---
_id: '40499'
abstract:
- lang: eng
text: September 2021
author:
- first_name: Petra
full_name: Büker, Petra
id: '21978'
last_name: Büker
- first_name: Birgit
full_name: Hüpping, Birgit
last_name: Hüpping
citation:
ama: 'Büker P, Hüpping B. Children as (Co)Researchers as an Opportunity to influence
School Life: A Didactic Approach and its Relevance in the Perspective of Children.
Beitrag im Rahmen des Symposiums: Participation to Connect Members of the School
Community an der ECER (European Conference on Educational Research), University
of Geneva. Online. In: ; 2021.'
apa: 'Büker, P., & Hüpping, B. (2021). Children as (Co)Researchers as an
Opportunity to influence School Life: A Didactic Approach and its Relevance in
the Perspective of Children. Beitrag im Rahmen des Symposiums: Participation to
Connect Members of the School Community an der ECER (European Conference on Educational
Research), University of Geneva. Online.'
bibtex: '@inproceedings{Büker_Hüpping_2021, title={Children as (Co)Researchers as
an Opportunity to influence School Life: A Didactic Approach and its Relevance
in the Perspective of Children. Beitrag im Rahmen des Symposiums: Participation
to Connect Members of the School Community an der ECER (European Conference on
Educational Research), University of Geneva. Online}, author={Büker, Petra and
Hüpping, Birgit}, year={2021} }'
chicago: 'Büker, Petra, and Birgit Hüpping. “Children as (Co)Researchers as an Opportunity
to Influence School Life: A Didactic Approach and Its Relevance in the Perspective
of Children. Beitrag Im Rahmen Des Symposiums: Participation to Connect Members
of the School Community an Der ECER (European Conference on Educational Research),
University of Geneva. Online,” 2021.'
ieee: 'P. Büker and B. Hüpping, “Children as (Co)Researchers as an Opportunity to
influence School Life: A Didactic Approach and its Relevance in the Perspective
of Children. Beitrag im Rahmen des Symposiums: Participation to Connect Members
of the School Community an der ECER (European Conference on Educational Research),
University of Geneva. Online,” 2021.'
mla: 'Büker, Petra, and Birgit Hüpping. Children as (Co)Researchers as an Opportunity
to Influence School Life: A Didactic Approach and Its Relevance in the Perspective
of Children. Beitrag Im Rahmen Des Symposiums: Participation to Connect Members
of the School Community an Der ECER (European Conference on Educational Research),
University of Geneva. Online. 2021.'
short: 'P. Büker, B. Hüpping, in: 2021.'
date_created: 2023-01-27T11:11:37Z
date_updated: 2023-01-27T12:48:10Z
department:
- _id: '458'
language:
- iso: eng
status: public
title: 'Children as (Co)Researchers as an Opportunity to influence School Life: A
Didactic Approach and its Relevance in the Perspective of Children. Beitrag im Rahmen
des Symposiums: Participation to Connect Members of the School Community an der
ECER (European Conference on Educational Research), University of Geneva. Online'
type: conference
user_id: '26718'
year: '2021'
...
---
_id: '37609'
author:
- first_name: Petra
full_name: Büker, Petra
id: '21978'
last_name: Büker
- first_name: Birgit
full_name: Hüpping, Birgit
last_name: Hüpping
- first_name: Enikö
full_name: Zala-Mezö, Enikö
last_name: Zala-Mezö
citation:
ama: Büker P, Hüpping B, Zala-Mezö E. Partizipation als Veränderung. Eine Aufforderung
an Grundschule und Forschung. Zeitschrift für Grundschulforschung. 2021;14(2):391-406.
doi:10.1007/s42278-021-00117-8
apa: Büker, P., Hüpping, B., & Zala-Mezö, E. (2021). Partizipation als Veränderung.
Eine Aufforderung an Grundschule und Forschung. Zeitschrift für Grundschulforschung,
14(2), 391–406. https://doi.org/10.1007/s42278-021-00117-8
bibtex: '@article{Büker_Hüpping_Zala-Mezö_2021, title={Partizipation als Veränderung.
Eine Aufforderung an Grundschule und Forschung}, volume={14}, DOI={10.1007/s42278-021-00117-8 }, number={2}, journal={Zeitschrift für Grundschulforschung},
author={Büker, Petra and Hüpping, Birgit and Zala-Mezö, Enikö}, year={2021}, pages={391–406}
}'
chicago: 'Büker, Petra, Birgit Hüpping, and Enikö Zala-Mezö. “Partizipation als
Veränderung. Eine Aufforderung an Grundschule und Forschung.” Zeitschrift für
Grundschulforschung 14, no. 2 (2021): 391–406. https://doi.org/10.1007/s42278-021-00117-8 .'
ieee: 'P. Büker, B. Hüpping, and E. Zala-Mezö, “Partizipation als Veränderung. Eine
Aufforderung an Grundschule und Forschung,” Zeitschrift für Grundschulforschung,
vol. 14, no. 2, pp. 391–406, 2021, doi: 10.1007/s42278-021-00117-8 .'
mla: Büker, Petra, et al. “Partizipation als Veränderung. Eine Aufforderung an Grundschule
und Forschung.” Zeitschrift für Grundschulforschung, vol. 14, no. 2, 2021,
pp. 391–406, doi:10.1007/s42278-021-00117-8
.
short: P. Büker, B. Hüpping, E. Zala-Mezö, Zeitschrift für Grundschulforschung 14
(2021) 391–406.
date_created: 2023-01-19T14:42:23Z
date_updated: 2023-01-27T13:16:11Z
department:
- _id: '458'
doi: '10.1007/s42278-021-00117-8 '
intvolume: ' 14'
issue: '2'
language:
- iso: ger
page: 391-406
publication: Zeitschrift für Grundschulforschung
status: public
title: Partizipation als Veränderung. Eine Aufforderung an Grundschule und Forschung
type: journal_article
user_id: '26718'
volume: 14
year: '2021'
...
---
_id: '40541'
author:
- first_name: D.
full_name: Itner, D.
last_name: Itner
- first_name: H.
full_name: Gravenkamp, H.
last_name: Gravenkamp
- first_name: Dmitrij
full_name: Dreiling, Dmitrij
id: '32616'
last_name: Dreiling
- first_name: Nadine
full_name: Feldmann, Nadine
id: '23082'
last_name: Feldmann
- first_name: Bernd
full_name: Henning, Bernd
id: '213'
last_name: Henning
citation:
ama: 'Itner D, Gravenkamp H, Dreiling D, Feldmann N, Henning B. Simulation of Guided
Waves in Cylinders Subject to Arbitrary Boundary Conditions Using the Scaled Boundary
Finite Element Method. In: 14th WCCM-ECCOMAS Congress. Vol 700. Numerical
Methods and Algorithms in Science and Engineering. CIMNE; 2021. doi:10.23967/wccm-eccomas.2020.307'
apa: Itner, D., Gravenkamp, H., Dreiling, D., Feldmann, N., & Henning, B. (2021).
Simulation of Guided Waves in Cylinders Subject to Arbitrary Boundary Conditions
Using the Scaled Boundary Finite Element Method. 14th WCCM-ECCOMAS Congress,
700. https://doi.org/10.23967/wccm-eccomas.2020.307
bibtex: '@inproceedings{Itner_Gravenkamp_Dreiling_Feldmann_Henning_2021, series={Numerical
Methods and Algorithms in Science and Engineering}, title={Simulation of Guided
Waves in Cylinders Subject to Arbitrary Boundary Conditions Using the Scaled Boundary
Finite Element Method}, volume={700}, DOI={10.23967/wccm-eccomas.2020.307},
booktitle={14th WCCM-ECCOMAS Congress}, publisher={CIMNE}, author={Itner, D. and
Gravenkamp, H. and Dreiling, Dmitrij and Feldmann, Nadine and Henning, Bernd},
year={2021}, collection={Numerical Methods and Algorithms in Science and Engineering}
}'
chicago: Itner, D., H. Gravenkamp, Dmitrij Dreiling, Nadine Feldmann, and Bernd
Henning. “Simulation of Guided Waves in Cylinders Subject to Arbitrary Boundary
Conditions Using the Scaled Boundary Finite Element Method.” In 14th WCCM-ECCOMAS
Congress, Vol. 700. Numerical Methods and Algorithms in Science and Engineering.
CIMNE, 2021. https://doi.org/10.23967/wccm-eccomas.2020.307.
ieee: 'D. Itner, H. Gravenkamp, D. Dreiling, N. Feldmann, and B. Henning, “Simulation
of Guided Waves in Cylinders Subject to Arbitrary Boundary Conditions Using the
Scaled Boundary Finite Element Method,” in 14th WCCM-ECCOMAS Congress,
2021, vol. 700, doi: 10.23967/wccm-eccomas.2020.307.'
mla: Itner, D., et al. “Simulation of Guided Waves in Cylinders Subject to Arbitrary
Boundary Conditions Using the Scaled Boundary Finite Element Method.” 14th
WCCM-ECCOMAS Congress, vol. 700, CIMNE, 2021, doi:10.23967/wccm-eccomas.2020.307.
short: 'D. Itner, H. Gravenkamp, D. Dreiling, N. Feldmann, B. Henning, in: 14th
WCCM-ECCOMAS Congress, CIMNE, 2021.'
conference:
end_date: 2021-01-15
name: 14th World Congress on Computational Mechanics (WCCM)
start_date: 2021-01-11
date_created: 2023-01-27T15:08:47Z
date_updated: 2023-01-27T15:28:35Z
department:
- _id: '49'
doi: 10.23967/wccm-eccomas.2020.307
intvolume: ' 700'
language:
- iso: eng
license: https://creativecommons.org/licenses/by-nc-sa/3.0/
main_file_link:
- open_access: '1'
url: https://www.scipedia.com/public/Itner_et_al_2021a
oa: '1'
project:
- _id: '89'
grant_number: '409779252'
name: 'VaMP: Vollständige Bestimmung der akustischen Materialparameter von Polymeren'
publication: 14th WCCM-ECCOMAS Congress
publication_status: published
publisher: CIMNE
series_title: Numerical Methods and Algorithms in Science and Engineering
status: public
title: Simulation of Guided Waves in Cylinders Subject to Arbitrary Boundary Conditions
Using the Scaled Boundary Finite Element Method
type: conference
user_id: '32616'
volume: 700
year: '2021'
...
