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M., &#38; Buhl, H. M. (2024). Elterliche Unterstützung beim Lernen mit digitalen Medien . In S. Aßmann, S. Grafe , &#38; A. Martin (Eds.), <i>Medien - Bildung - Forschung. Integrative und interdisziplinäre Perspektiven</i>. Julius Klinkhardt.","ama":"Kamin A-M, Meister DM, Buhl HM. Elterliche Unterstützung beim Lernen mit digitalen Medien . In: Aßmann S, Grafe  S, Martin A, eds. <i>Medien - Bildung - Forschung. Integrative Und Interdisziplinäre Perspektiven</i>. Julius Klinkhardt; 2024.","short":"A.-M. Kamin, D.M. Meister, H.M. Buhl, in: S. Aßmann, S. Grafe , A. Martin (Eds.), Medien - Bildung - Forschung. Integrative Und Interdisziplinäre Perspektiven, Julius Klinkhardt, Bad Heilbrunn, 2024.","mla":"Kamin, Anna-Maria, et al. “Elterliche Unterstützung Beim Lernen Mit Digitalen Medien .” <i>Medien - Bildung - Forschung. 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While the total number of speakers in a meeting may be known, it is usually not known on a per-segment level. With the proposed speaker counting, joint diarization and source separation can be done segment-by-segment, and the permutation problem across segments is solved, thus allowing for block-online processing in the future. Experimental results on the LibriCSS meeting corpus show that the integrated approach outperforms a cascaded approach of diarization and speech enhancement in terms of WER, both on a per-segment and on a per-meeting level.","lang":"eng"}],"publication":"ICASSP 2025 - 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)","language":[{"iso":"eng"}],"ddc":["000"],"keyword":["diarization","source separation","mixture model","meeting"],"year":"2024","title":"Simultaneous Diarization and Separation of Meetings through the Integration of Statistical Mixture Models","date_created":"2024-11-14T09:32:38Z","status":"public","type":"conference","file_date_updated":"2025-08-14T08:11:57Z","user_id":"44393","department":[{"_id":"54"}],"project":[{"name":"PC2: Computing Resources Provided by the Paderborn Center for Parallel Computing","_id":"52"},{"_id":"508","name":"Automatische Transkription von Gesprächssituationen"}],"_id":"57085","citation":{"apa":"Cord-Landwehr, T., Boeddeker, C., &#38; Haeb-Umbach, R. (2024). Simultaneous Diarization and Separation of Meetings through the Integration of Statistical Mixture Models. <i>ICASSP 2025 - 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)</i>. 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP), Hyderabad, India. <a href=\"https://doi.org/10.1109/ICASSP49660.2025.10888445\">https://doi.org/10.1109/ICASSP49660.2025.10888445</a>","short":"T. Cord-Landwehr, C. Boeddeker, R. Haeb-Umbach, in: ICASSP 2025 - 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP), 2024.","mla":"Cord-Landwehr, Tobias, et al. “Simultaneous Diarization and Separation of Meetings through the Integration of Statistical Mixture Models.” <i>ICASSP 2025 - 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)</i>, 2024, doi:<a href=\"https://doi.org/10.1109/ICASSP49660.2025.10888445\">10.1109/ICASSP49660.2025.10888445</a>.","bibtex":"@inproceedings{Cord-Landwehr_Boeddeker_Haeb-Umbach_2024, title={Simultaneous Diarization and Separation of Meetings through the Integration of Statistical Mixture Models}, DOI={<a href=\"https://doi.org/10.1109/ICASSP49660.2025.10888445\">10.1109/ICASSP49660.2025.10888445</a>}, booktitle={ICASSP 2025 - 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)}, author={Cord-Landwehr, Tobias and Boeddeker, Christoph and Haeb-Umbach, Reinhold}, year={2024} }","ama":"Cord-Landwehr T, Boeddeker C, Haeb-Umbach R. Simultaneous Diarization and Separation of Meetings through the Integration of Statistical Mixture Models. In: <i>ICASSP 2025 - 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)</i>. ; 2024. doi:<a href=\"https://doi.org/10.1109/ICASSP49660.2025.10888445\">10.1109/ICASSP49660.2025.10888445</a>","ieee":"T. Cord-Landwehr, C. Boeddeker, and R. Haeb-Umbach, “Simultaneous Diarization and Separation of Meetings through the Integration of Statistical Mixture Models,” presented at the 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP), Hyderabad, India, 2024, doi: <a href=\"https://doi.org/10.1109/ICASSP49660.2025.10888445\">10.1109/ICASSP49660.2025.10888445</a>.","chicago":"Cord-Landwehr, Tobias, Christoph Boeddeker, and Reinhold Haeb-Umbach. “Simultaneous Diarization and Separation of Meetings through the Integration of Statistical Mixture Models.” In <i>ICASSP 2025 - 2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)</i>, 2024. <a href=\"https://doi.org/10.1109/ICASSP49660.2025.10888445\">https://doi.org/10.1109/ICASSP49660.2025.10888445</a>."