[{"date_created":"2021-01-20T08:40:04Z","department":[{"_id":"15"}],"type":"journal_article","publication":"Optica","issue":"5","language":[{"iso":"eng"}],"article_number":"534-550","doi":"10.1364/optica.5.000534","publication_identifier":{"issn":["2334-2536"]},"author":[{"full_name":"Ansari, Vahid","last_name":"Ansari","first_name":"Vahid"},{"last_name":"Donohue","first_name":"John M.","full_name":"Donohue, John M."},{"id":"27150","first_name":"Benjamin","orcid":"0000-0003-4140-0556 ","last_name":"Brecht","full_name":"Brecht, Benjamin"},{"full_name":"Silberhorn, Christine","last_name":"Silberhorn","first_name":"Christine","id":"26263"}],"year":"2018","title":"Tailoring nonlinear processes for quantum optics with pulsed temporal-mode encodings","intvolume":"         5","publication_status":"published","date_updated":"2022-01-06T06:54:42Z","citation":{"ama":"Ansari V, Donohue JM, Brecht B, Silberhorn C. Tailoring nonlinear processes for quantum optics with pulsed temporal-mode encodings. <i>Optica</i>. 2018;5(5). doi:<a href=\"https://doi.org/10.1364/optica.5.000534\">10.1364/optica.5.000534</a>","bibtex":"@article{Ansari_Donohue_Brecht_Silberhorn_2018, title={Tailoring nonlinear processes for quantum optics with pulsed temporal-mode encodings}, volume={5}, DOI={<a href=\"https://doi.org/10.1364/optica.5.000534\">10.1364/optica.5.000534</a>}, number={5534–550}, journal={Optica}, author={Ansari, Vahid and Donohue, John M. and Brecht, Benjamin and Silberhorn, Christine}, year={2018} }","mla":"Ansari, Vahid, et al. “Tailoring Nonlinear Processes for Quantum Optics with Pulsed Temporal-Mode Encodings.” <i>Optica</i>, vol. 5, no. 5, 534–550, 2018, doi:<a href=\"https://doi.org/10.1364/optica.5.000534\">10.1364/optica.5.000534</a>.","short":"V. Ansari, J.M. Donohue, B. Brecht, C. Silberhorn, Optica 5 (2018).","chicago":"Ansari, Vahid, John M. Donohue, Benjamin Brecht, and Christine Silberhorn. “Tailoring Nonlinear Processes for Quantum Optics with Pulsed Temporal-Mode Encodings.” <i>Optica</i> 5, no. 5 (2018). <a href=\"https://doi.org/10.1364/optica.5.000534\">https://doi.org/10.1364/optica.5.000534</a>.","apa":"Ansari, V., Donohue, J. M., Brecht, B., &#38; Silberhorn, C. (2018). Tailoring nonlinear processes for quantum optics with pulsed temporal-mode encodings. <i>Optica</i>, <i>5</i>(5). <a href=\"https://doi.org/10.1364/optica.5.000534\">https://doi.org/10.1364/optica.5.000534</a>","ieee":"V. Ansari, J. M. Donohue, B. Brecht, and C. Silberhorn, “Tailoring nonlinear processes for quantum optics with pulsed temporal-mode encodings,” <i>Optica</i>, vol. 5, no. 5, 2018."},"project":[{"_id":"71","name":"TRR 142 - Subproject C1"}],"_id":"21028","volume":5,"user_id":"27150","status":"public"},{"date_created":"2018-03-23T13:14:51Z","department":[{"_id":"15"},{"_id":"230"}],"type":"journal_article","publication":"Nanophotonics","issue":"6","language":[{"iso":"eng"}],"main_file_link":[{"url":"https://www.degruyter.com/view/journals/nanoph/7/6/article-p1169.xml","open_access":"1"}],"doi":"10.1515/nanoph-2017-0118","author":[{"full_name":"Huang, Lingling","first_name":"Lingling","last_name":"Huang"},{"first_name":"Shuang","last_name":"Zhang","full_name":"Zhang, Shuang"},{"id":"30525","last_name":"Zentgraf","first_name":"Thomas","orcid":"0000-0002-8662-1101","full_name":"Zentgraf, Thomas"}],"publication_identifier":{"issn":["2192-8614"]},"year":"2018","title":"Metasurface holography: from