---
_id: '40601'
abstract:
- lang: eng
text: "Abstract\r\n Background
and aims\r\n One reason for the controversial
discussion of whether the dual task (DT) walking paradigm has an added value for
diagnosis in clinical conditions might be the use of different gait measurement
systems. Therefore, the purpose was 1) to detect DT effects of central gait parameters
obtained from five different gait analysis devices in young and old adults, 2)
to assess the consistency of the measurement systems, and 3) to determine if the
absolut and proportional DT costs (DTC) are greater than the system-measurement
error under ST.\r\n \r\n Methods\r\n
\ Twelve old (72.2 ± 7.9y) and 14 young adults (28.3 ± 6.2y)
walked a 14.7-m distance under ST and DT at a self-selected gait velocity. Interrater
reliability, precision of the measurement and sensitivity to change were calculated
under ST and DT.\r\n \r\n Results\r\n
\ An age effect was observed in almost all gait parameters
for the ST condition. For DT only differences for stride length (p < .029,
ɳ2p = .239) as well as single and double
limb support (p = .036, ɳ2p = .227;
p = .034, ɳ2p = .218)
remained. The measurement systems showed a lower absolute agreement compared to
consistency across all systems.\r\n \r\n
\ Conclusions\r\n When
reporting DT effects, the real changes in performance and random measurement errors
should always be accounted for. These findings have strong implications for interpreting
DT effects.\r\n "
article_number: '17'
author:
- first_name: Thomas Jürgen
full_name: Klotzbier, Thomas Jürgen
last_name: Klotzbier
- first_name: Bettina
full_name: Wollesen, Bettina
last_name: Wollesen
- first_name: Oliver
full_name: Vogel, Oliver
last_name: Vogel
- first_name: Julian
full_name: Rudisch, Julian
last_name: Rudisch
- first_name: Thomas
full_name: Cordes, Thomas
last_name: Cordes
- first_name: Thomas
full_name: Jöllenbeck, Thomas
last_name: Jöllenbeck
- first_name: Lutz
full_name: Vogt, Lutz
last_name: Vogt
citation:
ama: Klotzbier TJ, Wollesen B, Vogel O, et al. An interrater reliability study of
gait analysis systems with the dual task paradigm in healthy young and older adults.
European Review of Aging and Physical Activity. 2021;18(1). doi:10.1186/s11556-021-00271-z
apa: Klotzbier, T. J., Wollesen, B., Vogel, O., Rudisch, J., Cordes, T., Jöllenbeck,
T., & Vogt, L. (2021). An interrater reliability study of gait analysis systems
with the dual task paradigm in healthy young and older adults. European Review
of Aging and Physical Activity, 18(1), Article 17. https://doi.org/10.1186/s11556-021-00271-z
bibtex: '@article{Klotzbier_Wollesen_Vogel_Rudisch_Cordes_Jöllenbeck_Vogt_2021,
title={An interrater reliability study of gait analysis systems with the dual
task paradigm in healthy young and older adults}, volume={18}, DOI={10.1186/s11556-021-00271-z},
number={117}, journal={European Review of Aging and Physical Activity}, publisher={Springer
Science and Business Media LLC}, author={Klotzbier, Thomas Jürgen and Wollesen,
Bettina and Vogel, Oliver and Rudisch, Julian and Cordes, Thomas and Jöllenbeck,
Thomas and Vogt, Lutz}, year={2021} }'
chicago: Klotzbier, Thomas Jürgen, Bettina Wollesen, Oliver Vogel, Julian Rudisch,
Thomas Cordes, Thomas Jöllenbeck, and Lutz Vogt. “An Interrater Reliability Study
of Gait Analysis Systems with the Dual Task Paradigm in Healthy Young and Older
Adults.” European Review of Aging and Physical Activity 18, no. 1 (2021).
https://doi.org/10.1186/s11556-021-00271-z.
ieee: 'T. J. Klotzbier et al., “An interrater reliability study of gait analysis
systems with the dual task paradigm in healthy young and older adults,” European
Review of Aging and Physical Activity, vol. 18, no. 1, Art. no. 17, 2021,
doi: 10.1186/s11556-021-00271-z.'
mla: Klotzbier, Thomas Jürgen, et al. “An Interrater Reliability Study of Gait Analysis
Systems with the Dual Task Paradigm in Healthy Young and Older Adults.” European
Review of Aging and Physical Activity, vol. 18, no. 1, 17, Springer Science
and Business Media LLC, 2021, doi:10.1186/s11556-021-00271-z.
short: T.J. Klotzbier, B. Wollesen, O. Vogel, J. Rudisch, T. Cordes, T. Jöllenbeck,
L. Vogt, European Review of Aging and Physical Activity 18 (2021).
date_created: 2023-01-27T16:42:16Z
date_updated: 2023-01-27T16:42:28Z
department:
- _id: '266'
doi: 10.1186/s11556-021-00271-z
intvolume: ' 18'
issue: '1'
keyword:
- Geriatrics and Gerontology
language:
- iso: eng
publication: European Review of Aging and Physical Activity
publication_identifier:
issn:
- 1813-7253
- 1861-6909
publication_status: published
publisher: Springer Science and Business Media LLC
status: public
title: An interrater reliability study of gait analysis systems with the dual task
paradigm in healthy young and older adults
type: journal_article
user_id: '75770'
volume: 18
year: '2021'
...
---
_id: '40598'
author:
- first_name: Julian
full_name: Rudisch, Julian
last_name: Rudisch
- first_name: Thomas
full_name: Jöllenbeck, Thomas
last_name: Jöllenbeck
- first_name: Lutz
full_name: Vogt, Lutz
last_name: Vogt
- first_name: Thomas
full_name: Cordes, Thomas
last_name: Cordes
- first_name: Thomas Jürgen
full_name: Klotzbier, Thomas Jürgen
last_name: Klotzbier
- first_name: Oliver
full_name: Vogel, Oliver
last_name: Vogel
- first_name: Bettina
full_name: Wollesen, Bettina
last_name: Wollesen
citation:
ama: Rudisch J, Jöllenbeck T, Vogt L, et al. Agreement and consistency of five different
clinical gait analysis systems in the assessment of spatiotemporal gait parameters.
Gait & Posture. 2021;85:55-64. doi:10.1016/j.gaitpost.2021.01.013
apa: Rudisch, J., Jöllenbeck, T., Vogt, L., Cordes, T., Klotzbier, T. J., Vogel,
O., & Wollesen, B. (2021). Agreement and consistency of five different clinical
gait analysis systems in the assessment of spatiotemporal gait parameters. Gait
& Posture, 85, 55–64. https://doi.org/10.1016/j.gaitpost.2021.01.013
bibtex: '@article{Rudisch_Jöllenbeck_Vogt_Cordes_Klotzbier_Vogel_Wollesen_2021,
title={Agreement and consistency of five different clinical gait analysis systems
in the assessment of spatiotemporal gait parameters}, volume={85}, DOI={10.1016/j.gaitpost.2021.01.013},
journal={Gait & Posture}, publisher={Elsevier BV}, author={Rudisch, Julian
and Jöllenbeck, Thomas and Vogt, Lutz and Cordes, Thomas and Klotzbier, Thomas
Jürgen and Vogel, Oliver and Wollesen, Bettina}, year={2021}, pages={55–64} }'
chicago: 'Rudisch, Julian, Thomas Jöllenbeck, Lutz Vogt, Thomas Cordes, Thomas Jürgen
Klotzbier, Oliver Vogel, and Bettina Wollesen. “Agreement and Consistency of Five
Different Clinical Gait Analysis Systems in the Assessment of Spatiotemporal Gait
Parameters.” Gait & Posture 85 (2021): 55–64. https://doi.org/10.1016/j.gaitpost.2021.01.013.'
ieee: 'J. Rudisch et al., “Agreement and consistency of five different clinical
gait analysis systems in the assessment of spatiotemporal gait parameters,” Gait
& Posture, vol. 85, pp. 55–64, 2021, doi: 10.1016/j.gaitpost.2021.01.013.'
mla: Rudisch, Julian, et al. “Agreement and Consistency of Five Different Clinical
Gait Analysis Systems in the Assessment of Spatiotemporal Gait Parameters.” Gait
& Posture, vol. 85, Elsevier BV, 2021, pp. 55–64, doi:10.1016/j.gaitpost.2021.01.013.
short: J. Rudisch, T. Jöllenbeck, L. Vogt, T. Cordes, T.J. Klotzbier, O. Vogel,
B. Wollesen, Gait & Posture 85 (2021) 55–64.
date_created: 2023-01-27T16:37:34Z
date_updated: 2023-01-27T16:37:56Z
department:
- _id: '266'
doi: 10.1016/j.gaitpost.2021.01.013
intvolume: ' 85'
keyword:
- Rehabilitation
- Orthopedics and Sports Medicine
- Biophysics
language:
- iso: eng
page: 55-64
publication: Gait & Posture
publication_identifier:
issn:
- 0966-6362
publication_status: published
publisher: Elsevier BV
status: public
title: Agreement and consistency of five different clinical gait analysis systems
in the assessment of spatiotemporal gait parameters
type: journal_article
user_id: '75770'
volume: 85
year: '2021'
...
---
_id: '39794'
abstract:
- lang: ger
text: "In der Herausforderung Unterricht inklusionsbezogen weiterzuentwickeln, manifestiert
sich unter anderem die Forderung nach der Qualifizierung von (angehenden) Lehrkräften
bzgl. der Anwendung und Umsetzung einer alltagsintegrierten Diagnostik mit dem
Ziel, Kinder individualisiert und gleichzeitig mit Bezug auf einen gemeinsamen
Lerngegenstand zu unterrichten. Dabei ist ein didaktisch-diagnostisches Handeln
aller Lehrkräfte gefordert, welches im Kontext einer professionellen und inklusionsorientierten
Gestaltung sowie einer angemessenen Begleitung und Förderung von Lern- und Entwicklungsprozessen
steht. In der Konzeption entsprechender Aus- und Weiterbildungsformate setzt das
geplante Projekt DiPoSa (Didaktisch-diagnostische Potentiale des inklusionsorientierten
Sachunterrichts) an. Ziel ist es durch einen Design-Based-Research-Ansatz (DBR)
Videovignetten zu erstellen und zu evaluieren, mittels derer entsprechende Kompetenzen
von (angehenden) Lehrkräften im Sachunterricht weiterentwickelt werden können.
Dabei bietet insbesondere der Sachunterricht als vielperspektivisches Integrationsfach
der Grundschule einen passenden Rahmen, kindliche Lernpotentiale als Ausgangspunkt
für didaktisch-diagnostisches Handeln nutzbar zu machen. Denn in aktuellen inklusionsorientierten
Ansätzen des Sachunterrichts sind sowohl reformpädagogisch orientierte als auch
offene Konzepte und Modelle des adaptiven Unterrichts zu finden, die sich an den
unterschiedlichen Programmatiken der Umsetzung von individueller Förderung orientieren.
Im folgenden Beitrag werden die dem geplanten Projekt zugrundeliegenden theoretischen
und empirischen Zugänge erläutert und die forschungsmethodische Umsetzung durch
einen DBR-Ansatz als methodologische Basis für eine Theorie-Praxis-verzahnende
Forschungsperspektive auf diagnostisches Handeln sowie die Förderung diagnostischer
Handlungskompetenzen durch Videovignetten im Kontext der Aus- und Weiterbildung
von (Sachunterrichts-)Lehrkräften diskutiert.\r\n \r\nAbstract\r\nThe challenge
to further promote practices of inclusive teaching, requires the development of
assessment literacy. Combined with the aim to teach all children in a collaborative
learning environment, qualification of teachers (in training) in the application
and implementation of formative assessment as an integrated daily routine is needed.
