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Höfer, Journal of Physics: Condensed Matter 17 (2005) S221–S244.","bibtex":"@article{Meier_Reichelt_Koch_Höfer_2005, title={Femtosecond time-resolved five-wave mixing at silicon surfaces}, volume={17}, DOI={<a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">10.1088/0953-8984/17/8/003</a>}, number={8}, journal={Journal of Physics: Condensed Matter}, author={Meier, Torsten and Reichelt, Matthias and Koch, S W and Höfer, U}, year={2005}, pages={S221–S244} }","mla":"Meier, Torsten, et al. “Femtosecond Time-Resolved Five-Wave Mixing at Silicon Surfaces.” <i>Journal of Physics: Condensed Matter</i>, vol. 17, no. 8, 2005, pp. S221–44, doi:<a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">10.1088/0953-8984/17/8/003</a>.","chicago":"Meier, Torsten, Matthias Reichelt, S W Koch, and U Höfer. “Femtosecond Time-Resolved Five-Wave Mixing at Silicon Surfaces.” <i>Journal of Physics: Condensed Matter</i> 17, no. 8 (2005): S221–44. <a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">https://doi.org/10.1088/0953-8984/17/8/003</a>.","ieee":"T. Meier, M. Reichelt, S. W. Koch, and U. Höfer, “Femtosecond time-resolved five-wave mixing at silicon surfaces,” <i>Journal of Physics: Condensed Matter</i>, vol. 17, no. 8, pp. S221–S244, 2005, doi: <a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">10.1088/0953-8984/17/8/003</a>.","ama":"Meier T, Reichelt M, Koch SW, Höfer U. Femtosecond time-resolved five-wave mixing at silicon surfaces. <i>Journal of Physics: Condensed Matter</i>. 2005;17(8):S221-S244. doi:<a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">10.1088/0953-8984/17/8/003</a>"},"page":"S221-S244","intvolume":"        17","date_updated":"2023-04-24T06:14:12Z","date_created":"2021-08-24T09:20:43Z","author":[{"first_name":"Torsten","orcid":"0000-0001-8864-2072","last_name":"Meier","id":"344","full_name":"Meier, Torsten"},{"last_name":"Reichelt","id":"138","full_name":"Reichelt, Matthias","first_name":"Matthias"},{"last_name":"Koch","full_name":"Koch, S W","first_name":"S W"},{"first_name":"U","full_name":"Höfer, U","last_name":"Höfer"}],"volume":17,"title":"Femtosecond time-resolved five-wave mixing at silicon surfaces","doi":"10.1088/0953-8984/17/8/003","type":"journal_article","publication":"Journal of Physics: Condensed Matter","abstract":[{"lang":"eng","text":"The ultrafast dynamics of photoexcitations at silicon surfaces is investigated using a surface-sensitive purely optical technique. In the experiments, the diffracted second harmonic generated by sequences of ultrashort laser pulses is detected as a function of the time delay between the pulses. It is demonstrated that this five-wave-mixing technique can be used to measure the temporal evolution of the optical polarization and the photoexcited populations at the surface. The experimental results can be reproduced by numerical solutions of optical Bloch equations. The theoretical analysis allows one to investigate which dephasing times and relaxation processes are compatible with experiment. Furthermore, it is outlined how one can describe optical nonlinearities at surfaces using a microscopic theory within the framework of semiconductor Bloch equations."}],"status":"public","_id":"23498","user_id":"49063","department":[{"_id":"15"},{"_id":"170"},{"_id":"293"},{"_id":"230"}],"language":[{"iso":"eng"}],"extern":"1"},{"language":[{"iso":"eng"}],"extern":"1","_id":"23499","department":[{"_id":"15"},{"_id":"170"},{"_id":"293"}],"user_id":"49063","abstract":[{"lang":"eng","text":"The ultrafast dynamics of photoexcitations at silicon surfaces is investigated using a surface-sensitive purely optical technique. In the experiments, the diffracted second harmonic generated by sequences of ultrashort laser pulses is detected as a function of the time delay between the pulses. It is demonstrated that this five-wave-mixing technique can be used to measure the temporal evolution of the optical polarization and the photoexcited populations at the surface. The experimental results can be reproduced by numerical solutions of optical Bloch equations. The theoretical analysis allows one to investigate which dephasing times and relaxation processes are compatible with experiment. Furthermore, it is outlined how one can describe optical nonlinearities at surfaces using a microscopic theory within the framework of semiconductor Bloch equations."}],"status":"public","publication":"Journal of Physics: Condensed Matter","type":"journal_article","title":"Femtosecond time-resolved five-wave mixing at silicon surfaces","doi":"10.1088/0953-8984/17/8/003","date_updated":"2023-04-24T06:14:11Z","volume":17,"date_created":"2021-08-24T09:21:43Z","author":[{"first_name":"Torsten","orcid":"0000-0001-8864-2072","last_name":"Meier","full_name":"Meier, Torsten","id":"344"},{"full_name":"Reichelt, Matthias","id":"138","last_name":"Reichelt","first_name":"Matthias"},{"first_name":"S W","last_name":"Koch","full_name":"Koch, S W"},{"first_name":"U","full_name":"Höfer, U","last_name":"Höfer"}],"year":"2005","page":"S221-S244","intvolume":"        17","citation":{"ama":"Meier T, Reichelt M, Koch SW, Höfer U. 