469-9969 publication_status: published publisher: American Physical Society (APS) status: public title: 'Impact of ion exchange on vibrational modes in Rb-doped KTiOPO4: A Raman spectroscopy study on the interplay between ion exchange and polarization switching' type: journal_article user_id: '22501' volume: 110 year: '2024' ... --- _id: '59275' abstract: - lang: eng text: Studying and understanding many‐body interactions, particularly electron‐boson interactions, is essential for a deeper elucidation of fundamental physical phenomena and the development of novel material functionalities. Here, this aspect is explored in the weak itinerant ferromagnet LaCo2P2 by means of momentum‐resolved photoelectron spectroscopy (ARPES) and first‐principles calculations. The detailed ARPES patterns enable to unveil bulk and surface bands, spin splittings due to Rashba and exchange interactions, as well as the evolution of bands with temperature, which altogether creates a solid foundation for theoretical studies. The latter has allowed to establish the impact of electron‐boson interactions on the electronic structure, that are reflected in its strong renormalization driven by electron‐magnon interaction and the emergence of distinctive kinks of surface and bulk electron bands due to significant electron‐phonon coupling. Our results highlight the distinct impact of electron‐boson interactions on the electronic structure, particularly on the itinerant d states. Similar electronic states are observed in the isostructural iron pnictides, where electron‐boson interactions play a crucial role in the emergence of superconductivity. It is believed that further studies of material systems involving both magnetically active d‐ and f‐sublattices will reveal more advanced phenomena in the bulk and at distinct surfaces, driven by a combination of factors including Rashba and Kondo effects, exchange magnetism, and electron‐boson interactions. author: - first_name: D. Yu. full_name: Usachov, D. Yu. last_name: Usachov - first_name: K. full_name: Ali, K. last_name: Ali - first_name: G. full_name: Poelchen, G. last_name: Poelchen - first_name: M. full_name: Mende, M. last_name: Mende - first_name: S. full_name: Schulz, S. last_name: Schulz - first_name: M. full_name: Peters, M. last_name: Peters - first_name: K. full_name: Bokai, K. last_name: Bokai - first_name: I. Yu. full_name: Sklyadneva, I. Yu. last_name: Sklyadneva - first_name: V. full_name: Stolyarov, V. last_name: Stolyarov - first_name: E. V. full_name: Chulkov, E. V. last_name: Chulkov - first_name: K. full_name: Kliemt, K. last_name: Kliemt - first_name: S. full_name: Paischer, S. last_name: Paischer - first_name: P. A. full_name: Buczek, P. A. last_name: Buczek - first_name: R. full_name: Heid, R. last_name: Heid - first_name: F. full_name: Hempel, F. last_name: Hempel - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: A. full_name: Ernst, A. last_name: Ernst - first_name: C. full_name: Krellner, C. last_name: Krellner - first_name: S. V. full_name: Eremeev, S. V. last_name: Eremeev - first_name: D. V. full_name: Vyalikh, D. V. last_name: Vyalikh citation: ama: Usachov DYu, Ali K, Poelchen G, et al. Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2. Advanced Physics Research. Published online 2024. doi:10.1002/apxr.202400137 apa: Usachov, D. Yu., Ali, K., Poelchen, G., Mende, M., Schulz, S., Peters, M., Bokai, K., Sklyadneva, I. Yu., Stolyarov, V., Chulkov, E. V., Kliemt, K., Paischer, S., Buczek, P. A., Heid, R., Hempel, F., Rüsing, M., Ernst, A., Krellner, C., Eremeev, S. V., & Vyalikh, D. V. (2024). Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2. Advanced Physics Research. https://doi.org/10.1002/apxr.202400137 bibtex: '@article{Usachov_Ali_Poelchen_Mende_Schulz_Peters_Bokai_Sklyadneva_Stolyarov_Chulkov_et al._2024, title={Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2}, DOI={10.1002/apxr.202400137}, journal={Advanced Physics Research}, publisher={Wiley}, author={Usachov, D. Yu. and Ali, K. and Poelchen, G. and Mende, M. and Schulz, S. and Peters, M. and Bokai, K. and Sklyadneva, I. Yu. and Stolyarov, V. and Chulkov, E. V. and et al.}, year={2024} }' chicago: Usachov, D. Yu., K. Ali, G. Poelchen, M. Mende, S. Schulz, M. Peters, K. Bokai, et al. “Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2.” Advanced Physics Research, 2024. https://doi.org/10.1002/apxr.202400137. ieee: 'D. Yu. Usachov et al., “Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2,” Advanced Physics Research, 2024, doi: 10.1002/apxr.202400137.' mla: Usachov, D. Yu., et al. “Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2.” Advanced Physics Research, Wiley, 2024, doi:10.1002/apxr.202400137. short: D.Yu. Usachov, K. Ali, G. Poelchen, M. Mende, S. Schulz, M. Peters, K. Bokai, I.Yu. Sklyadneva, V. Stolyarov, E.V. Chulkov, K. Kliemt, S. Paischer, P.A. Buczek, R. Heid, F. Hempel, M. Rüsing, A. Ernst, C. Krellner, S.V. Eremeev, D.V. Vyalikh, Advanced Physics Research (2024). date_created: 2025-04-02T16:18:56Z date_updated: 2025-04-02T16:20:41Z department: - _id: '288' - _id: '623' - _id: '15' doi: 10.1002/apxr.202400137 language: - iso: eng publication: Advanced Physics Research publication_identifier: issn: - 2751-1200 - 2751-1200 publication_status: published publisher: Wiley quality_controlled: '1' status: public title: Unveiling Electron‐Phonon and Electron‐Magnon Interactions in the Weak Itinerant Ferromagnet LaCo2P2 type: journal_article user_id: '22501' year: '2024' ... --- _id: '54966' abstract: - lang: eng text: Piezoresponse force microscopy (PFM) is one of the most widespread methods for investigating and visualizing ferroelectric domain structures down to the nanometer length scale. PFM makes use of the direct coupling of the piezoelectric response to the crystal lattice, and hence, it is most often applied to spatially map the three-dimensional (3D) near-surface domain distribution of any polar or ferroic sample. Nonetheless, since most samples investigated by PFM are at least semiconducting or fully insulating, the electric ac field emerging from the conductive scanning force microscopy (SFM) tip penetrates the sample and, hence, may also couple to polar features that are deeply buried into the bulk of the sample under investigation. Thus, in the work presented here, we experimentally and theoretically explore the contrast and depth resolution capabilities of PFM, by analyzing the dependence of several key parameters. These key parameters include the depth of the buried feature, i.e., here a domain wall (DW), as well as PFM-relevant technical parameters such as the tip radius, the PFM drive voltage and frequency, and the signal-to-noise ratio. The theoretical predictions are experimentally verified using x-cut periodically poled lithium niobate single crystals that are specially prepared into wedge-shaped samples, in order to allow the buried feature, here the DW, to be “positioned” at any depth into the bulk. This inspection essentially contributes to the fundamental understanding in PFM contrast analysis and to the reconstruction of 3D domain structures down to a 1 μm-penetration depth into the sample. article_type: original author: - first_name: Matthias full_name: Roeper, Matthias last_name: Roeper - first_name: Samuel D. full_name: Seddon, Samuel D. last_name: Seddon - first_name: Zeeshan H. full_name: Amber, Zeeshan H. last_name: Amber - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Lukas M. full_name: Eng, Lukas M. last_name: Eng citation: ama: Roeper M, Seddon SD, Amber ZH, Rüsing M, Eng LM. Depth resolution in piezoresponse force microscopy. Journal of Applied Physics. 