[{"abstract":[{"text":"Single-entity electrochemistry allows for assessing electrocatalytic activities of individual material entities such as nanoparticles (NPs). Thus, it becomes possible to consider intrinsic electrochemical properties of nanocatalysts when researching how activity relates to physical and structural material properties. Conversely, conventional electrochemical techniques provide a normalized sum current referring to a huge ensemble of NPs constituting, along with additives (e.g., binders), a complete catalyst-coated electrode. Accordingly, recording electrocatalytic responses of single NPs avoids interferences of ensemble effects and reduces the complexity of electrocatalytic processes, thus enabling detailed description and modelling. Herein, we present insights into the oxygen evolution catalysis at individual cubic Co3O4 NPs impacting microelectrodes of different support materials. Simulating diffusion at supported nanocubes, measured step current signals can be analyzed, providing edge lengths, corresponding size distributions, and interference-free turnover frequencies. The provided nano-impact investigation of (electro-)catalyst-support effects contradicts assumptions on a low number of highly active sites.","lang":"eng"}],"publication":"International Journal of Molecular Sciences","keyword":["electrocatalysis","oxygen evolution reaction","cobalt spinel","single-entity electrochemistry"],"language":[{"iso":"eng"}],"year":"2021","quality_controlled":"1","issue":"23","title":"Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects","publisher":"MDPI AG","date_created":"2025-12-03T15:35:52Z","status":"public","type":"journal_article","article_type":"original","article_number":"13137","extern":"1","_id":"62805","department":[{"_id":"985"}],"user_id":"116779","intvolume":"        22","citation":{"chicago":"Liu, Zhibin, Manuel Corva, Hatem M. A. Amin, Niclas Blanc, Julia Linnemann, and Kristina Tschulik. “Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects.” <i>International Journal of Molecular Sciences</i> 22, no. 23 (2021). <a href=\"https://doi.org/10.3390/ijms222313137\">https://doi.org/10.3390/ijms222313137</a>.","ieee":"Z. Liu, M. Corva, H. M. A. Amin, N. Blanc, J. Linnemann, and K. Tschulik, “Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects,” <i>International Journal of Molecular Sciences</i>, vol. 22, no. 23, Art. no. 13137, 2021, doi: <a href=\"https://doi.org/10.3390/ijms222313137\">10.3390/ijms222313137</a>.","ama":"Liu Z, Corva M, Amin HMA, Blanc N, Linnemann J, Tschulik K. Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects. <i>International Journal of Molecular Sciences</i>. 2021;22(23). doi:<a href=\"https://doi.org/10.3390/ijms222313137\">10.3390/ijms222313137</a>","apa":"Liu, Z., Corva, M., Amin, H. M. A., Blanc, N., Linnemann, J., &#38; Tschulik, K. (2021). Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects. <i>International Journal of Molecular Sciences</i>, <i>22</i>(23), Article 13137. <a href=\"https://doi.org/10.3390/ijms222313137\">https://doi.org/10.3390/ijms222313137</a>","bibtex":"@article{Liu_Corva_Amin_Blanc_Linnemann_Tschulik_2021, title={Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects}, volume={22}, DOI={<a href=\"https://doi.org/10.3390/ijms222313137\">10.3390/ijms222313137</a>}, number={2313137}, journal={International Journal of Molecular Sciences}, publisher={MDPI AG}, author={Liu, Zhibin and Corva, Manuel and Amin, Hatem M. A. and Blanc, Niclas and Linnemann, Julia and Tschulik, Kristina}, year={2021} }","mla":"Liu, Zhibin, et al. “Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects.” <i>International Journal of Molecular Sciences</i>, vol. 22, no. 23, 13137, MDPI AG, 2021, doi:<a href=\"https://doi.org/10.3390/ijms222313137\">10.3390/ijms222313137</a>.","short":"Z. Liu, M. Corva, H.M.A. Amin, N. Blanc, J. Linnemann, K. Tschulik, International Journal of Molecular Sciences 22 (2021)."},"publication_identifier":{"issn":["1422-0067"]},"publication_status":"published","doi":"10.3390/ijms222313137","main_file_link":[{"open_access":"1"}],"date_updated":"2025-12-03T16:52:35Z","oa":"1","volume":22,"author":[{"first_name":"Zhibin","last_name":"Liu","full_name":"Liu, Zhibin"},{"first_name":"Manuel","full_name":"Corva, Manuel","last_name":"Corva"},{"first_name":"Hatem M. A.","last_name":"Amin","full_name":"Amin, Hatem M. A."},{"first_name":"Niclas","full_name":"Blanc, Niclas","last_name":"Blanc"},{"orcid":"0000-0001-6883-5424","last_name":"Linnemann","id":"116779","full_name":"Linnemann, Julia","first_name":"Julia"},{"full_name":"Tschulik, Kristina","last_name":"Tschulik","first_name":"Kristina"}]},{"language":[{"iso":"eng"}],"publication":"Inorganic Chemistry","abstract":[{"lang":"eng","text":"To reduce high-level radiotoxic waste generated by nuclear power plants, highly selective separation agents for minor actinides are mandatory. The mixed N,O-donor ligand N,N,N′,N′-tetrakis[(6-carboxypyridin-2-yl)methyl]ethylenediamine (H4TPAEN; 1) has shown good performance as a masking agent in Am3+/Eu3+ separation studies. Adjustments on the pyridyl backbone to raise the hydrophilicity led to a decrease in selectivity and a decrease in M3+–Nam interactions. An enhanced basicity of the pyridyl N-donors was given as a cause. In this work, we examine whether a decrease in O-donor basicity can promote the M3+–Nam interactions. Therefore, we replace the deprotonated “charged” carboxylic acid groups of TPAEN4– by neutral amide groups and introduce N,N,N′,N’-tetrakis[(6-N″,N′′-diethylcarbamoylpyridin-2-yl)methyl]ethylenediamine (TPAMEN; 2) as a new ligand. TPAMEN was crystallized with Eu(OTf)3 and Eu(NO3)3·6H2O to form positively charged 1:1 [Eu(TPAMEN)]3+ complexes in the solid state. Alterations in the M–O/N bond distances are compared to [Eu(TPAEN)]− and investigated by DFT calculations to expose the differences in charge/energy density distributions at europium(III) and the donor functionalities of the TPAEN4– and TPAMEN. On the basis of estimations of the bond orders, atomic charges spin populations, and density of states in the Eu and potential Am and Cm complexes, the specific contributions of the donor–metal interaction are analyzed. The prediction of complex formation energy differences for the [M(TPAEN)]− and [M(TPAMEN)]3+ (M3+ = Eu3+, Am3+) complexes provide an outlook on the potential performance of TPAMEN in Am3+/Eu3+ separation."