@article{22549, author = {{Gebhard, Maximilian and Mai, Lukas and Banko, Lars and Mitschker, Felix and Hoppe, Christian and Jaritz, Montgomery and Kirchheim, Dennis and Zekorn, Christoph and de los Arcos de Pedro, Maria Teresa and Grochla, Dario and Dahlmann, Rainer and Grundmeier, Guido and Awakowicz, Peter and Ludwig, Alfred and Devi, Anjana}}, issn = {{1944-8244}}, journal = {{ACS Applied Materials & Interfaces}}, pages = {{7422--7434}}, title = {{{PEALD of SiO2 and Al2O3 Thin Films on Polypropylene: Investigations of the Film Growth at the Interface, Stress, and Gas Barrier Properties of Dyads}}}, doi = {{10.1021/acsami.7b14916}}, year = {{2018}}, } @article{22551, author = {{Gebhard, Maximilian and Mai, Lukas and Banko, Lars and Mitschker, Felix and Hoppe, Christian and Jaritz, Montgomery and Kirchheim, Dennis and Zekorn, Christoph and de los Arcos de Pedro, Maria Teresa and Grochla, Dario and Dahlmann, Rainer and Grundmeier, Guido and Awakowicz, Peter and Ludwig, Alfred and Devi, Anjana}}, issn = {{1944-8244}}, journal = {{ACS Applied Materials & Interfaces}}, pages = {{7422--7434}}, title = {{{PEALD of SiO2 and Al2O3 Thin Films on Polypropylene: Investigations of the Film Growth at the Interface, Stress, and Gas Barrier Properties of Dyads}}}, doi = {{10.1021/acsami.7b14916}}, year = {{2018}}, } @article{22548, author = {{Dietrich, J. and Hoppe, C. and de los Arcos de Pedro, Maria Teresa and Grundmeier, Guido}}, issn = {{0863-1042}}, journal = {{Contributions to Plasma Physics}}, pages = {{377--383}}, title = {{{Combined in situ infrared reflection absorption spectroscopy-quartz crystal microbalance investigation of the initial growth stages of plasma-deposited SiO x on polypropylene}}}, doi = {{10.1002/ctpp.201700036}}, year = {{2018}}, } @article{22547, author = {{Budde, Maik and Corbella, Carles and Große-Kreul, Simon and de los Arcos de Pedro, Maria Teresa and Grundmeier, Guido and von Keudell, Achim}}, issn = {{1612-8850}}, journal = {{Plasma Processes and Polymers}}, title = {{{Decoupling of ion- and photon-activation mechanisms in polymer surfaces exposed to low-temperature plasmas}}}, doi = {{10.1002/ppap.201700230}}, year = {{2018}}, } @article{22557, abstract = {{

A new water assisted atomic layer deposition (ALD) process was developed using the yttrium tris-guanidinate precursor which resulted in device quality thin films.

}}, author = {{Mai, Lukas and Boysen, Nils and Subaşı, Ersoy and de los Arcos de Pedro, Maria Teresa and Rogalla, Detlef and Grundmeier, Guido and Bock, Claudia and Lu, Hong-Liang and Devi, Anjana}}, issn = {{2046-2069}}, journal = {{RSC Advances}}, pages = {{4987--4994}}, title = {{{Water assisted atomic layer deposition of yttrium oxide using tris(N,N′-diisopropyl-2-dimethylamido-guanidinato) yttrium(iii): process development, film characterization and functional properties}}}, doi = {{10.1039/c7ra13417g}}, year = {{2018}}, } @article{22558, author = {{Mitschker, F and Schücke, L and Hoppe, Ch and Jaritz, M and Dahlmann, R and de los Arcos de Pedro, Maria Teresa and Hopmann, Ch and Grundmeier, Guido and Awakowicz, P}}, issn = {{0022-3727}}, journal = {{Journal of Physics D: Applied Physics}}, title = {{{Comparative study on the deposition of silicon oxide permeation barrier coatings for polymers using hexamethyldisilazane (HMDSN) and hexamethyldisiloxane (HMDSO)}}}, doi = {{10.1088/1361-6463/aac0ab}}, year = {{2018}}, } @article{22559, author = {{Mitschker, F and Wißing, J and Hoppe, Ch and de los Arcos de Pedro, Maria Teresa and Grundmeier, Guido and Awakowicz, P}}, issn = {{0022-3727}}, journal = {{Journal of Physics D: Applied Physics}}, title = {{{Influence of average ion energy and atomic oxygen flux per Si atom on the formation of silicon oxide permeation barrier coatings on PET}}}, doi = {{10.1088/1361-6463/aab1dd}}, year = {{2018}}, } @article{22556, author = {{Layes, Vincent and Corbella, Carles and Monjé, Sascha and Schulz-von der Gathen, Volker and von Keudell, Achim and de los Arcos de Pedro, Maria Teresa}}, issn = {{1361-6595}}, journal = {{Plasma Sources Science and Technology}}, title = {{{Connection between target poisoning and current waveforms in reactive high-power impulse magnetron sputtering of chromium}}}, doi = {{10.1088/1361-6595/aad0e2}}, year = {{2018}}, } @article{22554, author = {{González-Orive, A. and Giner, I. and de los Arcos de Pedro, Maria Teresa and Keller, Adrian and Grundmeier, Guido}}, issn = {{0169-4332}}, journal = {{Applied Surface Science}}, pages = {{581--594}}, title = {{{Analysis of polymer/oxide interfaces under ambient conditions – An experimental perspective}}}, doi = {{10.1016/j.apsusc.2018.02.155}}, year = {{2018}}, } @article{22552, author = {{González-Orive, A. and Giner, I. and de los Arcos de Pedro, Maria Teresa and Keller, A. and Grundmeier, Guido}}, issn = {{0169-4332}}, journal = {{Applied Surface Science}}, pages = {{581--594}}, title = {{{Analysis of polymer/oxide interfaces under ambient conditions – An experimental perspective}}}, doi = {{10.1016/j.apsusc.2018.02.155}}, year = {{2018}}, } @article{22553, author = {{González-Orive, A. and Giner, I. and de los Arcos de Pedro, Maria Teresa and Keller, A. and Grundmeier, G.