[{"year":"2021","title":"Lamellar carbon-aluminosilicate nanocomposites with macroscopic orientation","status":"public","publication_identifier":{"issn":["2040-3364","2040-3372"]},"author":[{"first_name":"Dragana","last_name":"Paripović","full_name":"Paripović, Dragana"},{"first_name":"Lucia","last_name":"Hartmann","full_name":"Hartmann, Lucia"},{"id":"84268","orcid":"0000-0001-6373-0877","last_name":"Steinrück","first_name":"Hans-Georg","full_name":"Steinrück, Hans-Georg"},{"full_name":"Magerl, Andreas","last_name":"Magerl","first_name":"Andreas"},{"first_name":"Giovanni","last_name":"Li-Destri","full_name":"Li-Destri, Giovanni"},{"last_name":"Fontana","first_name":"Yannik","full_name":"Fontana, Yannik"},{"full_name":"Fontcuberta i Morral, Anna","first_name":"Anna","last_name":"Fontcuberta i Morral"},{"full_name":"Oveisi, Emad","last_name":"Oveisi","first_name":"Emad"},{"full_name":"Bomal, Enzo","first_name":"Enzo","last_name":"Bomal"},{"full_name":"Frauenrath, Holger","last_name":"Frauenrath","first_name":"Holger"}],"publication_status":"published","date_updated":"2022-01-06T06:55:57Z","intvolume":"        13","page":"13650-13657","_id":"23614","language":[{"iso":"eng"}],"user_id":"84268","doi":"10.1039/d1nr00807b","volume":13,"publication":"Nanoscale","citation":{"short":"D. Paripović, L. Hartmann, H.-G. Steinrück, A. Magerl, G. Li-Destri, Y. Fontana, A. Fontcuberta i Morral, E. Oveisi, E. Bomal, H. Frauenrath, Nanoscale 13 (2021) 13650–13657.","chicago":"Paripović, Dragana, Lucia Hartmann, Hans-Georg Steinrück, Andreas Magerl, Giovanni Li-Destri, Yannik Fontana, Anna Fontcuberta i Morral, Emad Oveisi, Enzo Bomal, and Holger Frauenrath. “Lamellar Carbon-Aluminosilicate Nanocomposites with Macroscopic Orientation.” <i>Nanoscale</i> 13 (2021): 13650–57. <a href=\"https://doi.org/10.1039/d1nr00807b\">https://doi.org/10.1039/d1nr00807b</a>.","ieee":"D. Paripović <i>et al.</i>, “Lamellar carbon-aluminosilicate nanocomposites with macroscopic orientation,” <i>Nanoscale</i>, vol. 13, pp. 13650–13657, 2021, doi: <a href=\"https://doi.org/10.1039/d1nr00807b\">10.1039/d1nr00807b</a>.","apa":"Paripović, D., Hartmann, L., Steinrück, H.-G., Magerl, A., Li-Destri, G., Fontana, Y., Fontcuberta i Morral, A., Oveisi, E., Bomal, E., &#38; Frauenrath, H. (2021). Lamellar carbon-aluminosilicate nanocomposites with macroscopic orientation. <i>Nanoscale</i>, <i>13</i>, 13650–13657. <a href=\"https://doi.org/10.1039/d1nr00807b\">https://doi.org/10.1039/d1nr00807b</a>","bibtex":"@article{Paripović_Hartmann_Steinrück_Magerl_Li-Destri_Fontana_Fontcuberta i Morral_Oveisi_Bomal_Frauenrath_2021, title={Lamellar carbon-aluminosilicate nanocomposites with macroscopic orientation}, volume={13}, DOI={<a href=\"https://doi.org/10.1039/d1nr00807b\">10.1039/d1nr00807b</a>}, journal={Nanoscale}, author={Paripović, Dragana and Hartmann, Lucia and Steinrück, Hans-Georg and Magerl, Andreas and Li-Destri, Giovanni and Fontana, Yannik and Fontcuberta i Morral, Anna and Oveisi, Emad and Bomal, Enzo and Frauenrath, Holger}, year={2021}, pages={13650–13657} }","ama":"Paripović D, Hartmann L, Steinrück H-G, et al. Lamellar carbon-aluminosilicate nanocomposites with macroscopic orientation. <i>Nanoscale</i>. 2021;13:13650-13657. doi:<a href=\"https://doi.org/10.1039/d1nr00807b\">10.1039/d1nr00807b</a>","mla":"Paripović, Dragana, et al. “Lamellar Carbon-Aluminosilicate Nanocomposites with Macroscopic Orientation.” <i>Nanoscale</i>, vol. 13, 2021, pp. 13650–57, doi:<a href=\"https://doi.org/10.1039/d1nr00807b\">10.1039/d1nr00807b</a>."},"abstract":[{"text":"<jats:p>A liquid-crystalline hexaphenylene amphiphile and an aluminosilicate precursor were co-assembled and pyrolyzed to form carbon-aluminosilicate nanocomposites with controlled lamellar orientation and macroscopic order.</jats:p>","lang":"eng"}],"date_created":"2021-09-01T09:09:41Z","type":"journal_article","department":[{"_id":"633"}]},{"title":"Quantification of heterogeneous, irreversible lithium plating in extreme fast charging of lithium-ion batteries","year":"2021","status":"public","publication_identifier":{"issn":["1754-5692","1754-5706"]},"author":[{"full_name":"Paul, Partha P.","first_name":"Partha P.","last_name":"Paul"},{"full_name":"Thampy, Vivek","first_name":"Vivek","last_name":"Thampy"},{"full_name":"Cao, Chuntian","last_name":"Cao","first_name":"Chuntian"},{"last_name":"Steinrück","first_name":"Hans-Georg","orcid":"0000-0001-6373-0877","full_name":"Steinrück, Hans-Georg","id":"84268"},{"first_name":"Tanvir R.","last_name":"Tanim","full_name":"Tanim, Tanvir R."},{"full_name":"Dunlop, Alison R.","first_name":"Alison R.","last_name":"Dunlop"},{"first_name":"Eric J.","last_name":"Dufek","full_name":"Dufek, Eric J."},{"first_name":"Stephen E.","last_name":"Trask","full_name":"Trask, Stephen E."},{"full_name":"Jansen, Andrew N.","first_name":"Andrew N.","last_name":"Jansen"},{"full_name":"Toney, Michael F.","first_name":"Michael F.","last_name":"Toney"},{"last_name":"Nelson Weker","first_name":"Johanna","full_name":"Nelson Weker, Johanna"}],"publication_status":"published","date_updated":"2022-01-06T06:55:57Z","intvolume":"        14","page":"4979-4988","_id":"23615","language":[{"iso":"eng"}],"user_id":"84268","doi":"10.1039/d1ee01216a","volume":14,"publication":"Energy & Environmental Science","citation":{"ama":"Paul PP, Thampy V, Cao C, et al. Quantification of heterogeneous, irreversible lithium plating in extreme fast charging of lithium-ion batteries. <i>Energy &#38; Environmental Science</i>. 2021;14:4979-4988. doi:<a href=\"https://doi.org/10.1039/d1ee01216a\">10.1039/d1ee01216a</a>","short":"P.P. Paul, V. Thampy, C. Cao, H.-G. Steinrück, T.R. Tanim, A.R. Dunlop, E.J. Dufek, S.E. Trask, A.N. Jansen, M.F. Toney, J. Nelson Weker, Energy &#38; Environmental Science 14 (2021) 4979–4988.","chicago":"Paul, Partha P., Vivek Thampy, Chuntian Cao, Hans-Georg Steinrück, Tanvir R. Tanim, Alison R. Dunlop, Eric J. Dufek, et al. “Quantification of Heterogeneous, Irreversible Lithium Plating in Extreme Fast Charging of Lithium-Ion Batteries.” <i>Energy &#38; Environmental Science</i> 14 (2021): 4979–88. <a href=\"https://doi.org/10.1039/d1ee01216a\">https://doi.org/10.1039/d1ee01216a</a>.","bibtex":"@article{Paul_Thampy_Cao_Steinrück_Tanim_Dunlop_Dufek_Trask_Jansen_Toney_et al._2021, title={Quantification of heterogeneous, irreversible lithium plating in extreme fast charging of lithium-ion batteries}, volume={14}, DOI={<a href=\"https://doi.org/10.1039/d1ee01216a\">10.1039/d1ee01216a</a>}, journal={Energy &#38; Environmental Science}, author={Paul, Partha P. and Thampy, Vivek and Cao, Chuntian and Steinrück, Hans-Georg and Tanim, Tanvir R. and Dunlop, Alison R. and Dufek, Eric J. and Trask, Stephen E. and Jansen, Andrew N. and Toney, Michael F. and et al.