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Höfer, “Femtosecond time-resolved five-wave mixing at silicon surfaces,” <i>Journal of Physics: Condensed Matter</i>, vol. 17, no. 8, pp. S221–S244, 2005, doi: <a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">10.1088/0953-8984/17/8/003</a>.","bibtex":"@article{Meier_Reichelt_Koch_Höfer_2005, title={Femtosecond time-resolved five-wave mixing at silicon surfaces}, volume={17}, DOI={<a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">10.1088/0953-8984/17/8/003</a>}, number={8}, journal={Journal of Physics: Condensed Matter}, author={Meier, Torsten and Reichelt, Matthias and Koch, S W and Höfer, U}, year={2005}, pages={S221–S244} }","mla":"Meier, Torsten, et al. “Femtosecond Time-Resolved Five-Wave Mixing at Silicon Surfaces.” <i>Journal of Physics: Condensed Matter</i>, vol. 17, no. 8, 2005, pp. S221–44, doi:<a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">10.1088/0953-8984/17/8/003</a>.","short":"T. Meier, M. Reichelt, S.W. Koch, U. 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Femtosecond time-resolved five-wave mixing at silicon surfaces. <i>Journal of Physics: Condensed Matter</i>, <i>17</i>(8), S221–S244. <a href=\"https://doi.org/10.1088/0953-8984/17/8/003\">https://doi.org/10.1088/0953-8984/17/8/003</a>"},"publication_identifier":{"issn":["0953-8984","1361-648X"]},"publication_status":"published","issue":"8"},{"year":"2005","citation":{"bibtex":"@inproceedings{Meier_Reichelt_Pasenow_Stroucken_Koch_2005, series={Verhandlungen der Deutschen Physikalischen Gesellschaft}, title={Optical properties of semiconductor photonic-crystal structures: spatially-inhomogeneous excitonic resonances and optical gain}, volume={40}, booktitle={2005 annual conference of the German Physical Society (DPG) during the World year of physics}, author={Meier, Torsten and Reichelt, Matthias and Pasenow, B. and Stroucken, T. and Koch, S.W.}, year={2005}, collection={Verhandlungen der Deutschen Physikalischen Gesellschaft} }","mla":"Meier, Torsten, et al. “Optical Properties of Semiconductor Photonic-Crystal Structures: Spatially-Inhomogeneous Excitonic Resonances and Optical Gain.” <i>2005 Annual Conference of the German Physical Society (DPG) during the World Year of Physics</i>, vol. 40, 2005.","short":"T. Meier, M. Reichelt, B. Pasenow, T. Stroucken, S.W. Koch, in: 2005 Annual Conference of the German Physical Society (DPG) during the World Year of Physics, 2005.","apa":"Meier, T., Reichelt, M., Pasenow, B., Stroucken, T., &#38; Koch, S. W. (2005). Optical properties of semiconductor photonic-crystal structures: spatially-inhomogeneous excitonic resonances and optical gain. <i>2005 Annual Conference of the German Physical Society (DPG) during the World Year of Physics</i>, <i>40</i>.","ama":"Meier T, Reichelt M, Pasenow B, Stroucken T, Koch SW. Optical properties of semiconductor photonic-crystal structures: spatially-inhomogeneous excitonic resonances and optical gain. In: <i>2005 Annual Conference of the German Physical Society (DPG) during the World Year of Physics</i>. Vol 40. Verhandlungen der Deutschen Physikalischen Gesellschaft. ; 2005.","chicago":"Meier, Torsten, Matthias Reichelt, B. Pasenow, T. Stroucken, and S.W. Koch. “Optical Properties of Semiconductor Photonic-Crystal Structures: Spatially-Inhomogeneous Excitonic Resonances and Optical Gain.” In <i>2005 Annual Conference of the German Physical Society (DPG) during the World Year of Physics</i>, Vol. 40. Verhandlungen Der Deutschen Physikalischen Gesellschaft, 2005.","ieee":"T. Meier, M. Reichelt, B. Pasenow, T. Stroucken, and S. W. Koch, “Optical properties of semiconductor photonic-crystal structures: spatially-inhomogeneous excitonic resonances and optical gain,” in <i>2005 annual conference of the German Physical Society (DPG) during the World year of physics</i>, Berlin, Germany, 2005, vol. 40."},"intvolume":"        40","publication_status":"published","title":"Optical properties of semiconductor photonic-crystal structures: spatially-inhomogeneous excitonic resonances and optical gain","main_file_link":[{"url":"https://www.dpg-verhandlungen.de/year/2005/conference/berlin/part/hl/session/37/contribution/2"}],"conference":{"location":"Berlin, Germany","end_date":"2005-03-09","start_date":"2005-03-04","name":"2005 annual conference of the German Physical Society (DPG) during the World year of physics"},"date_updated":"2023-05-01T13:25:46Z","date_created":"2023-05-01T13:25:43Z","author":[{"orcid":"0000-0001-8864-2072","last_name":"Meier","id":"344","full_name":"Meier, Torsten","first_name":"Torsten"},{"first_name":"Matthias","id":"138","full_name":"Reichelt, Matthias","last_name":"Reichelt"},{"full_name":"Pasenow, B.","last_name":"Pasenow","first_name":"B."},{"first_name":"T.","last_name":"Stroucken","full_name":"Stroucken, T."