fundamentals to applications","intvolume":"         7","date_updated":"2022-01-06T06:53:16Z","publication_status":"published","oa":"1","citation":{"bibtex":"@article{Huang_Zhang_Zentgraf_2018, title={Metasurface holography: from fundamentals to applications}, volume={7}, DOI={<a href=\"https://doi.org/10.1515/nanoph-2017-0118\">10.1515/nanoph-2017-0118</a>}, number={6}, journal={Nanophotonics}, publisher={Walter de Gruyter GmbH}, author={Huang, Lingling and Zhang, Shuang and Zentgraf, Thomas}, year={2018}, pages={1169–1190} }","chicago":"Huang, Lingling, Shuang Zhang, and Thomas Zentgraf. “Metasurface Holography: From Fundamentals to Applications.” <i>Nanophotonics</i> 7, no. 6 (2018): 1169–90. <a href=\"https://doi.org/10.1515/nanoph-2017-0118\">https://doi.org/10.1515/nanoph-2017-0118</a>.","short":"L. Huang, S. Zhang, T. Zentgraf, Nanophotonics 7 (2018) 1169–1190.","ama":"Huang L, Zhang S, Zentgraf T. Metasurface holography: from fundamentals to applications. <i>Nanophotonics</i>. 2018;7(6):1169-1190. doi:<a href=\"https://doi.org/10.1515/nanoph-2017-0118\">10.1515/nanoph-2017-0118</a>","ieee":"L. Huang, S. Zhang, and T. Zentgraf, “Metasurface holography: from fundamentals to applications,” <i>Nanophotonics</i>, vol. 7, no. 6, pp. 1169–1190, 2018.","apa":"Huang, L., Zhang, S., &#38; Zentgraf, T. (2018). Metasurface holography: from fundamentals to applications. <i>Nanophotonics</i>, <i>7</i>(6), 1169–1190. <a href=\"https://doi.org/10.1515/nanoph-2017-0118\">https://doi.org/10.1515/nanoph-2017-0118</a>","mla":"Huang, Lingling, et al. “Metasurface Holography: From Fundamentals to Applications.” <i>Nanophotonics</i>, vol. 7, no. 6, Walter de Gruyter GmbH, 2018, pp. 1169–90, doi:<a href=\"https://doi.org/10.1515/nanoph-2017-0118\">10.1515/nanoph-2017-0118</a>."},"quality_controlled":"1","_id":"1765","publisher":"Walter de Gruyter GmbH","page":"1169-1190","volume":7,"user_id":"30525","status":"public"},{"language":[{"iso":"eng"}],"_id":"23623","page":"26972-26981","volume":20,"user_id":"84268","doi":"10.1021/acsami.8b04573","author":[{"full_name":"Chen, Lin","last_name":"Chen","first_name":"Lin"},{"last_name":"Chen","first_name":"Kan-Sheng","full_name":"Chen, Kan-Sheng"},{"full_name":"Chen, Xinjie","first_name":"Xinjie","last_name":"Chen"},{"full_name":"Ramirez, Giovanni","last_name":"Ramirez","first_name":"Giovanni"},{"last_name":"Huang","first_name":"Zhennan","full_name":"Huang, Zhennan"},{"last_name":"Geise","first_name":"Natalie R.","full_name":"Geise, Natalie R."},{"orcid":"0000-0001-6373-0877","first_name":"Hans-Georg","last_name":"Steinrück","full_name":"Steinrück, Hans-Georg","id":"84268"},{"full_name":"Fisher, Brandon L.","first_name":"Brandon L.","last_name":"Fisher"},{"first_name":"Reza","last_name":"Shahbazian-Yassar","full_name":"Shahbazian-Yassar, Reza"},{"full_name":"Toney, Michael F.","last_name":"Toney","first_name":"Michael F."},{"last_name":"Hersam","first_name":"Mark C.","full_name":"Hersam, Mark C."},{"full_name":"Elam, Jeffrey W.","last_name":"Elam","first_name":"Jeffrey W."}],"publication_identifier":{"issn":["1944-8244","1944-8252"]},"title":"Novel ALD Chemistry Enabled Low-Temperature Synthesis of Lithium Fluoride Coatings for Durable Lithium Anodes","year":"2018","status":"public","intvolume":"        20","publication_status":"published","date_updated":"2022-01-06T06:55:57Z","date_created":"2021-09-01T09:47:02Z","department":[{"_id":"633"}],"type":"journal_article","citation":{"ama":"Chen L, Chen K-S, Chen X, et al. Novel ALD Chemistry Enabled Low-Temperature Synthesis of Lithium Fluoride Coatings for Durable Lithium Anodes. <i>ACS Applied Materials &#38; Interfaces</i>. 