}, year={2021}, pages={4979–4988} }","mla":"Paul, Partha P., et al. “Quantification of Heterogeneous, Irreversible Lithium Plating in Extreme Fast Charging of Lithium-Ion Batteries.” <i>Energy &#38; Environmental Science</i>, vol. 14, 2021, pp. 4979–88, doi:<a href=\"https://doi.org/10.1039/d1ee01216a\">10.1039/d1ee01216a</a>.","apa":"Paul, P. P., Thampy, V., Cao, C., Steinrück, H.-G., Tanim, T. R., Dunlop, A. R., Dufek, E. J., Trask, S. E., Jansen, A. N., Toney, M. F., &#38; Nelson Weker, J. (2021). Quantification of heterogeneous, irreversible lithium plating in extreme fast charging of lithium-ion batteries. <i>Energy &#38; Environmental Science</i>, <i>14</i>, 4979–4988. <a href=\"https://doi.org/10.1039/d1ee01216a\">https://doi.org/10.1039/d1ee01216a</a>","ieee":"P. P. Paul <i>et al.</i>, “Quantification of heterogeneous, irreversible lithium plating in extreme fast charging of lithium-ion batteries,” <i>Energy &#38; Environmental Science</i>, vol. 14, pp. 4979–4988, 2021, doi: <a href=\"https://doi.org/10.1039/d1ee01216a\">10.1039/d1ee01216a</a>."},"abstract":[{"lang":"eng","text":"<p>Realization of extreme fast charging (XFC, ≤15 minutes) of lithium-ion batteries is imperative for the widespread adoption of electric vehicles.</p>"}],"date_created":"2021-09-01T09:09:48Z","type":"journal_article","department":[{"_id":"633"}]},{"date_created":"2021-09-01T09:09:55Z","type":"journal_article","department":[{"_id":"633"}],"publication":"Macromolecules","citation":{"mla":"Galluzzo, Michael D., et al. “Orientation-Dependent Distortion of Lamellae in a Block Copolymer Electrolyte under DC Polarization.” <i>Macromolecules</i>, vol. 54, 2021, pp. 7808–24, doi:<a href=\"https://doi.org/10.1021/acs.macromol.1c01295\">10.1021/acs.macromol.1c01295</a>.","bibtex":"@article{Galluzzo_Grundy_Takacs_Cao_Steinrück_Fu_Rivas Valadez_Toney_Balsara_2021, title={Orientation-Dependent Distortion of Lamellae in a Block Copolymer Electrolyte under DC Polarization}, volume={54}, DOI={<a href=\"https://doi.org/10.1021/acs.macromol.1c01295\">10.1021/acs.macromol.1c01295</a>}, journal={Macromolecules}, author={Galluzzo, Michael D. and Grundy, Lorena S. and Takacs, Christopher J. and Cao, Chuntian and Steinrück, Hans-Georg and Fu, Sean and Rivas Valadez, Michael A. and Toney, Michael F. and Balsara, Nitash P.}, year={2021}, pages={7808–7824} }","ama":"Galluzzo MD, Grundy LS, Takacs CJ, et al. Orientation-Dependent Distortion of Lamellae in a Block Copolymer Electrolyte under DC Polarization. <i>Macromolecules</i>. 2021;54:7808-7824. doi:<a href=\"https://doi.org/10.1021/acs.macromol.1c01295\">10.1021/acs.macromol.1c01295</a>","ieee":"M. D. Galluzzo <i>et al.</i>, “Orientation-Dependent Distortion of Lamellae in a Block Copolymer Electrolyte under DC Polarization,” <i>Macromolecules</i>, vol. 54, pp. 7808–7824, 2021, doi: <a href=\"https://doi.org/10.1021/acs.macromol.1c01295\">10.1021/acs.macromol.1c01295</a>.","apa":"Galluzzo, M. D., Grundy, L. S., Takacs, C. J., Cao, C., Steinrück, H.-G., Fu, S., Rivas Valadez, M. A., Toney, M. F., &#38; Balsara, N. P. (2021). Orientation-Dependent Distortion of Lamellae in a Block Copolymer Electrolyte under DC Polarization. <i>Macromolecules</i>, <i>54</i>, 7808–7824. <a href=\"https://doi.org/10.1021/acs.macromol.1c01295\">https://doi.org/10.1021/acs.macromol.1c01295</a>","chicago":"Galluzzo, Michael D., Lorena S. Grundy, Christopher J. Takacs, Chuntian Cao, Hans-Georg Steinrück, Sean Fu, Michael A. Rivas Valadez, Michael F. Toney, and Nitash P. Balsara. “Orientation-Dependent Distortion of Lamellae in a Block Copolymer Electrolyte under DC Polarization.” <i>Macromolecules</i> 54 (2021): 7808–24. <a href=\"https://doi.org/10.1021/acs.macromol.1c01295\">https://doi.org/10.1021/acs.macromol.1c01295</a>.","short":"M.D. Galluzzo, L.S. Grundy, C.J. Takacs, C. Cao, H.-G. Steinrück, S. Fu, M.A. Rivas Valadez, M.F. Toney, N.P. Balsara, Macromolecules 54 (2021) 7808–7824."},"page":"7808-7824","language":[{"iso":"eng"}],"_id":"23616","user_id":"84268","doi":"10.1021/acs.macromol.1c01295","volume":54,"title":"Orientation-Dependent Distortion of Lamellae in a Block Copolymer Electrolyte under DC Polarization","year":"2021","status":"public","publication_identifier":{"issn":["0024-9297","1520-5835"]},"author":[{"full_name":"Galluzzo, Michael D.","first_name":"Michael D.","last_name":"Galluzzo"},{"full_name":"Grundy, Lorena S.","last_name":"Grundy","first_name":"Lorena S."},{"full_name":"Takacs, Christopher J.","last_name":"Takacs","first_name":"Christopher J."},{"last_name":"Cao","first_name":"Chuntian","full_name":"Cao, Chuntian"},{"full_name":"Steinrück, Hans-Georg","first_name":"Hans-Georg","last_name":"Steinrück","orcid":"0000-0001-6373-0877","id":"84268"},{"first_name":"Sean","last_name":"Fu","full_name":"Fu, Sean"},{"full_name":"Rivas Valadez, Michael A.","first_name":"Michael A.","last_name":"Rivas Valadez"},{"last_name":"Toney","first_name":"Michael F.","full_name":"Toney, Michael F."},{"full_name":"Balsara, Nitash P.","last_name":"Balsara","first_name":"Nitash P."}],"publication_status":"published","date_updated":"2022-01-06T06:55:57Z","intvolume":"        54"},{"abstract":[{"text":"<jats:p>The effects that solid–liquid interfaces exert on the aggregation of proteins and peptides are of high relevance for various fields of basic and applied research, ranging from molecular biology and biomedicine to nanotechnology. While the influence of surface chemistry has received a lot of attention in this context, the role of surface topography has mostly been neglected so far. In this work, therefore, we investigate the aggregation of the type 2 diabetes-associated peptide hormone hIAPP in contact with flat and nanopatterned silicon oxide surfaces. The nanopatterned surfaces are produced by ion beam irradiation, resulting in well-defined anisotropic ripple patterns with heights and periodicities of about 1.5 and 30 nm, respectively. Using time-lapse atomic force microscopy, the morphology of the hIAPP aggregates is characterized quantitatively. Aggregation results in both amorphous aggregates and amyloid fibrils, with the presence of the nanopatterns leading to retarded fibrillization and stronger amorphous aggregation. This is attributed to structural differences in the amorphous aggregates formed at the nanopatterned surface, which result in a lower propensity for nucleating amyloid fibrillization. Our results demonstrate that nanoscale surface topography may modulate peptide and protein aggregation pathways in complex and intricate ways.