2024;135(22). doi:10.1063/5.0206784 apa: Roeper, M., Seddon, S. D., Amber, Z. H., Rüsing, M., & Eng, L. M. (2024). Depth resolution in piezoresponse force microscopy. Journal of Applied Physics, 135(22). https://doi.org/10.1063/5.0206784 bibtex: '@article{Roeper_Seddon_Amber_Rüsing_Eng_2024, title={Depth resolution in piezoresponse force microscopy}, volume={135}, DOI={10.1063/5.0206784}, number={22}, journal={Journal of Applied Physics}, publisher={AIP Publishing}, author={Roeper, Matthias and Seddon, Samuel D. and Amber, Zeeshan H. and Rüsing, Michael and Eng, Lukas M.}, year={2024} }' chicago: Roeper, Matthias, Samuel D. Seddon, Zeeshan H. Amber, Michael Rüsing, and Lukas M. Eng. “Depth Resolution in Piezoresponse Force Microscopy.” Journal of Applied Physics 135, no. 22 (2024). https://doi.org/10.1063/5.0206784. ieee: 'M. Roeper, S. D. Seddon, Z. H. Amber, M. Rüsing, and L. M. Eng, “Depth resolution in piezoresponse force microscopy,” Journal of Applied Physics, vol. 135, no. 22, 2024, doi: 10.1063/5.0206784.' mla: Roeper, Matthias, et al. “Depth Resolution in Piezoresponse Force Microscopy.” Journal of Applied Physics, vol. 135, no. 22, AIP Publishing, 2024, doi:10.1063/5.0206784. short: M. Roeper, S.D. Seddon, Z.H. Amber, M. Rüsing, L.M. Eng, Journal of Applied Physics 135 (2024). date_created: 2024-07-01T21:00:43Z date_updated: 2025-04-03T12:35:34Z department: - _id: '15' - _id: '169' - _id: '288' - _id: '623' doi: 10.1063/5.0206784 intvolume: ' 135' issue: '22' keyword: - Ferroelectrics - lithium niobate - piezoresponse force microscopy language: - iso: eng main_file_link: - open_access: '1' url: https://doi.org/10.1063/5.0206784 oa: '1' publication: Journal of Applied Physics publication_identifier: issn: - 0021-8979 - 1089-7550 publication_status: published publisher: AIP Publishing quality_controlled: '1' status: public title: Depth resolution in piezoresponse force microscopy type: journal_article user_id: '22501' volume: 135 year: '2024' ... --- _id: '59259' author: - first_name: Tobias full_name: Schwabe, Tobias id: '39217' last_name: Schwabe - first_name: Michael full_name: Rüsing, Michael id: '22501' last_name: Rüsing orcid: 0000-0003-4682-4577 - first_name: Niels full_name: Staal, Niels last_name: Staal - first_name: Max full_name: Schwengelbeck, Max last_name: Schwengelbeck - first_name: Laura full_name: Bollmers, Laura id: '61375' last_name: Bollmers - first_name: Laura full_name: Padberg, Laura id: '40300' last_name: Padberg - first_name: Christof full_name: Eigner, Christof id: '13244' last_name: Eigner orcid: https://orcid.org/0000-0002-5693-3083 - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn - first_name: J. Christoph full_name: Scheytt, J. Christoph id: '37144' last_name: Scheytt orcid: '0000-0002-5950-6618 ' citation: ama: Schwabe T, Rüsing M, Staal N, et al. Quantum Photonic Systems in CMOS Compatible Silicon Nitride Technology . Zenodo; 2024. doi:10.5281/zenodo.15124929 apa: Schwabe, T., Rüsing, M., Staal, N., Schwengelbeck, M., Bollmers, L., Padberg, L., Eigner, C., Silberhorn, C., & Scheytt, J. C. (2024). Quantum photonic systems in CMOS compatible silicon nitride technology . Zenodo. https://doi.org/10.5281/zenodo.15124929 bibtex: '@book{Schwabe_Rüsing_Staal_Schwengelbeck_Bollmers_Padberg_Eigner_Silberhorn_Scheytt_2024, title={Quantum photonic systems in CMOS compatible silicon nitride technology }, DOI={10.5281/zenodo.15124929}, publisher={Zenodo}, author={Schwabe, Tobias and Rüsing, Michael and Staal, Niels and Schwengelbeck, Max and Bollmers, Laura and Padberg, Laura and Eigner, Christof and Silberhorn, Christine and Scheytt, J. Christoph}, year={2024} }' chicago: Schwabe, Tobias, Michael Rüsing, Niels Staal, Max Schwengelbeck, Laura Bollmers, Laura Padberg, Christof Eigner, Christine Silberhorn, and J. Christoph Scheytt. Quantum Photonic Systems in CMOS Compatible Silicon Nitride Technology . Zenodo, 