},"has_accepted_license":"1","main_file_link":[{"url":"https://arxiv.org/pdf/2410.21455","open_access":"1"}],"conference":{"location":"Hyderabad, India","name":"2025 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)"},"doi":"10.1109/ICASSP49660.2025.10888445","author":[{"first_name":"Tobias","id":"44393","full_name":"Cord-Landwehr, Tobias","last_name":"Cord-Landwehr"},{"first_name":"Christoph","last_name":"Boeddeker","id":"40767","full_name":"Boeddeker, Christoph"},{"first_name":"Reinhold","full_name":"Haeb-Umbach, Reinhold","id":"242","last_name":"Haeb-Umbach"}],"oa":"1","date_updated":"2025-08-14T08:12:22Z"},{"_id":"53659","project":[{"_id":"52","name":"PC2: Computing Resources Provided by the Paderborn Center for Parallel Computing"},{"name":"Automatische Transkription von Gesprächssituationen","_id":"508"}],"department":[{"_id":"54"}],"user_id":"44393","file_date_updated":"2025-08-14T08:09:52Z","type":"conference","status":"public","date_updated":"2025-08-14T08:11:07Z","author":[{"first_name":"Tobias","id":"44393","full_name":"Cord-Landwehr, Tobias","last_name":"Cord-Landwehr"},{"first_name":"Christoph","last_name":"Boeddeker","full_name":"Boeddeker, Christoph","id":"40767"},{"last_name":"Zorilă","full_name":"Zorilă, Cătălin","first_name":"Cătălin"},{"last_name":"Doddipatla","full_name":"Doddipatla, Rama","first_name":"Rama"},{"full_name":"Haeb-Umbach, Reinhold","id":"242","last_name":"Haeb-Umbach","first_name":"Reinhold"}],"doi":"10.1109/icassp48485.2024.10445911","conference":{"location":"Seoul","name":"2024 IEEE International Conference on Acoustics, Speech, and Signal Processing (ICASSP)"},"has_accepted_license":"1","publication_status":"published","citation":{"chicago":"Cord-Landwehr, Tobias, Christoph Boeddeker, Cătălin Zorilă, Rama Doddipatla, and Reinhold Haeb-Umbach. “Geodesic Interpolation of Frame-Wise Speaker Embeddings for the Diarization of Meeting Scenarios.” In <i>ICASSP 2024 - 2024 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)</i>. IEEE, 2024. <a href=\"https://doi.org/10.1109/icassp48485.2024.10445911\">https://doi.org/10.1109/icassp48485.2024.10445911</a>.","ieee":"T. Cord-Landwehr, C. Boeddeker, C. Zorilă, R. Doddipatla, and R. Haeb-Umbach, “Geodesic Interpolation of Frame-Wise Speaker Embeddings for the Diarization of Meeting Scenarios,” presented at the 2024 IEEE International Conference on Acoustics, Speech, and Signal Processing (ICASSP), Seoul, 2024, doi: <a href=\"https://doi.org/10.1109/icassp48485.2024.10445911\">10.1109/icassp48485.2024.10445911</a>.","ama":"Cord-Landwehr T, Boeddeker C, Zorilă C, Doddipatla R, Haeb-Umbach R. Geodesic Interpolation of Frame-Wise Speaker Embeddings for the Diarization of Meeting Scenarios. In: <i>ICASSP 2024 - 2024 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)</i>. IEEE; 2024. doi:<a href=\"https://doi.org/10.1109/icassp48485.2024.10445911\">10.1109/icassp48485.2024.10445911</a>","bibtex":"@inproceedings{Cord-Landwehr_Boeddeker_Zorilă_Doddipatla_Haeb-Umbach_2024, title={Geodesic Interpolation of Frame-Wise Speaker Embeddings for the Diarization of Meeting Scenarios}, DOI={<a href=\"https://doi.org/10.1109/icassp48485.2024.10445911\">10.1109/icassp48485.2024.10445911</a>}, booktitle={ICASSP 2024 - 2024 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)}, publisher={IEEE}, author={Cord-Landwehr, Tobias and Boeddeker, Christoph and Zorilă, Cătălin and Doddipatla, Rama and Haeb-Umbach, Reinhold}, year={2024} }","mla":"Cord-Landwehr, Tobias, et al. “Geodesic Interpolation of Frame-Wise Speaker Embeddings for the Diarization of Meeting Scenarios.” <i>ICASSP 2024 - 2024 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)</i>, IEEE, 2024, doi:<a href=\"https://doi.org/10.1109/icassp48485.2024.10445911\">10.1109/icassp48485.2024.10445911</a>.","short":"T. Cord-Landwehr, C. Boeddeker, C. Zorilă, R. Doddipatla, R. Haeb-Umbach, in: ICASSP 2024 - 2024 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP), IEEE, 2024.","apa":"Cord-Landwehr, T., Boeddeker, C., Zorilă, C., Doddipatla, R., &#38; Haeb-Umbach, R. (2024). Geodesic Interpolation of Frame-Wise Speaker Embeddings for the Diarization of Meeting Scenarios. <i>ICASSP 2024 - 2024 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)</i>. 