}],"publisher":"American Chemical Society (ACS)","date_created":"2025-12-04T12:06:36Z","title":"Effect of Oxygen-Donor Charge on Adjacent Nitrogen-Donor Interactions in Eu<sup>3+</sup> Complexes of Mixed N,O-Donor Ligands Demonstrated on a 10-Fold [Eu(TPAMEN)]<sup>3+</sup> Chelate Complex","quality_controlled":"1","issue":"4","year":"2021","_id":"62851","department":[{"_id":"985"}],"user_id":"117735","extern":"1","type":"journal_article","status":"public","date_updated":"2025-12-04T12:19:31Z","volume":60,"author":[{"first_name":"Kathleen","last_name":"Schnaars","full_name":"Schnaars, Kathleen","id":"117735"},{"full_name":"Kaneko, Masashi","last_name":"Kaneko","first_name":"Masashi"},{"first_name":"Kiyoshi","last_name":"Fujisawa","full_name":"Fujisawa, Kiyoshi"}],"doi":"10.1021/acs.inorgchem.0c03405","publication_identifier":{"issn":["0020-1669","1520-510X"]},"publication_status":"published","page":"2477-2491","intvolume":"        60","citation":{"chicago":"Schnaars, Kathleen, Masashi Kaneko, and Kiyoshi Fujisawa. “Effect of Oxygen-Donor Charge on Adjacent Nitrogen-Donor Interactions in Eu<sup>3+</sup> Complexes of Mixed N,O-Donor Ligands Demonstrated on a 10-Fold [Eu(TPAMEN)]<sup>3+</sup> Chelate Complex.” <i>Inorganic Chemistry</i> 60, no. 4 (2021): 2477–91. <a href=\"https://doi.org/10.1021/acs.inorgchem.0c03405\">https://doi.org/10.1021/acs.inorgchem.0c03405</a>.","ieee":"K. Schnaars, M. Kaneko, and K. Fujisawa, “Effect of Oxygen-Donor Charge on Adjacent Nitrogen-Donor Interactions in Eu<sup>3+</sup> Complexes of Mixed N,O-Donor Ligands Demonstrated on a 10-Fold [Eu(TPAMEN)]<sup>3+</sup> Chelate Complex,” <i>Inorganic Chemistry</i>, vol. 60, no. 4, pp. 2477–2491, 2021, doi: <a href=\"https://doi.org/10.1021/acs.inorgchem.0c03405\">10.1021/acs.inorgchem.0c03405</a>.","ama":"Schnaars K, Kaneko M, Fujisawa K. Effect of Oxygen-Donor Charge on Adjacent Nitrogen-Donor Interactions in Eu<sup>3+</sup> Complexes of Mixed N,O-Donor Ligands Demonstrated on a 10-Fold [Eu(TPAMEN)]<sup>3+</sup> Chelate Complex. <i>Inorganic Chemistry</i>. 2021;60(4):2477-2491. doi:<a href=\"https://doi.org/10.1021/acs.inorgchem.0c03405\">10.1021/acs.inorgchem.0c03405</a>","apa":"Schnaars, K., Kaneko, M., &#38; Fujisawa, K. (2021). Effect of Oxygen-Donor Charge on Adjacent Nitrogen-Donor Interactions in Eu<sup>3+</sup> Complexes of Mixed N,O-Donor Ligands Demonstrated on a 10-Fold [Eu(TPAMEN)]<sup>3+</sup> Chelate Complex. <i>Inorganic Chemistry</i>, <i>60</i>(4), 2477–2491. <a href=\"https://doi.org/10.1021/acs.inorgchem.0c03405\">https://doi.org/10.1021/acs.inorgchem.0c03405</a>","bibtex":"@article{Schnaars_Kaneko_Fujisawa_2021, title={Effect of Oxygen-Donor Charge on Adjacent Nitrogen-Donor Interactions in Eu<sup>3+</sup> Complexes of Mixed N,O-Donor Ligands Demonstrated on a 10-Fold [Eu(TPAMEN)]<sup>3+</sup> Chelate Complex}, volume={60}, DOI={<a href=\"https://doi.org/10.1021/acs.inorgchem.0c03405\">10.1021/acs.inorgchem.0c03405</a>}, number={4}, journal={Inorganic Chemistry}, publisher={American Chemical Society (ACS)}, author={Schnaars, Kathleen and Kaneko, Masashi and Fujisawa, Kiyoshi}, year={2021}, pages={2477–2491} }","mla":"Schnaars, Kathleen, et al. “Effect of Oxygen-Donor Charge on Adjacent Nitrogen-Donor Interactions in Eu<sup>3+</sup> Complexes of Mixed N,O-Donor Ligands Demonstrated on a 10-Fold [Eu(TPAMEN)]<sup>3+</sup> Chelate Complex.” <i>Inorganic Chemistry</i>, vol. 60, no. 4, American Chemical Society (ACS), 2021, pp. 2477–91, doi:<a href=\"https://doi.org/10.1021/acs.inorgchem.0c03405\">10.1021/acs.inorgchem.0c03405</a>.","short":"K. Schnaars, M. Kaneko, K. Fujisawa, Inorganic Chemistry 60 (2021) 2477–2491."}},{"year":"2020","citation":{"apa":"Scherer, B., Kottenstedde, I. L., Bremser, W., &#38; Matysik, F.-M. (2020). Analytical characterization of polyamide 11 used in the context of selective laser sintering: Physico-chemical correlations. <i>Polymer Testing</i>, Article 106786. <a href=\"https://doi.org/10.1016/j.polymertesting.2020.106786\">https://doi.org/10.1016/j.polymertesting.2020.106786</a>","bibtex":"@article{Scherer_Kottenstedde_Bremser_Matysik_2020, title={Analytical characterization of polyamide 11 used in the context of selective laser sintering: Physico-chemical correlations}, DOI={<a href=\"https://doi.org/10.1016/j.polymertesting.2020.106786\">10.1016/j.polymertesting.2020.106786</a>}, number={106786}, journal={Polymer Testing}, author={Scherer, Beate and Kottenstedde, Ingo Leonard and Bremser, Wolfgang and Matysik, Frank-Michael}, year={2020} }","short":"B. Scherer, I.L. Kottenstedde, W. Bremser, F.-M. Matysik, Polymer Testing (2020).","mla":"Scherer, Beate, et al. “Analytical Characterization of Polyamide 11 Used in the Context of Selective Laser Sintering: Physico-Chemical Correlations.” <i>Polymer Testing</i>, 106786, 2020, doi:<a href=\"https://doi.org/10.1016/j.polymertesting.2020.106786\">10.1016/j.polymertesting.2020.106786</a>.","ieee":"B. Scherer, I. L. Kottenstedde, W. Bremser, and F.-M. Matysik, “Analytical characterization of polyamide 11 used in the context of selective laser sintering: Physico-chemical correlations,” <i>Polymer Testing</i>, Art. no. 106786, 2020, doi: <a href=\"https://doi.org/10.1016/j.polymertesting.2020.106786\">10.1016/j.polymertesting.2020.106786</a>.","chicago":"Scherer, Beate, Ingo Leonard Kottenstedde, Wolfgang Bremser, and Frank-Michael Matysik. “Analytical Characterization of Polyamide 11 Used in the Context of Selective Laser Sintering: Physico-Chemical Correlations.” <i>Polymer Testing</i>, 2020. <a href=\"https://doi.org/10.1016/j.polymertesting.2020.106786\">https://doi.org/10.1016/j.polymertesting.2020.106786</a>.","ama":"Scherer B, Kottenstedde IL, Bremser W, Matysik F-M. Analytical characterization of polyamide 11 used in the context of selective laser sintering: Physico-chemical correlations. <i>Polymer Testing</i>. Published online 2020. doi:<a href=\"https://doi.org/10.1016/j.polymertesting.2020.106786\">10.1016/j.polymertesting.2020.106786</a>"},"publication_status":"published","publication_identifier":{"issn":["0142-9418"]},"title":"Analytical characterization of polyamide 11 used in the context of selective laser sintering: Physico-chemical correlations","doi":"10.1016/j.polymertesting.2020.106786","date_updated":"2022-01-06T06:57:00Z","author":[{"full_name":"Scherer, Beate","last_name":"Scherer","first_name":"Beate"},{"last_name":"Kottenstedde","full_name":"Kottenstedde, Ingo Leonard","first_name":"Ingo Leonard"},{"first_name":"Wolfgang","last_name":"Bremser","full_name":"Bremser, Wolfgang","id":"32"},{"last_name":"Matysik","full_name":"Matysik, Frank-Michael","first_name":"Frank-Michael"}],"date_created":"2021-10-04T13:18:54Z","status":"public","type":"journal_article","publication":"Polymer Testing","article_number":"106786","language":[{"iso":"eng"}],"_id":"25301","user_id":"32","department":[{"_id":"321"},{"_id":"301"}]},{"department":[{"_id":"633"}],"user_id":"84268","_id":"23599","language":[{"iso":"eng"}],"publication":"Journal of Applied Crystallography","type":"journal_article","status":"public","abstract":[{"text":"<jats:p>Grazing-incidence wide-angle X-ray scattering (GIWAXS) has become an increasingly popular technique for quantitative structural characterization and comparison of thin films. For this purpose, accurate intensity normalization and peak position determination are crucial. At present, few tools exist to estimate the uncertainties of these measurements. Here, a simulation package is introduced called <jats:italic>GIWAXS-SIIRkit</jats:italic>, where SIIR stands for scattering intensity, indexing and refraction. The package contains several tools that are freely available for download and can be executed in MATLAB. The package includes three functionalities: estimation of the relative scattering intensity and the corresponding uncertainty based on experimental setup and sample dimensions; extraction and indexing of peak positions to approximate the crystal structure of organic materials starting from calibrated GIWAXS patterns; and analysis of the effects of refraction on peak positions. Each tool is based on a graphical user interface and designed to have a short learning curve. A user guide is provided with detailed usage instruction, tips for adding functionality and customization, and exemplary files.