2024. https://doi.org/10.5281/zenodo.15124929. ieee: T. Schwabe et al., Quantum photonic systems in CMOS compatible silicon nitride technology . Zenodo, 2024. mla: Schwabe, Tobias, et al. Quantum Photonic Systems in CMOS Compatible Silicon Nitride Technology . Zenodo, 2024, doi:10.5281/zenodo.15124929. short: T. Schwabe, M. Rüsing, N. Staal, M. Schwengelbeck, L. Bollmers, L. Padberg, C. Eigner, C. Silberhorn, J.C. Scheytt, Quantum Photonic Systems in CMOS Compatible Silicon Nitride Technology , Zenodo, 2024. date_created: 2025-04-02T11:24:23Z date_updated: 2025-04-03T12:34:56Z department: - _id: '288' - _id: '15' - _id: '623' doi: 10.5281/zenodo.15124929 language: - iso: eng publisher: Zenodo status: public title: 'Quantum photonic systems in CMOS compatible silicon nitride technology ' type: misc user_id: '22501' year: '2024' ... --- _id: '56267' author: - first_name: Laura full_name: Serino, Laura id: '88242' last_name: Serino - first_name: Werner full_name: Ridder, Werner id: '63574' last_name: Ridder - first_name: Abhinandan full_name: Bhattacharjee, Abhinandan id: '95902' last_name: Bhattacharjee - first_name: Jano full_name: Gil López, Jano id: '51223' last_name: Gil López - first_name: Benjamin full_name: Brecht, Benjamin id: '27150' last_name: Brecht orcid: '0000-0003-4140-0556 ' - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn citation: ama: 'Serino L, Ridder W, Bhattacharjee A, Gil López J, Brecht B, Silberhorn C. Orchestrating time and color: a programmable source of high-dimensional entanglement. Optica Quantum. Published online 2024. doi:10.1364/opticaq.532334' apa: 'Serino, L., Ridder, W., Bhattacharjee, A., Gil López, J., Brecht, B., & Silberhorn, C. (2024). Orchestrating time and color: a programmable source of high-dimensional entanglement. Optica Quantum. https://doi.org/10.1364/opticaq.532334' bibtex: '@article{Serino_Ridder_Bhattacharjee_Gil López_Brecht_Silberhorn_2024, title={Orchestrating time and color: a programmable source of high-dimensional entanglement}, DOI={10.1364/opticaq.532334}, journal={Optica Quantum}, publisher={Optica Publishing Group}, author={Serino, Laura and Ridder, Werner and Bhattacharjee, Abhinandan and Gil López, Jano and Brecht, Benjamin and Silberhorn, Christine}, year={2024} }' chicago: 'Serino, Laura, Werner Ridder, Abhinandan Bhattacharjee, Jano Gil López, Benjamin Brecht, and Christine Silberhorn. “Orchestrating Time and Color: A Programmable Source of High-Dimensional Entanglement.” Optica Quantum, 2024. https://doi.org/10.1364/opticaq.532334.' ieee: 'L. Serino, W. Ridder, A. Bhattacharjee, J. Gil López, B. Brecht, and C. Silberhorn, “Orchestrating time and color: a programmable source of high-dimensional entanglement,” Optica Quantum, 2024, doi: 10.1364/opticaq.532334.' mla: 'Serino, Laura, et al. “Orchestrating Time and Color: A Programmable Source of High-Dimensional Entanglement.” Optica Quantum, Optica Publishing Group, 2024, doi:10.1364/opticaq.532334.' short: L. Serino, W. Ridder, A. Bhattacharjee, J. Gil López, B. Brecht, C. Silberhorn, Optica Quantum (2024). date_created: 2024-09-27T11:46:59Z date_updated: 2025-12-01T08:49:46Z department: - _id: '288' - _id: '623' - _id: '288' doi: 10.1364/opticaq.532334 language: - iso: eng project: - _id: '211' name: 'QuICHE: Quanteninformation und Quantenkommunikation mit hochdimensionaler Informationskodierung (QuICHE)' publication: Optica Quantum publication_identifier: issn: - 2837-6714 publication_status: published publisher: Optica Publishing Group status: public title: 'Orchestrating time and color: a programmable source of high-dimensional entanglement' type: journal_article user_id: '63574' year: '2024' ... --- _id: '54288' abstract: - lang: eng text: "The ability to apply user-chosen large-scale unitary operations with high fidelity to a quantum state is key to realizing