},{"first_name":"S.W.","last_name":"Koch","full_name":"Koch, S.W."}],"volume":40,"status":"public","type":"conference","publication":"2005 annual conference of the German Physical Society (DPG) during the World year of physics","language":[{"iso":"eng"}],"extern":"1","_id":"44297","series_title":"Verhandlungen der Deutschen Physikalischen Gesellschaft","user_id":"49063","department":[{"_id":"293"}]},{"author":[{"last_name":"Thiel","full_name":"Thiel, Ansgar","first_name":"Ansgar"},{"first_name":"Hilke","full_name":"Teubert, Hilke","id":"41891","last_name":"Teubert"},{"last_name":"Cachay","full_name":"Cachay, Klaus","first_name":"Klaus"}],"date_created":"2024-10-09T11:36:12Z","publisher":"Czwalina","date_updated":"2024-10-09T11:54:43Z","title":"Verbundsysteme in der Nachwuchsförderung – Effiziente Kopplung von Spitzensport und Schule als Abstimmungs- und Akzeptanzprobleme","page":"195-210","citation":{"chicago":"Thiel, Ansgar, Hilke Teubert, and Klaus Cachay. “Verbundsysteme in Der Nachwuchsförderung – Effiziente Kopplung von Spitzensport Und Schule Als Abstimmungs- Und Akzeptanzprobleme.” In <i>Fußball in Geschichte Und Gesellschaft</i>, edited by Michael Krüger and Bernd Schulze, 195–210. Czwalina, 2005.","ieee":"A. Thiel, H. Teubert, and K. Cachay, “Verbundsysteme in der Nachwuchsförderung – Effiziente Kopplung von Spitzensport und Schule als Abstimmungs- und Akzeptanzprobleme,” in <i>Fußball in Geschichte und Gesellschaft</i>, M. Krüger and B. Schulze, Eds. Czwalina, 2005, pp. 195–210.","ama":"Thiel A, Teubert H, Cachay K. Verbundsysteme in der Nachwuchsförderung – Effiziente Kopplung von Spitzensport und Schule als Abstimmungs- und Akzeptanzprobleme. In: Krüger M, Schulze B, eds. <i>Fußball in Geschichte Und Gesellschaft</i>. Czwalina; 2005:195-210.","apa":"Thiel, A., Teubert, H., &#38; Cachay, K. (2005). Verbundsysteme in der Nachwuchsförderung – Effiziente Kopplung von Spitzensport und Schule als Abstimmungs- und Akzeptanzprobleme. In M. Krüger &#38; B. Schulze (Eds.), <i>Fußball in Geschichte und Gesellschaft</i> (pp. 195–210). 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Spitzensport als Schulprofil? <i>Sportunterricht</i>. 2005;54:297-302.","chicago":"Borggrefe, Carmen, Hilke Teubert, Klaus Cachay, and Ansgar Thiel. “Spitzensport Als Schulprofil?” <i>Sportunterricht</i> 54 (2005): 297–302.","ieee":"C. Borggrefe, H. Teubert, K. Cachay, and A. Thiel, “Spitzensport als Schulprofil?,” <i>Sportunterricht</i>, vol. 54, pp. 297–302, 2005.","apa":"Borggrefe, C., Teubert, H., Cachay, K., &#38; Thiel, A. (2005). Spitzensport als Schulprofil? <i>Sportunterricht</i>, <i>54</i>, 297–302.","mla":"Borggrefe, Carmen, et al. “Spitzensport Als Schulprofil?” <i>Sportunterricht</i>, vol. 54, 2005, pp. 297–302.","bibtex":"@article{Borggrefe_Teubert_Cachay_Thiel_2005, title={Spitzensport als Schulprofil?}, volume={54}, journal={Sportunterricht}, author={Borggrefe, Carmen and Teubert, Hilke and Cachay, Klaus and Thiel, Ansgar}, year={2005}, pages={297–302} }","short":"C. Borggrefe, H. Teubert, K. Cachay, A. Thiel, Sportunterricht 54 (2005) 297–302."},"intvolume":"        54","page":"297-302","year":"2005","title":"Spitzensport als Schulprofil?","date_created":"2024-10-09T11:39:35Z","author":[{"full_name":"Borggrefe, Carmen","last_name":"Borggrefe","first_name":"Carmen"},{"last_name":"Teubert","id":"41891","full_name":"Teubert, Hilke","first_name":"Hilke"},{"first_name":"Klaus","last_name":"Cachay","full_name":"Cachay, Klaus"},{"first_name":"Ansgar","full_name":"Thiel, Ansgar","last_name":"Thiel"}],"volume":54,"date_updated":"2024-10-09T11:54:11Z","status":"public","type":"journal_article","publication":"Sportunterricht","language":[{"iso":"eng"}],"user_id":"41891","department":[{"_id":"174"},{"_id":"320"}],"_id":"56463"},{"type":"book_chapter","publication":"Qualität im Schulsport","status":"public","editor":[{"last_name":"Gogoll","full_name":"Gogoll, André","first_name":"André"},{"first_name":"Andrea","full_name":"Menze-Sonneck, Andrea","last_name":"Menze-Sonneck"}],"user_id":"41891","department":[{"_id":"174"},{"_id":"320"}],"_id":"56465","language":[{"iso":"eng"}],"citation":{"apa":"Teubert, H., Thiel, A., &#38; Kleindienst-Cachay, C. (2005). Die „Bewegte Schule“ auf dem Prüfstand – Qualitätsmerkmale einer grundschulpädagogischen Innovation. In A. Gogoll &#38; A. Menze-Sonneck (Eds.), <i>Qualität im Schulsport</i> (pp. 148–153). Czwalina.","bibtex":"@inbook{Teubert_Thiel_Kleindienst-Cachay_2005, title={Die „Bewegte Schule“ auf dem Prüfstand – Qualitätsmerkmale einer grundschulpädagogischen Innovation.}, booktitle={Qualität im Schulsport}, publisher={Czwalina}, author={Teubert, Hilke and Thiel, Ansgar and Kleindienst-Cachay, Christa}, editor={Gogoll, André and Menze-Sonneck, Andrea}, year={2005}, pages={148–153} }","short":"H. Teubert, A. Thiel, C. Kleindienst-Cachay, in: A. Gogoll, A. 