2024 IEEE International Conference on Acoustics, Speech, and Signal Processing (ICASSP), Seoul. <a href=\"https://doi.org/10.1109/icassp48485.2024.10445911\">https://doi.org/10.1109/icassp48485.2024.10445911</a>"},"ddc":["000"],"language":[{"iso":"eng"}],"publication":"ICASSP 2024 - 2024 IEEE International Conference on Acoustics, Speech and Signal Processing (ICASSP)","file":[{"relation":"main_file","success":1,"content_type":"application/pdf","access_level":"closed","file_name":"main.pdf","file_id":"60929","file_size":254478,"date_created":"2025-08-14T08:09:52Z","creator":"cord","date_updated":"2025-08-14T08:09:52Z"}],"publisher":"IEEE","date_created":"2024-04-25T12:57:22Z","title":"Geodesic Interpolation of Frame-Wise Speaker Embeddings for the Diarization of Meeting Scenarios","year":"2024"},{"keyword":["Photo"],"language":[{"iso":"eng"}],"_id":"56075","user_id":"48467","department":[{"_id":"306"}],"abstract":[{"text":"An isostructural series of FeII, FeIII, and Fe(IV)complexes [Fe(ImP)2]0/+/2+ utilizing the ImP 1,1′-(1,3-phenylene)-bis(3-methyl-1-imidazol-2-ylidene) ligand, combining N-heterocy-clic carbenes and cyclometalating functions, is presented. The strong donor motif stabilizes the high-valent Fe(IV) oxidation state yet keeps the FeII oxidation state accessible from the parent Fe(III)compound. Chemical oxidation of [Fe(ImP)2]+ yields stable [FeIV(ImP)2]2+. In contrast, [FeII(ImP)2]0, obtained by reduction,is highly sensitive toward oxygen. Exhaustive ground state characterization by single-crystal X-ray diffraction, 1H NMR,Mössbauer spectroscopy, temperature-dependent magnetic measurements, a combination of X-ray absorption near edge structureand valence-to-core, as well as core-to-core X-ray emission spectroscopy, complemented by detailed density functional theory (DFT) analysis, reveals that the three complexes[Fe(ImP)2]0/+/2+ can be unequivocally attributed to low-spin d6, d5, and d4 complexes. The excited state landscape of the Fe(II) and Fe(IV) complexes is characterized by short-lived 3MLCT and 3LMCT states, with lifetimes of 5.1 and 1.4 ps, respectively. In the FeII-compound, an energetically low-lying MC state leads to fast deactivation of the MLCT state. The distorted square-pyramidal state, where one carbene is dissociated, can not only relax into the ground state, but also into a singlet dissociated state. Its formation was investigated with time-dependent optical spectroscopy, while insights into its structure were gained by NMR spectroscopy.","lang":"eng"}],"status":"public","type":"journal_article","publication":"Inorganic Chemistry","title":"Isostructural Series of a Cyclometalated Iron Complex in Three Oxidation States","doi":"10.1021/acs.inorgchem.4c02576","publisher":"American Chemical Society (ACS)","date_updated":"2025-08-15T12:17:35Z","date_created":"2024-09-05T11:34:20Z","author":[{"first_name":"Jakob","last_name":"Steube","orcid":"0000-0003-3178-4429","id":"40342","full_name":"Steube, Jakob"},{"first_name":"Lorena","id":"44418","full_name":"Fritsch, Lorena","last_name":"Fritsch"},{"first_name":"Ayla","last_name":"Kruse","full_name":"Kruse, Ayla"},{"full_name":"Bokareva, Olga S.","last_name":"Bokareva","first_name":"Olga S."},{"last_name":"Demeshko","full_name":"Demeshko, Serhiy","first_name":"Serhiy"},{"id":"60250","full_name":"Elgabarty, Hossam","last_name":"Elgabarty","orcid":"0000-0002-4945-1481","first_name":"Hossam"},{"first_name":"Roland","full_name":"Schoch, Roland","id":"48467","orcid":"0000-0003-2061-7289","last_name":"Schoch"},{"first_name":"Mohammad","last_name":"Alaraby","full_name":"Alaraby, Mohammad"},{"first_name":"Hans","last_name":"Egold","full_name":"Egold, Hans","id":"101"},{"first_name":"Bastian Johannes","full_name":"Bracht, Bastian Johannes","id":"86707","last_name":"Bracht"},{"last_name":"Schmitz","full_name":"Schmitz, Lennart","id":"53140","first_name":"Lennart"},{"first_name":"Stephan","last_name":"Hohloch","full_name":"Hohloch, Stephan"},{"last_name":"Kühne","full_name":"Kühne, Thomas D.","first_name":"Thomas D."