future photonic quantum technologies. Here, we realize the implementation of programmable unitary operations on up to 64 frequency-bin modes. To benchmark the performance of our system, we probe different quantum walk unitary operations, in particular, Grover walks on four-dimensional hypercubes with similarities exceeding 95% and quantum walks with 400 steps on circles and finite lines with similarities of 98%. Our results open a path toward implementing high-quality unitary operations, which can form the basis for applications in complex tasks, such as Gaussian boson sampling.\r\n \r\n \ \r\n \r\n \r\n \ Published by the American Physical Society\r\n \ 2024\r\n \r\n \ \r\n " article_number: L022040 author: - first_name: Syamsundar full_name: De, Syamsundar last_name: De - first_name: Vahid full_name: Ansari, Vahid last_name: Ansari - first_name: Jan full_name: Sperling, Jan id: '75127' last_name: Sperling orcid: 0000-0002-5844-3205 - first_name: Sonja full_name: Barkhofen, Sonja id: '48188' last_name: Barkhofen - first_name: Benjamin full_name: Brecht, Benjamin id: '27150' last_name: Brecht orcid: '0000-0003-4140-0556 ' - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn citation: ama: De S, Ansari V, Sperling J, Barkhofen S, Brecht B, Silberhorn C. Realization of high-fidelity unitary operations on up to 64 frequency bins. Physical Review Research. 2024;6(2). doi:10.1103/physrevresearch.6.l022040 apa: De, S., Ansari, V., Sperling, J., Barkhofen, S., Brecht, B., & Silberhorn, C. (2024). Realization of high-fidelity unitary operations on up to 64 frequency bins. Physical Review Research, 6(2), Article L022040. https://doi.org/10.1103/physrevresearch.6.l022040 bibtex: '@article{De_Ansari_Sperling_Barkhofen_Brecht_Silberhorn_2024, title={Realization of high-fidelity unitary operations on up to 64 frequency bins}, volume={6}, DOI={10.1103/physrevresearch.6.l022040}, number={2L022040}, journal={Physical Review Research}, publisher={American Physical Society (APS)}, author={De, Syamsundar and Ansari, Vahid and Sperling, Jan and Barkhofen, Sonja and Brecht, Benjamin and Silberhorn, Christine}, year={2024} }' chicago: De, Syamsundar, Vahid Ansari, Jan Sperling, Sonja Barkhofen, Benjamin Brecht, and Christine Silberhorn. “Realization of High-Fidelity Unitary Operations on up to 64 Frequency Bins.” Physical Review Research 6, no. 2 (2024). https://doi.org/10.1103/physrevresearch.6.l022040. ieee: 'S. De, V. Ansari, J. Sperling, S. Barkhofen, B. Brecht, and C. Silberhorn, “Realization of high-fidelity unitary operations on up to 64 frequency bins,” Physical Review Research, vol. 6, no. 2, Art. no. L022040, 2024, doi: 10.1103/physrevresearch.6.l022040.' mla: De, Syamsundar, et al. “Realization of High-Fidelity Unitary Operations on up to 64 Frequency Bins.” Physical Review Research, vol. 6, no. 2, L022040, American Physical Society (APS), 2024, doi:10.1103/physrevresearch.6.l022040. short: S. De, V. Ansari, J. Sperling, S. Barkhofen, B. Brecht, C. Silberhorn, Physical Review Research 6 (2024). date_created: 2024-05-14T12:40:48Z date_updated: 2025-12-18T16:14:39Z department: - _id: '623' - _id: '288' - _id: '15' doi: 10.1103/physrevresearch.6.l022040 intvolume: ' 6' issue: '2' language: - iso: eng project: - _id: '216' name: 'QuPoPCoRN: QUPOPCORN: Quantum Particles on Programmable Complex Reconfigurable Networks' publication: Physical Review Research publication_identifier: issn: - 2643-1564 publication_status: published publisher: American Physical Society (APS) status: public title: Realization of high-fidelity unitary operations on up to 64 frequency bins type: journal_article user_id: '27150' volume: 6 year: '2024' ... --- _id: '54815' abstract: - lang: eng text: "Broadband quantum light is a vital resource for quantum metrology and spectroscopy applications such as quantum optical coherence tomography