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Linking Top Sports and Schools to Foster the Next Generation of Athletes in Competitive Sports – Considerations on the Example of the Integrated Systems. <i>European Journal for Sport and Society</i>. 2005;2(2):121-138.","chicago":"Thiel, Ansgar, Hilke Teubert, and Klaus Cachay. “Linking Top Sports and Schools to Foster the Next Generation of Athletes in Competitive Sports – Considerations on the Example of the Integrated Systems.” <i>European Journal for Sport and Society</i> 2, no. 2 (2005): 121–38.","ieee":"A. Thiel, H. Teubert, and K. Cachay, “Linking Top Sports and Schools to Foster the Next Generation of Athletes in Competitive Sports – Considerations on the Example of the Integrated Systems,” <i>European Journal for Sport and Society</i>, vol. 2, no. 2, pp. 121–138, 2005.","apa":"Thiel, A., Teubert, H., &#38; Cachay, K. (2005). Linking Top Sports and Schools to Foster the Next Generation of Athletes in Competitive Sports – Considerations on the Example of the Integrated Systems. <i>European Journal for Sport and Society</i>, <i>2</i>(2), 121–138.","short":"A. Thiel, H. Teubert, K. Cachay, European Journal for Sport and Society 2 (2005) 121–138.","bibtex":"@article{Thiel_Teubert_Cachay_2005, title={Linking Top Sports and Schools to Foster the Next Generation of Athletes in Competitive Sports – Considerations on the Example of the Integrated Systems}, volume={2}, number={2}, journal={European Journal for Sport and Society}, author={Thiel, Ansgar and Teubert, Hilke and Cachay, Klaus}, year={2005}, pages={121–138} }","mla":"Thiel, Ansgar, et al. “Linking Top Sports and Schools to Foster the Next Generation of Athletes in Competitive Sports – Considerations on the Example of the Integrated Systems.” <i>European Journal for Sport and Society</i>, vol. 2, no. 2, 2005, pp. 121–38."},"issue":"2"},{"_id":"56473","user_id":"41891","department":[{"_id":"174"},{"_id":"320"}],"language":[{"iso":"ger"}],"type":"book_chapter","publication":"Spitzensport im Jahr der olympischen Sommerspiele 2004 – Strukturen und Wissen","editor":[{"first_name":"J","last_name":"Mester","full_name":"Mester, J"},{"full_name":"Knuth, S","last_name":"Knuth","first_name":"S"}],"status":"public","publisher":"Meyer & Meyer","date_updated":"2024-11-05T07:46:34Z","date_created":"2024-10-09T12:30:19Z","author":[{"first_name":"Hilke","last_name":"Teubert","id":"41891","full_name":"Teubert, Hilke"},{"last_name":"Thiel","full_name":"Thiel, Ansgar","first_name":"Ansgar"},{"last_name":"Halle","full_name":"Halle, Arne","first_name":"Arne"},{"first_name":"Klaus","full_name":"Cachay, Klaus","last_name":"Cachay"}],"title":"Abstimmung und Akzeptanz der Verbindung von Schule und Leistungssport – Zu den Basisvoraussetzungen effizienter Verbundsysteme","year":"2005","citation":{"apa":"Teubert, H., Thiel, A., Halle, A., &#38; Cachay, K. (2005). Abstimmung und Akzeptanz der Verbindung von Schule und Leistungssport – Zu den Basisvoraussetzungen effizienter Verbundsysteme. In J. Mester &#38; S. Knuth (Eds.), <i>Spitzensport im Jahr der olympischen Sommerspiele 2004 – Strukturen und Wissen</i> (pp. 120–153). Meyer &#38; Meyer.","short":"H. Teubert, A. Thiel, A. Halle, K. Cachay, in: J. Mester, S. Knuth (Eds.), Spitzensport im Jahr der olympischen Sommerspiele 2004 – Strukturen und Wissen, Meyer &#38; Meyer, 2005, pp. 120–153.","mla":"Teubert, Hilke, et al. “Abstimmung und Akzeptanz der Verbindung von Schule und Leistungssport – Zu den Basisvoraussetzungen effizienter Verbundsysteme.” <i>Spitzensport im Jahr der olympischen Sommerspiele 2004 – Strukturen und Wissen</i>, edited by J Mester and S Knuth, Meyer &#38; Meyer, 2005, pp. 120–53.","bibtex":"@inbook{Teubert_Thiel_Halle_Cachay_2005, title={Abstimmung und Akzeptanz der Verbindung von Schule und Leistungssport – Zu den Basisvoraussetzungen effizienter Verbundsysteme}, booktitle={Spitzensport im Jahr der olympischen Sommerspiele 2004 – Strukturen und Wissen}, publisher={Meyer &#38; Meyer}, author={Teubert, Hilke and Thiel, Ansgar and Halle, Arne and Cachay, Klaus}, editor={Mester, J and Knuth, S}, year={2005}, pages={120–153} }","ieee":"H. Teubert, A. Thiel, A. Halle, and K. Cachay, “Abstimmung und Akzeptanz der Verbindung von Schule und Leistungssport – Zu den Basisvoraussetzungen effizienter Verbundsysteme,” in <i>Spitzensport im Jahr der olympischen Sommerspiele 2004 – Strukturen und Wissen</i>, J. Mester and S. Knuth, Eds. Meyer &#38; Meyer, 2005, pp. 120–153.","chicago":"Teubert, Hilke, Ansgar Thiel, Arne Halle, and Klaus Cachay. “Abstimmung und Akzeptanz der Verbindung von Schule und Leistungssport – Zu den Basisvoraussetzungen effizienter Verbundsysteme.” In <i>Spitzensport im Jahr der olympischen Sommerspiele 2004 – Strukturen und Wissen</i>, edited by J Mester and S Knuth, 120–53. Meyer &#38; Meyer, 2005.","ama":"Teubert H, Thiel A, Halle A, Cachay K. Abstimmung und Akzeptanz der Verbindung von Schule und Leistungssport – Zu den Basisvoraussetzungen effizienter Verbundsysteme. In: Mester J, Knuth S, eds. <i>Spitzensport im Jahr der olympischen Sommerspiele 2004 – Strukturen und Wissen</i>. Meyer &#38; Meyer; 2005:120-153."