},{"first_name":"Franc","last_name":"Meyer","full_name":"Meyer, Franc"},{"first_name":"Oliver","last_name":"Kühn","full_name":"Kühn, Oliver"},{"first_name":"Stefan","full_name":"Lochbrunner, Stefan","last_name":"Lochbrunner"},{"first_name":"Matthias","id":"47241","full_name":"Bauer, Matthias","last_name":"Bauer","orcid":"0000-0002-9294-6076"}],"year":"2024","citation":{"ama":"Steube J, Fritsch L, Kruse A, et al. Isostructural Series of a Cyclometalated Iron Complex in Three Oxidation States. <i>Inorganic Chemistry</i>. Published online 2024. doi:<a href=\"https://doi.org/10.1021/acs.inorgchem.4c02576\">10.1021/acs.inorgchem.4c02576</a>","chicago":"Steube, Jakob, Lorena Fritsch, Ayla Kruse, Olga S. Bokareva, Serhiy Demeshko, Hossam Elgabarty, Roland Schoch, et al. “Isostructural Series of a Cyclometalated Iron Complex in Three Oxidation States.” <i>Inorganic Chemistry</i>, 2024. <a href=\"https://doi.org/10.1021/acs.inorgchem.4c02576\">https://doi.org/10.1021/acs.inorgchem.4c02576</a>.","ieee":"J. Steube <i>et al.</i>, “Isostructural Series of a Cyclometalated Iron Complex in Three Oxidation States,” <i>Inorganic Chemistry</i>, 2024, doi: <a href=\"https://doi.org/10.1021/acs.inorgchem.4c02576\">10.1021/acs.inorgchem.4c02576</a>.","mla":"Steube, Jakob, et al. “Isostructural Series of a Cyclometalated Iron Complex in Three Oxidation States.” <i>Inorganic Chemistry</i>, American Chemical Society (ACS), 2024, doi:<a href=\"https://doi.org/10.1021/acs.inorgchem.4c02576\">10.1021/acs.inorgchem.4c02576</a>.","bibtex":"@article{Steube_Fritsch_Kruse_Bokareva_Demeshko_Elgabarty_Schoch_Alaraby_Egold_Bracht_et al._2024, title={Isostructural Series of a Cyclometalated Iron Complex in Three Oxidation States}, DOI={<a href=\"https://doi.org/10.1021/acs.inorgchem.4c02576\">10.1021/acs.inorgchem.4c02576</a>}, journal={Inorganic Chemistry}, publisher={American Chemical Society (ACS)}, author={Steube, Jakob and Fritsch, Lorena and Kruse, Ayla and Bokareva, Olga S. and Demeshko, Serhiy and Elgabarty, Hossam and Schoch, Roland and Alaraby, Mohammad and Egold, Hans and Bracht, Bastian Johannes and et al.}, year={2024} }","short":"J. Steube, L. Fritsch, A. Kruse, O.S. Bokareva, S. Demeshko, H. Elgabarty, R. Schoch, M. Alaraby, H. Egold, B.J. Bracht, L. Schmitz, S. Hohloch, T.D. Kühne, F. Meyer, O. Kühn, S. Lochbrunner, M. Bauer, Inorganic Chemistry (2024).","apa":"Steube, J., Fritsch, L., Kruse, A., Bokareva, O. S., Demeshko, S., Elgabarty, H., Schoch, R., Alaraby, M., Egold, H., Bracht, B. J., Schmitz, L., Hohloch, S., Kühne, T. D., Meyer, F., Kühn, O., Lochbrunner, S., &#38; Bauer, M. (2024). Isostructural Series of a Cyclometalated Iron Complex in Three Oxidation States. <i>Inorganic Chemistry</i>. <a href=\"https://doi.org/10.1021/acs.inorgchem.4c02576\">https://doi.org/10.1021/acs.inorgchem.4c02576</a>"},"publication_status":"published","publication_identifier":{"issn":["0020-1669","1520-510X"]}},{"department":[{"_id":"306"}],"user_id":"48467","_id":"56074","language":[{"iso":"eng"}],"keyword":["Photo","Xray"],"publication":"Advanced Science","type":"journal_article","status":"public","abstract":[{"text":"Effective photoinduced charge transfer makes molecular bimetallic assemblies attractive for applications as active light‐induced proton reduction systems. Developing competitive base metal dyads is mandatory for a more sustainable future. However, the electron transfer mechanisms from the photosensitizer to the proton reduction catalyst in base metal dyads remain so far unexplored. A Fe─Co dyad that exhibits photocatalytic H2 production activity is studied using femtosecond X‐ray emission spectroscopy, complemented by ultrafast optical spectroscopy and theoretical time‐dependent DFT calculations, to understand the electronic and structural dynamics after photoexcitation and during the subsequent charge transfer process from the Fe(II) photosensitizer to the cobaloxime catalyst. This novel approach enables the simultaneous measurement of the transient X‐ray emission at the iron and cobalt K‐edges in a two‐color experiment. With this methodology, the excited state dynamics are correlated to the electron transfer processes, and evidence of the Fe→Co electron transfer as an initial step of proton reduction activity is unraveled.","lang":"eng"}],"author":[{"first_name":"Michał","id":"78878","full_name":"Nowakowski, Michał","last_name":"Nowakowski","orcid":"0000-0002-3734-7011"},{"full_name":"Huber‐Gedert, Marina","last_name":"Huber‐Gedert","first_name":"Marina"},{"first_name":"Hossam","orcid":"0000-0002-4945-1481","last_name":"Elgabarty","full_name":"Elgabarty, Hossam","id":"60250"},{"last_name":"Kalinko","full_name":"Kalinko, Aleksandr","first_name":"Aleksandr"},{"first_name":"Jacek","full_name":"Kubicki, Jacek","last_name":"Kubicki"},{"first_name":"Ahmet","full_name":"Kertmen, Ahmet","last_name":"Kertmen"},{"full_name":"Lindner, Natalia","last_name":"Lindner","first_name":"Natalia"},{"last_name":"Khakhulin","full_name":"Khakhulin, Dmitry","first_name":"Dmitry"},{"full_name":"Lima, Frederico A.","last_name":"Lima","first_name":"Frederico A."