or entangled two photon absorption. For entangled two photon absorption in particular, very high photon flux combined with high time-frequency entanglement is crucial for observing a signal. So far these conditions could be met by using high power lasers driving degenerate, type 0 bulk-crystal spontaneous parametric down conversion (SPDC) sources. This naturally limits the available wavelength ranges and precludes deterministic splitting of the generated output photons. In this work we demonstrate an integrated two-colour SPDC source utilising a group-velocity matched lithium niobate waveguide, reaching both exceptional brightness 1.52⋅106pairssmWGHz and large bandwidth (7.8 THz FWHM) while pumped with a few mW of continuous wave (CW) laser light. By converting a narrow band pump to broadband pulses the created photon pairs show correlation times of Δτ ≈ 120 fs while maintaining the narrow bandwidth Δω\r\n \ p\r\n  ≪ 1 MHz of the CW pump light, yielding strong time-frequency entanglement. Furthermore our process can be adapted to a wide range of central wavelengths." article_number: '23945' article_type: original author: - first_name: René full_name: Pollmann, René id: '78890' last_name: Pollmann - first_name: Franz full_name: Roeder, Franz id: '88149' last_name: Roeder - first_name: Victor full_name: Quiring, Victor last_name: Quiring - first_name: Raimund full_name: Ricken, Raimund last_name: Ricken - first_name: Christof full_name: Eigner, Christof id: '13244' last_name: Eigner orcid: https://orcid.org/0000-0002-5693-3083 - first_name: Benjamin full_name: Brecht, Benjamin id: '27150' last_name: Brecht orcid: '0000-0003-4140-0556 ' - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn citation: ama: Pollmann R, Roeder F, Quiring V, et al. Integrated, bright broadband, two-colour parametric down-conversion source. Optics Express. 2024;32(14). doi:10.1364/oe.522549 apa: Pollmann, R., Roeder, F., Quiring, V., Ricken, R., Eigner, C., Brecht, B., & Silberhorn, C. (2024). Integrated, bright broadband, two-colour parametric down-conversion source. Optics Express, 32(14), Article 23945. https://doi.org/10.1364/oe.522549 bibtex: '@article{Pollmann_Roeder_Quiring_Ricken_Eigner_Brecht_Silberhorn_2024, title={Integrated, bright broadband, two-colour parametric down-conversion source}, volume={32}, DOI={10.1364/oe.522549}, number={1423945}, journal={Optics Express}, publisher={Optica Publishing Group}, author={Pollmann, René and Roeder, Franz and Quiring, Victor and Ricken, Raimund and Eigner, Christof and Brecht, Benjamin and Silberhorn, Christine}, year={2024} }' chicago: Pollmann, René, Franz Roeder, Victor Quiring, Raimund Ricken, Christof Eigner, Benjamin Brecht, and Christine Silberhorn. “Integrated, Bright Broadband, Two-Colour Parametric down-Conversion Source.” Optics Express 32, no. 14 (2024). https://doi.org/10.1364/oe.522549. ieee: 'R. Pollmann et al., “Integrated, bright broadband, two-colour parametric down-conversion source,” Optics Express, vol. 32, no. 14, Art. no. 23945, 2024, doi: 10.1364/oe.522549.' mla: Pollmann, René, et al. “Integrated, Bright Broadband, Two-Colour Parametric down-Conversion Source.” Optics Express, vol. 32, no. 14, 23945, Optica Publishing Group, 2024, doi:10.1364/oe.522549. short: R. Pollmann, F. Roeder, V. Quiring, R. Ricken, C. Eigner, B. Brecht, C. Silberhorn, Optics Express 32 (2024). date_created: 2024-06-19T06:58:17Z date_updated: 2025-12-19T11:37:41Z department: - _id: '15' - _id: '623' - _id: '288' doi: 10.1364/oe.522549 intvolume: ' 32' issue: '14' language: - iso: eng publication: Optics Express publication_identifier: issn: - 1094-4087 publication_status: published publisher: Optica Publishing Group status: public title: Integrated, bright broadband, two-colour parametric down-conversion source type: journal_article user_id: '78890' volume: 32 