},"page":"120-153"},{"issue":"22","publication_identifier":{"issn":["1434-193X","1099-0690"]},"publication_status":"published","intvolume":"      2005","page":"4879-4890","citation":{"ama":"Herres‐Pawlis S, Neuba A, Seewald O, et al. A Library of Peralkylated Bis‐guanidine Ligands for Use in Biomimetic Coordination Chemistry. <i>European Journal of Organic Chemistry</i>. 2005;2005(22):4879-4890. doi:<a href=\"https://doi.org/10.1002/ejoc.200500340\">10.1002/ejoc.200500340</a>","ieee":"S. Herres‐Pawlis <i>et al.</i>, “A Library of Peralkylated Bis‐guanidine Ligands for Use in Biomimetic Coordination Chemistry,” <i>European Journal of Organic Chemistry</i>, vol. 2005, no. 22, pp. 4879–4890, 2005, doi: <a href=\"https://doi.org/10.1002/ejoc.200500340\">10.1002/ejoc.200500340</a>.","chicago":"Herres‐Pawlis, Sonja, Adam Neuba, Oliver Seewald, Tarimala Seshadri, Hans Egold, Ulrich Flörke, and Gerald Henkel. “A Library of Peralkylated Bis‐guanidine Ligands for Use in Biomimetic Coordination Chemistry.” <i>European Journal of Organic Chemistry</i> 2005, no. 22 (2005): 4879–90. <a href=\"https://doi.org/10.1002/ejoc.200500340\">https://doi.org/10.1002/ejoc.200500340</a>.","apa":"Herres‐Pawlis, S., Neuba, A., Seewald, O., Seshadri, T., Egold, H., Flörke, U., &#38; Henkel, G. (2005). A Library of Peralkylated Bis‐guanidine Ligands for Use in Biomimetic Coordination Chemistry. <i>European Journal of Organic Chemistry</i>, <i>2005</i>(22), 4879–4890. <a href=\"https://doi.org/10.1002/ejoc.200500340\">https://doi.org/10.1002/ejoc.200500340</a>","short":"S. Herres‐Pawlis, A. Neuba, O. Seewald, T. Seshadri, H. Egold, U. Flörke, G. Henkel, European Journal of Organic Chemistry 2005 (2005) 4879–4890.","mla":"Herres‐Pawlis, Sonja, et al. “A Library of Peralkylated Bis‐guanidine Ligands for Use in Biomimetic Coordination Chemistry.” <i>European Journal of Organic Chemistry</i>, vol. 2005, no. 22, Wiley, 2005, pp. 4879–90, doi:<a href=\"https://doi.org/10.1002/ejoc.200500340\">10.1002/ejoc.200500340</a>.","bibtex":"@article{Herres‐Pawlis_Neuba_Seewald_Seshadri_Egold_Flörke_Henkel_2005, title={A Library of Peralkylated Bis‐guanidine Ligands for Use in Biomimetic Coordination Chemistry}, volume={2005}, DOI={<a href=\"https://doi.org/10.1002/ejoc.200500340\">10.1002/ejoc.200500340</a>}, number={22}, journal={European Journal of Organic Chemistry}, publisher={Wiley}, author={Herres‐Pawlis, Sonja and Neuba, Adam and Seewald, Oliver and Seshadri, Tarimala and Egold, Hans and Flörke, Ulrich and Henkel, Gerald}, year={2005}, pages={4879–4890} }"},"year":"2005","volume":2005,"author":[{"first_name":"Sonja","full_name":"Herres‐Pawlis, Sonja","last_name":"Herres‐Pawlis"},{"full_name":"Neuba, Adam","last_name":"Neuba","first_name":"Adam"},{"first_name":"Oliver","last_name":"Seewald","full_name":"Seewald, Oliver","id":"495"},{"last_name":"Seshadri","full_name":"Seshadri, Tarimala","first_name":"Tarimala"},{"full_name":"Egold, Hans","last_name":"Egold","first_name":"Hans"},{"first_name":"Ulrich","last_name":"Flörke","full_name":"Flörke, Ulrich"},{"last_name":"Henkel","full_name":"Henkel, Gerald","first_name":"Gerald"}],"date_created":"2025-02-12T09:27:00Z","publisher":"Wiley","date_updated":"2025-02-12T09:30:43Z","doi":"10.1002/ejoc.200500340","title":"A Library of Peralkylated Bis‐guanidine Ligands for Use in Biomimetic Coordination Chemistry","publication":"European Journal of Organic Chemistry","type":"journal_article","status":"public","abstract":[{"text":"<jats:title>Abstract</jats:title><jats:p>A series of bis‐guanidine ligands designed for use in biomimetic coordination chemistry has been extended to a library matrix combining unprecedented substitutional flexibility within the guanidyl residues with a wide range of aliphatic and aromatic spacers connecting these functionalities. The underlying protocol can be used with predefined ureas as well as secondary amines to build up these units by reaction with phosgene if the ureas are otherwise unavailable. In the latter case, the resulting urea intermediates do not have to be isolated as the reaction proceeds further with additional phosgene to yield a chloroformamidinium chloride which is transformed into the bis‐guanidine functionality by subsequent reaction with a suitable primary diamine in the presence of triethylamine as an auxiliary base. This concept has been used to synthesise and characterise more then two dozen different bis‐guanidines based on 12 discrete monoguanidine units and seven different spacers. These spacers have been chosen such that the most important phenotypes have been dealt with and which range from rigid to more flexible scaffolds. In addition to spacers with no metal‐binding capabilities, other species containing further donor functions such as <jats:italic>N</jats:italic>‐methyldiphenyleneamine or pyridine‐2,6‐diyl have also been used. The substitution patterns of the guanidine residues can be classified