</jats:p>","lang":"eng"}],"volume":53,"date_created":"2021-09-01T09:07:00Z","author":[{"first_name":"Victoria","full_name":"Savikhin, Victoria","last_name":"Savikhin"},{"first_name":"Hans-Georg","id":"84268","full_name":"Steinrück, Hans-Georg","last_name":"Steinrück","orcid":"0000-0001-6373-0877"},{"first_name":"Ru-Ze","full_name":"Liang, Ru-Ze","last_name":"Liang"},{"full_name":"Collins, Brian A.","last_name":"Collins","first_name":"Brian A."},{"full_name":"Oosterhout, Stefan D.","last_name":"Oosterhout","first_name":"Stefan D."},{"first_name":"Pierre M.","full_name":"Beaujuge, Pierre M.","last_name":"Beaujuge"},{"first_name":"Michael F.","last_name":"Toney","full_name":"Toney, Michael F."}],"date_updated":"2022-01-06T06:55:57Z","doi":"10.1107/s1600576720005476","title":"GIWAXS-SIIRkit: scattering intensity, indexing and refraction calculation toolkit for grazing-incidence wide-angle X-ray scattering of organic materials","publication_identifier":{"issn":["1600-5767"]},"publication_status":"published","page":"1108-1129","intvolume":"        53","citation":{"ama":"Savikhin V, Steinrück H-G, Liang R-Z, et al. GIWAXS-SIIRkit: scattering intensity, indexing and refraction calculation toolkit for grazing-incidence wide-angle X-ray scattering of organic materials. <i>Journal of Applied Crystallography</i>. 2020;53:1108-1129. doi:<a href=\"https://doi.org/10.1107/s1600576720005476\">10.1107/s1600576720005476</a>","ieee":"V. Savikhin <i>et al.</i>, “GIWAXS-SIIRkit: scattering intensity, indexing and refraction calculation toolkit for grazing-incidence wide-angle X-ray scattering of organic materials,” <i>Journal of Applied Crystallography</i>, vol. 53, pp. 1108–1129, 2020, doi: <a href=\"https://doi.org/10.1107/s1600576720005476\">10.1107/s1600576720005476</a>.","chicago":"Savikhin, Victoria, Hans-Georg Steinrück, Ru-Ze Liang, Brian A. Collins, Stefan D. Oosterhout, Pierre M. Beaujuge, and Michael F. Toney. “GIWAXS-SIIRkit: Scattering Intensity, Indexing and Refraction Calculation Toolkit for Grazing-Incidence Wide-Angle X-Ray Scattering of Organic Materials.” <i>Journal of Applied Crystallography</i> 53 (2020): 1108–29. <a href=\"https://doi.org/10.1107/s1600576720005476\">https://doi.org/10.1107/s1600576720005476</a>.","apa":"Savikhin, V., Steinrück, H.-G., Liang, R.-Z., Collins, B. A., Oosterhout, S. D., Beaujuge, P. M., &#38; Toney, M. F. (2020). GIWAXS-SIIRkit: scattering intensity, indexing and refraction calculation toolkit for grazing-incidence wide-angle X-ray scattering of organic materials. <i>Journal of Applied Crystallography</i>, <i>53</i>, 1108–1129. <a href=\"https://doi.org/10.1107/s1600576720005476\">https://doi.org/10.1107/s1600576720005476</a>","short":"V. Savikhin, H.-G. Steinrück, R.-Z. Liang, B.A. Collins, S.D. Oosterhout, P.M. Beaujuge, M.F. Toney, Journal of Applied Crystallography 53 (2020) 1108–1129.","mla":"Savikhin, Victoria, et al. “GIWAXS-SIIRkit: Scattering Intensity, Indexing and Refraction Calculation Toolkit for Grazing-Incidence Wide-Angle X-Ray Scattering of Organic Materials.” <i>Journal of Applied Crystallography</i>, vol. 53, 2020, pp. 1108–29, doi:<a href=\"https://doi.org/10.1107/s1600576720005476\">10.1107/s1600576720005476</a>.","bibtex":"@article{Savikhin_Steinrück_Liang_Collins_Oosterhout_Beaujuge_Toney_2020, title={GIWAXS-SIIRkit: scattering intensity, indexing and refraction calculation toolkit for grazing-incidence wide-angle X-ray scattering of organic materials}, volume={53}, DOI={<a href=\"https://doi.org/10.1107/s1600576720005476\">10.1107/s1600576720005476</a>}, journal={Journal of Applied Crystallography}, author={Savikhin, Victoria and Steinrück, Hans-Georg and Liang, Ru-Ze and Collins, Brian A. and Oosterhout, Stefan D. and Beaujuge, Pierre M. and Toney, Michael F.}, year={2020}, pages={1108–1129} }"},"year":"2020"},{"user_id":"84268","department":[{"_id":"633"}],"_id":"23600","language":[{"iso":"eng"}],"type":"journal_article","publication":"Chemistry – A European Journal","status":"public","author":[{"full_name":"Gebers, Jan","last_name":"Gebers","first_name":"Jan"},{"full_name":"Özen, Bilal","last_name":"Özen","first_name":"Bilal"},{"first_name":"Lucia","last_name":"Hartmann","full_name":"Hartmann, Lucia"},{"first_name":"Michel","full_name":"Schaer, Michel","last_name":"Schaer"},{"full_name":"Suàrez, Stéphane","last_name":"Suàrez","first_name":"Stéphane"},{"full_name":"Bugnon, Philippe","last_name":"Bugnon","first_name":"Philippe"},{"first_name":"Rosario","last_name":"Scopelliti","full_name":"Scopelliti, Rosario"},{"first_name":"Hans-Georg","orcid":"0000-0001-6373-0877","last_name":"Steinrück","full_name":"Steinrück, Hans-Georg","id":"84268"},{"first_name":"Oleg","last_name":"Konovalov","full_name":"Konovalov, Oleg"},{"full_name":"Magerl, Andreas","last_name":"Magerl","first_name":"Andreas"},{"last_name":"Brinkmann","full_name":"Brinkmann, Martin","first_name":"Martin"},{"full_name":"Petraglia, Riccardo","last_name":"Petraglia","first_name":"Riccardo"},{"last_name":"Silva","full_name":"Silva, Piotr","first_name":"Piotr"},{"first_name":"Clémence","full_name":"Corminboeuf, Clémence","last_name":"Corminboeuf"},{"first_name":"Holger","last_name":"Frauenrath","full_name":"Frauenrath, Holger"}],"date_created":"2021-09-01T09:07:50Z","volume":26,"date_updated":"2022-01-06T06:55:57Z","doi":"10.1002/chem.201904562","title":"Crystallization and Organic Field‐Effect Transistor Performance of a Hydrogen‐Bonded Quaterthiophene","publication_status":"published","publication_identifier":{"issn":["0947-6539","1521-3765"]},"citation":{"apa":"Gebers, J., Özen, B., Hartmann, L., Schaer, M., Suàrez, S., Bugnon, P., Scopelliti, R., Steinrück, H.-G., Konovalov, O., Magerl, A., Brinkmann, M., Petraglia, R., Silva, P., Corminboeuf, C., &#38; Frauenrath, H. (2020). Crystallization and Organic Field‐Effect Transistor Performance of a Hydrogen‐Bonded Quaterthiophene. <i>Chemistry – A European Journal</i>, <i>26</i>, 10265–10275. <a href=\"https://doi.org/10.1002/chem.201904562\">https://doi.org/10.1002/chem.201904562</a>","mla":"Gebers, Jan, et al. “Crystallization and Organic Field‐Effect Transistor Performance of a Hydrogen‐Bonded Quaterthiophene.” <i>Chemistry – A European Journal</i>, vol. 26, 2020, pp. 10265–75, doi:<a href=\"https://doi.org/10.1002/chem.201904562\">10.1002/chem.201904562</a>.","short":"J. Gebers, B. Özen, L. Hartmann, M. Schaer, S. Suàrez, P. Bugnon, R. Scopelliti, H.-G. Steinrück, O. Konovalov, A. Magerl, M. Brinkmann, R. Petraglia, P. Silva, C. Corminboeuf, H. Frauenrath, Chemistry – A European Journal 26 (2020) 10265–10275.","bibtex":"@article{Gebers_Özen_Hartmann_Schaer_Suàrez_Bugnon_Scopelliti_Steinrück_Konovalov_Magerl_et al._2020, title={Crystallization and Organic Field‐Effect Transistor Performance of a Hydrogen‐Bonded Quaterthiophene}, volume={26}, DOI={<a href=\"https://doi.org/10.1002/chem.201904562\">10.1002/chem.201904562</a>}, journal={Chemistry – A European Journal}, author={Gebers, Jan and Özen, Bilal and Hartmann, Lucia and Schaer, Michel and Suàrez, Stéphane and Bugnon, Philippe and Scopelliti, Rosario and Steinrück, Hans-Georg and Konovalov, Oleg and Magerl, Andreas and et al.}, year={2020}, pages={10265–10275} }","ieee":"J. Gebers <i>et al.