Therefore, the project DiPoSa focuses on the development of appropriate training
and qualification formats. The project heads to create and evaluate video vignettes
using a design-based-research approach (DBR), which can then be used to further
develop assessment literacy of teachers in social studies and science in primary
education. As a multi-perspective integrative subject in elementary school social
studies and science in primary education offers a suitable framework for practices
of formative assessment taking children's learning potentials as a serious concern.
Foundations can be seen in current inclusive approaches to social studies and
science in primary education, where reform pedagogically orientation and open
concepts can as well be found as models of adaptive teaching. Although there are
different theoretical and programmatic implementations, both perspectives share
an orientation towards individual support of children. With this in mind the following
article tries to lay down the theoretical and empirical approaches of the planed
project DiPoSa and discusses methodological foundations of the project. The discussion
focuses on how assessment practices as well as assessment literacy can be promoted
through a DBR research-design using video vignettes in the context of teacher
education and qualification and rooting in a deepened science-practice partnership.Zusammenfassung
englisch"
alternative_title:
- Potentials of formative assessment practices in social studies and science in inclusive
primary education. Conceptual and methodological implications of a design-based-research-based
approach for teacher education
author:
- first_name: René
full_name: Schroeder, René
last_name: Schroeder
- first_name: Eva
full_name: Blumberg, Eva
last_name: Blumberg
- first_name: Brigitte
full_name: Kottmann, Brigitte
id: '82466'
last_name: Kottmann
- first_name: Susanne
full_name: Miller, Susanne
last_name: Miller
- first_name: Anne
full_name: Reh, Anne
last_name: Reh
citation:
ama: Schroeder R, Blumberg E, Kottmann B, Miller S, Reh A. Chancen des inklusionsorientierten
Sachunterrichts für didaktisch-diagnostisches Handeln. Konzeptionelle und methodologisch-methodische
Grundlagen eines forschungsbasierten Entwicklungsansatzes für die Lehrer*innenbildung.
QfI - Qualifizierung für Inklusion Online-Zeitschrift zur Forschung über Aus-,
Fort- und Weiterbildung pädagogischer Fachkräfte. 2021;3(2). doi:10.21248/qfi.74
apa: Schroeder, R., Blumberg, E., Kottmann, B., Miller, S., & Reh, A. (2021).
Chancen des inklusionsorientierten Sachunterrichts für didaktisch-diagnostisches
Handeln. Konzeptionelle und methodologisch-methodische Grundlagen eines forschungsbasierten
Entwicklungsansatzes für die Lehrer*innenbildung. QfI - Qualifizierung für
Inklusion. Online-Zeitschrift zur Forschung über Aus-, Fort- und Weiterbildung
pädagogischer Fachkräfte, 3(2). https://doi.org/10.21248/qfi.74
bibtex: '@article{Schroeder_Blumberg_Kottmann_Miller_Reh_2021, title={Chancen des
inklusionsorientierten Sachunterrichts für didaktisch-diagnostisches Handeln.
Konzeptionelle und methodologisch-methodische Grundlagen eines forschungsbasierten
Entwicklungsansatzes für die Lehrer*innenbildung}, volume={3}, DOI={10.21248/qfi.74},
number={2}, journal={QfI - Qualifizierung für Inklusion. Online-Zeitschrift zur
Forschung über Aus-, Fort- und Weiterbildung pädagogischer Fachkräfte}, author={Schroeder,
René and Blumberg, Eva and Kottmann, Brigitte and Miller, Susanne and Reh, Anne},
year={2021} }'
chicago: Schroeder, René, Eva Blumberg, Brigitte Kottmann, Susanne Miller, and Anne
Reh. “Chancen des inklusionsorientierten Sachunterrichts für didaktisch-diagnostisches
Handeln. Konzeptionelle und methodologisch-methodische Grundlagen eines forschungsbasierten
Entwicklungsansatzes für die Lehrer*innenbildung.” QfI - Qualifizierung für
Inklusion. Online-Zeitschrift zur Forschung über Aus-, Fort- und Weiterbildung
pädagogischer Fachkräfte 3, no. 2 (2021). https://doi.org/10.21248/qfi.74.
ieee: 'R. Schroeder, E. Blumberg, B. Kottmann, S. Miller, and A. Reh, “Chancen des
inklusionsorientierten Sachunterrichts für didaktisch-diagnostisches Handeln.
Konzeptionelle und methodologisch-methodische Grundlagen eines forschungsbasierten
Entwicklungsansatzes für die Lehrer*innenbildung,” QfI - Qualifizierung für
Inklusion. Online-Zeitschrift zur Forschung über Aus-, Fort- und Weiterbildung
pädagogischer Fachkräfte, vol. 3, no. 2, 2021, doi: 10.21248/qfi.74.'
mla: Schroeder, René, et al. “Chancen des inklusionsorientierten Sachunterrichts
für didaktisch-diagnostisches Handeln. Konzeptionelle und methodologisch-methodische
Grundlagen eines forschungsbasierten Entwicklungsansatzes für die Lehrer*innenbildung.”
QfI - Qualifizierung für Inklusion. Online-Zeitschrift zur Forschung über Aus-,
Fort- und Weiterbildung pädagogischer Fachkräfte, vol. 3, no. 2, 2021, doi:10.21248/qfi.74.
short: R. Schroeder, E. Blumberg, B. Kottmann, S. Miller, A. Reh, QfI - Qualifizierung
für Inklusion. Online-Zeitschrift zur Forschung über Aus-, Fort- und Weiterbildung
pädagogischer Fachkräfte 3 (2021).
date_created: 2023-01-24T20:03:43Z
date_updated: 2023-01-29T13:41:59Z
ddc:
- '370'
department:
- _id: '479'
doi: 10.21248/qfi.74
has_accepted_license: '1'
intvolume: ' 3'
issue: '2'
language:
- iso: ger
publication: QfI - Qualifizierung für Inklusion. Online-Zeitschrift zur Forschung
über Aus-, Fort- und Weiterbildung pädagogischer Fachkräfte
publication_identifier:
eissn:
- 2699-2477
publication_status: published
status: public
title: Chancen des inklusionsorientierten Sachunterrichts für didaktisch-diagnostisches
Handeln. Konzeptionelle und methodologisch-methodische Grundlagen eines forschungsbasierten
Entwicklungsansatzes für die Lehrer*innenbildung
type: journal_article
user_id: '77753'
volume: 3
year: '2021'
...
---
_id: '39809'
abstract:
- lang: ger
text: "In dem Beitrag wird ausgehend von der Notwendigkeit einer inklusionspädagogischen
Professionalisierung im Lehramtsstudium ein erziehungswissenschaftliches Projekt
dargestellt, das es den teilnehmenden Bachelor-Studierenden in besonderer Weise
ermöglicht, berufsspezifische Reflexionsprozesse zu durchlaufen. In dem Projekt
übernehmen Studierende die einjährige pädagogische Förderung von Grundschulkindern
mit bildungsrelevanten Benachteiligungsfaktoren, die häufig von Selektionspraktiken
und -maßnahmen bedroht sind. Die Bearbeitung von vorliegenden Common-Sense-Theorien
im inklusiven Kontext gilt dabei als ein relevantes Professionalisierungsziel
in der Lehramtsausbildung. Konkret werden Ausschnitte aus Praktikumsberichten
von zwei Studierenden mittels der dokumentarischen Methode ausgewertet und einander
gegenübergestellt, um daran herauszuarbeiten, inwiefern sich die Reflexionen unterscheiden.
Es zeigt sich anhand der Analysen, dass im Rahmen der Praxisphase eine Reflection-on-Action
und auch die vertiefte Reflexion eigener Common-Sense-Theorien grundsätzlich möglich,
jedoch nicht voraussetzungslos ist. Insbesondere kann auch anhand der gewählten
Einzelfälle verdeutlicht werden, wie individuell inklusionsbezogene Professionalisierungsprozesse
im Rahmen der vorliegenden Praxisphase verlaufen können. Die Analyse offenbart
multiple Professionalisierungschancen in Abhängigkeit von den Rahmenbedingungen
des Projekts, den individuellen Schwerpunkten der pädagogischen Arbeit oder den
individuellen Reflexionen der Studierenden.\r\nAbstract\r\nBased on the necessity
of an inclusive pedagogical professionalisation in the teacher training program,
this article presents an educational science project that enables the participating
Bachelor students in a unique manner to go through profession-specific reflection
processes. In the project, students take on the one-year pedagogical support of
primary school children with educational disadvantage factors, who are often threatened
by selection practices and measures. In this context, working through present
common-sense theories in an inclusive context is considered a relevant professionalization
goal in teacher education. Specifically, excerpts from internship reports of two
students are analysed by means of the documentary method and compared to each
other in order to work out the extent to which the reflections differ. The analyses
show that reflection-on-action and in-depth reflection on one's own common-sense
theories are generally possible during the practical phase, but not without preconditions.
In particular, the selected individual cases can be used to illustrate how individual
inclusion-related professionalisation processes can take place within the framework
of the present practical phase. The analysis reveals multiple opportunities for
professionalisation depending on the general framework of the project, the individual
focal points of the pedagogical work or the individual reflections of the students."
author:
- first_name: Anne
full_name: Reh, Anne
last_name: Reh
- first_name: Brigitte
full_name: Kottmann, Brigitte
id: '82466'
last_name: Kottmann
- first_name: Susanne
full_name: Miller, Susanne
last_name: Miller
citation:
ama: 'Reh A, Kottmann B, Miller S. Berufsspezifische Reflexionsprozesse durch Einzelfallarbeit
im Projekt „Schule für alle": Analyse von zwei Praxisberichten mittels der Dokumentarischen
Methode. QfI - Qualifizierung für Inklusion. 2021;3(1). doi:10.21248/qfi.56'
apa: 'Reh, A., Kottmann, B., & Miller, S. (2021). Berufsspezifische Reflexionsprozesse
durch Einzelfallarbeit im Projekt „Schule für alle": Analyse von zwei Praxisberichten
mittels der Dokumentarischen Methode. QfI - Qualifizierung für Inklusion,
3(1). https://doi.org/10.21248/qfi.56'
bibtex: '@article{Reh_Kottmann_Miller_2021, title={Berufsspezifische Reflexionsprozesse
durch Einzelfallarbeit im Projekt „Schule für alle": Analyse von zwei Praxisberichten
mittels der Dokumentarischen Methode}, volume={3}, DOI={10.21248/qfi.56},
number={1}, journal={QfI - Qualifizierung für Inklusion}, author={Reh, Anne and
Kottmann, Brigitte and Miller, Susanne}, year={2021} }'
chicago: 'Reh, Anne, Brigitte Kottmann, and Susanne Miller. “Berufsspezifische Reflexionsprozesse
durch Einzelfallarbeit im Projekt „Schule für alle": Analyse von zwei Praxisberichten
mittels der Dokumentarischen Methode.” QfI - Qualifizierung für Inklusion
3, no. 1 (2021). https://doi.org/10.21248/qfi.56.'