</jats:p>","lang":"eng"}],"publication":"International Journal of Molecular Sciences","citation":{"apa":"Hanke, M., Yang, Y., Ji, Y., Grundmeier, G., &#38; Keller, A. (2021). Nanoscale Surface Topography Modulates hIAPP Aggregation Pathways at Solid–Liquid Interfaces. <i>International Journal of Molecular Sciences</i>, <i>22</i>, 5142. <a href=\"https://doi.org/10.3390/ijms22105142\">https://doi.org/10.3390/ijms22105142</a>","ieee":"M. Hanke, Y. Yang, Y. Ji, G. Grundmeier, and A. Keller, “Nanoscale Surface Topography Modulates hIAPP Aggregation Pathways at Solid–Liquid Interfaces,” <i>International Journal of Molecular Sciences</i>, vol. 22, p. 5142, 2021.","short":"M. Hanke, Y. Yang, Y. Ji, G. Grundmeier, A. Keller, International Journal of Molecular Sciences 22 (2021) 5142.","chicago":"Hanke, Marcel, Yu Yang, Yuxin Ji, Guido Grundmeier, and Adrian Keller. “Nanoscale Surface Topography Modulates HIAPP Aggregation Pathways at Solid–Liquid Interfaces.” <i>International Journal of Molecular Sciences</i> 22 (2021): 5142. <a href=\"https://doi.org/10.3390/ijms22105142\">https://doi.org/10.3390/ijms22105142</a>.","mla":"Hanke, Marcel, et al. “Nanoscale Surface Topography Modulates HIAPP Aggregation Pathways at Solid–Liquid Interfaces.” <i>International Journal of Molecular Sciences</i>, vol. 22, 2021, p. 5142, doi:<a href=\"https://doi.org/10.3390/ijms22105142\">10.3390/ijms22105142</a>.","ama":"Hanke M, Yang Y, Ji Y, Grundmeier G, Keller A. Nanoscale Surface Topography Modulates hIAPP Aggregation Pathways at Solid–Liquid Interfaces. <i>International Journal of Molecular Sciences</i>. 2021;22:5142. doi:<a href=\"https://doi.org/10.3390/ijms22105142\">10.3390/ijms22105142</a>","bibtex":"@article{Hanke_Yang_Ji_Grundmeier_Keller_2021, title={Nanoscale Surface Topography Modulates hIAPP Aggregation Pathways at Solid–Liquid Interfaces}, volume={22}, DOI={<a href=\"https://doi.org/10.3390/ijms22105142\">10.3390/ijms22105142</a>}, journal={International Journal of Molecular Sciences}, author={Hanke, Marcel and Yang, Yu and Ji, Yuxin and Grundmeier, Guido and Keller, Adrian}, year={2021}, pages={5142} }"},"type":"journal_article","department":[{"_id":"302"}],"date_created":"2021-07-08T11:43:14Z","date_updated":"2022-01-06T06:55:37Z","publication_status":"published","intvolume":"        22","status":"public","title":"Nanoscale Surface Topography Modulates hIAPP Aggregation Pathways at Solid–Liquid Interfaces","year":"2021","author":[{"last_name":"Hanke","first_name":"Marcel","full_name":"Hanke, Marcel"},{"full_name":"Yang, Yu","last_name":"Yang","first_name":"Yu"},{"full_name":"Ji, Yuxin","last_name":"Ji","first_name":"Yuxin"},{"id":"194","last_name":"Grundmeier","first_name":"Guido","full_name":"Grundmeier, Guido"},{"first_name":"Adrian","last_name":"Keller","orcid":"0000-0001-7139-3110","full_name":"Keller, Adrian","id":"48864"}],"publication_identifier":{"issn":["1422-0067"]},"doi":"10.3390/ijms22105142","user_id":"48864","volume":22,"page":"5142","language":[{"iso":"eng"}],"_id":"22636"},{"citation":{"apa":"Ijäs, H., Shen, B., Heuer-Jungemann, A., Keller, A., Kostiainen, M. A., Liedl, T., … Linko, V. (2021). Unraveling the interaction between doxorubicin and DNA origami nanostructures for customizable chemotherapeutic drug release. <i>Nucleic Acids Research</i>, <i>49</i>, 3048–3062. <a href=\"https://doi.org/10.1093/nar/gkab097\">https://doi.org/10.1093/nar/gkab097</a>","ieee":"H. Ijäs <i>et al.</i>, “Unraveling the interaction between doxorubicin and DNA origami nanostructures for customizable chemotherapeutic drug release,” <i>Nucleic Acids Research</i>, vol. 49, pp. 3048–3062, 2021.","chicago":"Ijäs, Heini, Boxuan Shen, Amelie Heuer-Jungemann, Adrian Keller, Mauri A Kostiainen, Tim Liedl, Janne A Ihalainen, and Veikko Linko. “Unraveling the Interaction between Doxorubicin and DNA Origami Nanostructures for Customizable Chemotherapeutic Drug Release.” <i>Nucleic Acids Research</i> 49 (2021): 3048–62. <a href=\"https://doi.org/10.1093/nar/gkab097\">https://doi.org/10.1093/nar/gkab097</a>.","short":"H. Ijäs, B. Shen, A. Heuer-Jungemann, A. Keller, M.A. Kostiainen, T. Liedl, J.A. Ihalainen, V. Linko, Nucleic Acids Research 49 (2021) 3048–3062.","mla":"Ijäs, Heini, et al. “Unraveling the Interaction between Doxorubicin and DNA Origami Nanostructures for Customizable Chemotherapeutic Drug Release.” <i>Nucleic Acids Research</i>, vol. 49, 2021, pp. 3048–62, doi:<a href=\"https://doi.org/10.1093/nar/gkab097\">10.1093/nar/gkab097</a>.","ama":"Ijäs H, Shen B, Heuer-Jungemann A, et al. Unraveling the interaction between doxorubicin and DNA origami nanostructures for customizable chemotherapeutic drug release. <i>Nucleic Acids Research</i>. 2021;49:3048-3062. doi:<a href=\"https://doi.org/10.1093/nar/gkab097\">10.1093/nar/gkab097</a>","bibtex":"@article{Ijäs_Shen_Heuer-Jungemann_Keller_Kostiainen_Liedl_Ihalainen_Linko_2021, title={Unraveling the interaction between doxorubicin and DNA origami nanostructures for customizable chemotherapeutic drug release}, volume={49}, DOI={<a href=\"https://doi.org/10.1093/nar/gkab097\">10.1093/nar/gkab097</a>}, journal={Nucleic Acids Research}, author={Ijäs, Heini and Shen, Boxuan and Heuer-Jungemann, Amelie and Keller, Adrian and Kostiainen, Mauri A and Liedl, Tim and Ihalainen, Janne A and Linko, Veikko}, year={2021}, pages={3048–3062} }"},"publication":"Nucleic Acids Research","abstract":[{"lang":"eng","text":"<jats:title>Abstract</jats:title>\r\n               <jats:p>Doxorubicin (DOX) is a common drug in cancer chemotherapy, and its high DNA-binding affinity can be harnessed in preparing DOX-loaded DNA nanostructures for targeted delivery and therapeutics. Although DOX has been widely studied, the existing literature of DOX-loaded DNA-carriers remains limited and incoherent. Here, based on an in-depth spectroscopic analysis, we characterize and optimize the DOX loading into different 2D and 3D scaffolded DNA origami nanostructures (DONs). In our experimental conditions, all DONs show similar DOX binding capacities (one DOX molecule per two to three base pairs), and the binding equilibrium is reached within seconds, remarkably faster than previously acknowledged. To characterize drug release profiles, DON degradation and DOX release from the complexes upon DNase I digestion was studied. For the employed DONs, the relative doses (DOX molecules released per unit time) may vary by two orders of magnitude depending on the DON superstructure. In addition, we identify DOX aggregation mechanisms and spectral changes linked to pH, magnesium, and DOX concentration. These features have been largely ignored in experimenting with DNA nanostructures, but are probably the major sources of the incoherence of the experimental results so far. Therefore, we believe this work can act as a guide to tailoring the release profiles and developing better drug delivery systems based on DNA-carriers.