</i>, “Crystallization and Organic Field‐Effect Transistor Performance of a Hydrogen‐Bonded Quaterthiophene,” <i>Chemistry – A European Journal</i>, vol. 26, pp. 10265–10275, 2020, doi: <a href=\"https://doi.org/10.1002/chem.201904562\">10.1002/chem.201904562</a>.","chicago":"Gebers, Jan, Bilal Özen, Lucia Hartmann, Michel Schaer, Stéphane Suàrez, Philippe Bugnon, Rosario Scopelliti, et al. “Crystallization and Organic Field‐Effect Transistor Performance of a Hydrogen‐Bonded Quaterthiophene.” <i>Chemistry – A European Journal</i> 26 (2020): 10265–75. <a href=\"https://doi.org/10.1002/chem.201904562\">https://doi.org/10.1002/chem.201904562</a>.","ama":"Gebers J, Özen B, Hartmann L, et al. Crystallization and Organic Field‐Effect Transistor Performance of a Hydrogen‐Bonded Quaterthiophene. <i>Chemistry – A European Journal</i>. 2020;26:10265-10275. doi:<a href=\"https://doi.org/10.1002/chem.201904562\">10.1002/chem.201904562</a>"},"page":"10265-10275","intvolume":"        26","year":"2020"},{"date_created":"2021-09-01T09:08:01Z","author":[{"last_name":"Abdelsamie","full_name":"Abdelsamie, Maged","first_name":"Maged"},{"last_name":"Xu","full_name":"Xu, Junwei","first_name":"Junwei"},{"last_name":"Bruening","full_name":"Bruening, Karsten","first_name":"Karsten"},{"full_name":"Tassone, Christopher J.","last_name":"Tassone","first_name":"Christopher J."},{"last_name":"Steinrück","orcid":"0000-0001-6373-0877","full_name":"Steinrück, Hans-Georg","id":"84268","first_name":"Hans-Georg"},{"full_name":"Toney, Michael F.","last_name":"Toney","first_name":"Michael F."}],"volume":30,"date_updated":"2022-01-06T06:55:57Z","doi":"10.1002/adfm.202001752","title":"Impact of Processing on Structural and Compositional Evolution in Mixed Metal Halide Perovskites during Film Formation","publication_status":"published","publication_identifier":{"issn":["1616-301X","1616-3028"]},"citation":{"ama":"Abdelsamie M, Xu J, Bruening K, Tassone CJ, Steinrück H-G, Toney MF. 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Mackanic, Yuchi Tsao, et al. “Interfacial Speciation Determines Interfacial Chemistry: X‐ray‐Induced Lithium Fluoride Formation from Water‐in‐salt Electrolytes on Solid Surfaces.” <i>Angewandte Chemie International Edition</i> 59 (2020): 23180–87. <a href=\"https://doi.org/10.1002/anie.202007745\">https://doi.org/10.1002/anie.202007745</a>."},"page":"23180-23187","intvolume":"        59","year":"2020","user_id":"84268","department":[{"_id":"633"}],"_id":"23606","language":[{"iso":"eng"}],"type":"journal_article","publication":"Angewandte Chemie International Edition","status":"public"},{"status":"public","abstract":[{"text":"<p>Direct measurements of concentration and velocity profiles in a polymeric lithium-ion battery electrolyte provide insights into the transference number.</p>","lang":"eng"}],"type":"journal_article","publication":"Energy & Environmental Science","language":[{"iso":"eng"}],"user_id":"84268","department":[{"_id":"633"}],"_id":"23607","citation":{"apa":"Steinrück, H.-G., Takacs, C. J., Kim, H.-K., Mackanic, D. G., Holladay, B., Cao, C., Narayanan, S., Dufresne, E. M., Chushkin, Y., Ruta, B., Zontone, F., Will, J., Borodin, O., Sinha, S. K., Srinivasan, V., &#38; Toney, M. F. (2020). Concentration and velocity profiles in a polymeric lithium-ion battery electrolyte. <i>Energy &#38; Environmental Science</i>, <i>13</i>, 4312–4321. <a href=\"https://doi.org/10.1039/d0ee02193h\">https://doi.org/10.1039/d0ee02193h</a>","bibtex":"@article{Steinrück_Takacs_Kim_Mackanic_Holladay_Cao_Narayanan_Dufresne_Chushkin_Ruta_et al._2020, title={Concentration and velocity profiles in a polymeric lithium-ion battery electrolyte}, volume={13}, DOI={<a href=\"https://doi.org/10.1039/d0ee02193h\">10.1039/d0ee02193h</a>}, journal={Energy &#38; Environmental Science}, author={Steinrück, Hans-Georg and Takacs, Christopher J. and Kim, Hong-Keun and Mackanic, David G. and Holladay, Benjamin and Cao, Chuntian and Narayanan, Suresh and Dufresne, Eric M. and Chushkin, Yuriy and Ruta, Beatrice and et al.}, year={2020}, pages={4312–4321} }","short":"H.-G. Steinrück, C.J. Takacs, H.-K. Kim, D.G. Mackanic, B. Holladay, C. Cao, S. Narayanan, E.M. Dufresne, Y. Chushkin, B. Ruta, F. Zontone, J. Will, O. Borodin, S.K. Sinha, V. Srinivasan, M.F. Toney, Energy &#38; Environmental Science 13 (2020) 4312–4321.","mla":"Steinrück, Hans-Georg, et al. “Concentration and Velocity Profiles in a Polymeric Lithium-Ion Battery Electrolyte.” <i>Energy &#38; Environmental Science</i>, vol. 13, 2020, pp. 4312–21, doi:<a href=\"https://doi.org/10.1039/d0ee02193h\">10.1039/d0ee02193h</a>.","ama":"Steinrück H-G, Takacs CJ, Kim H-K, et al. Concentration and velocity profiles in a polymeric lithium-ion battery electrolyte. <i>Energy &#38; Environmental Science</i>. 2020;13:4312-4321. doi:<a href=\"https://doi.org/10.1039/d0ee02193h\">10.1039/d0ee02193h</a>","ieee":"H.-G. Steinrück <i>et al.</i>, “Concentration and velocity profiles in a polymeric lithium-ion battery electrolyte,” <i>Energy &#38; Environmental Science</i>, vol. 13, pp. 4312–4321, 2020, doi: <a href=\"https://doi.org/10.1039/d0ee02193h\">10.1039/d0ee02193h</a>.","chicago":"Steinrück, Hans-Georg, Christopher J. Takacs, Hong-Keun Kim, David G. Mackanic, Benjamin Holladay, Chuntian Cao, Suresh Narayanan, et al. “Concentration and Velocity Profiles in a Polymeric Lithium-Ion Battery Electrolyte.” <i>Energy &#38; Environmental Science</i> 13 (2020): 4312–21. <a href=\"https://doi.org/10.1039/d0ee02193h\">https://doi.org/10.1039/d0ee02193h</a>."},"intvolume":"        13","page":"4312-4321","year":"2020","publication_status":"published","publication_identifier":{"issn":["1754-5692","1754-5706"]},"doi":"10.1039/d0ee02193h","title":"Concentration and velocity profiles in a polymeric lithium-ion battery electrolyte","author":[{"id":"84268","full_name":"Steinrück, Hans-Georg","last_name":"Steinrück","orcid":"0000-0001-6373-0877","first_name":"Hans-Georg"},{"full_name":"Takacs, Christopher J.","last_name":"Takacs","first_name":"Christopher J."},{"first_name":"Hong-Keun","full_name":"Kim, Hong-Keun","last_name":"Kim"},{"first_name":"David G.","full_name":"Mackanic, David G.","last_name":"Mackanic"},{"full_name":"Holladay, Benjamin","last_name":"Holladay","first_name":"Benjamin"},{"last_name":"Cao","full_name":"Cao, Chuntian","first_name":"Chuntian"},{"first_name":"Suresh","full_name":"Narayanan, Suresh","last_name":"Narayanan"},{"first_name":"Eric M.","last_name":"Dufresne","full_name":"Dufresne, Eric M."},{"full_name":"Chushkin, Yuriy","last_name":"Chushkin","first_name":"Yuriy"},{"full_name":"Ruta, Beatrice","last_name":"Ruta","first_name":"Beatrice"},{"first_name":"Federico","full_name":"Zontone, Federico","last_name":"Zontone"},{"first_name":"Johannes","last_name":"Will","full_name":"Will, Johannes"},{"first_name":"Oleg","last_name":"Borodin","full_name":"Borodin, Oleg"},{"last_name":"Sinha","full_name":"Sinha, Sunil K.","first_name":"Sunil K."