ieee: 'A. Reh, B. Kottmann, and S. Miller, “Berufsspezifische Reflexionsprozesse
durch Einzelfallarbeit im Projekt „Schule für alle": Analyse von zwei Praxisberichten
mittels der Dokumentarischen Methode,” QfI - Qualifizierung für Inklusion,
vol. 3, no. 1, 2021, doi: 10.21248/qfi.56.'
mla: 'Reh, Anne, et al. “Berufsspezifische Reflexionsprozesse durch Einzelfallarbeit
im Projekt „Schule für alle": Analyse von zwei Praxisberichten mittels der Dokumentarischen
Methode.” QfI - Qualifizierung für Inklusion, vol. 3, no. 1, 2021, doi:10.21248/qfi.56.'
short: A. Reh, B. Kottmann, S. Miller, QfI - Qualifizierung für Inklusion 3 (2021).
date_created: 2023-01-24T20:30:10Z
date_updated: 2023-01-29T13:41:18Z
ddc:
- '370'
department:
- _id: '479'
doi: 10.21248/qfi.56
has_accepted_license: '1'
intvolume: ' 3'
issue: '1'
language:
- iso: ger
publication: QfI - Qualifizierung für Inklusion
publication_status: published
status: public
title: 'Berufsspezifische Reflexionsprozesse durch Einzelfallarbeit im Projekt „Schule
für alle": Analyse von zwei Praxisberichten mittels der Dokumentarischen Methode'
type: journal_article
user_id: '77753'
volume: 3
year: '2021'
...
---
_id: '39804'
author:
- first_name: Brigitte
full_name: Kottmann, Brigitte
id: '82466'
last_name: Kottmann
citation:
ama: 'Kottmann B. Übergänge begleiten. Peer-Beratung beim Übergang für Lernende
mit Förderbedarf. In: Streese B, Werning R, eds. Schule inklusiv - Vielfalt
nutzen - Bildungsgerechtigkeit schaffen. Vol 3. ; 2021:32-34.'
apa: Kottmann, B. (2021). Übergänge begleiten. Peer-Beratung beim Übergang für Lernende
mit Förderbedarf. In B. Streese & R. Werning (Eds.), Schule inklusiv -
Vielfalt nutzen - Bildungsgerechtigkeit schaffen (Vol. 3, pp. 32–34).
bibtex: '@inbook{Kottmann_2021, title={Übergänge begleiten. Peer-Beratung beim Übergang
für Lernende mit Förderbedarf}, volume={3}, booktitle={Schule inklusiv - Vielfalt
nutzen - Bildungsgerechtigkeit schaffen}, author={Kottmann, Brigitte}, editor={Streese,
Bettina and Werning, Rolf}, year={2021}, pages={32–34} }'
chicago: Kottmann, Brigitte. “Übergänge begleiten. Peer-Beratung beim Übergang für
Lernende mit Förderbedarf.” In Schule inklusiv - Vielfalt nutzen - Bildungsgerechtigkeit
schaffen, edited by Bettina Streese and Rolf Werning, 3:32–34, 2021.
ieee: B. Kottmann, “Übergänge begleiten. Peer-Beratung beim Übergang für Lernende
mit Förderbedarf,” in Schule inklusiv - Vielfalt nutzen - Bildungsgerechtigkeit
schaffen, vol. 3, B. Streese and R. Werning, Eds. 2021, pp. 32–34.
mla: Kottmann, Brigitte. “Übergänge begleiten. Peer-Beratung beim Übergang für Lernende
mit Förderbedarf.” Schule inklusiv - Vielfalt nutzen - Bildungsgerechtigkeit
schaffen, edited by Bettina Streese and Rolf Werning, vol. 3, 2021, pp. 32–34.
short: 'B. Kottmann, in: B. Streese, R. Werning (Eds.), Schule inklusiv - Vielfalt
nutzen - Bildungsgerechtigkeit schaffen, 2021, pp. 32–34.'
date_created: 2023-01-24T20:27:40Z
date_updated: 2023-01-29T13:44:51Z
department:
- _id: '479'
editor:
- first_name: Bettina
full_name: Streese, Bettina
last_name: Streese
- first_name: Rolf
full_name: Werning, Rolf
last_name: Werning
intvolume: ' 3'
language:
- iso: ger
page: 32-34
publication: Schule inklusiv - Vielfalt nutzen - Bildungsgerechtigkeit schaffen
publication_status: published
status: public
title: Übergänge begleiten. Peer-Beratung beim Übergang für Lernende mit Förderbedarf
type: book_chapter
user_id: '77753'
volume: 3
year: '2021'
...
---
_id: '39814'
author:
- first_name: Brigitte
full_name: Kottmann, Brigitte
id: '82466'
last_name: Kottmann
citation:
ama: 'Kottmann B. Rezension des Buches: "Sonderschule im Nationalsozialismus. Die
Magdeburger Hilfsschule als Modell von Dagmar Hänsel (2019). Zeitschrift für
Heilpädagogik. 2021;4(2021):211-212.'
apa: 'Kottmann, B. (2021). Rezension des Buches: "Sonderschule im Nationalsozialismus.
Die Magdeburger Hilfsschule als Modell von Dagmar Hänsel (2019). Zeitschrift
für Heilpädagogik, 4(2021), 211–212.'
bibtex: '@article{Kottmann_2021, title={Rezension des Buches: "Sonderschule im Nationalsozialismus.
Die Magdeburger Hilfsschule als Modell von Dagmar Hänsel (2019)}, volume={4},
number={2021}, journal={Zeitschrift für Heilpädagogik}, author={Kottmann, Brigitte},
year={2021}, pages={211–212} }'
chicago: 'Kottmann, Brigitte. “Rezension des Buches: "Sonderschule im Nationalsozialismus.
Die Magdeburger Hilfsschule als Modell von Dagmar Hänsel (2019).” Zeitschrift
für Heilpädagogik 4, no. 2021 (2021): 211–12.'
ieee: 'B. Kottmann, “Rezension des Buches: "Sonderschule im Nationalsozialismus.
Die Magdeburger Hilfsschule als Modell von Dagmar Hänsel (2019),” Zeitschrift
für Heilpädagogik, vol. 4, no. 2021, pp. 211–212, 2021.'
mla: 'Kottmann, Brigitte. “Rezension des Buches: "Sonderschule im Nationalsozialismus.
Die Magdeburger Hilfsschule als Modell von Dagmar Hänsel (2019).” Zeitschrift
für Heilpädagogik, vol. 4, no. 2021, 2021, pp. 211–12.'
short: B. Kottmann, Zeitschrift für Heilpädagogik 4 (2021) 211–212.
date_created: 2023-01-24T20:45:20Z
date_updated: 2023-01-29T13:43:58Z
department:
- _id: '479'
intvolume: ' 4'
issue: '2021'
language:
- iso: ger
page: 211-212
publication: Zeitschrift für Heilpädagogik
publication_status: published
status: public
title: 'Rezension des Buches: "Sonderschule im Nationalsozialismus. Die Magdeburger
Hilfsschule als Modell von Dagmar Hänsel (2019)'
type: journal_article
user_id: '77753'
volume: 4
year: '2021'
...
---
_id: '35758'
author:
- first_name: Elnaz
full_name: Meydani, Elnaz
last_name: Meydani
- first_name: Christoph
full_name: Düsing, Christoph
last_name: Düsing
- first_name: Matthias
full_name: Trier, Matthias
id: '72744'
last_name: Trier
citation:
ama: 'Meydani E, Düsing C, Trier M. Towards a Trust-Aware Item Recommendation System
on a Graph Autoencoder with Attention Mechanism. In: Lecture Notes in Information
Systems and Organisation. Springer International Publishing; 2021. doi:10.1007/978-3-030-86797-3_5'
apa: Meydani, E., Düsing, C., & Trier, M. (2021). Towards a Trust-Aware Item
Recommendation System on a Graph Autoencoder with Attention Mechanism. In Lecture
Notes in Information Systems and Organisation. Springer International Publishing.
https://doi.org/10.1007/978-3-030-86797-3_5
bibtex: '@inbook{Meydani_Düsing_Trier_2021, place={Cham}, title={Towards a Trust-Aware
Item Recommendation System on a Graph Autoencoder with Attention Mechanism}, DOI={10.1007/978-3-030-86797-3_5},
booktitle={Lecture Notes in Information Systems and Organisation}, publisher={Springer
International Publishing}, author={Meydani, Elnaz and Düsing, Christoph and Trier,
Matthias}, year={2021} }'
chicago: 'Meydani, Elnaz, Christoph Düsing, and Matthias Trier. “Towards a Trust-Aware
Item Recommendation System on a Graph Autoencoder with Attention Mechanism.” In
Lecture Notes in Information Systems and Organisation. Cham: Springer International
Publishing, 2021. https://doi.org/10.1007/978-3-030-86797-3_5.'
ieee: 'E. Meydani, C. Düsing, and M. Trier, “Towards a Trust-Aware Item Recommendation
System on a Graph Autoencoder with Attention Mechanism,” in Lecture Notes in
Information Systems and Organisation, Cham: Springer International Publishing,
2021.'
mla: Meydani, Elnaz, et al. “Towards a Trust-Aware Item Recommendation System on
a Graph Autoencoder with Attention Mechanism.” Lecture Notes in Information
Systems and Organisation, Springer International Publishing, 2021, doi:10.1007/978-3-030-86797-3_5.
short: 'E. Meydani, C. Düsing, M. Trier, in: Lecture Notes in Information Systems
and Organisation, Springer International Publishing, Cham, 2021.'
date_created: 2023-01-10T10:27:20Z
date_updated: 2023-01-29T23:19:40Z
department:
- _id: '198'
doi: 10.1007/978-3-030-86797-3_5
language:
- iso: eng
place: Cham
publication: Lecture Notes in Information Systems and Organisation
publication_identifier:
isbn:
- '9783030867966'
- '9783030867973'
issn:
- 2195-4968
- 2195-4976
publication_status: published
publisher: Springer International Publishing
status: public
title: Towards a Trust-Aware Item Recommendation System on a Graph Autoencoder with
Attention Mechanism
type: book_chapter
user_id: '14931'
year: '2021'
...