</jats:p>"}],"date_created":"2021-07-08T11:46:53Z","department":[{"_id":"302"}],"type":"journal_article","publication_identifier":{"issn":["0305-1048","1362-4962"]},"author":[{"full_name":"Ijäs, Heini","first_name":"Heini","last_name":"Ijäs"},{"first_name":"Boxuan","last_name":"Shen","full_name":"Shen, Boxuan"},{"last_name":"Heuer-Jungemann","first_name":"Amelie","full_name":"Heuer-Jungemann, Amelie"},{"id":"48864","full_name":"Keller, Adrian","first_name":"Adrian","last_name":"Keller","orcid":"0000-0001-7139-3110"},{"full_name":"Kostiainen, Mauri A","first_name":"Mauri A","last_name":"Kostiainen"},{"first_name":"Tim","last_name":"Liedl","full_name":"Liedl, Tim"},{"full_name":"Ihalainen, Janne A","first_name":"Janne A","last_name":"Ihalainen"},{"last_name":"Linko","first_name":"Veikko","full_name":"Linko, Veikko"}],"title":"Unraveling the interaction between doxorubicin and DNA origami nanostructures for customizable chemotherapeutic drug release","status":"public","year":"2021","intvolume":"        49","date_updated":"2022-01-06T06:55:37Z","publication_status":"published","_id":"22637","language":[{"iso":"eng"}],"page":"3048-3062","volume":49,"doi":"10.1093/nar/gkab097","user_id":"48864"},{"citation":{"mla":"Xin, Y., et al. “Scaling Up DNA Origami Lattice Assembly.” <i>Chemistry – A European Journal</i>, vol. 27, no. 33, 2021, pp. 8564–71, doi:<a href=\"https://doi.org/10.1002/chem.202100784\">10.1002/chem.202100784</a>.","bibtex":"@article{Xin_Shen_Kostiainen_Grundmeier_Castro_Linko_Keller_2021, title={Scaling Up DNA Origami Lattice Assembly.}, volume={27}, DOI={<a href=\"https://doi.org/10.1002/chem.202100784\">10.1002/chem.202100784</a>}, number={33}, journal={Chemistry – A European Journal}, author={Xin, Y and Shen, B and Kostiainen, MA and Grundmeier, Guido and Castro, M and Linko, V and Keller, Adrian}, year={2021}, pages={8564–8571} }","ama":"Xin Y, Shen B, Kostiainen M, et al. Scaling Up DNA Origami Lattice Assembly. <i>Chemistry – A European Journal</i>. 2021;27(33):8564-8571. doi:<a href=\"https://doi.org/10.1002/chem.202100784\">10.1002/chem.202100784</a>","ieee":"Y. Xin <i>et al.</i>, “Scaling Up DNA Origami Lattice Assembly.,” <i>Chemistry – A European Journal</i>, vol. 27, no. 33, pp. 8564–8571, 2021.","apa":"Xin, Y., Shen, B., Kostiainen, M., Grundmeier, G., Castro, M., Linko, V., &#38; Keller, A. (2021). Scaling Up DNA Origami Lattice Assembly. <i>Chemistry – A European Journal</i>, <i>27</i>(33), 8564–8571. <a href=\"https://doi.org/10.1002/chem.202100784\">https://doi.org/10.1002/chem.202100784</a>","chicago":"Xin, Y, B Shen, MA Kostiainen, Guido Grundmeier, M Castro, V Linko, and Adrian Keller. “Scaling Up DNA Origami Lattice Assembly.” <i>Chemistry – A European Journal</i> 27, no. 33 (2021): 8564–71. <a href=\"https://doi.org/10.1002/chem.202100784\">https://doi.org/10.1002/chem.202100784</a>.","short":"Y. Xin, B. Shen, M. Kostiainen, G. Grundmeier, M. Castro, V. Linko, A. 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N. and Arcos de Pedro, Maria Teresa and Grundmeier, Guido}, year={2021}, pages={1237–1245} }","ama":"Knust S, Ruhm L, Kuhlmann A, et al. In situ backside Raman spectroscopy of zinc oxide nanorods in an atmospheric‐pressure dielectric barrier discharge plasma. <i>Journal of Raman Spectroscopy</i>. 2021:1237-1245. doi:<a href=\"https://doi.org/10.1002/jrs.6123\">10.1002/jrs.6123</a>","mla":"Knust, Steffen, et al. “In Situ Backside Raman Spectroscopy of Zinc Oxide Nanorods in an Atmospheric‐pressure Dielectric Barrier Discharge Plasma.” <i>Journal of Raman Spectroscopy</i>, 2021, pp. 1237–45, doi:<a href=\"https://doi.org/10.1002/jrs.6123\">10.1002/jrs.6123</a>.","chicago":"Knust, Steffen, Lukas Ruhm, Andreas Kuhlmann, Dennis Meinderink, Julius Bürger, Jörg K. N. Lindner, Maria Teresa Arcos de Pedro, and Guido Grundmeier. “In Situ Backside Raman Spectroscopy of Zinc Oxide Nanorods in an Atmospheric‐pressure Dielectric Barrier Discharge Plasma.” <i>Journal of Raman Spectroscopy</i>, 2021, 1237–45. <a href=\"https://doi.org/10.1002/jrs.6123\">https://doi.org/10.1002/jrs.6123</a>.","short":"S. Knust, L. Ruhm, A. Kuhlmann, D. Meinderink, J. Bürger, J.K.N. Lindner, M.T. Arcos de Pedro, G. Grundmeier, Journal of Raman Spectroscopy (2021) 1237–1245.","ieee":"S. Knust <i>et al.</i>, “In situ backside Raman spectroscopy of zinc oxide nanorods in an atmospheric‐pressure dielectric barrier discharge plasma,” <i>Journal of Raman Spectroscopy</i>, pp. 1237–1245, 2021.","apa":"Knust, S., Ruhm, L., Kuhlmann, A., Meinderink, D., Bürger, J., Lindner, J. K. N., … Grundmeier, G. (2021). In situ backside Raman spectroscopy of zinc oxide nanorods in an atmospheric‐pressure dielectric barrier discharge plasma. <i>Journal of Raman Spectroscopy</i>, 1237–1245. <a href=\"https://doi.org/10.1002/jrs.6123\">https://doi.org/10.1002/jrs.6123</a>"},"date_created":"2021-07-09T12:31:06Z","type":"journal_article","department":[{"_id":"302"}],"year":"2021","status":"public","title":"In situ backside Raman spectroscopy of zinc oxide nanorods in an atmospheric‐pressure dielectric barrier discharge plasma","publication_identifier":{"issn":["0377-0486","1097-4555"]},"author":[{"full_name":"Knust, Steffen","last_name":"Knust","first_name":"Steffen"},{"last_name":"Ruhm","first_name":"Lukas","full_name":"Ruhm, Lukas"},{"first_name":"Andreas","last_name":"Kuhlmann","full_name":"Kuhlmann, Andreas"},{"id":"32378","full_name":"Meinderink, Dennis","orcid":"0000-0002-2755-6514","first_name":"Dennis","last_name":"Meinderink"},{"full_name":"Bürger, Julius","first_name":"Julius","last_name":"Bürger","id":"46952"},{"last_name":"Lindner","first_name":"Jörg K. N.","full_name":"Lindner, Jörg K. N."},{"full_name":"Arcos de Pedro, Maria Teresa","first_name":"Maria Teresa","last_name":"Arcos de Pedro"},{"id":"194","full_name":"Grundmeier, Guido","first_name":"Guido","last_name":"Grundmeier"}],"publication_status":"published","date_updated":"2022-01-06T06:55:38Z","page":"1237-1245","language":[{"iso":"eng"}],"_id":"22697","user_id":"32378","doi":"10.1002/jrs.6123"},{"publication_status":"published","date_updated":"2022-01-06T06:55:40Z","intvolume":"        11","title":"Ion Beam Nanopatterning of Biomaterial Surfaces","year":"2021","status":"public","publication_identifier":{"issn":["2076-3417"]},"author":[{"last_name":"Yang","first_name":"Yu","full_name":"Yang, Yu"},{"orcid":"0000-0001-7139-3110","first_name":"Adrian","last_name":"Keller","full_name":"Keller, Adrian","id":"48864"}],"user_id":"48864","doi":"10.3390/app11146575","volume":11,"page":"6575","language":[{"iso":"eng"}],"_id":"22773","abstract":[{"text":"<jats:p>Ion beam irradiation of solid surfaces may result in the self-organized formation of well-defined topographic nanopatterns. Depending on the irradiation conditions and the material properties, isotropic or anisotropic patterns of differently shaped features may be obtained. Most intriguingly, the periodicities of these patterns can be adjusted in the range between less than twenty and several hundred nanometers, which covers the dimensions of many cellular and extracellular features. However, even though ion beam nanopatterning has been studied for several decades and is nowadays widely employed in the fabrication of functional surfaces, it has found its way into the biomaterials field only recently. This review provides a brief overview of the basics of ion beam nanopatterning, emphasizes aspects of particular relevance for biomaterials applications, and summarizes a number of recent studies that investigated the effects of such nanopatterned surfaces on the adsorption of biomolecules and the response of adhering cells. Finally, promising future directions and potential translational challenges are identified.