},{"last_name":"Srinivasan","full_name":"Srinivasan, Venkat","first_name":"Venkat"},{"first_name":"Michael F.","full_name":"Toney, Michael F.","last_name":"Toney"}],"date_created":"2021-09-01T09:08:45Z","volume":13,"date_updated":"2022-01-06T06:55:57Z"},{"language":[{"iso":"eng"}],"department":[{"_id":"633"}],"user_id":"84268","_id":"23608","status":"public","publication":"Langmuir","type":"journal_article","doi":"10.1021/acs.langmuir.0c02745","title":"Interface between Water–Solvent Mixtures and a Hydrophobic Surface","volume":36,"date_created":"2021-09-01T09:08:51Z","author":[{"last_name":"Prihoda","full_name":"Prihoda, Annemarie","first_name":"Annemarie"},{"first_name":"Johannes","full_name":"Will, Johannes","last_name":"Will"},{"first_name":"Patrick","full_name":"Duchstein, Patrick","last_name":"Duchstein"},{"full_name":"Becit, Bahanur","last_name":"Becit","first_name":"Bahanur"},{"first_name":"Felix","full_name":"Lossin, Felix","last_name":"Lossin"},{"first_name":"Torben","last_name":"Schindler","full_name":"Schindler, Torben"},{"first_name":"Marvin","full_name":"Berlinghof, Marvin","last_name":"Berlinghof"},{"first_name":"Hans-Georg","full_name":"Steinrück, Hans-Georg","id":"84268","last_name":"Steinrück","orcid":"0000-0001-6373-0877"},{"full_name":"Bertram, Florian","last_name":"Bertram","first_name":"Florian"},{"first_name":"Dirk","last_name":"Zahn","full_name":"Zahn, Dirk"},{"full_name":"Unruh, Tobias","last_name":"Unruh","first_name":"Tobias"}],"date_updated":"2022-01-06T06:55:57Z","page":"12077-12086","intvolume":"        36","citation":{"ama":"Prihoda A, Will J, Duchstein P, et al. Interface between Water–Solvent Mixtures and a Hydrophobic Surface. <i>Langmuir</i>. 2020;36:12077-12086. doi:<a href=\"https://doi.org/10.1021/acs.langmuir.0c02745\">10.1021/acs.langmuir.0c02745</a>","chicago":"Prihoda, Annemarie, Johannes Will, Patrick Duchstein, Bahanur Becit, Felix Lossin, Torben Schindler, Marvin Berlinghof, et al. “Interface between Water–Solvent Mixtures and a Hydrophobic Surface.” <i>Langmuir</i> 36 (2020): 12077–86. <a href=\"https://doi.org/10.1021/acs.langmuir.0c02745\">https://doi.org/10.1021/acs.langmuir.0c02745</a>.","ieee":"A. Prihoda <i>et al.</i>, “Interface between Water–Solvent Mixtures and a Hydrophobic Surface,” <i>Langmuir</i>, vol. 36, pp. 12077–12086, 2020, doi: <a href=\"https://doi.org/10.1021/acs.langmuir.0c02745\">10.1021/acs.langmuir.0c02745</a>.","apa":"Prihoda, A., Will, J., Duchstein, P., Becit, B., Lossin, F., Schindler, T., Berlinghof, M., Steinrück, H.-G., Bertram, F., Zahn, D., &#38; Unruh, T. (2020). Interface between Water–Solvent Mixtures and a Hydrophobic Surface. <i>Langmuir</i>, <i>36</i>, 12077–12086. <a href=\"https://doi.org/10.1021/acs.langmuir.0c02745\">https://doi.org/10.1021/acs.langmuir.0c02745</a>","short":"A. Prihoda, J. Will, P. Duchstein, B. Becit, F. Lossin, T. Schindler, M. Berlinghof, H.-G. Steinrück, F. Bertram, D. Zahn, T. Unruh, Langmuir 36 (2020) 12077–12086.","bibtex":"@article{Prihoda_Will_Duchstein_Becit_Lossin_Schindler_Berlinghof_Steinrück_Bertram_Zahn_et al._2020, title={Interface between Water–Solvent Mixtures and a Hydrophobic Surface}, volume={36}, DOI={<a href=\"https://doi.org/10.1021/acs.langmuir.0c02745\">10.1021/acs.langmuir.0c02745</a>}, journal={Langmuir}, author={Prihoda, Annemarie and Will, Johannes and Duchstein, Patrick and Becit, Bahanur and Lossin, Felix and Schindler, Torben and Berlinghof, Marvin and Steinrück, Hans-Georg and Bertram, Florian and Zahn, Dirk and et al.}, year={2020}, pages={12077–12086} }","mla":"Prihoda, Annemarie, et al. “Interface between Water–Solvent Mixtures and a Hydrophobic Surface.” <i>Langmuir</i>, vol. 36, 2020, pp. 12077–86, doi:<a href=\"https://doi.org/10.1021/acs.langmuir.0c02745\">10.1021/acs.langmuir.0c02745</a>."},"year":"2020","publication_identifier":{"issn":["0743-7463","1520-5827"]},"publication_status":"published"},{"type":"journal_article","publication":"Joule","status":"public","_id":"23617","user_id":"84268","department":[{"_id":"633"}],"language":[{"iso":"eng"}],"publication_status":"published","publication_identifier":{"issn":["2542-4351"]},"year":"2020","citation":{"ama":"Chen H, Pei A, Wan J, et al. Tortuosity Effects in Lithium-Metal Host Anodes. <i>Joule</i>. 2020;4:938-952. doi:<a href=\"https://doi.org/10.1016/j.joule.2020.03.008\">10.1016/j.joule.2020.03.008</a>","ieee":"H. Chen <i>et al.</i>, “Tortuosity Effects in Lithium-Metal Host Anodes,” <i>Joule</i>, vol. 4, pp. 938–952, 2020, doi: <a href=\"https://doi.org/10.1016/j.joule.2020.03.008\">10.1016/j.joule.2020.03.008</a>.","chicago":"Chen, Hao, Allen Pei, Jiayu Wan, Dingchang Lin, Rafael Vilá, Hongxia Wang, David Mackanic, et al. “Tortuosity Effects in Lithium-Metal Host Anodes.” <i>Joule</i> 4 (2020): 938–52. <a href=\"https://doi.org/10.1016/j.joule.2020.03.008\">https://doi.org/10.1016/j.joule.2020.03.008</a>.","apa":"Chen, H., Pei, A., Wan, J., Lin, D., Vilá, R., Wang, H., Mackanic, D., Steinrück, H.-G., Huang, W., Li, Y., Yang, A., Xie, J., Wu, Y., Wang, H., &#38; Cui, Y. (2020). Tortuosity Effects in Lithium-Metal Host Anodes. <i>Joule</i>, <i>4</i>, 938–952. <a href=\"https://doi.org/10.1016/j.joule.2020.03.008\">https://doi.org/10.1016/j.joule.2020.03.008</a>","short":"H. Chen, A. Pei, J. Wan, D. Lin, R. Vilá, H. Wang, D. Mackanic, H.-G. Steinrück, W. Huang, Y. Li, A. Yang, J. Xie, Y. Wu, H. Wang, Y. Cui, Joule 4 (2020) 938–952.","bibtex":"@article{Chen_Pei_Wan_Lin_Vilá_Wang_Mackanic_Steinrück_Huang_Li_et al._2020, title={Tortuosity Effects in Lithium-Metal Host Anodes}, volume={4}, DOI={<a href=\"https://doi.org/10.1016/j.joule.2020.03.008\">10.1016/j.joule.2020.03.008</a>}, journal={Joule}, author={Chen, Hao and Pei, Allen and Wan, Jiayu and Lin, Dingchang and Vilá, Rafael and Wang, Hongxia and Mackanic, David and Steinrück, Hans-Georg and Huang, William and Li, Yuzhang and et al.}, year={2020}, pages={938–952} }","mla":"Chen, Hao, et al. “Tortuosity Effects in Lithium-Metal Host Anodes.” <i>Joule</i>, vol. 4, 2020, pp. 938–52, doi:<a href=\"https://doi.org/10.1016/j.joule.2020.03.008\">10.1016/j.joule.2020.03.008</a>."},"page":"938-952","intvolume":"         4","date_updated":"2022-01-06T06:55:57Z","date_created":"2021-09-01T09:46:28Z","author":[{"first_name":"Hao","last_name":"Chen","full_name":"Chen, Hao"},{"first_name":"Allen","full_name":"Pei, Allen","last_name":"Pei"},{"first_name":"Jiayu","full_name":"Wan, Jiayu","last_name":"Wan"},{"last_name":"Lin","full_name":"Lin, Dingchang","first_name":"Dingchang"},{"last_name":"Vilá","full_name":"Vilá, Rafael","first_name":"Rafael"},{"first_name":"Hongxia","last_name":"Wang","full_name":"Wang, Hongxia"},{"full_name":"Mackanic, David","last_name":"Mackanic","first_name":"David"},{"full_name":"Steinrück, Hans-Georg","id":"84268","orcid":"0000-0001-6373-0877","last_name":"Steinrück","first_name":"Hans-Georg"},{"first_name":"William","last_name":"Huang","full_name":"Huang, William"},{"last_name":"Li","full_name":"Li, Yuzhang","first_name":"Yuzhang"},{"full_name":"Yang, Ankun","last_name":"Yang","first_name":"Ankun"},{"full_name":"Xie, Jin","last_name":"Xie","first_name":"Jin"},{"first_name":"Yecun","last_name":"Wu","full_name":"Wu, Yecun"},{"full_name":"Wang, Hansen","last_name":"Wang","first_name":"Hansen"},{"first_name":"Yi","full_name":"Cui, Yi","last_name":"Cui"}],"volume":4,"title":"Tortuosity Effects in Lithium-Metal Host Anodes","doi":"10.1016/j.joule.2020.03.008"},{"language":[{"iso":"eng"}],"department":[{"_id":"633"}],"user_id":"84268","_id":"23618","status":"public","publication":"The Journal of Chemical Physics","type":"journal_article","doi":"10.1063/1.5142643","title":"Toward quantifying capacity losses due to solid electrolyte interphase evolution in silicon thin film batteries","volume":152,"date_created":"2021-09-01T09:46:33Z","author":[{"first_name":"Hans-Georg","orcid":"0000-0001-6373-0877","last_name":"Steinrück","full_name":"Steinrück, Hans-Georg","id":"84268"},{"full_name":"Cao, Chuntian","last_name":"Cao","first_name":"Chuntian"},{"full_name":"Veith, Gabriel M.","last_name":"Veith","first_name":"Gabriel M."