2018;20:26972-26981. doi:<a href=\"https://doi.org/10.1021/acsami.8b04573\">10.1021/acsami.8b04573</a>","bibtex":"@article{Chen_Chen_Chen_Ramirez_Huang_Geise_Steinrück_Fisher_Shahbazian-Yassar_Toney_et al._2018, title={Novel ALD Chemistry Enabled Low-Temperature Synthesis of Lithium Fluoride Coatings for Durable Lithium Anodes}, volume={20}, DOI={<a href=\"https://doi.org/10.1021/acsami.8b04573\">10.1021/acsami.8b04573</a>}, journal={ACS Applied Materials &#38; Interfaces}, author={Chen, Lin and Chen, Kan-Sheng and Chen, Xinjie and Ramirez, Giovanni and Huang, Zhennan and Geise, Natalie R. and Steinrück, Hans-Georg and Fisher, Brandon L. and Shahbazian-Yassar, Reza and Toney, Michael F. and et al.}, year={2018}, pages={26972–26981} }","mla":"Chen, Lin, et al. “Novel ALD Chemistry Enabled Low-Temperature Synthesis of Lithium Fluoride Coatings for Durable Lithium Anodes.” <i>ACS Applied Materials &#38; Interfaces</i>, vol. 20, 2018, pp. 26972–81, doi:<a href=\"https://doi.org/10.1021/acsami.8b04573\">10.1021/acsami.8b04573</a>.","short":"L. Chen, K.-S. Chen, X. Chen, G. Ramirez, Z. Huang, N.R. Geise, H.-G. Steinrück, B.L. Fisher, R. Shahbazian-Yassar, M.F. Toney, M.C. Hersam, J.W. Elam, ACS Applied Materials &#38; Interfaces 20 (2018) 26972–26981.","chicago":"Chen, Lin, Kan-Sheng Chen, Xinjie Chen, Giovanni Ramirez, Zhennan Huang, Natalie R. Geise, Hans-Georg Steinrück, et al. “Novel ALD Chemistry Enabled Low-Temperature Synthesis of Lithium Fluoride Coatings for Durable Lithium Anodes.” <i>ACS Applied Materials &#38; Interfaces</i> 20 (2018): 26972–81. <a href=\"https://doi.org/10.1021/acsami.8b04573\">https://doi.org/10.1021/acsami.8b04573</a>.","apa":"Chen, L., Chen, K.-S., Chen, X., Ramirez, G., Huang, Z., Geise, N. R., Steinrück, H.-G., Fisher, B. L., Shahbazian-Yassar, R., Toney, M. F., Hersam, M. C., &#38; Elam, J. W. (2018). Novel ALD Chemistry Enabled Low-Temperature Synthesis of Lithium Fluoride Coatings for Durable Lithium Anodes. <i>ACS Applied Materials &#38; Interfaces</i>, <i>20</i>, 26972–26981. <a href=\"https://doi.org/10.1021/acsami.8b04573\">https://doi.org/10.1021/acsami.8b04573</a>","ieee":"L. Chen <i>et al.</i>, “Novel ALD Chemistry Enabled Low-Temperature Synthesis of Lithium Fluoride Coatings for Durable Lithium Anodes,” <i>ACS Applied Materials &#38; Interfaces</i>, vol. 20, pp. 26972–26981, 2018, doi: <a href=\"https://doi.org/10.1021/acsami.8b04573\">10.1021/acsami.8b04573</a>."},"publication":"ACS Applied Materials & Interfaces"},{"author":[{"first_name":"Yonatan","last_name":"Horowitz","full_name":"Horowitz, Yonatan"},{"last_name":"Steinrück","first_name":"Hans-Georg","orcid":"0000-0001-6373-0877","full_name":"Steinrück, Hans-Georg","id":"84268"},{"last_name":"Han","first_name":"Hui-Ling","full_name":"Han, Hui-Ling"},{"last_name":"Cao","first_name":"Chuntian","full_name":"Cao, Chuntian"},{"last_name":"Abate","first_name":"Iwnetim Iwnetu","full_name":"Abate, Iwnetim Iwnetu"},{"full_name":"Tsao, Yuchi","last_name":"Tsao","first_name":"Yuchi"},{"first_name":"Michael F.","last_name":"Toney","full_name":"Toney, Michael F."},{"last_name":"Somorjai","first_name":"Gabor A.","full_name":"Somorjai, Gabor A."