</jats:p>","lang":"eng"}],"publication":"Applied Sciences","citation":{"mla":"Yang, Yu, and Adrian Keller. “Ion Beam Nanopatterning of Biomaterial Surfaces.” <i>Applied Sciences</i>, vol. 11, 2021, p. 6575, doi:<a href=\"https://doi.org/10.3390/app11146575\">10.3390/app11146575</a>.","bibtex":"@article{Yang_Keller_2021, title={Ion Beam Nanopatterning of Biomaterial Surfaces}, volume={11}, DOI={<a href=\"https://doi.org/10.3390/app11146575\">10.3390/app11146575</a>}, journal={Applied Sciences}, author={Yang, Yu and Keller, Adrian}, year={2021}, pages={6575} }","ama":"Yang Y, Keller A. Ion Beam Nanopatterning of Biomaterial Surfaces. <i>Applied Sciences</i>. 2021;11:6575. doi:<a href=\"https://doi.org/10.3390/app11146575\">10.3390/app11146575</a>","ieee":"Y. Yang and A. Keller, “Ion Beam Nanopatterning of Biomaterial Surfaces,” <i>Applied Sciences</i>, vol. 11, p. 6575, 2021.","apa":"Yang, Y., &#38; Keller, A. (2021). Ion Beam Nanopatterning of Biomaterial Surfaces. <i>Applied Sciences</i>, <i>11</i>, 6575. <a href=\"https://doi.org/10.3390/app11146575\">https://doi.org/10.3390/app11146575</a>","short":"Y. Yang, A. Keller, Applied Sciences 11 (2021) 6575.","chicago":"Yang, Yu, and Adrian Keller. “Ion Beam Nanopatterning of Biomaterial Surfaces.” <i>Applied Sciences</i> 11 (2021): 6575. <a href=\"https://doi.org/10.3390/app11146575\">https://doi.org/10.3390/app11146575</a>."},"type":"journal_article","department":[{"_id":"302"}],"date_created":"2021-07-21T09:25:55Z"},{"type":"journal_article","department":[{"_id":"302"}],"date_created":"2021-08-03T06:07:33Z","abstract":[{"lang":"eng","text":"<jats:p>Implant-associated infections are an increasingly severe burden on healthcare systems worldwide and many research activities currently focus on inhibiting microbial colonization of biomedically relevant surfaces. To obtain molecular-level understanding of the involved processes and interactions, we investigate the adsorption of synthetic adhesin-like peptide sequences derived from the type IV pili of the Pseudomonas aeruginosa strains PAK and PAO at abiotic model surfaces, i.e., Au, SiO2, and oxidized Ti. These peptides correspond to the sequences of the receptor-binding domain 128–144 of the major pilin protein, which is known to facilitate P. aeruginosa adhesion at biotic and abiotic surfaces. Using quartz crystal microbalance with dissipation monitoring (QCM-D), we find that peptide adsorption is material- as well as strain-dependent. At the Au surface, PAO(128–144) shows drastically stronger adsorption than PAK(128–144), whereas adsorption of both peptides is markedly reduced at the oxide surfaces with less drastic differences between the two sequences. These observations suggest that peptide adsorption is influenced by not only the peptide sequence, but also peptide conformation. Our results furthermore highlight the importance of molecular-level investigations to understand and ultimately control microbial colonization of surfaces.</jats:p>"}],"publication":"Micro","issue":"1","doi":"10.3390/micro1010010","language":[{"iso":"eng"}],"date_updated":"2022-01-06T06:55:43Z","publication_status":"published","intvolume":"         1","title":"Strain-Dependent Adsorption of Pseudomonas aeruginosa-Derived Adhesin-like Peptides at Abiotic Surfaces","year":"2021","author":[{"first_name":"Yu","last_name":"Yang","full_name":"Yang, Yu"},{"first_name":"Sabrina","last_name":"Schwiderek","full_name":"Schwiderek, Sabrina"},{"last_name":"Grundmeier","first_name":"Guido","full_name":"Grundmeier, Guido","id":"194"},{"last_name":"Keller","first_name":"Adrian","orcid":"0000-0001-7139-3110","full_name":"Keller, Adrian","id":"48864"}],"publication_identifier":{"issn":["2673-8023"]},"citation":{"short":"Y. Yang, S. Schwiderek, G. Grundmeier, A. Keller, Micro 1 (2021) 129–139.","chicago":"Yang, Yu, Sabrina Schwiderek, Guido Grundmeier, and Adrian Keller. “Strain-Dependent Adsorption of Pseudomonas Aeruginosa-Derived Adhesin-like Peptides at Abiotic Surfaces.” <i>Micro</i> 1, no. 1 (2021): 129–39. <a href=\"https://doi.org/10.3390/micro1010010\">https://doi.org/10.3390/micro1010010</a>.","apa":"Yang, Y., Schwiderek, S., Grundmeier, G., &#38; Keller, A. (2021). Strain-Dependent Adsorption of Pseudomonas aeruginosa-Derived Adhesin-like Peptides at Abiotic Surfaces. <i>Micro</i>, <i>1</i>(1), 129–139. <a href=\"https://doi.org/10.3390/micro1010010\">https://doi.org/10.3390/micro1010010</a>","ieee":"Y. Yang, S. Schwiderek, G. Grundmeier, and A. Keller, “Strain-Dependent Adsorption of Pseudomonas aeruginosa-Derived Adhesin-like Peptides at Abiotic Surfaces,” <i>Micro</i>, vol. 1, no. 1, pp. 129–139, 2021.","ama":"Yang Y, Schwiderek S, Grundmeier G, Keller A. Strain-Dependent Adsorption of Pseudomonas aeruginosa-Derived Adhesin-like Peptides at Abiotic Surfaces. <i>Micro</i>. 2021;1(1):129-139. doi:<a href=\"https://doi.org/10.3390/micro1010010\">10.3390/micro1010010</a>","bibtex":"@article{Yang_Schwiderek_Grundmeier_Keller_2021, title={Strain-Dependent Adsorption of Pseudomonas aeruginosa-Derived Adhesin-like Peptides at Abiotic Surfaces}, volume={1}, DOI={<a href=\"https://doi.org/10.3390/micro1010010\">10.3390/micro1010010</a>}, number={1}, journal={Micro}, author={Yang, Yu and Schwiderek, Sabrina and Grundmeier, Guido and Keller, Adrian}, year={2021}, pages={129–139} }","mla":"Yang, Yu, et al. “Strain-Dependent Adsorption of Pseudomonas Aeruginosa-Derived Adhesin-like Peptides at Abiotic Surfaces.” <i>Micro</i>, vol. 1, no. 1, 2021, pp. 129–39, doi:<a href=\"https://doi.org/10.3390/micro1010010\">10.3390/micro1010010</a>."},"user_id":"48864","volume":1,"page":"129-139","_id":"22926","status":"public"},{"citation":{"ieee":"Y. Xin, A. A. Zargariantabrizi, G. Grundmeier, and A. Keller, “Magnesium-Free Immobilization of DNA Origami Nanostructures at Mica Surfaces for Atomic Force Microscopy,” <i>Molecules</i>, vol. 26, p. 4798, 2021.","apa":"Xin, Y., Zargariantabrizi, A. A., Grundmeier, G., &#38; Keller, A. (2021). Magnesium-Free Immobilization of DNA Origami Nanostructures at Mica Surfaces for Atomic Force Microscopy. <i>Molecules</i>, <i>26</i>, 4798. <a href=\"https://doi.org/10.3390/molecules26164798\">https://doi.org/10.3390/molecules26164798</a>","chicago":"Xin, Yang, Amir Ardalan Zargariantabrizi, Guido Grundmeier, and Adrian Keller. “Magnesium-Free Immobilization of DNA Origami Nanostructures at Mica Surfaces for Atomic Force Microscopy.” <i>Molecules</i> 26 (2021): 4798. <a href=\"https://doi.org/10.3390/molecules26164798\">https://doi.org/10.3390/molecules26164798</a>.","short":"Y. Xin, A.A. Zargariantabrizi, G. Grundmeier, A. Keller, Molecules 26 (2021) 4798.","mla":"Xin, Yang, et al. “Magnesium-Free Immobilization of DNA Origami Nanostructures at Mica Surfaces for Atomic Force Microscopy.” <i>Molecules</i>, vol. 26, 2021, p. 4798, doi:<a href=\"https://doi.org/10.3390/molecules26164798\">10.3390/molecules26164798</a>.","bibtex":"@article{Xin_Zargariantabrizi_Grundmeier_Keller_2021, title={Magnesium-Free Immobilization of DNA Origami Nanostructures at Mica Surfaces for Atomic Force Microscopy}, volume={26}, DOI={<a href=\"https://doi.org/10.3390/molecules26164798\">10.3390/molecules26164798</a>}, journal={Molecules}, author={Xin, Yang and Zargariantabrizi, Amir Ardalan and Grundmeier, Guido and Keller, Adrian}, year={2021}, pages={4798} }","ama":"Xin Y, Zargariantabrizi AA, Grundmeier G, Keller A. Magnesium-Free Immobilization of DNA Origami Nanostructures at Mica Surfaces for Atomic Force Microscopy. <i>Molecules</i>. 