},{"first_name":"Michael F.","last_name":"Toney","full_name":"Toney, Michael F."}],"date_updated":"2022-01-06T06:55:57Z","page":"084702","intvolume":"       152","citation":{"ama":"Steinrück H-G, Cao C, Veith GM, Toney MF. Toward quantifying capacity losses due to solid electrolyte interphase evolution in silicon thin film batteries. <i>The Journal of Chemical Physics</i>. 2020;152:084702. doi:<a href=\"https://doi.org/10.1063/1.5142643\">10.1063/1.5142643</a>","chicago":"Steinrück, Hans-Georg, Chuntian Cao, Gabriel M. Veith, and Michael F. Toney. “Toward Quantifying Capacity Losses Due to Solid Electrolyte Interphase Evolution in Silicon Thin Film Batteries.” <i>The Journal of Chemical Physics</i> 152 (2020): 084702. <a href=\"https://doi.org/10.1063/1.5142643\">https://doi.org/10.1063/1.5142643</a>.","ieee":"H.-G. Steinrück, C. Cao, G. M. Veith, and M. F. Toney, “Toward quantifying capacity losses due to solid electrolyte interphase evolution in silicon thin film batteries,” <i>The Journal of Chemical Physics</i>, vol. 152, p. 084702, 2020, doi: <a href=\"https://doi.org/10.1063/1.5142643\">10.1063/1.5142643</a>.","short":"H.-G. Steinrück, C. Cao, G.M. Veith, M.F. Toney, The Journal of Chemical Physics 152 (2020) 084702.","mla":"Steinrück, Hans-Georg, et al. “Toward Quantifying Capacity Losses Due to Solid Electrolyte Interphase Evolution in Silicon Thin Film Batteries.” <i>The Journal of Chemical Physics</i>, vol. 152, 2020, p. 084702, doi:<a href=\"https://doi.org/10.1063/1.5142643\">10.1063/1.5142643</a>.","bibtex":"@article{Steinrück_Cao_Veith_Toney_2020, title={Toward quantifying capacity losses due to solid electrolyte interphase evolution in silicon thin film batteries}, volume={152}, DOI={<a href=\"https://doi.org/10.1063/1.5142643\">10.1063/1.5142643</a>}, journal={The Journal of Chemical Physics}, author={Steinrück, Hans-Georg and Cao, Chuntian and Veith, Gabriel M. and Toney, Michael F.}, year={2020}, pages={084702} }","apa":"Steinrück, H.-G., Cao, C., Veith, G. M., &#38; Toney, M. F. (2020). Toward quantifying capacity losses due to solid electrolyte interphase evolution in silicon thin film batteries. <i>The Journal of Chemical Physics</i>, <i>152</i>, 084702. <a href=\"https://doi.org/10.1063/1.5142643\">https://doi.org/10.1063/1.5142643</a>"},"year":"2020","publication_identifier":{"issn":["0021-9606","1089-7690"]},"publication_status":"published"},{"user_id":"48864","department":[{"_id":"302"}],"_id":"22644","language":[{"iso":"eng"}],"type":"journal_article","publication":"Nanomaterials","status":"public","abstract":[{"lang":"eng","text":"<jats:p>The aggregation of human islet amyloid polypeptide (hIAPP) plays a major role in the pathogenesis of type 2 diabetes mellitus (T2DM), and numerous strategies for controlling hIAPP aggregation have been investigated so far. In particular, several organic and inorganic nanoparticles (NPs) have shown the potential to influence the aggregation of hIAPP and other amyloidogenic proteins and peptides. In addition to conventional NPs, DNA nanostructures are receiving more and more attention from the biomedical field. Therefore, in this work, we investigated the effects of two different DNA origami nanostructures on hIAPP aggregation. To this end, we employed in situ turbidity measurements and ex situ atomic force microscopy (AFM). The turbidity measurements revealed a retarding effect of the DNA nanostructures on hIAPP aggregation, while the AFM results showed the co-aggregation of hIAPP with the DNA origami nanostructures into hybrid peptide–DNA aggregates. We assume that this was caused by strong electrostatic interactions between the negatively charged DNA origami nanostructures and the positively charged peptide. Most intriguingly, the influence of the DNA origami nanostructures on hIAPP aggregation differed from that of genomic double-stranded DNA (dsDNA) and appeared to depend on DNA origami superstructure. DNA origami nanostructures may thus represent a novel route for modulating amyloid aggregation in vivo.</jats:p>"}],"author":[{"last_name":"Hanke","full_name":"Hanke, Marcel","first_name":"Marcel"},{"last_name":"Gonzalez Orive","full_name":"Gonzalez Orive, Alejandro","first_name":"Alejandro"},{"full_name":"Grundmeier, Guido","id":"194","last_name":"Grundmeier","first_name":"Guido"},{"last_name":"Keller","orcid":"0000-0001-7139-3110","full_name":"Keller, Adrian","id":"48864","first_name":"Adrian"}],"date_created":"2021-07-08T11:59:01Z","volume":10,"date_updated":"2022-01-06T06:55:37Z","doi":"10.3390/nano10112200","title":"Effect of DNA Origami Nanostructures on hIAPP Aggregation","publication_status":"published","publication_identifier":{"issn":["2079-4991"]},"citation":{"chicago":"Hanke, Marcel, Alejandro Gonzalez Orive, Guido Grundmeier, and Adrian Keller. “Effect of DNA Origami Nanostructures on HIAPP Aggregation.” <i>Nanomaterials</i> 10 (2020): 2200. <a href=\"https://doi.org/10.3390/nano10112200\">https://doi.org/10.3390/nano10112200</a>.","ieee":"M. Hanke, A. Gonzalez Orive, G. Grundmeier, and A. Keller, “Effect of DNA Origami Nanostructures on hIAPP Aggregation,” <i>Nanomaterials</i>, vol. 10, p. 2200, 2020.","ama":"Hanke M, Gonzalez Orive A, Grundmeier G, Keller A. Effect of DNA Origami Nanostructures on hIAPP Aggregation. <i>Nanomaterials</i>. 2020;10:2200. doi:<a href=\"https://doi.org/10.3390/nano10112200\">10.3390/nano10112200</a>","bibtex":"@article{Hanke_Gonzalez Orive_Grundmeier_Keller_2020, title={Effect of DNA Origami Nanostructures on hIAPP Aggregation}, volume={10}, DOI={<a href=\"https://doi.org/10.3390/nano10112200\">10.3390/nano10112200</a>}, journal={Nanomaterials}, author={Hanke, Marcel and Gonzalez Orive, Alejandro and Grundmeier, Guido and Keller, Adrian}, year={2020}, pages={2200} }","short":"M. Hanke, A. Gonzalez Orive, G. Grundmeier, A. Keller, Nanomaterials 10 (2020) 2200.","mla":"Hanke, Marcel, et al. “Effect of DNA Origami Nanostructures on HIAPP Aggregation.” <i>Nanomaterials</i>, vol. 10, 2020, p. 2200, doi:<a href=\"https://doi.org/10.3390/nano10112200\">10.3390/nano10112200</a>.","apa":"Hanke, M., Gonzalez Orive, A., Grundmeier, G., &#38; Keller, A. (2020). Effect of DNA Origami Nanostructures on hIAPP Aggregation. <i>Nanomaterials</i>, <i>10</i>, 2200. <a href=\"https://doi.org/10.3390/nano10112200\">https://doi.org/10.3390/nano10112200</a>"},"page":"2200","intvolume":"        10","year":"2020"},{"status":"public","abstract":[{"text":"<jats:p>Immobile Holliday junctions represent not only the most fundamental building block of structural DNA nanotechnology but are also of tremendous importance for the in vitro investigation of genetic recombination and epigenetics. Here, we present a detailed study on the room-temperature assembly of immobile Holliday junctions with the help of the single-strand annealing protein Redβ. Individual DNA single strands are initially coated with protein monomers and subsequently hybridized to form a rigid blunt-ended four-arm junction. We investigate the efficiency of this approach for different DNA/protein ratios, as well as for different DNA sequence lengths. Furthermore, we also evaluate the potential of Redβ to anneal sticky-end modified Holliday junctions into hierarchical assemblies. We demonstrate the Redβ-mediated annealing of Holliday junction dimers, multimers, and extended networks several microns in size. While these hybrid DNA–protein nanostructures may find applications in the crystallization of DNA–protein complexes, our work shows the great potential of Redβ to aid in the synthesis of functional DNA nanostructures under mild reaction conditions.