---
_id: '37936'
author:
- first_name: Emanuele
full_name: Pelucchi, Emanuele
last_name: Pelucchi
- first_name: Giorgos
full_name: Fagas, Giorgos
last_name: Fagas
- first_name: Igor
full_name: Aharonovich, Igor
last_name: Aharonovich
- first_name: Dirk
full_name: Englund, Dirk
last_name: Englund
- first_name: Eden
full_name: Figueroa, Eden
last_name: Figueroa
- first_name: Qihuang
full_name: Gong, Qihuang
last_name: Gong
- first_name: Hübel
full_name: Hannes, Hübel
last_name: Hannes
- first_name: Jin
full_name: Liu, Jin
last_name: Liu
- first_name: Chao-Yang
full_name: Lu, Chao-Yang
last_name: Lu
- first_name: Nobuyuki
full_name: Matsuda, Nobuyuki
last_name: Matsuda
- first_name: Jian-Wei
full_name: Pan, Jian-Wei
last_name: Pan
- first_name: Florian
full_name: Schreck, Florian
last_name: Schreck
- first_name: Fabio
full_name: Sciarrino, Fabio
last_name: Sciarrino
- first_name: Christine
full_name: Silberhorn, Christine
id: '26263'
last_name: Silberhorn
- first_name: Jianwei
full_name: Wang, Jianwei
last_name: Wang
- first_name: Klaus
full_name: Jöns, Klaus
id: '85353'
last_name: Jöns
citation:
ama: Pelucchi E, Fagas G, Aharonovich I, et al. The potential and global outlook
of integrated photonics for quantum technologies. Nature Reviews Physics.
2021;4(3):194-208. doi:10.1038/s42254-021-00398-z
apa: Pelucchi, E., Fagas, G., Aharonovich, I., Englund, D., Figueroa, E., Gong,
Q., Hannes, H., Liu, J., Lu, C.-Y., Matsuda, N., Pan, J.-W., Schreck, F., Sciarrino,
F., Silberhorn, C., Wang, J., & Jöns, K. (2021). The potential and global
outlook of integrated photonics for quantum technologies. Nature Reviews Physics,
4(3), 194–208. https://doi.org/10.1038/s42254-021-00398-z
bibtex: '@article{Pelucchi_Fagas_Aharonovich_Englund_Figueroa_Gong_Hannes_Liu_Lu_Matsuda_et
al._2021, title={The potential and global outlook of integrated photonics for
quantum technologies}, volume={4}, DOI={10.1038/s42254-021-00398-z},
number={3}, journal={Nature Reviews Physics}, publisher={Springer Science and
Business Media LLC}, author={Pelucchi, Emanuele and Fagas, Giorgos and Aharonovich,
Igor and Englund, Dirk and Figueroa, Eden and Gong, Qihuang and Hannes, Hübel
and Liu, Jin and Lu, Chao-Yang and Matsuda, Nobuyuki and et al.}, year={2021},
pages={194–208} }'
chicago: 'Pelucchi, Emanuele, Giorgos Fagas, Igor Aharonovich, Dirk Englund, Eden
Figueroa, Qihuang Gong, Hübel Hannes, et al. “The Potential and Global Outlook
of Integrated Photonics for Quantum Technologies.” Nature Reviews Physics
4, no. 3 (2021): 194–208. https://doi.org/10.1038/s42254-021-00398-z.'
ieee: 'E. Pelucchi et al., “The potential and global outlook of integrated
photonics for quantum technologies,” Nature Reviews Physics, vol. 4, no.
3, pp. 194–208, 2021, doi: 10.1038/s42254-021-00398-z.'
mla: Pelucchi, Emanuele, et al. “The Potential and Global Outlook of Integrated
Photonics for Quantum Technologies.” Nature Reviews Physics, vol. 4, no.
3, Springer Science and Business Media LLC, 2021, pp. 194–208, doi:10.1038/s42254-021-00398-z.
short: E. Pelucchi, G. Fagas, I. Aharonovich, D. Englund, E. Figueroa, Q. Gong,
H. Hannes, J. Liu, C.-Y. Lu, N. Matsuda, J.-W. Pan, F. Schreck, F. Sciarrino,
C. Silberhorn, J. Wang, K. Jöns, Nature Reviews Physics 4 (2021) 194–208.
date_created: 2023-01-22T17:46:36Z
date_updated: 2023-01-30T11:13:42Z
department:
- _id: '288'
- _id: '15'
- _id: '623'
- _id: '230'
doi: 10.1038/s42254-021-00398-z
intvolume: ' 4'
issue: '3'
keyword:
- General Physics and Astronomy
language:
- iso: eng
page: 194-208
publication: Nature Reviews Physics
publication_identifier:
issn:
- 2522-5820
publication_status: published
publisher: Springer Science and Business Media LLC
status: public
title: The potential and global outlook of integrated photonics for quantum technologies
type: journal_article
user_id: '26263'
volume: 4
year: '2021'
...
---
_id: '40673'
author:
- first_name: Mohammad
full_name: Soleymani, Mohammad
last_name: Soleymani
- first_name: Ignacio
full_name: Santamaria, Ignacio
last_name: Santamaria
- first_name: Peter J
full_name: Schreier, Peter J
last_name: Schreier
citation:
ama: Soleymani M, Santamaria I, Schreier PJ. Distributed Algorithms for Spectral
and Energy-Efficiency Maximization of $K$-User Interference Channels. IEEE
Access. 2021;9:96948–96963.
apa: Soleymani, M., Santamaria, I., & Schreier, P. J. (2021). Distributed Algorithms
for Spectral and Energy-Efficiency Maximization of $K$-User Interference Channels.
IEEE Access, 9, 96948–96963.
bibtex: '@article{Soleymani_Santamaria_Schreier_2021, title={Distributed Algorithms
for Spectral and Energy-Efficiency Maximization of $K$-User Interference Channels},
volume={9}, journal={IEEE Access}, publisher={IEEE}, author={Soleymani, Mohammad
and Santamaria, Ignacio and Schreier, Peter J}, year={2021}, pages={96948–96963}
}'
chicago: 'Soleymani, Mohammad, Ignacio Santamaria, and Peter J Schreier. “Distributed
Algorithms for Spectral and Energy-Efficiency Maximization of $K$-User Interference
Channels.” IEEE Access 9 (2021): 96948–96963.'
ieee: M. Soleymani, I. Santamaria, and P. J. Schreier, “Distributed Algorithms for
Spectral and Energy-Efficiency Maximization of $K$-User Interference Channels,”
IEEE Access, vol. 9, pp. 96948–96963, 2021.
mla: Soleymani, Mohammad, et al. “Distributed Algorithms for Spectral and Energy-Efficiency
Maximization of $K$-User Interference Channels.” IEEE Access, vol. 9, IEEE,
2021, pp. 96948–96963.
short: M. Soleymani, I. Santamaria, P.J. Schreier, IEEE Access 9 (2021) 96948–96963.
date_created: 2023-01-30T11:51:35Z
date_updated: 2023-01-30T12:03:37Z
department:
- _id: '263'
intvolume: ' 9'
page: 96948–96963
publication: IEEE Access
publisher: IEEE
status: public
title: Distributed Algorithms for Spectral and Energy-Efficiency Maximization of $K$-User
Interference Channels
type: journal_article
user_id: '43497'
volume: 9
year: '2021'
...
---
_id: '40677'
author:
- first_name: Mohammad
full_name: Soleymani, Mohammad
last_name: Soleymani
- first_name: Ignacio
full_name: Santamaria, Ignacio
last_name: Santamaria
- first_name: Behrouz
full_name: Maham, Behrouz
last_name: Maham
- first_name: Peter J
full_name: Schreier, Peter J
last_name: Schreier
citation:
ama: 'Soleymani M, Santamaria I, Maham B, Schreier PJ. Rate Region of the $K$-user
MIMO Interference Channel with Imperfect Transmitters. In: Proc. 28th European
Signal Processing Conference (EUSIPCO). ; 2021:1638–1642.'
apa: Soleymani, M., Santamaria, I., Maham, B., & Schreier, P. J. (2021). Rate
Region of the $K$-user MIMO Interference Channel with Imperfect Transmitters.
Proc. 28th European Signal Processing Conference (EUSIPCO), 1638–1642.
bibtex: '@inproceedings{Soleymani_Santamaria_Maham_Schreier_2021, title={Rate Region
of the $K$-user MIMO Interference Channel with Imperfect Transmitters}, booktitle={Proc.
28th European Signal Processing Conference (EUSIPCO)}, author={Soleymani, Mohammad
and Santamaria, Ignacio and Maham, Behrouz and Schreier, Peter J}, year={2021},
pages={1638–1642} }'
chicago: Soleymani, Mohammad, Ignacio Santamaria, Behrouz Maham, and Peter J Schreier.
“Rate Region of the $K$-User MIMO Interference Channel with Imperfect Transmitters.”
In Proc. 28th European Signal Processing Conference (EUSIPCO), 1638–1642,
2021.
ieee: M. Soleymani, I. Santamaria, B. Maham, and P. J. Schreier, “Rate Region of
the $K$-user MIMO Interference Channel with Imperfect Transmitters,” in Proc.
28th European Signal Processing Conference (EUSIPCO), 2021, pp. 1638–1642.
mla: Soleymani, Mohammad, et al. “Rate Region of the $K$-User MIMO Interference
Channel with Imperfect Transmitters.” Proc. 28th European Signal Processing
Conference (EUSIPCO), 2021, pp. 1638–1642.
short: 'M. Soleymani, I. Santamaria, B. Maham, P.J. Schreier, in: Proc. 28th European
Signal Processing Conference (EUSIPCO), 2021, pp. 1638–1642.'
date_created: 2023-01-30T11:51:35Z
date_updated: 2023-01-30T12:03:35Z
department:
- _id: '263'
page: 1638–1642
publication: Proc. 28th European Signal Processing Conference (EUSIPCO)
status: public
title: Rate Region of the $K$-user MIMO Interference Channel with Imperfect Transmitters
type: conference
user_id: '43497'
year: '2021'
...
---
_id: '41002'
abstract:
- lang: eng
text: Homogeneous catalysts immobilized on metal oxides often have different catalytic
properties than in homogeneous solution. This can be either activating or deactivating
and is often attributed to interactions of catalyst species with the metal oxide
surface. However, few studies have ever demonstrated the effect that close associations
of active sites with surfaces have on the catalytic activity. In this paper, we
immobilize H2Ru(PPh3)2(Ph2P)2N–C3H6–Si(OEt)3 (3) on SiO2, Al2O3, and ZnO and interrogate
the relationship to the surface using IR, MAS NMR, 1H–31P HETCOR, and XAS spectroscopies.