}],"publication_identifier":{"issn":["1530-6984","1530-6992"]},"year":"2018","title":"Fluoroethylene Carbonate Induces Ordered Electrolyte Interface on Silicon and Sapphire Surfaces as Revealed by Sum Frequency Generation Vibrational Spectroscopy and X-ray Reflectivity","status":"public","intvolume":"        18","date_updated":"2022-01-06T06:55:57Z","publication_status":"published","language":[{"iso":"eng"}],"_id":"23624","page":"2105-2111","volume":18,"doi":"10.1021/acs.nanolett.8b00298","user_id":"84268","citation":{"short":"Y. Horowitz, H.-G. Steinrück, H.-L. Han, C. Cao, I.I. Abate, Y. Tsao, M.F. Toney, G.A. Somorjai, Nano Letters 18 (2018) 2105–2111.","chicago":"Horowitz, Yonatan, Hans-Georg Steinrück, Hui-Ling Han, Chuntian Cao, Iwnetim Iwnetu Abate, Yuchi Tsao, Michael F. Toney, and Gabor A. Somorjai. “Fluoroethylene Carbonate Induces Ordered Electrolyte Interface on Silicon and Sapphire Surfaces as Revealed by Sum Frequency Generation Vibrational Spectroscopy and X-Ray Reflectivity.” <i>Nano Letters</i> 18 (2018): 2105–11. <a href=\"https://doi.org/10.1021/acs.nanolett.8b00298\">https://doi.org/10.1021/acs.nanolett.8b00298</a>.","apa":"Horowitz, Y., Steinrück, H.-G., Han, H.-L., Cao, C., Abate, I. I., Tsao, Y., Toney, M. F., &#38; Somorjai, G. A. (2018). Fluoroethylene Carbonate Induces Ordered Electrolyte Interface on Silicon and Sapphire Surfaces as Revealed by Sum Frequency Generation Vibrational Spectroscopy and X-ray Reflectivity. <i>Nano Letters</i>, <i>18</i>, 2105–2111. <a href=\"https://doi.org/10.1021/acs.nanolett.8b00298\">https://doi.org/10.1021/acs.nanolett.8b00298</a>","ieee":"Y. Horowitz <i>et al.</i>, “Fluoroethylene Carbonate Induces Ordered Electrolyte Interface on Silicon and Sapphire Surfaces as Revealed by Sum Frequency Generation Vibrational Spectroscopy and X-ray Reflectivity,” <i>Nano Letters</i>, vol. 18, pp. 2105–2111, 2018, doi: <a href=\"https://doi.org/10.1021/acs.nanolett.8b00298\">10.1021/acs.nanolett.8b00298</a>.","ama":"Horowitz Y, Steinrück H-G, Han H-L, et al. Fluoroethylene Carbonate Induces Ordered Electrolyte Interface on Silicon and Sapphire Surfaces as Revealed by Sum Frequency Generation Vibrational Spectroscopy and X-ray Reflectivity. <i>Nano Letters</i>. 2018;18:2105-2111. doi:<a href=\"https://doi.org/10.1021/acs.nanolett.8b00298\">10.1021/acs.nanolett.8b00298</a>","bibtex":"@article{Horowitz_Steinrück_Han_Cao_Abate_Tsao_Toney_Somorjai_2018, title={Fluoroethylene Carbonate Induces Ordered Electrolyte Interface on Silicon and Sapphire Surfaces as Revealed by Sum Frequency Generation Vibrational Spectroscopy and X-ray Reflectivity}, volume={18}, DOI={<a href=\"https://doi.org/10.1021/acs.nanolett.8b00298\">10.1021/acs.nanolett.8b00298</a>}, journal={Nano Letters}, author={Horowitz, Yonatan and Steinrück, Hans-Georg and Han, Hui-Ling and Cao, Chuntian and Abate, Iwnetim Iwnetu and Tsao, Yuchi and Toney, Michael F. and Somorjai, Gabor A.}, year={2018}, pages={2105–2111} }","mla":"Horowitz, Yonatan, et al. “Fluoroethylene Carbonate Induces Ordered Electrolyte Interface on Silicon and Sapphire Surfaces as Revealed by Sum Frequency Generation Vibrational Spectroscopy and X-Ray Reflectivity.” <i>Nano Letters</i>, vol. 18, 2018, pp. 2105–11, doi:<a href=\"https://doi.org/10.1021/acs.nanolett.8b00298\">10.1021/acs.nanolett.8b00298</a>."