year: '2024' ... --- _id: '57862' abstract: - lang: eng text: The latest applications in ultrafast quantum metrology require bright, broadband bi-photon sources with one of the photons in the mid-infrared and the other in the visible to near infrared. However, existing sources based on bulk crystals are limited in brightness due to the short interaction length and only allow for limited dispersion engineering. Here, we present an integrated PDC source based on a Ti:LiNbO3 waveguide that generates broadband bi-photons with central wavelengths at 860 nm and 2800 nm. Their spectral bandwidth exceeds 25 THz and is achieved by simultaneous matching of the group velocities (GVs) and cancellation of GV dispersion for the signal and idler field. We provide an intuitive understanding of the process by studying our source’s behavior at different temperatures and pump wavelengths, which agrees well with simulations. article_number: '123025' article_type: original author: - first_name: Franz full_name: Roeder, Franz id: '88149' last_name: Roeder - first_name: Abira full_name: Gnanavel, Abira last_name: Gnanavel - first_name: René full_name: Pollmann, René id: '78890' last_name: Pollmann - first_name: Olga full_name: Brecht, Olga last_name: Brecht - first_name: Michael full_name: Stefszky, Michael id: '42777' last_name: Stefszky - first_name: Laura full_name: Padberg, Laura id: '40300' last_name: Padberg - first_name: Christof full_name: Eigner, Christof id: '13244' last_name: Eigner orcid: https://orcid.org/0000-0002-5693-3083 - first_name: Christine full_name: Silberhorn, Christine id: '26263' last_name: Silberhorn - first_name: Benjamin full_name: Brecht, Benjamin id: '27150' last_name: Brecht orcid: '0000-0003-4140-0556 ' citation: ama: Roeder F, Gnanavel A, Pollmann R, et al. Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared. New Journal of Physics. 2024;26(12). doi:10.1088/1367-2630/ad9f98 apa: Roeder, F., Gnanavel, A., Pollmann, R., Brecht, O., Stefszky, M., Padberg, L., Eigner, C., Silberhorn, C., & Brecht, B. (2024). Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared. New Journal of Physics, 26(12), Article 123025. https://doi.org/10.1088/1367-2630/ad9f98 bibtex: '@article{Roeder_Gnanavel_Pollmann_Brecht_Stefszky_Padberg_Eigner_Silberhorn_Brecht_2024, title={Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared}, volume={26}, DOI={10.1088/1367-2630/ad9f98}, number={12123025}, journal={New Journal of Physics}, publisher={IOP Publishing}, author={Roeder, Franz and Gnanavel, Abira and Pollmann, René and Brecht, Olga and Stefszky, Michael and Padberg, Laura and Eigner, Christof and Silberhorn, Christine and Brecht, Benjamin}, year={2024} }' chicago: Roeder, Franz, Abira Gnanavel, René Pollmann, Olga Brecht, Michael Stefszky, Laura Padberg, Christof Eigner, Christine Silberhorn, and Benjamin Brecht. “Ultra-Broadband Non-Degenerate Guided-Wave Bi-Photon Source in the near and Mid-Infrared.” New Journal of Physics 26, no. 12 (2024). https://doi.org/10.1088/1367-2630/ad9f98. ieee: 'F. Roeder et al., “Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared,” New Journal of Physics, vol. 26, no. 12, Art. no. 123025, 2024, doi: 10.1088/1367-2630/ad9f98.' mla: Roeder, Franz, et al. “Ultra-Broadband Non-Degenerate Guided-Wave Bi-Photon Source in the near and Mid-Infrared.” New Journal of Physics, vol. 26, no. 12, 123025, IOP Publishing, 2024, doi:10.1088/1367-2630/ad9f98. short: F. Roeder, A. Gnanavel, R. Pollmann, O. Brecht, M. Stefszky, L. Padberg, C. Eigner, C. Silberhorn, B. Brecht, New Journal of Physics 26 (2024). date_created: 2024-12-27T19:01:14Z date_updated: 2025-12-19T11:36:36Z department: - _id: '288' - _id: '623' - _id: '15' doi: 10.1088/1367-2630/ad9f98 intvolume: ' 26' issue: '12' language: - iso: eng project: - _id: '571' name: 'MIRAQLS: MIRAQLS: Mid-infrared Quantum Technology