We found that while there are close contacts between the P atoms of the complex
and all three metal oxide surfaces, the Ru–H bond only reacts with oxygen bridges
on SiO2 and Al2O3, forming new Ru–O bonds. In contrast, complex 3 stays intact
on ZnO. Comparison of the catalytic activities of our immobilized species for
CO2 hydrogenation to ethyl formate showed that Lewis acidic metal oxides activate,
rather than deactivate, complex 3 in the order Al2O3 > ZnO > SiO2. The Lewis acidic
sites on the metal oxide surfaces most likely increase the productivity by increasing
the rate of esterification of formate intermediates.
article_type: original
author:
- first_name: Hoang-Huy
full_name: Nguyen, Hoang-Huy
last_name: Nguyen
- first_name: Zheng
full_name: Li, Zheng
last_name: Li
- first_name: Toni
full_name: Enenkel, Toni
last_name: Enenkel
- first_name: Joachim
full_name: Hildebrand, Joachim
last_name: Hildebrand
- first_name: Matthias
full_name: Bauer, Matthias
id: '47241'
last_name: Bauer
orcid: 0000-0002-9294-6076
- first_name: Michael
full_name: Dyballa, Michael
last_name: Dyballa
- first_name: Deven P.
full_name: Estes, Deven P.
last_name: Estes
citation:
ama: 'Nguyen H-H, Li Z, Enenkel T, et al. Probing the Interactions of Immobilized
Ruthenium Dihydride Complexes with Metal Oxide Surfaces by MAS NMR: Effects on
CO2 Hydrogenation. The Journal of Physical Chemistry C. 2021;125(27):14627-14635.
doi:10.1021/acs.jpcc.1c02074'
apa: 'Nguyen, H.-H., Li, Z., Enenkel, T., Hildebrand, J., Bauer, M., Dyballa, M.,
& Estes, D. P. (2021). Probing the Interactions of Immobilized Ruthenium Dihydride
Complexes with Metal Oxide Surfaces by MAS NMR: Effects on CO2 Hydrogenation.
The Journal of Physical Chemistry C, 125(27), 14627–14635. https://doi.org/10.1021/acs.jpcc.1c02074'
bibtex: '@article{Nguyen_Li_Enenkel_Hildebrand_Bauer_Dyballa_Estes_2021, title={Probing
the Interactions of Immobilized Ruthenium Dihydride Complexes with Metal Oxide
Surfaces by MAS NMR: Effects on CO2 Hydrogenation}, volume={125}, DOI={10.1021/acs.jpcc.1c02074},
number={27}, journal={The Journal of Physical Chemistry C}, publisher={American
Chemical Society (ACS)}, author={Nguyen, Hoang-Huy and Li, Zheng and Enenkel,
Toni and Hildebrand, Joachim and Bauer, Matthias and Dyballa, Michael and Estes,
Deven P.}, year={2021}, pages={14627–14635} }'
chicago: 'Nguyen, Hoang-Huy, Zheng Li, Toni Enenkel, Joachim Hildebrand, Matthias
Bauer, Michael Dyballa, and Deven P. Estes. “Probing the Interactions of Immobilized
Ruthenium Dihydride Complexes with Metal Oxide Surfaces by MAS NMR: Effects on
CO2 Hydrogenation.” The Journal of Physical Chemistry C 125,
no. 27 (2021): 14627–35. https://doi.org/10.1021/acs.jpcc.1c02074.'
ieee: 'H.-H. Nguyen et al., “Probing the Interactions of Immobilized Ruthenium
Dihydride Complexes with Metal Oxide Surfaces by MAS NMR: Effects on CO2
Hydrogenation,” The Journal of Physical Chemistry C, vol. 125, no. 27,
pp. 14627–14635, 2021, doi: 10.1021/acs.jpcc.1c02074.'
mla: 'Nguyen, Hoang-Huy, et al. “Probing the Interactions of Immobilized Ruthenium
Dihydride Complexes with Metal Oxide Surfaces by MAS NMR: Effects on CO2
Hydrogenation.” The Journal of Physical Chemistry C, vol. 125, no. 27,
American Chemical Society (ACS), 2021, pp. 14627–35, doi:10.1021/acs.jpcc.1c02074.'
short: H.-H. Nguyen, Z. Li, T. Enenkel, J. Hildebrand, M. Bauer, M. Dyballa, D.P.
Estes, The Journal of Physical Chemistry C 125 (2021) 14627–14635.
date_created: 2023-01-30T16:49:18Z
date_updated: 2023-01-31T08:06:00Z
department:
- _id: '35'
- _id: '306'
doi: 10.1021/acs.jpcc.1c02074
intvolume: ' 125'
issue: '27'
keyword:
- Surfaces
- Coatings and Films
- Physical and Theoretical Chemistry
- General Energy
- Electronic
- Optical and Magnetic Materials
language:
- iso: eng
page: 14627-14635
publication: The Journal of Physical Chemistry C
publication_identifier:
issn:
- 1932-7447
- 1932-7455
publication_status: published
publisher: American Chemical Society (ACS)
status: public
title: 'Probing the Interactions of Immobilized Ruthenium Dihydride Complexes with
Metal Oxide Surfaces by MAS NMR: Effects on CO2 Hydrogenation'
type: journal_article
user_id: '48467'
volume: 125
year: '2021'
...
---
_id: '40998'
abstract:
- lang: eng
text: Covalent organic frameworks (COFs) offer vast structural and chemical diversity
enabling a wide and growing range of applications. While COFs are well-established
as heterogeneous catalysts, so far, their high and ordered porosity has scarcely
been utilized to its full potential when it comes to spatially confined reactions
in COF pores to alter the outcome of reactions. Here, we present a highly porous
and crystalline, large-pore COF as catalytic support in α,ω-diene ring-closing
metathesis reactions, leading to increased macrocyclization selectivity. COF pore-wall
modification by immobilization of a Grubbs-Hoveyda-type catalyst via a mild silylation
reaction provides a molecularly precise heterogeneous olefin metathesis catalyst.
An increased macro(mono)cyclization (MMC) selectivity over oligomerization (O)
for the heterogeneous COF-catalyst (MMC:O=1.35) of up to 51 % compared to the
homogeneous catalyst (MMC:O=0.90) was observed along with a substrate-size dependency
in selectivity, pointing to diffusion limitations induced by the pore confinement.
article_type: original
author:
- first_name: Sebastian T.
full_name: Emmerling, Sebastian T.
last_name: Emmerling
- first_name: Felix
full_name: Ziegler, Felix
last_name: Ziegler
- first_name: Felix R.
full_name: Fischer, Felix R.
last_name: Fischer
- first_name: Roland
full_name: Schoch, Roland
id: '48467'
last_name: Schoch
orcid: 0000-0003-2061-7289
- first_name: Matthias
full_name: Bauer, Matthias
id: '47241'
last_name: Bauer
orcid: 0000-0002-9294-6076
- first_name: Bernd
full_name: Plietker, Bernd
last_name: Plietker
- first_name: Michael R.
full_name: Buchmeiser, Michael R.
last_name: Buchmeiser
- first_name: Bettina V.
full_name: Lotsch, Bettina V.
last_name: Lotsch
citation:
ama: 'Emmerling ST, Ziegler F, Fischer FR, et al. Olefin Metathesis in Confinement:
Towards Covalent Organic Framework Scaffolds for Increased Macrocyclization Selectivity.
Chemistry – A European Journal. 2021;28(8). doi:10.1002/chem.202104108'
apa: 'Emmerling, S. T., Ziegler, F., Fischer, F. R., Schoch, R., Bauer, M., Plietker,
B., Buchmeiser, M. R., & Lotsch, B. V. (2021). Olefin Metathesis in Confinement:
Towards Covalent Organic Framework Scaffolds for Increased Macrocyclization Selectivity.
Chemistry – A European Journal, 28(8). https://doi.org/10.1002/chem.202104108'
bibtex: '@article{Emmerling_Ziegler_Fischer_Schoch_Bauer_Plietker_Buchmeiser_Lotsch_2021,
title={Olefin Metathesis in Confinement: Towards Covalent Organic Framework Scaffolds
for Increased Macrocyclization Selectivity}, volume={28}, DOI={10.1002/chem.202104108},
number={8}, journal={Chemistry – A European Journal}, publisher={Wiley}, author={Emmerling,
Sebastian T. and Ziegler, Felix and Fischer, Felix R. and Schoch, Roland and Bauer,
Matthias and Plietker, Bernd and Buchmeiser, Michael R. and Lotsch, Bettina V.},
year={2021} }'
chicago: 'Emmerling, Sebastian T., Felix Ziegler, Felix R. Fischer, Roland Schoch,
Matthias Bauer, Bernd Plietker, Michael R. Buchmeiser, and Bettina V. Lotsch.
“Olefin Metathesis in Confinement: Towards Covalent Organic Framework Scaffolds
for Increased Macrocyclization Selectivity.” Chemistry – A European Journal
28, no. 8 (2021). https://doi.org/10.1002/chem.202104108.'
ieee: 'S. T. Emmerling et al., “Olefin Metathesis in Confinement: Towards
Covalent Organic Framework Scaffolds for Increased Macrocyclization Selectivity,”
Chemistry – A European Journal, vol. 28, no. 8, 2021, doi: 10.1002/chem.202104108.'
mla: 'Emmerling, Sebastian T., et al. “Olefin Metathesis in Confinement: Towards
Covalent Organic Framework Scaffolds for Increased Macrocyclization Selectivity.”
Chemistry – A European Journal, vol. 28, no. 8, Wiley, 2021, doi:10.1002/chem.202104108.'
short: S.T. Emmerling, F. Ziegler, F.R. Fischer, R. Schoch, M. Bauer, B. Plietker,
M.R. Buchmeiser, B.V. Lotsch, Chemistry – A European Journal 28 (2021).
date_created: 2023-01-30T16:48:22Z
date_updated: 2023-01-31T08:05:07Z
department:
- _id: '35'
- _id: '306'
doi: 10.1002/chem.202104108
intvolume: ' 28'
issue: '8'
keyword:
- General Chemistry
- Catalysis
- Organic Chemistry
language:
- iso: eng
publication: Chemistry – A European Journal
publication_identifier:
issn:
- 0947-6539
- 1521-3765
publication_status: published
publisher: Wiley
status: public
title: 'Olefin Metathesis in Confinement: Towards Covalent Organic Framework Scaffolds
for Increased Macrocyclization Selectivity'
type: journal_article
user_id: '48467'
volume: 28
year: '2021'
...