</jats:p>","lang":"eng"}],"publication":"Molecules","type":"journal_article","language":[{"iso":"eng"}],"department":[{"_id":"302"}],"user_id":"48864","_id":"22645","intvolume":"        25","page":"5099","citation":{"ama":"Ramakrishnan S, Subramaniam S, Kielar C, Grundmeier G, Stewart AF, Keller A. Protein-Assisted Room-Temperature Assembly of Rigid, Immobile Holliday Junctions and Hierarchical DNA Nanostructures. <i>Molecules</i>. 2020;25:5099. doi:<a href=\"https://doi.org/10.3390/molecules25215099\">10.3390/molecules25215099</a>","chicago":"Ramakrishnan, Saminathan, Sivaraman Subramaniam, Charlotte Kielar, Guido Grundmeier, A. Francis Stewart, and Adrian Keller. “Protein-Assisted Room-Temperature Assembly of Rigid, Immobile Holliday Junctions and Hierarchical DNA Nanostructures.” <i>Molecules</i> 25 (2020): 5099. <a href=\"https://doi.org/10.3390/molecules25215099\">https://doi.org/10.3390/molecules25215099</a>.","ieee":"S. Ramakrishnan, S. Subramaniam, C. Kielar, G. Grundmeier, A. F. Stewart, and A. Keller, “Protein-Assisted Room-Temperature Assembly of Rigid, Immobile Holliday Junctions and Hierarchical DNA Nanostructures,” <i>Molecules</i>, vol. 25, p. 5099, 2020.","apa":"Ramakrishnan, S., Subramaniam, S., Kielar, C., Grundmeier, G., Stewart, A. F., &#38; Keller, A. (2020). Protein-Assisted Room-Temperature Assembly of Rigid, Immobile Holliday Junctions and Hierarchical DNA Nanostructures. <i>Molecules</i>, <i>25</i>, 5099. <a href=\"https://doi.org/10.3390/molecules25215099\">https://doi.org/10.3390/molecules25215099</a>","mla":"Ramakrishnan, Saminathan, et al. “Protein-Assisted Room-Temperature Assembly of Rigid, Immobile Holliday Junctions and Hierarchical DNA Nanostructures.” <i>Molecules</i>, vol. 25, 2020, p. 5099, doi:<a href=\"https://doi.org/10.3390/molecules25215099\">10.3390/molecules25215099</a>.","short":"S. Ramakrishnan, S. Subramaniam, C. Kielar, G. Grundmeier, A.F. Stewart, A. Keller, Molecules 25 (2020) 5099.","bibtex":"@article{Ramakrishnan_Subramaniam_Kielar_Grundmeier_Stewart_Keller_2020, title={Protein-Assisted Room-Temperature Assembly of Rigid, Immobile Holliday Junctions and Hierarchical DNA Nanostructures}, volume={25}, DOI={<a href=\"https://doi.org/10.3390/molecules25215099\">10.3390/molecules25215099</a>}, journal={Molecules}, author={Ramakrishnan, Saminathan and Subramaniam, Sivaraman and Kielar, Charlotte and Grundmeier, Guido and Stewart, A. Francis and Keller, Adrian}, year={2020}, pages={5099} }"},"year":"2020","publication_identifier":{"issn":["1420-3049"]},"publication_status":"published","doi":"10.3390/molecules25215099","title":"Protein-Assisted Room-Temperature Assembly of Rigid, Immobile Holliday Junctions and Hierarchical DNA Nanostructures","volume":25,"date_created":"2021-07-08T11:59:55Z","author":[{"last_name":"Ramakrishnan","full_name":"Ramakrishnan, Saminathan","first_name":"Saminathan"},{"last_name":"Subramaniam","full_name":"Subramaniam, Sivaraman","first_name":"Sivaraman"},{"last_name":"Kielar","full_name":"Kielar, Charlotte","first_name":"Charlotte"},{"last_name":"Grundmeier","id":"194","full_name":"Grundmeier, Guido","first_name":"Guido"},{"full_name":"Stewart, A. Francis","last_name":"Stewart","first_name":"A. Francis"},{"id":"48864","full_name":"Keller, Adrian","orcid":"0000-0001-7139-3110","last_name":"Keller","first_name":"Adrian"}],"date_updated":"2022-01-06T06:55:37Z"},{"year":"2020","citation":{"apa":"Xin, Y., Martinez Rivadeneira, S., Grundmeier, G., Castro, M., &#38; Keller, A. (2020). Self-assembly of highly ordered DNA origami lattices at solid-liquid interfaces by controlling cation binding and exchange. <i>Nano Research</i>, <i>13</i>, 3142–3150. <a href=\"https://doi.org/10.1007/s12274-020-2985-4\">https://doi.org/10.1007/s12274-020-2985-4</a>","bibtex":"@article{Xin_Martinez Rivadeneira_Grundmeier_Castro_Keller_2020, title={Self-assembly of highly ordered DNA origami lattices at solid-liquid interfaces by controlling cation binding and exchange}, volume={13}, DOI={<a href=\"https://doi.org/10.1007/s12274-020-2985-4\">10.1007/s12274-020-2985-4</a>}, journal={Nano Research}, author={Xin, Yang and Martinez Rivadeneira, Salvador and Grundmeier, Guido and Castro, Mario and Keller, Adrian}, year={2020}, pages={3142–3150} }","mla":"Xin, Yang, et al. “Self-Assembly of Highly Ordered DNA Origami Lattices at Solid-Liquid Interfaces by Controlling Cation Binding and Exchange.” <i>Nano Research</i>, vol. 13, 2020, pp. 3142–50, doi:<a href=\"https://doi.org/10.1007/s12274-020-2985-4\">10.1007/s12274-020-2985-4</a>.","short":"Y. Xin, S. Martinez Rivadeneira, G. Grundmeier, M. Castro, A. Keller, Nano Research 13 (2020) 3142–3150.","ama":"Xin Y, Martinez Rivadeneira S, Grundmeier G, Castro M, Keller A. Self-assembly of highly ordered DNA origami lattices at solid-liquid interfaces by controlling cation binding and exchange. <i>Nano Research</i>. 2020;13:3142-3150. doi:<a href=\"https://doi.org/10.1007/s12274-020-2985-4\">10.1007/s12274-020-2985-4</a>","chicago":"Xin, Yang, Salvador Martinez Rivadeneira, Guido Grundmeier, Mario Castro, and Adrian Keller. “Self-Assembly of Highly Ordered DNA Origami Lattices at Solid-Liquid Interfaces by Controlling Cation Binding and Exchange.” <i>Nano Research</i> 13 (2020): 3142–50. <a href=\"https://doi.org/10.1007/s12274-020-2985-4\">https://doi.org/10.1007/s12274-020-2985-4</a>.","ieee":"Y. Xin, S. Martinez Rivadeneira, G. Grundmeier, M. Castro, and A. Keller, “Self-assembly of highly ordered DNA origami lattices at solid-liquid interfaces by controlling cation binding and exchange,” <i>Nano Research</i>, vol. 13, pp. 3142–3150, 2020."},"intvolume":"        13","page":"3142-3150","publication_status":"published","publication_identifier":{"issn":["1998-0124","1998-0000"]},"title":"Self-assembly of highly ordered DNA origami lattices at solid-liquid interfaces by controlling cation binding and exchange","doi":"10.1007/s12274-020-2985-4","date_updated":"2022-01-06T06:55:37Z","author":[{"first_name":"Yang","full_name":"Xin, Yang","last_name":"Xin"},{"full_name":"Martinez Rivadeneira, Salvador","last_name":"Martinez Rivadeneira","first_name":"Salvador"},{"full_name":"Grundmeier, Guido","id":"194","last_name":"Grundmeier","first_name":"Guido"},{"first_name":"Mario","last_name":"Castro","full_name":"Castro, Mario"},{"last_name":"Keller","orcid":"0000-0001-7139-3110","id":"48864","full_name":"Keller, Adrian","first_name":"Adrian"}],"date_created":"2021-07-08T12:01:03Z","volume":13,"abstract":[{"lang":"eng","text":"<jats:title>Abstract</jats:title>\r\n<jats:p>The surface-assisted hierarchical self-assembly of DNA origami lattices represents a versatile and straightforward method for the organization of functional nanoscale objects such as proteins and nanoparticles. Here, we demonstrate