},{"first_name":"Tae‐Kyu","full_name":"Choi, Tae‐Kyu","last_name":"Choi"},{"last_name":"Biednov","full_name":"Biednov, Mykola","first_name":"Mykola"},{"first_name":"Lennart","last_name":"Schmitz","id":"53140","full_name":"Schmitz, Lennart"},{"first_name":"Natalia","last_name":"Piergies","full_name":"Piergies, Natalia"},{"full_name":"Zalden, Peter","last_name":"Zalden","first_name":"Peter"},{"full_name":"Kubicek, Katerina","last_name":"Kubicek","first_name":"Katerina"},{"full_name":"Rodriguez‐Fernandez, Angel","last_name":"Rodriguez‐Fernandez","first_name":"Angel"},{"first_name":"Mohammad Alaraby","full_name":"Salem, Mohammad Alaraby","last_name":"Salem"},{"last_name":"Canton","full_name":"Canton, Sophie E.","first_name":"Sophie E."},{"first_name":"Christian","last_name":"Bressler","full_name":"Bressler, Christian"},{"last_name":"Kühne","full_name":"Kühne, Thomas D.","first_name":"Thomas D."},{"full_name":"Gawelda, Wojciech","last_name":"Gawelda","first_name":"Wojciech"},{"first_name":"Matthias","id":"47241","full_name":"Bauer, Matthias","last_name":"Bauer","orcid":"0000-0002-9294-6076"}],"date_created":"2024-09-05T11:31:30Z","date_updated":"2025-08-15T12:49:56Z","publisher":"Wiley","doi":"10.1002/advs.202404348","title":"Ultrafast Two‐Color X‐Ray Emission Spectroscopy Reveals Excited State Landscape in a Base Metal Dyad","publication_identifier":{"issn":["2198-3844","2198-3844"]},"publication_status":"published","citation":{"short":"M. Nowakowski, M. Huber‐Gedert, H. Elgabarty, A. Kalinko, J. Kubicki, A. Kertmen, N. Lindner, D. Khakhulin, F.A. Lima, T. Choi, M. Biednov, L. Schmitz, N. Piergies, P. Zalden, K. Kubicek, A. Rodriguez‐Fernandez, M.A. Salem, S.E. Canton, C. Bressler, T.D. Kühne, W. Gawelda, M. Bauer, Advanced Science (2024).","mla":"Nowakowski, Michał, et al. “Ultrafast Two‐Color X‐Ray Emission Spectroscopy Reveals Excited State Landscape in a Base Metal Dyad.” <i>Advanced Science</i>, Wiley, 2024, doi:<a href=\"https://doi.org/10.1002/advs.202404348\">10.1002/advs.202404348</a>.","bibtex":"@article{Nowakowski_Huber‐Gedert_Elgabarty_Kalinko_Kubicki_Kertmen_Lindner_Khakhulin_Lima_Choi_et al._2024, title={Ultrafast Two‐Color X‐Ray Emission Spectroscopy Reveals Excited State Landscape in a Base Metal Dyad}, DOI={<a href=\"https://doi.org/10.1002/advs.202404348\">10.1002/advs.202404348</a>}, journal={Advanced Science}, publisher={Wiley}, author={Nowakowski, Michał and Huber‐Gedert, Marina and Elgabarty, Hossam and Kalinko, Aleksandr and Kubicki, Jacek and Kertmen, Ahmet and Lindner, Natalia and Khakhulin, Dmitry and Lima, Frederico A. and Choi, Tae‐Kyu and et al.}, year={2024} }","apa":"Nowakowski, M., Huber‐Gedert, M., Elgabarty, H., Kalinko, A., Kubicki, J., Kertmen, A., Lindner, N., Khakhulin, D., Lima, F. A., Choi, T., Biednov, M., Schmitz, L., Piergies, N., Zalden, P., Kubicek, K., Rodriguez‐Fernandez, A., Salem, M. A., Canton, S. E., Bressler, C., … Bauer, M. (2024). Ultrafast Two‐Color X‐Ray Emission Spectroscopy Reveals Excited State Landscape in a Base Metal Dyad. <i>Advanced Science</i>. <a href=\"https://doi.org/10.1002/advs.202404348\">https://doi.org/10.1002/advs.202404348</a>","chicago":"Nowakowski, Michał, Marina Huber‐Gedert, Hossam Elgabarty, Aleksandr Kalinko, Jacek Kubicki, Ahmet Kertmen, Natalia Lindner, et al. “Ultrafast Two‐Color X‐Ray Emission Spectroscopy Reveals Excited State Landscape in a Base Metal Dyad.” <i>Advanced Science</i>, 2024. <a href=\"https://doi.org/10.1002/advs.202404348\">https://doi.org/10.1002/advs.202404348</a>.","ieee":"M. Nowakowski <i>et al.</i>, “Ultrafast Two‐Color X‐Ray Emission Spectroscopy Reveals Excited State Landscape in a Base Metal Dyad,” <i>Advanced Science</i>, 2024, doi: <a href=\"https://doi.org/10.1002/advs.202404348\">10.1002/advs.202404348</a>.","ama":"Nowakowski M, Huber‐Gedert M, Elgabarty H, et al. Ultrafast Two‐Color X‐Ray Emission Spectroscopy Reveals Excited State Landscape in a Base Metal Dyad. <i>Advanced Science</i>. Published online 2024. doi:<a href=\"https://doi.org/10.1002/advs.202404348\">10.1002/advs.202404348</a>"},"year":"2024"},{"language":[{"iso":"eng"}],"keyword":["Xray"],"department":[{"_id":"306"}],"user_id":"48467","_id":"52346","status":"public","abstract":[{"text":"Promising cathode materials for fluoride-ion batteries (FIBs) are 