}}, issn = {{0169-4332}}, journal = {{Applied Surface Science}}, pages = {{581--594}}, title = {{{Analysis of polymer/oxide interfaces under ambient conditions – An experimental perspective}}}, doi = {{10.1016/j.apsusc.2018.02.155}}, year = {{2018}}, } @article{25276, author = {{Wolk, Andreas and Rosenthal, Marta and Neuhaus, Stephan and Huber, Klaus and Brassat, Katharina and Lindner, Jörg K. N. and Grothe, Richard and Grundmeier, Guido and Bremser, Wolfgang and Wilhelm, René}}, issn = {{2045-2322}}, journal = {{Scientific Reports}}, title = {{{A Novel Lubricant Based on Covalent Functionalized Graphene Oxide Quantum Dots}}}, doi = {{10.1038/s41598-018-24062-2}}, year = {{2018}}, } @article{25911, abstract = {{Different types of reduced graphene oxide and graphene oxide particles have been studied regarding their influence on the curing behaviour of epoxy-amine resins. Especially the specific surface area of reduced graphene oxide was selectively influenced by controlled drying of the material. The different types of reduced graphene oxide particles were used to produce epoxy-amine composites that significantly change their curing behaviour and mechanical properties. A variety of surface areas and compositions were prepared by combination of a fast heating rate and different drying methods. The combination of freeze drying with a fast heating rate leads to a large specific surface area of 680 m2/g. The morphologies of the particles were observed by scanning electron microscope and the BET surface area was measured with nitrogen-physisorption. The exfoliation quality was measured by XRD. The generated graphene oxide and thermally reduced graphene oxide particles were mixed with epoxy-amine resin. The curing behaviour was studied with rheological and differential scanning calorimetry (DSC) measurements. We observed that different surface functionalities lowers the Glass transition temperature and the gel time of an epoxy-amine curing system. In addition, we found that generated graphene oxide acts as flexibilizer. An increase of the deformation from 2.5 mm to 3.1 mm was measured by Erichsen Cupping Test.}}, author = {{Wolk, Andreas and Rosenthal, Marta and Weiß, Julia and Voigt, Markus and Wesendahl, Jan-Niklas and Hartmann, Marc and Grundmeier, Guido and Wilhelm, Rene and Meschut, Gerson and Tiemann, Michael and Bremser, Wolfgang}}, issn = {{0300-9440}}, journal = {{Progress in Organic Coatings}}, pages = {{280--289}}, title = {{{Graphene oxide as flexibilizer for epoxy amine resins}}}, doi = {{10.1016/j.porgcoat.2018.05.028}}, year = {{2018}}, } @article{62802, abstract = {{Since the resurgence of interest in lithium–sulfur (Li–S) batteries at the end of the 2000s, research in the field has grown rapidly. Li–S batteries hold great promise as the upcoming post-lithium-ion batteries owing to their notably high theoretical specific energy density of 2600 W h kg−1, nearly five-fold larger than that of current lithium-ion batteries. However, one of their major technical problems is found in the shuttling of soluble polysulfides between the electrodes, resulting in rapid capacity fading and poor cycling stability. This review spotlights the foremost findings and the recent progress in enhancing the electrochemical performance of Li–S batteries by using nanoscaled metal compounds and metals. Based on an overview of reported functional metal-based materials and their specific employment in certain parts of Li–S batteries, the underlying mechanisms of enhanced adsorption and improved reaction kinetics are critically discussed involving both experimental and computational research findings. Thus, material design principles and possible interdisciplinary research approaches providing the chance to jointly advance with related fields such as electrocatalysis are identified. Particularly, we elucidate additives, sulfur hosts, current collectors and functional interlayers/hybrid separators containing metal oxides, hydroxides and sulfides as well as metal–organic frameworks, bare metal and further metal nitrides, metal carbides and MXenes. Throughout this review article, we emphasize the close relationship between the intrinsic properties of metal-based nanostructured materials, the (electro)chemical interaction with lithium (poly)sulfides and the subsequent effect on the battery performance. Concluding the review, prospects for the future development of practical Li–S batteries with metal-based nanomaterials are discussed.