into acyclic and cyclic types. Among the cyclic types, one subset is characterised by five‐ or six‐membered heterocycles containing both the amino nitrogen atoms and another one by individual N‐heterocyclic systems for each amino nitrogen. Structurally characterised examples are 2‐{2‐[2‐(tetramethylguanidi­no)ethoxy]ethoxy}‐1‐(tetramethylguanidino)ethane (TMG<jats:sub>2</jats:sub>doo) in its diprotonated form and 2,2′‐bis[2<jats:italic>N</jats:italic>‐(1,1′,3,3′‐tetramethylguanidine)]diphenyleneamine (TMG<jats:sub>2</jats:sub>PA) as wellas <jats:italic>N</jats:italic><jats:sup>1</jats:sup>,<jats:italic>N</jats:italic><jats:sup>3</jats:sup>‐bis(dimorpholinomethylene)propane‐1,3‐diamine (DMorphG<jats:sub>2</jats:sub>p) as free bases. For the permethylated bis‐guanidine derivatives, the barrier to rotation around the (C=N)<jats:sub>guanidine</jats:sub> bond has been determined by means of temperature‐dependent EXSY <jats:sup>1</jats:sup>H NMR spectroscopy to range between 54 and 79 kJ mol<jats:sup>–1</jats:sup> depending on the type of spacer. (© Wiley‐VCH Verlag GmbH &amp; Co. KGaA, 69451 Weinheim, Germany, 2005)</jats:p>","lang":"eng"}],"department":[{"_id":"321"},{"_id":"35"},{"_id":"301"}],"user_id":"495","_id":"58598","language":[{"iso":"eng"}]},{"language":[{"iso":"eng"}],"publication":"Zeitschrift für anorganische und allgemeine Chemie","abstract":[{"text":"<jats:title>Abstract</jats:title><jats:p><jats:bold>Syntheses and Structure of Chiral Metallatetrahedron Complexes of the Type [Re<jats:sub>2</jats:sub>(M<jats:sup>1</jats:sup>PPh<jats:sub>3</jats:sub>)(M<jats:sup>2</jats:sup>PPh<jats:sub>3</jats:sub>)(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>C≡CPh] (M<jats:sup>1</jats:sup> = Ag, Au; M<jats:sup>2</jats:sup> = Cu, Ag, Au)</jats:bold></jats:p><jats:p>From the reaction of Li[Re<jats:sub>2</jats:sub>(μ‐H)(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>(C(Ph)O)] (<jats:bold>1</jats:bold>) with Ph<jats:sub>3</jats:sub>AuC≡CPh both benzaldehyde and the trinuclear complex Li[Re<jats:sub>2</jats:sub>(AuPPh<jats:sub>3</jats:sub>)(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>C≡CPh] (<jats:bold>2a</jats:bold>) were obtained in high yield. The complex anion was isolated as its PPh<jats:sub>4</jats:sub>‐salt <jats:bold>2b</jats:bold>. The latter reacts with coinage metal complexes PPh<jats:sub>3</jats:sub>M<jats:sup>2</jats:sup>Cl [M<jats:sup>2</jats:sup> = Cu, Ag, Au] to give chiral heterometallatetrahedranes of the general formula [Re<jats:sub>2</jats:sub>(AuPPh<jats:sub>3</jats:sub>)(M<jats:sup>2</jats:sup>PPh<jats:sub>3</jats:sub>)(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>C≡CPh] (M<jats:sup>2</jats:sup> = Cu <jats:bold>3a</jats:bold>, Ag <jats:bold>3b</jats:bold>, Au <jats:bold>3c</jats:bold>). The corresponding complex [Re<jats:sub>2</jats:sub>(AgPPh<jats:sub>3</jats:sub>)<jats:sub>2</jats:sub>(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>C≡CPh] (<jats:bold>3d</jats:bold>) is obtained from the reaction of [Re<jats:sub>2</jats:sub>(AgPPh<jats:sub>3</jats:sub>)<jats:sub>2</jats:sub>(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>Cl] (<jats:bold>4</jats:bold>) with LiC≡CPh. <jats:bold>3d</jats:bold> undergoes a metathesis reaction in the presence of PPh<jats:sub>3</jats:sub>CuCl giving [Re<jats:sub>2</jats:sub>(AgPPh<jats:sub>3</jats:sub>)(CuPPh<jats:sub>3</jats:sub>)(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>C≡CPh] (<jats:bold>3e</jats:bold>) and PPh<jats:sub>3</jats:sub>AgCl. Analogous metathesis reactions are observed when <jats:bold>3c</jats:bold> is reacted with PPh<jats:sub>3</jats:sub>AgCl or PPh<jats:sub>3</jats:sub>CuCl giving <jats:bold>3a</jats:bold> or <jats:bold>3b</jats:bold>, respectively. The reaction of <jats:bold>1</jats:bold> with PPh<jats:sub>3</jats:sub>AuCl gives benzaldehyde and Li[Re<jats:sub>2</jats:sub>(AuPPh<jats:sub>3</jats:sub>)(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>Cl] (<jats:bold>5a</jats:bold>) which upon reaction with PhLi forms the trinuclear complex Li[Re<jats:sub>2</jats:sub>(AuPPh<jats:sub>3</jats:sub>)(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>Ph] (<jats:bold>6a</jats:bold>). Again this complex was isolated as its PPh<jats:sub>4</jats:sub>‐salt <jats:bold>6b</jats:bold>. In contrast to <jats:bold>2b</jats:bold>, <jats:bold>6b</jats:bold> reacts with one equivalent of Ph<jats:sub>3</jats:sub>PAuCl by transmetalation to give Ph<jats:sub>3</jats:sub>PAuPh and PPh<jats:sub>4</jats:sub>[Re<jats:sub>2</jats:sub>(AuPPh<jats:sub>3</jats:sub>)(μ‐PCy<jats:sub>2</jats:sub>)(CO)<jats:sub>7</jats:sub>Cl] (<jats:bold>5b</jats:bold>). The X‐ray structures of the compounds <jats:bold>3a</jats:bold>, <jats:bold>3b</jats:bold>, <jats:bold>3e</jats:bold> and <jats:bold>4</jats:bold> are reported.