3d transition metal containing oxides with Ruddlesden-Popper-type structure. So far, multi-elemental compositions were not investigated, but could alternate electrochemical performance similar to what has been found for cathode materials for lithium-ion batteries. Within this study, we investigate RP type La2Ni0.75Co0.25O4.08 as an intercalation-based active cathode material for all-solid-state FIBs. We determine the structural changes of La2Ni0.75Co0.25O4.08 during fluoride intercalation / de-intercalation by ex-situ X-ray diffraction, which showed that F- insertion leads to transformation of the parent phase to three different phases. Changes in Ni and Co oxidation states and coordination environment were examined by X-ray absorption spectroscopy and magnetic measurements in order to understand the complex reaction behaviour of the phases in detail, showing that the two transition metals behave differently in the charging and discharging process. Under optimized operating conditions, a cycle life of 120 cycles at a critical cut-off capacity of 40 mAh g-1 against Pb/PbF2 was obtained, which is one of the highest observed for intercalation electrode materials in FIBs so far. The average Coulombic efficiencies ranged from 85% to 90%. Thus, La2Ni0.75Co0.25O4.08 could be a promising candidate for cycling-stable high-energy cathode materials for all-solid-state FIBs","lang":"eng"}],"publication":"Journal of Materials Chemistry A","type":"journal_article","doi":"10.1039/d4ta00704b","title":"Insights into the First Multi-Transition-Metal Containing Ruddlesden Popper-Type Cathode for all-solid-state Fluoride Ion Batteries","author":[{"full_name":"Vanita, Vanita","last_name":"Vanita","first_name":"Vanita"},{"full_name":"Waidha, Aamir Iqbal","last_name":"Waidha","first_name":"Aamir Iqbal"},{"first_name":"Sami","last_name":"Vasala","full_name":"Vasala, Sami"},{"last_name":"Puphal","full_name":"Puphal, Pascal","first_name":"Pascal"},{"first_name":"Roland","id":"48467","full_name":"Schoch, Roland","last_name":"Schoch","orcid":"0000-0003-2061-7289"},{"full_name":"Glatzel, Pieter","last_name":"Glatzel","first_name":"Pieter"},{"id":"47241","full_name":"Bauer, Matthias","last_name":"Bauer","orcid":"0000-0002-9294-6076","first_name":"Matthias"},{"full_name":"Clemens, Oliver","last_name":"Clemens","first_name":"Oliver"}],"date_created":"2024-03-07T10:01:09Z","date_updated":"2025-08-15T12:50:31Z","publisher":"Royal Society of Chemistry (RSC)","citation":{"short":"V. Vanita, A.I. Waidha, S. Vasala, P. Puphal, R. Schoch, P. Glatzel, M. Bauer, O. Clemens, Journal of Materials Chemistry A (2024).","mla":"Vanita, Vanita, et al. “Insights into the First Multi-Transition-Metal Containing Ruddlesden Popper-Type Cathode for All-Solid-State Fluoride Ion Batteries.” <i>Journal of Materials Chemistry A</i>, no. 12, Royal Society of Chemistry (RSC), 2024, doi:<a href=\"https://doi.org/10.1039/d4ta00704b\">10.1039/d4ta00704b</a>.","bibtex":"@article{Vanita_Waidha_Vasala_Puphal_Schoch_Glatzel_Bauer_Clemens_2024, title={Insights into the First Multi-Transition-Metal Containing Ruddlesden Popper-Type Cathode for all-solid-state Fluoride Ion Batteries}, DOI={<a href=\"https://doi.org/10.1039/d4ta00704b\">10.1039/d4ta00704b</a>}, number={12}, journal={Journal of Materials Chemistry A}, publisher={Royal Society of Chemistry (RSC)}, author={Vanita, Vanita and Waidha, Aamir Iqbal and Vasala, Sami and Puphal, Pascal and Schoch, Roland and Glatzel, Pieter and Bauer, Matthias and Clemens, Oliver}, year={2024} }","apa":"Vanita, V., Waidha, A. I., Vasala, S., Puphal, P., Schoch, R., Glatzel, P., Bauer, M., &#38; Clemens, O. (2024). Insights into the First Multi-Transition-Metal Containing Ruddlesden Popper-Type Cathode for all-solid-state Fluoride Ion Batteries. <i>Journal of Materials Chemistry A</i>, <i>12</i>. <a href=\"https://doi.org/10.1039/d4ta00704b\">https://doi.org/10.1039/d4ta00704b</a>","chicago":"Vanita, Vanita, Aamir Iqbal Waidha, Sami Vasala, Pascal Puphal, Roland Schoch, Pieter Glatzel, Matthias Bauer, and Oliver Clemens. “Insights into the First Multi-Transition-Metal Containing Ruddlesden Popper-Type Cathode for All-Solid-State Fluoride Ion Batteries.” <i>Journal of Materials Chemistry A</i>, no. 12 (2024). <a href=\"https://doi.org/10.1039/d4ta00704b\">https://doi.org/10.1039/d4ta00704b</a>.","ieee":"V. Vanita <i>et al.