for Sensing' - _id: '190' name: 'E2TPA: Exploiting Entangled Two-Photon Absorption' publication: New Journal of Physics publication_identifier: issn: - 1367-2630 publication_status: published publisher: IOP Publishing status: public title: Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared type: journal_article user_id: '78890' volume: 26 year: '2024' ... --- _id: '48349' abstract: - lang: eng text: We report a titanium indiffused waveguide resonator featuring an integrated electro-optic modulator for cavity length stabilisation that produces close to 5 dB of squeezed light at 1550 nm (2.4 dB directly measured). The resonator is locked on resonance for tens of minutes with 70 mW of SH light incident on the cavity, demonstrating that photorefraction can be mitigated. Squeezed light production concurrent with cavity length stabilisation utilising the integrated EOM is demonstrated. The device demonstrates the suitability of this platform for squeezed light generation in network applications, where stabilisation to the reference field is typically necessary. article_number: '34903' author: - first_name: M. full_name: Stefszky, M. last_name: Stefszky - first_name: F. full_name: vom Bruch, F. last_name: vom Bruch - first_name: M. full_name: Santandrea, M. last_name: Santandrea - first_name: R. full_name: Ricken, R. last_name: Ricken - first_name: V. full_name: Quiring, V. last_name: Quiring - first_name: C. full_name: Eigner, C. last_name: Eigner - first_name: H full_name: Herrmann, H last_name: Herrmann - first_name: C full_name: Silberhorn, C last_name: Silberhorn citation: ama: Stefszky M, vom Bruch F, Santandrea M, et al. Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications. Optics Express. 2023;31(21). doi:10.1364/oe.498423 apa: Stefszky, M., vom Bruch, F., Santandrea, M., Ricken, R., Quiring, V., Eigner, C., Herrmann, H., & Silberhorn, C. (2023). Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications. Optics Express, 31(21), Article 34903. https://doi.org/10.1364/oe.498423 bibtex: '@article{Stefszky_vom Bruch_Santandrea_Ricken_Quiring_Eigner_Herrmann_Silberhorn_2023, title={Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications}, volume={31}, DOI={10.1364/oe.498423}, number={2134903}, journal={Optics Express}, publisher={Optica Publishing Group}, author={Stefszky, M. and vom Bruch, F. and Santandrea, M. and Ricken, R. and Quiring, V. and Eigner, C. and Herrmann, H and Silberhorn, C}, year={2023} }' chicago: Stefszky, M., F. vom Bruch, M. Santandrea, R. Ricken, V. Quiring, C. Eigner, H Herrmann, and C Silberhorn. “Lithium Niobate Waveguide Squeezer with Integrated Cavity Length Stabilisation for Network Applications.” Optics Express 31, no. 21 (2023). https://doi.org/10.1364/oe.498423. ieee: 'M. Stefszky et al., “Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications,” Optics Express, vol. 31, no. 21, Art. no. 34903, 2023, doi: 10.1364/oe.498423.' mla: Stefszky, M., et al. “Lithium Niobate Waveguide Squeezer with Integrated Cavity Length Stabilisation for Network Applications.” Optics Express, vol. 31, no. 21, 34903, Optica Publishing Group, 2023, doi:10.1364/oe.498423. short: M. Stefszky, F. vom Bruch, M. Santandrea, R. Ricken, V. Quiring, C. Eigner, H. Herrmann, C. Silberhorn, Optics Express 31 (2023). date_created: 2023-10-19T14:22:59Z date_updated: 2023-11-02T09:26:42Z department: - _id: '288' - _id: '623' doi: 10.1364/oe.498423 intvolume: ' 31' issue: '21' keyword: - Atomic and Molecular Physics - and Optics language: - iso: eng publication: Optics Express publication_identifier: issn: - 1094-4087 publication_status: published publisher: Optica Publishing Group status: public title: Lithium niobate waveguide squeezer with integrated cavity length stabilisation for network applications type: journal_article user_id: '42777' volume: 31 year: '2023' ...