---
_id: '41003'
abstract:
- lang: eng
text: Combining strong σ-donating N-heterocyclic carbene ligands and π-accepting
pyridine ligands with a high octahedricity in rigid iron(II) complexes increases
the 3MLCT lifetime from 0.15 ps in the prototypical [Fe(tpy)2]2+ complex to 9.2
ps in [Fe(dpmi)2]2+12+. The tripodal CNN ligand dpmi (di(pyridine-2-yl)(3-methylimidazol-2-yl)methane)
forms six-membered chelate rings with the iron(II) centre leading to close to
90° bite angles and enhanced iron-ligand orbital overlap
article_type: original
author:
- first_name: Thomas
full_name: Reuter, Thomas
last_name: Reuter
- first_name: Ayla
full_name: Kruse, Ayla
last_name: Kruse
- first_name: Roland
full_name: Schoch, Roland
id: '48467'
last_name: Schoch
orcid: 0000-0003-2061-7289
- first_name: Stefan
full_name: Lochbrunner, Stefan
last_name: Lochbrunner
- first_name: Matthias
full_name: Bauer, Matthias
id: '47241'
last_name: Bauer
orcid: 0000-0002-9294-6076
- first_name: Katja
full_name: Heinze, Katja
last_name: Heinze
citation:
ama: Reuter T, Kruse A, Schoch R, Lochbrunner S, Bauer M, Heinze K. Higher MLCT
lifetime of carbene iron(<scp>ii</scp>) complexes by chelate ring
expansion. Chemical Communications. 2021;57(61):7541-7544. doi:10.1039/d1cc02173g
apa: Reuter, T., Kruse, A., Schoch, R., Lochbrunner, S., Bauer, M., & Heinze,
K. (2021). Higher MLCT lifetime of carbene iron(<scp>ii</scp>)
complexes by chelate ring expansion. Chemical Communications, 57(61),
7541–7544. https://doi.org/10.1039/d1cc02173g
bibtex: '@article{Reuter_Kruse_Schoch_Lochbrunner_Bauer_Heinze_2021, title={Higher
MLCT lifetime of carbene iron(<scp>ii</scp>) complexes by chelate
ring expansion}, volume={57}, DOI={10.1039/d1cc02173g},
number={61}, journal={Chemical Communications}, publisher={Royal Society of Chemistry
(RSC)}, author={Reuter, Thomas and Kruse, Ayla and Schoch, Roland and Lochbrunner,
Stefan and Bauer, Matthias and Heinze, Katja}, year={2021}, pages={7541–7544}
}'
chicago: 'Reuter, Thomas, Ayla Kruse, Roland Schoch, Stefan Lochbrunner, Matthias
Bauer, and Katja Heinze. “Higher MLCT Lifetime of Carbene Iron(<scp>ii</Scp>)
Complexes by Chelate Ring Expansion.” Chemical Communications 57, no. 61
(2021): 7541–44. https://doi.org/10.1039/d1cc02173g.'
ieee: 'T. Reuter, A. Kruse, R. Schoch, S. Lochbrunner, M. Bauer, and K. Heinze,
“Higher MLCT lifetime of carbene iron(<scp>ii</scp>) complexes
by chelate ring expansion,” Chemical Communications, vol. 57, no. 61, pp.
7541–7544, 2021, doi: 10.1039/d1cc02173g.'
mla: Reuter, Thomas, et al. “Higher MLCT Lifetime of Carbene Iron(<scp>ii</Scp>)
Complexes by Chelate Ring Expansion.” Chemical Communications, vol. 57,
no. 61, Royal Society of Chemistry (RSC), 2021, pp. 7541–44, doi:10.1039/d1cc02173g.
short: T. Reuter, A. Kruse, R. Schoch, S. Lochbrunner, M. Bauer, K. Heinze, Chemical
Communications 57 (2021) 7541–7544.
date_created: 2023-01-30T16:49:33Z
date_updated: 2023-01-31T08:06:16Z
department:
- _id: '35'
- _id: '306'
doi: 10.1039/d1cc02173g
intvolume: ' 57'
issue: '61'
keyword:
- Materials Chemistry
- Metals and Alloys
- Surfaces
- Coatings and Films
- General Chemistry
- Ceramics and Composites
- Electronic
- Optical and Magnetic Materials
- Catalysis
language:
- iso: eng
page: 7541-7544
publication: Chemical Communications
publication_identifier:
issn:
- 1359-7345
- 1364-548X
publication_status: published
publisher: Royal Society of Chemistry (RSC)
status: public
title: Higher MLCT lifetime of carbene iron(ii) complexes by chelate ring
expansion
type: journal_article
user_id: '48467'
volume: 57
year: '2021'
...
---
_id: '40997'
abstract:
- lang: eng
text: 'On transition metals such as iron rests lots of hope to replace precious
metal catalysts in the field of photochemistry for a more sustainable future.
Indeed, significant progress has been made in recent years in terms of lifetime
extension and emerging applications in catalysis. For this reason, recent synthetic
strategies of new photoactive iron compounds, which have proved to show particularly
promising properties, are reviewed here. The lifetime of the excited state serves
as a key parameter for comparison with the standard ruthenium complex, [Ru(bpy)3]2+,
to discuss the potential and performance of the iron complexes. This approach
is complemented by a more holistic examination of the sustainability of such a
substitution strategy in order to answer the question: when or at which point
can we assume that iron represents a more sustainable alternative for noble metals
in photochemical applications?'
article_type: review
author:
- first_name: Philipp
full_name: Dierks, Philipp
last_name: Dierks
- first_name: Yannik
full_name: Vukadinovic, Yannik
last_name: Vukadinovic
- first_name: Matthias
full_name: Bauer, Matthias
id: '47241'
last_name: Bauer
orcid: 0000-0002-9294-6076
citation:
ama: 'Dierks P, Vukadinovic Y, Bauer M. Photoactive iron complexes: more sustainable,
but still a challenge. Inorganic Chemistry Frontiers. 2021;9(2):206-220.
doi:10.1039/d1qi01112j'
apa: 'Dierks, P., Vukadinovic, Y., & Bauer, M. (2021). Photoactive iron complexes:
more sustainable, but still a challenge. Inorganic Chemistry Frontiers,
9(2), 206–220. https://doi.org/10.1039/d1qi01112j'
bibtex: '@article{Dierks_Vukadinovic_Bauer_2021, title={Photoactive iron complexes:
more sustainable, but still a challenge}, volume={9}, DOI={10.1039/d1qi01112j},
number={2}, journal={Inorganic Chemistry Frontiers}, publisher={Royal Society
of Chemistry (RSC)}, author={Dierks, Philipp and Vukadinovic, Yannik and Bauer,
Matthias}, year={2021}, pages={206–220} }'
chicago: 'Dierks, Philipp, Yannik Vukadinovic, and Matthias Bauer. “Photoactive
Iron Complexes: More Sustainable, but Still a Challenge.” Inorganic Chemistry
Frontiers 9, no. 2 (2021): 206–20. https://doi.org/10.1039/d1qi01112j.'
ieee: 'P. Dierks, Y. Vukadinovic, and M. Bauer, “Photoactive iron complexes: more
sustainable, but still a challenge,” Inorganic Chemistry Frontiers, vol.
9, no. 2, pp. 206–220, 2021, doi: 10.1039/d1qi01112j.'
mla: 'Dierks, Philipp, et al. “Photoactive Iron Complexes: More Sustainable, but
Still a Challenge.” Inorganic Chemistry Frontiers, vol. 9, no. 2, Royal
Society of Chemistry (RSC), 2021, pp. 206–20, doi:10.1039/d1qi01112j.'
short: P. Dierks, Y. Vukadinovic, M. Bauer, Inorganic Chemistry Frontiers 9 (2021)
206–220.
date_created: 2023-01-30T16:47:45Z
date_updated: 2023-01-31T08:04:56Z
department:
- _id: '35'
- _id: '306'
doi: 10.1039/d1qi01112j
intvolume: ' 9'
issue: '2'
keyword:
- Inorganic Chemistry
language:
- iso: eng
page: 206-220
publication: Inorganic Chemistry Frontiers
publication_identifier:
issn:
- 2052-1553
publication_status: published
publisher: Royal Society of Chemistry (RSC)
status: public
title: 'Photoactive iron complexes: more sustainable, but still a challenge'
type: journal_article
user_id: '48467'
volume: 9
year: '2021'
...
---
_id: '41000'
abstract:
- lang: eng
text: Metal-catalyzed C−H activations are environmentally and economically attractive
synthetic strategies for the construction of functional molecules as they obviate
the need for pre-functionalized substrates and minimize waste generation. Great
challenges reside in the control of selectivities, the utilization of unbiased
hydrocarbons, and the operation of atom-economical dehydrocoupling mechanisms.
An especially mild borylation of benzylic CH bonds was developed with the ligand-free
pre-catalyst Co[N(SiMe3)2]2 and the bench-stable and inexpensive borylation reagent
B2pin2 that produces H2 as the only by-product. A full set of kinetic, spectroscopic,
and preparative mechanistic studies are indicative of a tandem catalysis mechanism
of CH-borylation and dehydrocoupling via molecular CoI catalysts.
article_type: original
author:
- first_name: Pradip
full_name: Ghosh, Pradip
last_name: Ghosh
- first_name: Roland
full_name: Schoch, Roland
id: '48467'
last_name: Schoch
orcid: 0000-0003-2061-7289
- first_name: Matthias
full_name: Bauer, Matthias
id: '47241'
last_name: Bauer
orcid: 0000-0002-9294-6076
- first_name: Axel
full_name: Jacobi von Wangelin, Axel
last_name: Jacobi von Wangelin
citation:
ama: Ghosh P, Schoch R, Bauer M, Jacobi von Wangelin A. Selective Benzylic CH‐Borylations
by Tandem Cobalt Catalysis. Angewandte Chemie International Edition. 2021;61(1).
doi:10.1002/anie.202110821
apa: Ghosh, P., Schoch, R., Bauer, M., & Jacobi von Wangelin, A. (2021). Selective
Benzylic CH‐Borylations by Tandem Cobalt Catalysis. Angewandte Chemie International
Edition, 61(1). https://doi.org/10.1002/anie.202110821
bibtex: '@article{Ghosh_Schoch_Bauer_Jacobi von Wangelin_2021, title={Selective
Benzylic CH‐Borylations by Tandem Cobalt Catalysis}, volume={61}, DOI={10.1002/anie.202110821},
number={1}, journal={Angewandte Chemie International Edition}, publisher={Wiley},
author={Ghosh, Pradip and Schoch, Roland and Bauer, Matthias and Jacobi von Wangelin,
Axel}, year={2021} }'
chicago: Ghosh, Pradip, Roland Schoch, Matthias Bauer, and Axel Jacobi von Wangelin.
“Selective Benzylic CH‐Borylations by Tandem Cobalt Catalysis.” Angewandte
Chemie International Edition 61, no. 1 (2021). https://doi.org/10.1002/anie.202110821.
ieee: 'P. Ghosh, R. Schoch, M. Bauer, and A. Jacobi von Wangelin, “Selective Benzylic
CH‐Borylations by Tandem Cobalt Catalysis,” Angewandte Chemie International
Edition, vol. 61, no. 1, 2021, doi: 10.1002/anie.202110821.'
mla: Ghosh, Pradip, et al. “Selective Benzylic CH‐Borylations by Tandem Cobalt Catalysis.”
Angewandte Chemie International Edition, vol. 61, no. 1, Wiley, 2021, doi:10.1002/anie.202110821.
short: P. Ghosh, R. Schoch, M. Bauer, A. Jacobi von Wangelin, Angewandte Chemie
International Edition 61 (2021).
date_created: 2023-01-30T16:48:53Z
date_updated: 2023-01-31T08:05:26Z
department:
- _id: '35'
- _id: '306'
doi: 10.1002/anie.202110821
intvolume: ' 61'
issue: '1'
keyword:
- General Chemistry
- Catalysis
language:
- iso: eng
publication: Angewandte Chemie International Edition
publication_identifier:
issn:
- 1433-7851
- 1521-3773
publication_status: published
publisher: Wiley
status: public
title: Selective Benzylic CH‐Borylations by Tandem Cobalt Catalysis
type: journal_article
user_id: '48467'
volume: 61
year: '2021'
...