2021;26:4798. doi:<a href=\"https://doi.org/10.3390/molecules26164798\">10.3390/molecules26164798</a>"},"publication":"Molecules","abstract":[{"lang":"eng","text":"<jats:p>DNA origami nanostructures (DONs) are promising substrates for the single-molecule investigation of biomolecular reactions and dynamics by in situ atomic force microscopy (AFM). For this, they are typically immobilized on mica substrates by adding millimolar concentrations of Mg2+ ions to the sample solution, which enable the adsorption of the negatively charged DONs at the like-charged mica surface. These non-physiological Mg2+ concentrations, however, present a serious limitation in such experiments as they may interfere with the reactions and processes under investigation. Therefore, we here evaluate three approaches to efficiently immobilize DONs at mica surfaces under essentially Mg2+-free conditions. These approaches rely on the pre-adsorption of different multivalent cations, i.e., Ni2+, poly-l-lysine (PLL), and spermidine (Spdn). DON adsorption is studied in phosphate-buffered saline (PBS) and pure water. In general, Ni2+ shows the worst performance with heavily deformed DONs. For 2D DON triangles, adsorption at PLL- and in particular Spdn-modified mica may outperform even Mg2+-mediated adsorption in terms of surface coverage, depending on the employed solution. For 3D six-helix bundles, less pronounced differences between the individual strategies are observed. Our results provide some general guidance for the immobilization of DONs at mica surfaces under Mg2+-free conditions and may aid future in situ AFM studies.</jats:p>"}],"date_created":"2021-08-09T06:17:59Z","department":[{"_id":"302"}],"type":"journal_article","publication_identifier":{"issn":["1420-3049"]},"author":[{"full_name":"Xin, Yang","last_name":"Xin","first_name":"Yang"},{"first_name":"Amir Ardalan","last_name":"Zargariantabrizi","full_name":"Zargariantabrizi, Amir Ardalan"},{"last_name":"Grundmeier","first_name":"Guido","full_name":"Grundmeier, Guido","id":"194"},{"id":"48864","first_name":"Adrian","orcid":"0000-0001-7139-3110","last_name":"Keller","full_name":"Keller, Adrian"}],"year":"2021","title":"Magnesium-Free Immobilization of DNA Origami Nanostructures at Mica Surfaces for Atomic Force Microscopy","status":"public","intvolume":"        26","publication_status":"published","date_updated":"2022-01-06T06:55:45Z","language":[{"iso":"eng"}],"_id":"23023","page":"4798","volume":26,"user_id":"48864","doi":"10.3390/molecules26164798"},{"date_created":"2021-04-22T10:19:48Z","type":"conference","department":[{"_id":"157"},{"_id":"302"}],"citation":{"apa":"Schmolke, T., Teutenberg, D., Meschut, G., Meinderink, D., Koch, L., Ebbert, C., &#38; Grundmeier, G. (2021). Entwicklung einer Methode zur Bewertung einer stahlintensiven Mischbau-Klebverbindung eines Batteriegehäuses gegenüber mechanischer und medialer Belastung und Berücksichtigung der Interphasenstruktur. In DECHEMA, Gesellschaft für Chemische Technik und Biotechnologie e.V. (Ed.). Presented at the 21. Kolloquium Gemeinsame Forschung in der Klebtechnik , Online Event.","ieee":"T. Schmolke <i>et al.</i>, “Entwicklung einer Methode zur Bewertung einer stahlintensiven Mischbau-Klebverbindung eines Batteriegehäuses gegenüber mechanischer und medialer Belastung und Berücksichtigung der Interphasenstruktur,” presented at the 21. Kolloquium Gemeinsame Forschung in der Klebtechnik , Online Event, 2021.","short":"T. Schmolke, D. Teutenberg, G. Meschut, D. Meinderink, L. Koch, C. Ebbert, G. Grundmeier, in: DECHEMA, Gesellschaft für Chemische Technik und Biotechnologie e.V. (Ed.), 2021.","chicago":"Schmolke, Tobias, Dominik Teutenberg, Gerson Meschut, Dennis Meinderink, Leon  Koch, Christoph Ebbert, and Guido Grundmeier. “Entwicklung Einer Methode Zur Bewertung Einer Stahlintensiven Mischbau-Klebverbindung Eines Batteriegehäuses Gegenüber Mechanischer Und Medialer Belastung Und Berücksichtigung Der Interphasenstruktur.” edited by DECHEMA, Gesellschaft für Chemische Technik und Biotechnologie e.V., 2021.","mla":"Schmolke, Tobias, et al. <i>Entwicklung Einer Methode Zur Bewertung Einer Stahlintensiven Mischbau-Klebverbindung Eines Batteriegehäuses Gegenüber Mechanischer Und Medialer Belastung Und Berücksichtigung Der Interphasenstruktur</i>. Edited by DECHEMA, Gesellschaft für Chemische Technik und Biotechnologie e.V., 2021.","ama":"Schmolke T, Teutenberg D, Meschut G, et al. Entwicklung einer Methode zur Bewertung einer stahlintensiven Mischbau-Klebverbindung eines Batteriegehäuses gegenüber mechanischer und medialer Belastung und Berücksichtigung der Interphasenstruktur. In: DECHEMA, Gesellschaft für Chemische Technik und Biotechnologie e.V., ed. ; 2021.","bibtex":"@inproceedings{Schmolke_Teutenberg_Meschut_Meinderink_Koch_Ebbert_Grundmeier_2021, title={Entwicklung einer Methode zur Bewertung einer stahlintensiven Mischbau-Klebverbindung eines Batteriegehäuses gegenüber mechanischer und medialer Belastung und Berücksichtigung der Interphasenstruktur}, author={Schmolke, Tobias and Teutenberg, Dominik and Meschut, Gerson and Meinderink, Dennis and Koch, Leon  and Ebbert, Christoph and Grundmeier, Guido}, editor={DECHEMA, Gesellschaft für Chemische Technik und Biotechnologie e.V.Editor}, year={2021} }"},"_id":"21717","language":[{"iso":"eng"}],"user_id":"7266","status":"public","title":"Entwicklung einer Methode zur Bewertung einer stahlintensiven Mischbau-Klebverbindung eines Batteriegehäuses gegenüber mechanischer und medialer Belastung und Berücksichtigung der Interphasenstruktur","year":"2021","conference":{"location":"Online Event","name":"21. Kolloquium Gemeinsame Forschung in der Klebtechnik ","start_date":"2021-03-02","end_date":"2021-03-03"},"corporate_editor":["DECHEMA, Gesellschaft für Chemische Technik und Biotechnologie e.V."],"author":[{"first_name":"Tobias","last_name":"Schmolke","full_name":"Schmolke, Tobias","id":"44759"},{"full_name":"Teutenberg, Dominik","first_name":"Dominik","last_name":"Teutenberg","id":"537"},{"id":"32056","full_name":"Meschut, Gerson","last_name":"Meschut","orcid":"0000-0002-2763-1246","first_name":"Gerson"},{"first_name":"Dennis","orcid":"0000-0002-2755-6514","last_name":"Meinderink","full_name":"Meinderink, Dennis","id":"32378"},{"last_name":"Koch","first_name":"Leon ","full_name":"Koch, Leon "},{"id":"7266","last_name":"Ebbert","first_name":"Christoph","full_name":"Ebbert, Christoph"},{"id":"194","full_name":"Grundmeier, Guido","first_name":"Guido","last_name":"Grundmeier"}],"date_updated":"2022-01-06T06:55:11Z"},{"user_id":"71051","volume":33,"page":"2008752","_id":"22220","status":"public","project":[{"name":"Computing Resources Provided by the Paderborn Center for Parallel Computing","_id":"52"}],"citation":{"bibtex":"@article{Wang_Kormath Madam Raghupathy_Querebillo_Liao_Li_Lin_Hantusch_Sofer_Li_Zschech_et al._2021, title={Interfacial Covalent Bonds Regulated Electron-Deficient 2D Black Phosphorus for Electrocatalytic Oxygen Reactions}, volume={33}, DOI={<a href=\"https://doi.org/10.1002/adma.202008752\">https://doi.org/10.1002/adma.202008752</a>}, number={20}, journal={Advanced Materials}, author={Wang, Xia and Kormath Madam Raghupathy, Ramya and Querebillo, Christine Joy and Liao, Zhongquan and Li, Dongqi and Lin, Kui and Hantusch, Martin and Sofer, Zdeněk and Li, Baohua and Zschech, Ehrenfried and et al.}, year={2021}, pages={2008752} }","ama":"Wang X, Kormath Madam Raghupathy R, Querebillo CJ, et al. Interfacial Covalent Bonds Regulated Electron-Deficient 2D Black Phosphorus for Electrocatalytic Oxygen Reactions. <i>Advanced Materials</i>. 2021;33(20):2008752. doi:<a href=\"https://doi.org/10.1002/adma.202008752\">https://doi.org/10.1002/adma.202008752</a>","short":"X. Wang, R. Kormath Madam Raghupathy, C.J. Querebillo, Z. Liao, D. Li, K. Lin, M. Hantusch, Z. Sofer, B. Li, E. Zschech, I.M. Weidinger, T. Kühne, H. Mirhosseini, M. Yu, X. Feng, Advanced Materials 33 (2021) 2008752.","chicago":"Wang, Xia, Ramya Kormath Madam Raghupathy, Christine Joy Querebillo, Zhongquan Liao, Dongqi Li, Kui Lin, Martin Hantusch, et al. “Interfacial Covalent Bonds Regulated Electron-Deficient 2D Black Phosphorus for Electrocatalytic Oxygen Reactions.” <i>Advanced Materials</i> 33, no. 20 (2021): 2008752. <a href=\"https://doi.org/10.1002/adma.202008752\">https://doi.org/10.1002/adma.202008752</a>.","ieee":"X. Wang <i>et al.</i>, “Interfacial Covalent Bonds Regulated Electron-Deficient 2D Black Phosphorus for Electrocatalytic Oxygen Reactions,” <i>Advanced Materials</i>, vol. 33, no. 20, p. 2008752, 2021, doi: <a href=\"https://doi.org/10.1002/adma.202008752\">https://doi.org/10.1002/adma.202008752</a>.","mla":"Wang, Xia, et al. “Interfacial Covalent Bonds Regulated Electron-Deficient 2D Black Phosphorus for Electrocatalytic Oxygen Reactions.” <i>Advanced Materials</i>, vol. 33, no. 20, 2021, p. 2008752, doi:<a href=\"https://doi.org/10.1002/adma.202008752\">https://doi.org/10.1002/adma.202008752</a>.","apa":"Wang, X., Kormath Madam Raghupathy, R., Querebillo, C. J., Liao, Z., Li, D., Lin, K., Hantusch, M., Sofer, Z., Li, B., Zschech, E., Weidinger, I. M., Kühne, T., Mirhosseini, H., Yu, M., &#38; Feng, X. (2021). Interfacial Covalent Bonds Regulated Electron-Deficient 2D Black Phosphorus for Electrocatalytic Oxygen Reactions. <i>Advanced Materials</i>, <i>33</i>(20), 2008752. <a href=\"https://doi.org/10.1002/adma.202008752\">https://doi.org/10.1002/adma.202008752</a>"},"doi":"https://doi.org/10.1002/adma.202008752","language":[{"iso":"eng"}],"date_updated":"2022-07-21T09:25:33Z","intvolume":"        33","title":"Interfacial Covalent Bonds Regulated Electron-Deficient 2D Black Phosphorus for Electrocatalytic Oxygen Reactions","year":"2021","author":[{"last_name":"Wang","first_name":"Xia","full_name":"Wang, Xia"},{"full_name":"Kormath Madam Raghupathy, Ramya","last_name":"Kormath Madam Raghupathy","first_name":"Ramya","orcid":"https://orcid.org/0000-0003-4667-9744","id":"71692"},{"full_name":"Querebillo, Christine Joy","last_name":"Querebillo","first_name":"Christine Joy"},{"full_name":"Liao, Zhongquan","first_name":"Zhongquan","last_name":"Liao"},{"first_name":"Dongqi","last_name":"Li","full_name":"Li, Dongqi"},{"full_name":"Lin, Kui","last_name":"Lin","first_name":"Kui"},{"full_name":"Hantusch, Martin","last_name":"Hantusch","first_name":"Martin"},{"first_name":"Zdeněk","last_name":"Sofer","full_name":"Sofer, Zdeněk"},{"full_name":"Li, Baohua","first_name":"Baohua","last_name":"Li"},{"first_name":"Ehrenfried","last_name":"Zschech","full_name":"Zschech, Ehrenfried"},{"full_name":"Weidinger, Inez M.","last_name":"Weidinger","first_name":"Inez M."},{"id":"49079","full_name":"Kühne, Thomas","last_name":"Kühne","first_name":"Thomas"},{"full_name":"Mirhosseini, Hossein","last_name":"Mirhosseini","first_name":"Hossein","orcid":"0000-0001-6179-1545","id":"71051"},{"full_name":"Yu, Minghao","first_name":"Minghao","last_name":"Yu"},{"last_name":"Feng","first_name":"Xinliang","full_name":"Feng, Xinliang"}],"keyword":["2D materials","bifunctional oxygen electrocatalysts","black phosphorus","oxygen evolution reaction","zinc–air batteries"],"type":"journal_article","department":[{"_id":"304"}],"date_created":"2021-05-21T12:38:41Z","abstract":[{"text":"Abstract Developing resource-abundant and sustainable metal-free bifunctional oxygen electrocatalysts is essential for the practical application of zinc–air batteries (ZABs). 2D black phosphorus (BP) with fully exposed atoms and active lone pair electrons can be promising for oxygen electrocatalysts, which, however, suffers from low catalytic activity and poor electrochemical stability. Herein, guided by density functional theory (DFT) calculations, an efficient metal-free electrocatalyst is demonstrated via covalently bonding BP nanosheets with graphitic carbon nitride (denoted BP-CN-c). The polarized PN covalent bonds in BP-CN-c can efficiently regulate the electron transfer from BP to graphitic carbon nitride and significantly promote the OOH* adsorption on phosphorus atoms. Impressively, the oxygen evolution reaction performance of BP-CN-c (overpotential of 350 mV at 10 mA cm−2, 90\\% retention after 10 h operation) represents the state-of-the-art among the reported BP-based metal-free catalysts. Additionally, BP-CN-c exhibits a small half-wave overpotential of 390 mV for oxygen reduction reaction, representing the first bifunctional BP-based metal-free oxygen catalyst. Moreover, ZABs are assembled incorporating BP-CN-c cathodes, delivering a substantially higher peak power density (168.3 mW cm−2) than the Pt/C+RuO2-based ZABs (101.3 mW cm−2). The acquired insights into interfacial covalent bonds pave the way for the rational design of new and affordable metal-free catalysts.","lang":"eng"}],"issue":"20","publication":"Advanced Materials"},{"publication":"Phys. Chem. Chem. Phys.","citation":{"apa":"Ghasemi, A., Mirhosseini, H., &#38; Kühne, T. (2021). Thermodynamically stable polymorphs of nitrogen-rich carbon nitrides: a C3N5 study. <i>Phys. Chem. Chem. Phys.</i>, <i>23</i>, 6422–6432. <a href=\"https://doi.org/10.1039/D0CP06185A\">https://doi.org/10.1039/D0CP06185A</a>","mla":"Ghasemi, Alireza, et al. “Thermodynamically Stable Polymorphs of Nitrogen-Rich Carbon Nitrides: A C3N5 Study.” <i>Phys. Chem. Chem. Phys.