},"publication":"Nano Letters","date_created":"2021-09-01T09:47:06Z","department":[{"_id":"633"}],"type":"journal_article"},{"page":"594-602","language":[{"iso":"eng"}],"_id":"23625","user_id":"84268","doi":"10.1039/c7ee02724a","volume":11,"year":"2018","status":"public","title":"The nanoscale structure of the electrolyte–metal oxide interface","author":[{"full_name":"Steinrück, Hans-Georg","first_name":"Hans-Georg","orcid":"0000-0001-6373-0877","last_name":"Steinrück","id":"84268"},{"full_name":"Cao, Chuntian","first_name":"Chuntian","last_name":"Cao"},{"last_name":"Tsao","first_name":"Yuchi","full_name":"Tsao, Yuchi"},{"first_name":"Christopher J.","last_name":"Takacs","full_name":"Takacs, Christopher J."},{"full_name":"Konovalov, Oleg","first_name":"Oleg","last_name":"Konovalov"},{"full_name":"Vatamanu, Jenel","last_name":"Vatamanu","first_name":"Jenel"},{"full_name":"Borodin, Oleg","first_name":"Oleg","last_name":"Borodin"},{"full_name":"Toney, Michael F.","first_name":"Michael F.","last_name":"Toney"}],"publication_identifier":{"issn":["1754-5692","1754-5706"]},"publication_status":"published","date_updated":"2022-01-06T06:55:57Z","intvolume":"        11","date_created":"2021-09-01T09:47:13Z","type":"journal_article","department":[{"_id":"633"}],"publication":"Energy & Environmental Science","citation":{"mla":"Steinrück, Hans-Georg, et al. “The Nanoscale Structure of the Electrolyte–Metal Oxide Interface.” <i>Energy &#38; Environmental Science</i>, vol. 11, 2018, pp. 594–602, doi:<a href=\"https://doi.org/10.1039/c7ee02724a\">10.1039/c7ee02724a</a>.","bibtex":"@article{Steinrück_Cao_Tsao_Takacs_Konovalov_Vatamanu_Borodin_Toney_2018, title={The nanoscale structure of the electrolyte–metal oxide interface}, volume={11}, DOI={<a href=\"https://doi.org/10.1039/c7ee02724a\">10.1039/c7ee02724a</a>}, journal={Energy &#38; Environmental Science}, author={Steinrück, Hans-Georg and Cao, Chuntian and Tsao, Yuchi and Takacs, Christopher J. and Konovalov, Oleg and Vatamanu, Jenel and Borodin, Oleg and Toney, Michael F.}, year={2018}, pages={594–602} }","ama":"Steinrück H-G, Cao C, Tsao Y, et al. The nanoscale structure of the electrolyte–metal oxide interface. <i>Energy &#38; Environmental Science</i>. 2018;11:594-602. doi:<a href=\"https://doi.org/10.1039/c7ee02724a\">10.1039/c7ee02724a</a>","ieee":"H.-G. Steinrück <i>et al.</i>, “The nanoscale structure of the electrolyte–metal oxide interface,” <i>Energy &#38; Environmental Science</i>, vol. 11, pp. 594–602, 2018, doi: <a href=\"https://doi.org/10.1039/c7ee02724a\">10.1039/c7ee02724a</a>.","apa":"Steinrück, H.-G., Cao, C., Tsao, Y., Takacs, C. J., Konovalov, O., Vatamanu, J., Borodin, O., &#38; Toney, M. F. (2018). The nanoscale structure of the electrolyte–metal oxide interface. <i>Energy &#38; Environmental Science</i>, <i>11</i>, 594–602. <a href=\"https://doi.org/10.1039/c7ee02724a\">https://doi.org/10.1039/c7ee02724a</a>","short":"H.-G. Steinrück, C. Cao, Y. Tsao, C.J. Takacs, O. Konovalov, J. Vatamanu, O. Borodin, M.F. Toney, Energy &#38; Environmental Science 11 (2018) 594–602.","chicago":"Steinrück, Hans-Georg, Chuntian Cao, Yuchi Tsao, Christopher J. Takacs, Oleg Konovalov, Jenel Vatamanu, Oleg Borodin, and Michael F. Toney. “The Nanoscale Structure of the Electrolyte–Metal Oxide Interface.” <i>Energy &#38; Environmental Science</i> 11 (2018): 594–602. <a href=\"https://doi.org/10.1039/c7ee02724a\">https://doi.org/10.1039/c7ee02724a</a>."},"abstract":[{"text":"<p>Combined experimental and theoretical insights into electrolyte–electrode interfaces relevant to lithium ion batteries.