that controlling the binding and exchange of different monovalent and divalent cation species at the DNA-mica interface enables the self-assembly of highly ordered DNA origami lattices on mica surfaces. The development of lattice quality and order is quantified by a detailed topological analysis of high-speed atomic force microscopy (HS-AFM) images. We find that lattice formation and quality strongly depend on the monovalent cation species. Na<jats:sup>+</jats:sup> is more effective than Li<jats:sup>+</jats:sup> and K<jats:sup>+</jats:sup> in facilitating the assembly of high-quality DNA origami lattices, because it is replacing the divalent cations at their binding sites in the DNA backbone more efficiently. With regard to divalent cations, Ca<jats:sup>2+</jats:sup> can be displaced more easily from the backbone phosphates than Mg<jats:sup>2+</jats:sup> and is thus superior in guiding lattice assembly. By independently adjusting incubation time, DNA origami concentration, and cation species, we thus obtain a highly ordered DNA origami lattice with an unprecedented normalized correlation length of 8.2. Beyond the correlation length, we use computer vision algorithms to compute the time course of different topological observables that, overall, demonstrate that replacing MgCl<jats:sub>2</jats:sub> by CaCl<jats:sub>2</jats:sub> enables the synthesis of DNA origami lattices with drastically increased lattice order.</jats:p>"}],"status":"public","type":"journal_article","publication":"Nano Research","language":[{"iso":"eng"}],"_id":"22646","user_id":"48864","department":[{"_id":"302"}]},{"title":"Quantitative Assessment of Tip Effects in Single‐Molecule High‐Speed Atomic Force Microscopy Using DNA Origami Substrates","doi":"10.1002/anie.202005884","date_updated":"2022-01-06T06:55:38Z","volume":59,"author":[{"first_name":"Charlotte","full_name":"Kielar, Charlotte","last_name":"Kielar"},{"first_name":"Siqi","full_name":"Zhu, Siqi","last_name":"Zhu"},{"last_name":"Grundmeier","full_name":"Grundmeier, Guido","id":"194","first_name":"Guido"},{"full_name":"Keller, Adrian","id":"48864","orcid":"0000-0001-7139-3110","last_name":"Keller","first_name":"Adrian"}],"date_created":"2021-07-08T12:03:01Z","year":"2020","intvolume":"        59","page":"14336-14341","citation":{"mla":"Kielar, Charlotte, et al. “Quantitative Assessment of Tip Effects in Single‐Molecule High‐Speed Atomic Force Microscopy Using DNA Origami Substrates.” <i>Angewandte Chemie International Edition</i>, vol. 59, 2020, pp. 14336–41, doi:<a href=\"https://doi.org/10.1002/anie.202005884\">10.1002/anie.202005884</a>.","bibtex":"@article{Kielar_Zhu_Grundmeier_Keller_2020, title={Quantitative Assessment of Tip Effects in Single‐Molecule High‐Speed Atomic Force Microscopy Using DNA Origami Substrates}, volume={59}, DOI={<a href=\"https://doi.org/10.1002/anie.202005884\">10.1002/anie.202005884</a>}, journal={Angewandte Chemie International Edition}, author={Kielar, Charlotte and Zhu, Siqi and Grundmeier, Guido and Keller, Adrian}, year={2020}, pages={14336–14341} }","short":"C. Kielar, S. Zhu, G. Grundmeier, A. Keller, Angewandte Chemie International Edition 59 (2020) 14336–14341.","apa":"Kielar, C., Zhu, S., Grundmeier, G., &#38; Keller, A. (2020). Quantitative Assessment of Tip Effects in Single‐Molecule High‐Speed Atomic Force Microscopy Using DNA Origami Substrates. <i>Angewandte Chemie International Edition</i>, <i>59</i>, 14336–14341. <a href=\"https://doi.org/10.1002/anie.202005884\">https://doi.org/10.1002/anie.202005884</a>","chicago":"Kielar, Charlotte, Siqi Zhu, Guido Grundmeier, and Adrian Keller. “Quantitative Assessment of Tip Effects in Single‐Molecule High‐Speed Atomic Force Microscopy Using DNA Origami Substrates.” <i>Angewandte Chemie International Edition</i> 59 (2020): 14336–41. <a href=\"https://doi.org/10.1002/anie.202005884\">https://doi.org/10.1002/anie.202005884</a>.","ieee":"C. Kielar, S. Zhu, G. Grundmeier, and A. Keller, “Quantitative Assessment of Tip Effects in Single‐Molecule High‐Speed Atomic Force Microscopy Using DNA Origami Substrates,” <i>Angewandte Chemie International Edition</i>, vol. 59, pp. 14336–14341, 2020.","ama":"Kielar C, Zhu S, Grundmeier G, Keller A. Quantitative Assessment of Tip Effects in Single‐Molecule High‐Speed Atomic Force Microscopy Using DNA Origami Substrates. <i>Angewandte Chemie International Edition</i>. 2020;59:14336-14341. doi:<a href=\"https://doi.org/10.1002/anie.202005884\">10.1002/anie.202005884</a>"},"publication_identifier":{"issn":["1433-7851","1521-3773"]},"publication_status":"published","language":[{"iso":"eng"}],"_id":"22647","department":[{"_id":"302"}],"user_id":"48864","status":"public","publication":"Angewandte Chemie International Edition","type":"journal_article"},{"status":"public","abstract":[{"lang":"eng","text":"<p>DNA origami lattice formation at solid–liquid interfaces is surprisingly resilient toward the incorporation of DNA origami impurities with different shapes.</p>"}],"type":"journal_article","publication":"Nanoscale","language":[{"iso":"eng"}],"user_id":"48864","department":[{"_id":"302"}],"_id":"22648","citation":{"ieee":"Y. Xin, X. Ji, G. Grundmeier, and A. Keller, “Dynamics of lattice defects in mixed DNA origami monolayers,” <i>Nanoscale</i>, vol. 12, pp. 9733–9743, 2020.","chicago":"Xin, Yang, Xueyin Ji, Guido Grundmeier, and Adrian Keller. “Dynamics of Lattice Defects in Mixed DNA Origami Monolayers.” <i>Nanoscale</i> 12 (2020): 9733–43. <a href=\"https://doi.org/10.1039/d0nr01252a\">https://doi.org/10.1039/d0nr01252a</a>.","ama":"Xin Y, Ji X, Grundmeier G, Keller A. Dynamics of lattice defects in mixed DNA origami monolayers. <i>Nanoscale</i>. 2020;12:9733-9743. doi:<a href=\"https://doi.org/10.1039/d0nr01252a\">10.1039/d0nr01252a</a>","apa":"Xin, Y., Ji, X., Grundmeier, G., &#38; Keller, A. (2020). Dynamics of lattice defects in mixed DNA origami monolayers. <i>Nanoscale</i>, <i>12</i>, 9733–9743. <a href=\"https://doi.org/10.1039/d0nr01252a\">https://doi.org/10.1039/d0nr01252a</a>","bibtex":"@article{Xin_Ji_Grundmeier_Keller_2020, title={Dynamics of lattice defects in mixed DNA origami monolayers}, volume={12}, DOI={<a href=\"https://doi.org/10.1039/d0nr01252a\">10.1039/d0nr01252a</a>}, journal={Nanoscale}, author={Xin, Yang and Ji, Xueyin and Grundmeier, Guido and Keller, Adrian}, year={2020}, pages={9733–9743} }","mla":"Xin, Yang, et al. “Dynamics of Lattice Defects in Mixed DNA Origami Monolayers.” <i>Nanoscale</i>, vol. 12, 2020, pp. 9733–43, doi:<a href=\"https://doi.org/10.1039/d0nr01252a\">10.1039/d0nr01252a</a>.","short":"Y. Xin, X. Ji, G. Grundmeier, A. Keller, Nanoscale 12 (2020) 9733–9743."},"page":"9733-9743","intvolume":"        12","year":"2020","publication_status":"published","publication_identifier":{"issn":["2040-3364","2040-3372"]},"doi":"10.1039/d0nr01252a","title":"Dynamics of lattice defects in mixed DNA origami monolayers","author":[{"first_name":"Yang","last_name":"Xin","full_name":"Xin, Yang"},{"full_name":"Ji, Xueyin","last_name":"Ji","first_name":"Xueyin"},{"first_name":"Guido","full_name":"Grundmeier, Guido","id":"194","last_name":"Grundmeier"},{"first_name":"Adrian","id":"48864","full_name":"Keller, Adrian","last_name":"Keller","orcid":"0000-0001-7139-3110"}],"date_created":"2021-07-08T12:03:52Z","volume":12,"date_updated":"2022-01-06T06:55:38Z"}]