</jats:p>","lang":"eng"}],"date_created":"2025-02-12T09:26:12Z","publisher":"Wiley","title":"Synthese und Struktur chiraler Heterometallatetrahedrane des Typs [Re<sub>2</sub>(M<sup>1</sup>PPh<sub>3</sub>)(M<sup>2</sup>PPh<sub>3</sub>)(μ‐PCy<sub>2</sub>)(CO)<sub>7</sub>C≡CPh] (M<sup>1</sup> = Ag, Au; M<sup>2</sup> = Cu, Ag, Au)","issue":"2","year":"2005","department":[{"_id":"321"},{"_id":"35"},{"_id":"301"}],"user_id":"495","_id":"58597","type":"journal_article","status":"public","volume":632,"author":[{"last_name":"Seewald","id":"495","full_name":"Seewald, Oliver","first_name":"Oliver"},{"first_name":"Ulrich","last_name":"Flörke","full_name":"Flörke, Ulrich"},{"first_name":"Hans","full_name":"Egold, Hans","last_name":"Egold"},{"first_name":"Hans‐Jürgen","full_name":"Haupt, Hans‐Jürgen","last_name":"Haupt"},{"full_name":"Schwefer, Meinhard","last_name":"Schwefer","first_name":"Meinhard"}],"date_updated":"2025-02-12T09:30:52Z","doi":"10.1002/zaac.200500340","publication_identifier":{"issn":["0044-2313","1521-3749"]},"publication_status":"published","intvolume":"       632","page":"204-210","citation":{"mla":"Seewald, Oliver, et al. “Synthese Und Struktur Chiraler Heterometallatetrahedrane Des Typs [Re<sub>2</sub>(M<sup>1</sup>PPh<sub>3</sub>)(M<sup>2</sup>PPh<sub>3</sub>)(Μ‐PCy<sub>2</sub>)(CO)<sub>7</sub>C≡CPh] (M<sup>1</sup> = Ag, Au; M<sup>2</sup> = Cu, Ag, Au).” <i>Zeitschrift Für Anorganische Und Allgemeine Chemie</i>, vol. 632, no. 2, Wiley, 2005, pp. 204–10, doi:<a href=\"https://doi.org/10.1002/zaac.200500340\">10.1002/zaac.200500340</a>.","short":"O. Seewald, U. Flörke, H. Egold, H. Haupt, M. Schwefer, Zeitschrift Für Anorganische Und Allgemeine Chemie 632 (2005) 204–210.","bibtex":"@article{Seewald_Flörke_Egold_Haupt_Schwefer_2005, title={Synthese und Struktur chiraler Heterometallatetrahedrane des Typs [Re<sub>2</sub>(M<sup>1</sup>PPh<sub>3</sub>)(M<sup>2</sup>PPh<sub>3</sub>)(μ‐PCy<sub>2</sub>)(CO)<sub>7</sub>C≡CPh] (M<sup>1</sup> = Ag, Au; M<sup>2</sup> = Cu, Ag, Au)}, volume={632}, DOI={<a href=\"https://doi.org/10.1002/zaac.200500340\">10.1002/zaac.200500340</a>}, number={2}, journal={Zeitschrift für anorganische und allgemeine Chemie}, publisher={Wiley}, author={Seewald, Oliver and Flörke, Ulrich and Egold, Hans and Haupt, Hans‐Jürgen and Schwefer, Meinhard}, year={2005}, pages={204–210} }","apa":"Seewald, O., Flörke, U., Egold, H., Haupt, H., &#38; Schwefer, M. (2005). Synthese und Struktur chiraler Heterometallatetrahedrane des Typs [Re<sub>2</sub>(M<sup>1</sup>PPh<sub>3</sub>)(M<sup>2</sup>PPh<sub>3</sub>)(μ‐PCy<sub>2</sub>)(CO)<sub>7</sub>C≡CPh] (M<sup>1</sup> = Ag, Au; M<sup>2</sup> = Cu, Ag, Au). <i>Zeitschrift Für Anorganische Und Allgemeine Chemie</i>, <i>632</i>(2), 204–210. <a href=\"https://doi.org/10.1002/zaac.200500340\">https://doi.org/10.1002/zaac.200500340</a>","chicago":"Seewald, Oliver, Ulrich Flörke, Hans Egold, Hans‐Jürgen Haupt, and Meinhard Schwefer. “Synthese Und Struktur Chiraler Heterometallatetrahedrane Des Typs [Re<sub>2</sub>(M<sup>1</sup>PPh<sub>3</sub>)(M<sup>2</sup>PPh<sub>3</sub>)(Μ‐PCy<sub>2</sub>)(CO)<sub>7</sub>C≡CPh] (M<sup>1</sup> = Ag, Au; M<sup>2</sup> = Cu, Ag, Au).” <i>Zeitschrift Für Anorganische Und Allgemeine Chemie</i> 632, no. 2 (2005): 204–10. <a href=\"https://doi.org/10.1002/zaac.200500340\">https://doi.org/10.1002/zaac.200500340</a>.","ieee":"O. Seewald, U. Flörke, H. Egold, H. Haupt, and M. Schwefer, “Synthese und Struktur chiraler Heterometallatetrahedrane des Typs [Re<sub>2</sub>(M<sup>1</sup>PPh<sub>3</sub>)(M<sup>2</sup>PPh<sub>3</sub>)(μ‐PCy<sub>2</sub>)(CO)<sub>7</sub>C≡CPh] (M<sup>1</sup> = Ag, Au; M<sup>2</sup> = Cu, Ag, Au),” <i>Zeitschrift für anorganische und allgemeine Chemie</i>, vol. 632, no. 2, pp. 204–210, 2005, doi: <a href=\"https://doi.org/10.1002/zaac.200500340\">10.1002/zaac.200500340</a>.","ama":"Seewald O, Flörke U, Egold H, Haupt H, Schwefer M. Synthese und Struktur chiraler Heterometallatetrahedrane des Typs [Re<sub>2</sub>(M<sup>1</sup>PPh<sub>3</sub>)(M<sup>2</sup>PPh<sub>3</sub>)(μ‐PCy<sub>2</sub>)(CO)<sub>7</sub>C≡CPh] (M<sup>1</sup> = Ag, Au; M<sup>2</sup> = Cu, Ag, Au). <i>Zeitschrift für anorganische und allgemeine Chemie</i>. 2005;632(2):204-210. doi:<a href=\"https://doi.org/10.1002/zaac.200500340\">10.1002/zaac.200500340</a>"}},{"editor":[{"last_name":"Bräu","full_name":"Bräu, Karin","first_name":"Karin"},{"last_name":"Schwerdt","full_name":"Schwerdt, Ulrich","first_name":"Ulrich"}],"status":"public","type":"book_chapter","publication":"Heterogenität als Chance. Vom produktiven Umgang mit Gleichheit und Differenz in der Schule","language":[{"iso":"ger"}],"_id":"36078","user_id":"459","department":[{"_id":"35"},{"_id":"17"},{"_id":"22"},{"_id":"396"}],"year":"2005","place":"Münster","citation":{"ieee":"K. Schlegel-Matthies, “Fachdidaktische Perspektiven auf den Umgang mit Heterogenität im haushaltsbezogenen Unterricht,” in <i>Heterogenität als Chance. Vom produktiven Umgang mit Gleichheit und Differenz in der Schule</i>, K. Bräu and U. Schwerdt, Eds. Münster: Lit-Verlag, 2005, pp. 197–217.","chicago":"Schlegel-Matthies, Kirsten. “Fachdidaktische Perspektiven auf den Umgang mit Heterogenität im haushaltsbezogenen