</p>","lang":"eng"}]},{"publication":"Proceedings of the National Academy of Sciences","citation":{"mla":"Haddad, Julia, et al. “Surface Structure Evolution in a Homologous Series of Ionic Liquids.” <i>Proceedings of the National Academy of Sciences</i>, vol. 115, 2018, pp. E1100–07, doi:<a href=\"https://doi.org/10.1073/pnas.1716418115\">10.1073/pnas.1716418115</a>.","bibtex":"@article{Haddad_Pontoni_Murphy_Festersen_Runge_Magnussen_Steinrück_Reichert_Ocko_Deutsch_2018, title={Surface structure evolution in a homologous series of ionic liquids}, volume={115}, DOI={<a href=\"https://doi.org/10.1073/pnas.1716418115\">10.1073/pnas.1716418115</a>}, journal={Proceedings of the National Academy of Sciences}, author={Haddad, Julia and Pontoni, Diego and Murphy, Bridget M. and Festersen, Sven and Runge, Benjamin and Magnussen, Olaf M. and Steinrück, Hans-Georg and Reichert, Harald and Ocko, Benjamin M. and Deutsch, Moshe}, year={2018}, pages={E1100–E1107} }","ama":"Haddad J, Pontoni D, Murphy BM, et al. Surface structure evolution in a homologous series of ionic liquids. <i>Proceedings of the National Academy of Sciences</i>. 2018;115:E1100-E1107. doi:<a href=\"https://doi.org/10.1073/pnas.1716418115\">10.1073/pnas.1716418115</a>","ieee":"J. Haddad <i>et al.</i>, “Surface structure evolution in a homologous series of ionic liquids,” <i>Proceedings of the National Academy of Sciences</i>, vol. 115, pp. E1100–E1107, 2018, doi: <a href=\"https://doi.org/10.1073/pnas.1716418115\">10.1073/pnas.1716418115</a>.","apa":"Haddad, J., Pontoni, D., Murphy, B. M., Festersen, S., Runge, B., Magnussen, O. M., Steinrück, H.-G., Reichert, H., Ocko, B. M., &#38; Deutsch, M. (2018). Surface structure evolution in a homologous series of ionic liquids. <i>Proceedings of the National Academy of Sciences</i>, <i>115</i>, E1100–E1107. <a href=\"https://doi.org/10.1073/pnas.1716418115\">https://doi.org/10.1073/pnas.1716418115</a>","chicago":"Haddad, Julia, Diego Pontoni, Bridget M. Murphy, Sven Festersen, Benjamin Runge, Olaf M. Magnussen, Hans-Georg Steinrück, Harald Reichert, Benjamin M. Ocko, and Moshe Deutsch. “Surface Structure Evolution in a Homologous Series of Ionic Liquids.” <i>Proceedings of the National Academy of Sciences</i> 115 (2018): E1100–1107. <a href=\"https://doi.org/10.1073/pnas.1716418115\">https://doi.org/10.1073/pnas.1716418115</a>.","short":"J. Haddad, D. Pontoni, B.M. Murphy, S. Festersen, B. Runge, O.M. Magnussen, H.-G. Steinrück, H. Reichert, B.M. Ocko, M. Deutsch, Proceedings of the National Academy of Sciences 115 (2018) E1100–E1107."},"abstract":[{"lang":"eng","text":"<jats:p>Interfaces of room temperature ionic liquids (RTILs) are important for both applications and basic science and are therefore intensely studied. However, the evolution of their interface structure with the cation’s alkyl chain length n from Coulomb to van der Waals interaction domination has not yet been studied for even a single broad homologous RTIL series. We present here such a study of the liquid–air interface for <jats:inline-formula><m:math xmlns:m=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"><m:mrow><m:mpadded width=\"+1.7pt\"><m:mi>n</m:mi></m:mpadded><m:mo>=</m:mo><m:mrow><m:mpadded width=\"+1.7pt\"><m:mn>2</m:mn></m:mpadded><m:mtext>to</m:mtext><m:mo> </m:mo><m:mn>22</m:mn></m:mrow></m:mrow></m:math></jats:inline-formula>, using angstrom-resolution X-ray methods. For <jats:inline-formula><m:math xmlns:m=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"><m:mrow><m:mpadded width=\"+1.7pt\"><m:mi>n</m:mi></m:mpadded><m:mo mathvariant=\"bold\">&lt;</m:mo><m:mn>6</m:mn></m:mrow></m:math></jats:inline-formula>, a typical “simple liquid” monotonic surface-normal electron density profile <jats:inline-formula><m:math xmlns:m=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"><m:mrow><m:msub><m:mi>ρ</m:mi><m:mi>e</m:mi></m:msub><m:mrow><m:mo stretchy=\"false\">(</m:mo><m:mi>z</m:mi><m:mo stretchy=\"false\">)</m:mo></m:mrow></m:mrow></m:math></jats:inline-formula> is obtained, like those of water and organic solvents. For <jats:inline-formula><m:math xmlns:m=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"><m:mrow><m:mpadded width=\"+1.7pt\"><m:mi>n</m:mi></m:mpadded><m:mo mathvariant=\"bold\">&gt;</m:mo><m:mn>6</m:mn></m:mrow></m:math></jats:inline-formula>, increasingly more pronounced nanoscale self-segregation of the molecules’ charged moieties and apolar chains yields surface layering with alternating regions of headgroups and chains. The layering decays into the bulk over a few, to a few tens, of nanometers. The layering periods and decay lengths, their linear n dependence, and slopes are discussed within two models, one with partial-chain interdigitation and the other with liquid-like chains. No surface-parallel long-range order is found within the surface layer. For <jats:inline-formula><m:math xmlns:m=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"><m:mrow><m:mpadded width=\"+1.7pt\"><m:mi>n</m:mi></m:mpadded><m:mo>=</m:mo><m:mn>22</m:mn></m:mrow></m:math></jats:inline-formula>, a different surface phase is observed above melting. Our results also impact general liquid-phase issues like supramolecular self-aggregation and bulk–surface structure relations.</jats:p>"}],"date_created":"2021-09-01T09:47:27Z","type":"journal_article","department":[{"_id":"633"}],"title":"Surface structure evolution in a homologous series of ionic liquids","year":"2018","status":"public","publication_identifier":{"issn":["0027-8424","1091-6490"]},"author":[{"first_name":"Julia","last_name":"Haddad","full_name":"Haddad, Julia"},{"first_name":"Diego","last_name":"Pontoni","full_name":"Pontoni, Diego"},{"last_name":"Murphy","first_name":"Bridget M.","full_name":"Murphy, Bridget M."},{"last_name":"Festersen","first_name":"Sven","full_name":"Festersen, Sven"},{"full_name":"Runge, Benjamin","last_name":"Runge","first_name":"Benjamin"},{"first_name":"Olaf M.","last_name":"Magnussen","full_name":"Magnussen, Olaf M."},{"orcid":"0000-0001-6373-0877","last_name":"Steinrück","first_name":"Hans-Georg","full_name":"Steinrück, Hans-Georg","id":"84268"},{"last_name":"Reichert","first_name":"Harald","full_name":"Reichert, Harald"},{"last_name":"Ocko","first_name":"Benjamin M.","full_name":"Ocko, Benjamin M."},{"full_name":"Deutsch, Moshe","first_name":"Moshe","last_name":"Deutsch"}],"date_updated":"2022-01-06T06:55:57Z","publication_status":"published","intvolume":"       115","page":"E1100-E1107","language":[{"iso":"eng"}],"_id":"23626","doi":"10.1073/pnas.1716418115","user_id":"84268","volume":115},{"type":"book_chapter","department":[{"_id":"386"}],"date_created":"2021-09-03T12:14:38Z","place":"Berlin, Heidelberg","publication":"Theorien in der naturwissenschaftsdidaktischen Forschung","citation":{"ieee":"S. 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