</i>, “Insights into the First Multi-Transition-Metal Containing Ruddlesden Popper-Type Cathode for all-solid-state Fluoride Ion Batteries,” <i>Journal of Materials Chemistry A</i>, no. 12, 2024, doi: <a href=\"https://doi.org/10.1039/d4ta00704b\">10.1039/d4ta00704b</a>.","ama":"Vanita V, Waidha AI, Vasala S, et al. Insights into the First Multi-Transition-Metal Containing Ruddlesden Popper-Type Cathode for all-solid-state Fluoride Ion Batteries. <i>Journal of Materials Chemistry A</i>. 2024;(12). doi:<a href=\"https://doi.org/10.1039/d4ta00704b\">10.1039/d4ta00704b</a>"},"year":"2024","issue":"12","publication_identifier":{"issn":["2050-7488","2050-7496"]},"publication_status":"published"},{"citation":{"ieee":"M. Benz <i>et al.</i>, “Hydrogen spillover through hydride transfer: the reaction of ZnO and ZrO2 with strong hydride donors,” <i>Catalysis Science &#38; Technology</i>, vol. 14, no. 20, pp. 5854–5863, 2024, doi: <a href=\"https://doi.org/10.1039/d4cy00504j\">10.1039/d4cy00504j</a>.","chicago":"Benz, Michael, Osman Bunjaku, Michał Nowakowski, Alexander Allgaier, Indro Biswas, Joris van Slageren, Matthias Bauer, and Deven P. Estes. “Hydrogen Spillover through Hydride Transfer: The Reaction of ZnO and ZrO2 with Strong Hydride Donors.” <i>Catalysis Science &#38; Technology</i> 14, no. 20 (2024): 5854–63. <a href=\"https://doi.org/10.1039/d4cy00504j\">https://doi.org/10.1039/d4cy00504j</a>.","ama":"Benz M, Bunjaku O, Nowakowski M, et al. Hydrogen spillover through hydride transfer: the reaction of ZnO and ZrO2 with strong hydride donors. <i>Catalysis Science &#38; Technology</i>. 2024;14(20):5854-5863. doi:<a href=\"https://doi.org/10.1039/d4cy00504j\">10.1039/d4cy00504j</a>","bibtex":"@article{Benz_Bunjaku_Nowakowski_Allgaier_Biswas_van Slageren_Bauer_Estes_2024, title={Hydrogen spillover through hydride transfer: the reaction of ZnO and ZrO2 with strong hydride donors}, volume={14}, DOI={<a href=\"https://doi.org/10.1039/d4cy00504j\">10.1039/d4cy00504j</a>}, number={20}, journal={Catalysis Science &#38; Technology}, publisher={Royal Society of Chemistry (RSC)}, author={Benz, Michael and Bunjaku, Osman and Nowakowski, Michał and Allgaier, Alexander and Biswas, Indro and van Slageren, Joris and Bauer, Matthias and Estes, Deven P.}, year={2024}, pages={5854–5863} }","mla":"Benz, Michael, et al. “Hydrogen Spillover through Hydride Transfer: The Reaction of ZnO and ZrO2 with Strong Hydride Donors.” <i>Catalysis Science &#38; Technology</i>, vol. 14, no. 20, Royal Society of Chemistry (RSC), 2024, pp. 5854–63, doi:<a href=\"https://doi.org/10.1039/d4cy00504j\">10.1039/d4cy00504j</a>.","short":"M. Benz, O. Bunjaku, M. Nowakowski, A. Allgaier, I. Biswas, J. van Slageren, M. Bauer, D.P. Estes, Catalysis Science &#38; Technology 14 (2024) 5854–5863.","apa":"Benz, M., Bunjaku, O., Nowakowski, M., Allgaier, A., Biswas, I., van Slageren, J., Bauer, M., &#38; Estes, D. P. (2024). Hydrogen spillover through hydride transfer: the reaction of ZnO and ZrO2 with strong hydride donors. <i>Catalysis Science &#38; Technology</i>, <i>14</i>(20), 5854–5863. <a href=\"https://doi.org/10.1039/d4cy00504j\">https://doi.org/10.1039/d4cy00504j</a>"},"page":"5854-5863","intvolume":"        14","publication_status":"published","publication_identifier":{"issn":["2044-4753","2044-4761"]},"doi":"10.1039/d4cy00504j","date_updated":"2025-08-15T12:42:34Z","author":[{"last_name":"Benz","full_name":"Benz, Michael","first_name":"Michael"},{"first_name":"Osman","full_name":"Bunjaku, Osman","last_name":"Bunjaku"},{"first_name":"Michał","full_name":"Nowakowski, Michał","id":"78878","orcid":"0000-0002-3734-7011","last_name":"Nowakowski"},{"last_name":"Allgaier","full_name":"Allgaier, Alexander","first_name":"Alexander"},{"full_name":"Biswas, Indro","last_name":"Biswas","first_name":"Indro"},{"first_name":"Joris","full_name":"van Slageren, Joris","last_name":"van Slageren"},{"last_name":"Bauer","orcid":"0000-0002-9294-6076","full_name":"Bauer, Matthias","id":"47241","first_name":"Matthias"},{"last_name":"Estes","full_name":"Estes, Deven P.","first_name":"Deven P."}],"volume":14,"status":"public","type":"journal_article","_id":"60216","user_id":"48467","department":[{"_id":"306"}],"year":"2024","issue":"20","title":"Hydrogen spillover through hydride transfer: the reaction of ZnO and ZrO2 with strong hydride donors","publisher":"Royal Society of Chemistry (RSC)","date_created":"2025-06-16T08:55:24Z","abstract":[{"lang":"eng","text":"Hydride donors such as DIBAL or CuH react with ZnO and ZrO2 via hydrogen spillover. This suggests that hydrogen spillover in catalysts based on these metal oxides may take place via initial hydride transfer and not via proton–electron transfer."