Unterricht.” In <i>Heterogenität als Chance. Vom produktiven Umgang mit Gleichheit und Differenz in der Schule</i>, edited by Karin Bräu and Ulrich Schwerdt, 197–217. Münster: Lit-Verlag, 2005.","ama":"Schlegel-Matthies K. Fachdidaktische Perspektiven auf den Umgang mit Heterogenität im haushaltsbezogenen Unterricht. In: Bräu K, Schwerdt U, eds. <i>Heterogenität als Chance. Vom produktiven Umgang mit Gleichheit und Differenz in der Schule</i>. Lit-Verlag; 2005:197–217.","apa":"Schlegel-Matthies, K. (2005). Fachdidaktische Perspektiven auf den Umgang mit Heterogenität im haushaltsbezogenen Unterricht. In K. Bräu &#38; U. Schwerdt (Eds.), <i>Heterogenität als Chance. Vom produktiven Umgang mit Gleichheit und Differenz in der Schule</i> (pp. 197–217). Lit-Verlag.","mla":"Schlegel-Matthies, Kirsten. “Fachdidaktische Perspektiven auf den Umgang mit Heterogenität im haushaltsbezogenen Unterricht.” <i>Heterogenität als Chance. Vom produktiven Umgang mit Gleichheit und Differenz in der Schule</i>, edited by Karin Bräu and Ulrich Schwerdt, Lit-Verlag, 2005, pp. 197–217.","short":"K. Schlegel-Matthies, in: K. Bräu, U. Schwerdt (Eds.), Heterogenität als Chance. Vom produktiven Umgang mit Gleichheit und Differenz in der Schule, Lit-Verlag, Münster, 2005, pp. 197–217.","bibtex":"@inbook{Schlegel-Matthies_2005, place={Münster}, title={Fachdidaktische Perspektiven auf den Umgang mit Heterogenität im haushaltsbezogenen Unterricht}, booktitle={Heterogenität als Chance. 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Bechstedt. “Initial Stage of Si(001) Surface Oxidation from First-Principles Calculations.” <i>The Journal of Physical Chemistry B</i> 109 (2005): 17649–53. <a href=\"https://doi.org/10.1021/jp0501087\">https://doi.org/10.1021/jp0501087</a>."},"publication_identifier":{"issn":["1520-6106","1520-5207"]},"publication_status":"published","title":"Initial Stage of Si(001) Surface Oxidation from First-Principles Calculations","doi":"10.1021/jp0501087","date_updated":"2025-12-05T13:20:42Z","volume":109,"date_created":"2019-10-09T11:41:59Z","author":[{"first_name":"F.","full_name":"Fuchs, F.","last_name":"Fuchs"},{"first_name":"Wolf Gero","orcid":"0000-0002-2717-5076","last_name":"Schmidt","id":"468","full_name":"Schmidt, Wolf Gero"},{"first_name":"F.","full_name":"Bechstedt, F.","last_name":"Bechstedt"}]},{"publication_identifier":{"issn":["0031-9007","1079-7114"]},"publication_status":"published","issue":"18","year":"2005","intvolume":"        95","citation":{"short":"F. Ortmann, W.G. Schmidt, F. Bechstedt, Physical Review Letters 95 (2005).","bibtex":"@article{Ortmann_Schmidt_Bechstedt_2005, title={Attracted by Long-Range Electron Correlation: Adenine on Graphite}, volume={95}, DOI={<a href=\"https://doi.org/10.1103/physrevlett.95.186101\">10.1103/physrevlett.95.186101</a>}, number={18}, journal={Physical Review Letters}, author={Ortmann, F. and Schmidt, Wolf Gero and Bechstedt, F.}, year={2005} }","mla":"Ortmann, F., et al. “Attracted by Long-Range Electron Correlation: Adenine on Graphite.” <i>Physical Review Letters</i>, vol. 95, no. 18, 2005, doi:<a href=\"https://doi.org/10.1103/physrevlett.95.186101\">10.1103/physrevlett.95.186101</a>.","apa":"Ortmann, F., Schmidt, W. G., &#38; Bechstedt, F. (2005). Attracted by Long-Range Electron Correlation: Adenine on Graphite. <i>Physical Review Letters</i>, <i>95</i>(18). <a href=\"https://doi.org/10.1103/physrevlett.95.186101\">https://doi.org/10.1103/physrevlett.95.186101</a>","chicago":"Ortmann, F., Wolf Gero Schmidt, and F. Bechstedt. “Attracted by Long-Range Electron Correlation: Adenine on Graphite.” <i>Physical Review Letters</i> 95, no. 18 (2005). <a href=\"https://doi.org/10.1103/physrevlett.95.186101\">https://doi.org/10.1103/physrevlett.95.186101</a>.","ieee":"F. Ortmann, W. G. Schmidt, and F. Bechstedt, “Attracted by Long-Range Electron Correlation: Adenine on Graphite,” <i>Physical Review Letters</i>, vol. 95, no. 18, 2005, doi: <a href=\"https://doi.org/10.1103/physrevlett.95.186101\">10.1103/physrevlett.95.186101</a>.","ama":"Ortmann F, Schmidt WG, Bechstedt F. Attracted by Long-Range Electron Correlation: Adenine on Graphite. <i>Physical Review Letters</i>. 2005;95(18). doi:<a href=\"https://doi.org/10.1103/physrevlett.95.186101\">10.1103/physrevlett.95.186101</a>"},"date_updated":"2025-12-05T13:20:00Z","volume":95,"date_created":"2019-10-09T11:28:08Z","author":[{"full_name":"Ortmann, F.","last_name":"Ortmann","first_name":"F."},{"first_name":"Wolf Gero","full_name":"Schmidt, Wolf Gero","id":"468","last_name":"Schmidt","orcid":"0000-0002-2717-5076"},{"full_name":"Bechstedt, F.","last_name":"Bechstedt","first_name":"F."}],"title":"Attracted by Long-Range Electron Correlation: Adenine on Graphite","doi":"10.1103/physrevlett.95.186101","publication":"Physical Review Letters","type":"journal_article","status":"public","_id":"13697","department":[{"_id":"15"},{"_id":"170"},{"_id":"295"},{"_id":"35"},{"_id":"230"}],"user_id":"16199","language":[{"iso":"eng"}]}]