</i>, vol. 23, The Royal Society of Chemistry, 2021, pp. 6422–32, doi:<a href=\"https://doi.org/10.1039/D0CP06185A\">10.1039/D0CP06185A</a>.","ieee":"A. Ghasemi, H. Mirhosseini, and T. Kühne, “Thermodynamically stable polymorphs of nitrogen-rich carbon nitrides: a C3N5 study,” <i>Phys. Chem. Chem. Phys.</i>, vol. 23, pp. 6422–6432, 2021, doi: <a href=\"https://doi.org/10.1039/D0CP06185A\">10.1039/D0CP06185A</a>.","chicago":"Ghasemi, Alireza, Hossein Mirhosseini, and Thomas Kühne. “Thermodynamically Stable Polymorphs of Nitrogen-Rich Carbon Nitrides: A C3N5 Study.” <i>Phys. Chem. Chem. Phys.</i> 23 (2021): 6422–32. <a href=\"https://doi.org/10.1039/D0CP06185A\">https://doi.org/10.1039/D0CP06185A</a>.","ama":"Ghasemi A, Mirhosseini H, Kühne T. Thermodynamically stable polymorphs of nitrogen-rich carbon nitrides: a C3N5 study. <i>Phys Chem Chem Phys</i>. 2021;23:6422-6432. doi:<a href=\"https://doi.org/10.1039/D0CP06185A\">10.1039/D0CP06185A</a>","short":"A. Ghasemi, H. Mirhosseini, T. Kühne, Phys. Chem. Chem. Phys. 23 (2021) 6422–6432.","bibtex":"@article{Ghasemi_Mirhosseini_Kühne_2021, title={Thermodynamically stable polymorphs of nitrogen-rich carbon nitrides: a C3N5 study}, volume={23}, DOI={<a href=\"https://doi.org/10.1039/D0CP06185A\">10.1039/D0CP06185A</a>}, journal={Phys. Chem. Chem. Phys.}, publisher={The Royal Society of Chemistry}, author={Ghasemi, Alireza and Mirhosseini, Hossein and Kühne, Thomas}, year={2021}, pages={6422–6432} }"},"abstract":[{"text":"We have carried out an extensive search for stable polymorphs of carbon nitride with C3N5 stoichiometry using the minima hopping method. Contrary to the widely held opinion that stacked{,} planar{,} graphite-like structures are energetically the most stable carbon nitride polymorphs for various nitrogen contents{,} we find that this does not apply for nitrogen-rich materials owing to the high abundance of N–N bonds. In fact{,} our results disclose novel morphologies with moieties not previously considered for C3N5. We demonstrate that nitrogen-rich compounds crystallize in a large variety of different structures due to particular characteristics of their energy landscapes. The newly found low-energy structures of C3N5 have band gaps within good agreement with the values measured in experimental studies.","lang":"eng"}],"project":[{"_id":"52","name":"PC2: Computing Resources Provided by the Paderborn Center for Parallel Computing"}],"date_created":"2022-01-31T11:00:05Z","type":"journal_article","department":[{"_id":"304"}],"status":"public","year":"2021","title":"Thermodynamically stable polymorphs of nitrogen-rich carbon nitrides: a C3N5 study","author":[{"id":"77282","full_name":"Ghasemi, Alireza","first_name":"Alireza","last_name":"Ghasemi"},{"full_name":"Mirhosseini, Hossein","orcid":"0000-0001-6179-1545","first_name":"Hossein","last_name":"Mirhosseini","id":"71051"},{"full_name":"Kühne, Thomas","first_name":"Thomas","last_name":"Kühne","id":"49079"}],"date_updated":"2022-07-21T09:26:33Z","intvolume":"        23","page":"6422-6432","_id":"29700","publisher":"The Royal Society of Chemistry","language":[{"iso":"eng"}],"doi":"10.1039/D0CP06185A","user_id":"71051","volume":23},{"department":[{"_id":"311"}],"type":"journal_article","date_created":"2021-09-02T12:48:00Z","citation":{"ama":"Schoppa T, Jung D, Rust T, Mulac D, Kuckling D, Langer K. Light-responsive polymeric nanoparticles based on a novel nitropiperonal based polyester as drug delivery systems for photosensitizers in PDT. <i>International Journal of Pharmaceutics</i>. 2021;597. doi:<a href=\"https://doi.org/10.1016/j.ijpharm.2021.120326\">10.1016/j.ijpharm.2021.120326</a>","bibtex":"@article{Schoppa_Jung_Rust_Mulac_Kuckling_Langer_2021, title={Light-responsive polymeric nanoparticles based on a novel nitropiperonal based polyester as drug delivery systems for photosensitizers in PDT}, volume={597}, DOI={<a href=\"https://doi.org/10.1016/j.ijpharm.2021.120326\">10.1016/j.ijpharm.2021.120326</a>}, number={120326}, journal={International Journal of Pharmaceutics}, publisher={Elsevier}, author={Schoppa, Timo and Jung, Dimitri and Rust, Tarik and Mulac, Dennis and Kuckling, Dirk and Langer, Klaus}, year={2021} }","mla":"Schoppa, Timo, et al. “Light-Responsive Polymeric Nanoparticles Based on a Novel Nitropiperonal Based Polyester as Drug Delivery Systems for Photosensitizers in PDT.” <i>International Journal of Pharmaceutics</i>, vol. 597, 120326, Elsevier, 2021, doi:<a href=\"https://doi.org/10.1016/j.ijpharm.2021.120326\">10.1016/j.ijpharm.2021.120326</a>.","short":"T. Schoppa, D. Jung, T. Rust, D. Mulac, D. Kuckling, K. Langer, International Journal of Pharmaceutics 597 (2021).","chicago":"Schoppa, Timo, Dimitri Jung, Tarik Rust, Dennis Mulac, Dirk Kuckling, and Klaus Langer. “Light-Responsive Polymeric Nanoparticles Based on a Novel Nitropiperonal Based Polyester as Drug Delivery Systems for Photosensitizers in PDT.” <i>International Journal of Pharmaceutics</i> 597 (2021). <a href=\"https://doi.org/10.1016/j.ijpharm.2021.120326\">https://doi.org/10.1016/j.ijpharm.2021.120326</a>.","apa":"Schoppa, T., Jung, D., Rust, T., Mulac, D., Kuckling, D., &#38; Langer, K. (2021). Light-responsive polymeric nanoparticles based on a novel nitropiperonal based polyester as drug delivery systems for photosensitizers in PDT. <i>International Journal of Pharmaceutics</i>, <i>597</i>, Article 120326. <a href=\"https://doi.org/10.1016/j.ijpharm.2021.120326\">https://doi.org/10.1016/j.ijpharm.2021.120326</a>","ieee":"T. Schoppa, D. Jung, T. Rust, D. Mulac, D. Kuckling, and K. Langer, “Light-responsive polymeric nanoparticles based on a novel nitropiperonal based polyester as drug delivery systems for photosensitizers in PDT,” <i>International Journal of Pharmaceutics</i>, vol. 597, Art. no. 120326, 2021, doi: <a href=\"https://doi.org/10.1016/j.ijpharm.2021.120326\">10.1016/j.ijpharm.2021.120326</a>."},"publication":"International Journal of Pharmaceutics","volume":597,"user_id":"94","doi":"10.1016/j.ijpharm.2021.120326","language":[{"iso":"eng"}],"_id":"23701","publisher":"Elsevier","article_number":"120326","intvolume":"       597","publication_status":"published","date_updated":"2022-07-28T09:57:44Z","author":[{"full_name":"Schoppa, Timo","first_name":"Timo","last_name":"Schoppa"},{"full_name":"Jung, Dimitri","last_name":"Jung","first_name":"Dimitri"},{"full_name":"Rust, Tarik","last_name":"Rust","first_name":"Tarik"},{"full_name":"Mulac, Dennis","first_name":"Dennis","last_name":"Mulac"},{"id":"287","last_name":"Kuckling","first_name":"Dirk","full_name":"Kuckling, Dirk"},{"full_name":"Langer, Klaus","last_name":"Langer","first_name":"Klaus"}],"publication_identifier":{"issn":["0378-5173"]},"title":"Light-responsive polymeric nanoparticles based on a novel nitropiperonal based polyester as drug delivery systems for photosensitizers in PDT","status":"public","year":"2021"}]