}],"publication":"Catalysis Science & Technology","keyword":["Xray"],"language":[{"iso":"eng"}]},{"abstract":[{"text":"Transition metal complexes, particularly copper hydrides, play an important role in various catalytic processes and molecular inorganic chemistry. This study employs synchrotron hard X‐ray spectroscopy to gain insights into the geometric and electronic properties of copper hydrides as potential catalysts for CO2 hydrogenation. The potential of high energy resolution X‐ray absorption near‐edge structure (HERFD‐XANES) and valence‐to‐core X‐ray emission (VtC‐XES) is demonstrated with measurement on Stryker's reagent (Cu6H6) and [Cu3(μ3‐H)(dpmppe)2](PF6)2 (Cu3H), alongside a non‐hydride copper compound (Cu‐I). The XANES analysis reveals that coordination geometries strongly influence the spectra, providing only indirect details about hydride coordination. The VtC‐XES analysis exhibits a distinct signal around 8975 eV, offering a diagnostic tool to identify hydride ligands. Theoretical calculations support and extend these findings by comparing hydride‐containing complexes with their hydride‐free counterparts.","lang":"eng"}],"publication":"Chemistry – A European Journal","keyword":["Xray"],"language":[{"iso":"eng"}],"year":"2024","issue":"36","title":"Detection and Characterization of Hydride Ligands in Copper Complexes by Hard X‐ray Spectroscopy","publisher":"Wiley","date_created":"2024-05-07T08:41:11Z","status":"public","type":"journal_article","article_type":"original","_id":"54024","user_id":"48467","department":[{"_id":"306"}],"citation":{"apa":"Fritsch, L., Rehsies, P., Barakat, W., Estes, D. P., &#38; Bauer, M. (2024). Detection and Characterization of Hydride Ligands in Copper Complexes by Hard X‐ray Spectroscopy. <i>Chemistry – A European Journal</i>, <i>30</i>(36). <a href=\"https://doi.org/10.1002/chem.202400357\">https://doi.org/10.1002/chem.202400357</a>","short":"L. Fritsch, P. Rehsies, W. Barakat, D.P. Estes, M. Bauer, Chemistry – A European Journal 30 (2024).","mla":"Fritsch, Lorena, et al. “Detection and Characterization of Hydride Ligands in Copper Complexes by Hard X‐ray Spectroscopy.” <i>Chemistry – A European Journal</i>, vol. 30, no. 36, Wiley, 2024, doi:<a href=\"https://doi.org/10.1002/chem.202400357\">10.1002/chem.202400357</a>.","bibtex":"@article{Fritsch_Rehsies_Barakat_Estes_Bauer_2024, title={Detection and Characterization of Hydride Ligands in Copper Complexes by Hard X‐ray Spectroscopy}, volume={30}, DOI={<a href=\"https://doi.org/10.1002/chem.202400357\">10.1002/chem.202400357</a>}, number={36}, journal={Chemistry – A European Journal}, publisher={Wiley}, author={Fritsch, Lorena and Rehsies, Pia and Barakat, Wael and Estes, Deven P. and Bauer, Matthias}, year={2024} }","ieee":"L. Fritsch, P. Rehsies, W. Barakat, D. P. Estes, and M. Bauer, “Detection and Characterization of Hydride Ligands in Copper Complexes by Hard X‐ray Spectroscopy,” <i>Chemistry – A European Journal</i>, vol. 30, no. 36, 2024, doi: <a href=\"https://doi.org/10.1002/chem.202400357\">10.1002/chem.202400357</a>.","chicago":"Fritsch, Lorena, Pia Rehsies, Wael Barakat, Deven P. Estes, and Matthias Bauer. “Detection and Characterization of Hydride Ligands in Copper Complexes by Hard X‐ray Spectroscopy.” <i>Chemistry – A European Journal</i> 30, no. 36 (2024). <a href=\"https://doi.org/10.1002/chem.202400357\">https://doi.org/10.1002/chem.202400357</a>.","ama":"Fritsch L, Rehsies P, Barakat W, Estes DP, Bauer M. Detection and Characterization of Hydride Ligands in Copper Complexes by Hard X‐ray Spectroscopy. <i>Chemistry – A European Journal</i>. 2024;30(36). doi:<a href=\"https://doi.org/10.1002/chem.202400357\">10.1002/chem.202400357</a>"},"intvolume":"        30","publication_status":"published","publication_identifier":{"issn":["0947-6539","1521-3765"]},"doi":"10.1002/chem.202400357","date_updated":"2025-08-15T12:51:10Z","author":[{"id":"44418","full_name":"Fritsch, Lorena","last_name":"Fritsch","first_name":"Lorena"},{"first_name":"Pia","last_name":"Rehsies","full_name":"Rehsies, Pia","id":"46959"},{"last_name":"Barakat","full_name":"Barakat, Wael","first_name":"Wael"},{"full_name":"Estes, Deven P.","last_name":"Estes","first_name":"Deven P."},{"first_name":"Matthias","last_name":"Bauer","orcid":"0000-0002-9294-6076","id":"47241","full_name":"Bauer, Matthias"}],"volume":30}]