}}, author = {{Balach, Juan and Linnemann, Julia and Jaumann, Tony and Giebeler, Lars}}, issn = {{2050-7488}}, journal = {{Journal of Materials Chemistry A}}, keywords = {{lithium-sulfur battery}}, number = {{46}}, pages = {{23127--23168}}, publisher = {{Royal Society of Chemistry (RSC)}}, title = {{{Metal-based nanostructured materials for advanced lithium–sulfur batteries}}}, doi = {{10.1039/c8ta07220e}}, volume = {{6}}, year = {{2018}}, } @article{62809, abstract = {{Superhierarchically rough films are rapidly synthesised on metal substrates via electrochemically triggered self-assembly of meso/macroporous-structured metal-organic framework (MOF) crystals. These coatings are applied to immobilise a functional oil with low surface energy to provide stable coatings repellent to a wide range of hydrophobic as well as hydrophilic fluids. Such omniphobic surfaces are highly interesting for several applications such as anti-fouling, anti-icing, and dropwise condensation, and become easily scalable with the presented bottom-up fabrication approach. As investigated by environmental scanning electron microscopy (ESEM), the presented perfluorinated oil-infused Cu-BTC coating constitutes of a flat liquid-covered surface with protruding edges of octahedral superstructured MOF crystals. Water and non-polar diiodomethane droplets form considerably high contact angles and even low-surface-tension fluids, e.g. acetone, form droplets on the infused coating. The repellent properties towards the test fluids do not change upon extended water spraying in contrast to oil-infused porous copper oxide or native copper surfaces. It is discussed in detail, how the presented electrodeposited MOF films grow and provide a proficient surface morphology to stabilise the functional oil film due to hemiwicking.}}, author = {{Sablowski, Jakob and Linnemann, Julia and Hempel, Simone and Hoffmann, Volker and Unz, Simon and Beckmann, Michael and Giebeler, Lars}}, issn = {{2045-2322}}, journal = {{Scientific Reports}}, keywords = {{electrodeposition, metal-organic framework, MOF, drop-wise condensation, omniphobic coatings}}, number = {{1}}, publisher = {{Springer Science and Business Media LLC}}, title = {{{Electrodeposited metal-organic framework films as self-assembled hierarchically superstructured supports for stable omniphobic surface coatings}}}, doi = {{10.1038/s41598-018-33542-4}}, volume = {{8}}, year = {{2018}}, } @article{58588, author = {{Ressel, Joerg and Seewald, Oliver and Bremser, Wolfgang and Reicher, Hans-Peter and Strube, Oliver I.}}, issn = {{0300-9440}}, journal = {{Progress in Organic Coatings}}, pages = {{1--7}}, publisher = {{Elsevier BV}}, title = {{{Low friction poly(amide-imide) coatings with silicones as tethered liquids}}}, doi = {{10.1016/j.porgcoat.2018.07.029}}, volume = {{124}}, year = {{2018}}, } @article{25306, author = {{Büngeler, Anne and Hämisch, Benjamin and Huber, Klaus and Bremser, Wolfgang and Strube, Oliver I.}}, issn = {{0743-7463}}, journal = {{Langmuir}}, pages = {{6895--6901}}, title = {{{Insight into the Final Step of the Supramolecular Buildup of Eumelanin}}}, doi = {{10.1021/acs.langmuir.7b01634}}, year = {{2017}}, } @article{25307, author = {{Reichinger, M. and Bremser, Wolfgang and Dornbusch, M.}}, issn = {{0013-4686}}, journal = {{Electrochimica Acta}}, pages = {{135--152}}, title = {{{Interface and volume transport on technical cataphoretic painting: A comparison of steel, hot-dip galvanised steel and aluminium alloy}}}, doi = {{10.1016/j.electacta.2017.02.013}}, year = {{2017}}, } @article{24109, author = {{Wiesener, Markus and Peters, K. and Taube, Alexander and Keller, Adrian and Hoyer, Kay-Peter and Niendorf, Thomas and Grundmeier, Guido}}, issn = {{0947-5117}}, journal = {{Materials and Corrosion}}, pages = {{1028--1036}}, title = {{{Corrosion properties of bioresorbable FeMn-Ag alloys prepared by selective laser melting}}}, doi = {{10.1002/maco.201709478}}, year = {{2017}}, } @article{23627, author = {{Schmaltz, Thomas and Gothe, Bastian and Krause, Andreas and Leitherer, Susanne and Steinrück, Hans-Georg and Thoss, Michael and Clark, Timothy and Halik, Marcus}}, issn = {{1936-0851}}, journal = {{ACS Nano}}, pages = {{8747--8757}}, title = {{{Effect of Structure and Disorder on the Charge Transport in Defined Self-Assembled Monolayers of Organic Semiconductors}}}, doi = {{10.1021/acsnano.7b02394}}, volume = {{11}}, year = {{2017}}, }