---
_id: '41013'
abstract:
- lang: eng
text: Within this article, it is shown that an electrochemical defluorination and
additional fluorination of Ruddlesden–Popper-type La2NiO3F2 is possible within
all-solid-state fluoride-ion batteries. Structural changes within the reduced
and oxidized phases have been examined by X-ray diffraction studies at different
states of charging and discharging. The synthesis of the oxidized phase La2NiO3F2+x
proved to be successful by structural analysis using both X-ray powder diffraction
and automated electron diffraction tomography techniques. The structural reversibility
on re-fluorinating and re-defluorinating is also demonstrated. Moreover, the influence
of different sequences of consecutive reduction and oxidation steps on the formed
phases has been investigated. The observed structural changes have been compared
to changes in phases obtained via other topochemical modification approaches such
as hydride-based reduction and oxidative fluorination using F2 gas, highlighting
the potential of such electrochemical reactions as alternative synthesis routes.
Furthermore, the electrochemical routes represent safe and controllable synthesis
approaches for novel phases, which cannot be synthesized via other topochemical
methods. Additionally, side reactions, occurring alongside the desired electrochemical
reactions, have been addressed and the cycling performance has been studied.
article_type: original
author:
- first_name: Kerstin
full_name: Wissel, Kerstin
last_name: Wissel
- first_name: Roland
full_name: Schoch, Roland
id: '48467'
last_name: Schoch
orcid: 0000-0003-2061-7289
- first_name: Tobias
full_name: Vogel, Tobias
last_name: Vogel
- first_name: Manuel
full_name: Donzelli, Manuel
last_name: Donzelli
- first_name: Galina
full_name: Matveeva, Galina
last_name: Matveeva
- first_name: Ute
full_name: Kolb, Ute
last_name: Kolb
- first_name: Matthias
full_name: Bauer, Matthias
id: '47241'
last_name: Bauer
orcid: 0000-0002-9294-6076
- first_name: Peter R.
full_name: Slater, Peter R.
last_name: Slater
- first_name: Oliver
full_name: Clemens, Oliver
last_name: Clemens
citation:
ama: Wissel K, Schoch R, Vogel T, et al. Electrochemical Reduction and Oxidation
of Ruddlesden–Popper-Type La2NiO3F2 within Fluoride-Ion
Batteries. Chemistry of Materials. 2021;33(2):499-512. doi:10.1021/acs.chemmater.0c01762
apa: Wissel, K., Schoch, R., Vogel, T., Donzelli, M., Matveeva, G., Kolb, U., Bauer,
M., Slater, P. R., & Clemens, O. (2021). Electrochemical Reduction and Oxidation
of Ruddlesden–Popper-Type La2NiO3F2 within Fluoride-Ion
Batteries. Chemistry of Materials, 33(2), 499–512. https://doi.org/10.1021/acs.chemmater.0c01762
bibtex: '@article{Wissel_Schoch_Vogel_Donzelli_Matveeva_Kolb_Bauer_Slater_Clemens_2021,
title={Electrochemical Reduction and Oxidation of Ruddlesden–Popper-Type La2NiO3F2
within Fluoride-Ion Batteries}, volume={33}, DOI={10.1021/acs.chemmater.0c01762},
number={2}, journal={Chemistry of Materials}, publisher={American Chemical Society
(ACS)}, author={Wissel, Kerstin and Schoch, Roland and Vogel, Tobias and Donzelli,
Manuel and Matveeva, Galina and Kolb, Ute and Bauer, Matthias and Slater, Peter
R. and Clemens, Oliver}, year={2021}, pages={499–512} }'
chicago: 'Wissel, Kerstin, Roland Schoch, Tobias Vogel, Manuel Donzelli, Galina
Matveeva, Ute Kolb, Matthias Bauer, Peter R. Slater, and Oliver Clemens. “Electrochemical
Reduction and Oxidation of Ruddlesden–Popper-Type La2NiO3F2
within Fluoride-Ion Batteries.” Chemistry of Materials 33, no. 2 (2021):
499–512. https://doi.org/10.1021/acs.chemmater.0c01762.'
ieee: 'K. Wissel et al., “Electrochemical Reduction and Oxidation of Ruddlesden–Popper-Type
La2NiO3F2 within Fluoride-Ion Batteries,” Chemistry
of Materials, vol. 33, no. 2, pp. 499–512, 2021, doi: 10.1021/acs.chemmater.0c01762.'
mla: Wissel, Kerstin, et al. “Electrochemical Reduction and Oxidation of Ruddlesden–Popper-Type
La2NiO3F2 within Fluoride-Ion Batteries.” Chemistry
of Materials, vol. 33, no. 2, American Chemical Society (ACS), 2021, pp. 499–512,
doi:10.1021/acs.chemmater.0c01762.
short: K. Wissel, R. Schoch, T. Vogel, M. Donzelli, G. Matveeva, U. Kolb, M. Bauer,
P.R. Slater, O. Clemens, Chemistry of Materials 33 (2021) 499–512.
date_created: 2023-01-30T17:01:00Z
date_updated: 2023-01-31T08:07:28Z
department:
- _id: '35'
- _id: '306'
doi: 10.1021/acs.chemmater.0c01762
intvolume: ' 33'
issue: '2'
keyword:
- Materials Chemistry
- General Chemical Engineering
- General Chemistry
language:
- iso: eng
page: 499-512
publication: Chemistry of Materials
publication_identifier:
issn:
- 0897-4756
- 1520-5002
publication_status: published
publisher: American Chemical Society (ACS)
status: public
title: Electrochemical Reduction and Oxidation of Ruddlesden–Popper-Type La2NiO3F2
within Fluoride-Ion Batteries
type: journal_article
user_id: '48467'
volume: 33
year: '2021'
...
---
_id: '41010'
abstract:
- lang: eng
text: We present the η3-coordination of the 2-phosphaethynthiolate anion in the
complex (PN)2La(SCP) (2) [PN=N-(2-(diisopropylphosphanyl)-4-methylphenyl)-2,4,6-trimethylanilide)].
Structural comparison with dinuclear thiocyanate-bridged (PN)2La(μ-1,3-SCN)2La(PN)2
(3) and azide-bridged (PN)2La(μ-1,3-N3)2La(PN)2 (4) complexes indicates that the
[SCP]− coordination mode is mainly governed by electronic, rather than steric
factors. Quantum mechanical investigations reveal large contributions of the antibonding
π*-orbital of the [SCP]− ligand to the LUMO of complex 2, rendering it the ideal
precursor for the first functionalization of the [SCP]− anion. Complex 2 was therefore
reacted with CAACs which induced a selective rearrangement of the [SCP]− ligand
to form the first CAAC stabilized group 15–group 16 fulminate-type complexes (PN)2La{SPC(RCAAC)}
(5 a,b, R=Ad, Me). A detailed reaction mechanism for the SCP-to-SPC isomerization
is proposed based on DFT calculations.
article_type: original
author:
- first_name: Fabian A.
full_name: Watt, Fabian A.
last_name: Watt
- first_name: Lukas
full_name: Burkhardt, Lukas
last_name: Burkhardt
- first_name: Roland
full_name: Schoch, Roland
id: '48467'
last_name: Schoch
orcid: 0000-0003-2061-7289
- first_name: Stefan
full_name: Mitzinger, Stefan
last_name: Mitzinger
- first_name: Matthias
full_name: Bauer, Matthias
id: '47241'
last_name: Bauer
orcid: 0000-0002-9294-6076
- first_name: Florian
full_name: Weigend, Florian
last_name: Weigend
- first_name: Jose M.
full_name: Goicoechea, Jose M.
last_name: Goicoechea
- first_name: Frank
full_name: Tambornino, Frank
last_name: Tambornino
- first_name: Stephan
full_name: Hohloch, Stephan
last_name: Hohloch
citation:
ama: Watt FA, Burkhardt L, Schoch R, et al. η 3
‐Coordination and Functionalization of the 2‐Phosphaethynthiolate Anion at Lanthanum(III)**.
Angewandte Chemie International Edition. 2021;60(17):9534-9539. doi:10.1002/anie.202100559
apa: Watt, F. A., Burkhardt, L., Schoch, R., Mitzinger, S., Bauer, M., Weigend,
F., Goicoechea, J. M., Tambornino, F., & Hohloch, S. (2021). η
3 ‐Coordination and Functionalization of the 2‐Phosphaethynthiolate
Anion at Lanthanum(III)**. Angewandte Chemie International Edition, 60(17),
9534–9539. https://doi.org/10.1002/anie.202100559
bibtex: '@article{Watt_Burkhardt_Schoch_Mitzinger_Bauer_Weigend_Goicoechea_Tambornino_Hohloch_2021,
title={η 3 ‐Coordination and Functionalization
of the 2‐Phosphaethynthiolate Anion at Lanthanum(III)**}, volume={60}, DOI={10.1002/anie.202100559}, number={17},
journal={Angewandte Chemie International Edition}, publisher={Wiley}, author={Watt,
Fabian A. and Burkhardt, Lukas and Schoch, Roland and Mitzinger, Stefan and Bauer,
Matthias and Weigend, Florian and Goicoechea, Jose M. and Tambornino, Frank and
Hohloch, Stephan}, year={2021}, pages={9534–9539} }'
chicago: 'Watt, Fabian A., Lukas Burkhardt, Roland Schoch, Stefan Mitzinger, Matthias
Bauer, Florian Weigend, Jose M. Goicoechea, Frank Tambornino, and Stephan Hohloch.
“η 3 ‐Coordination and Functionalization of the
2‐Phosphaethynthiolate Anion at Lanthanum(III)**.” Angewandte Chemie International
Edition 60, no. 17 (2021): 9534–39. https://doi.org/10.1002/anie.202100559.'
ieee: 'F. A. Watt et al., “η 3 ‐Coordination
and Functionalization of the 2‐Phosphaethynthiolate Anion at Lanthanum(III)**,”
Angewandte Chemie International Edition, vol. 60, no. 17, pp. 9534–9539,
2021, doi: 10.1002/anie.202100559.'
mla: Watt, Fabian A., et al. “η 3 ‐Coordination
and Functionalization of the 2‐Phosphaethynthiolate Anion at Lanthanum(III)**.”
Angewandte Chemie International Edition, vol. 60, no. 17, Wiley, 2021,
pp. 9534–39, doi:10.1002/anie.202100559.
short: F.A. Watt, L. Burkhardt, R. Schoch, S. Mitzinger, M. Bauer, F. Weigend, J.M.
Goicoechea, F. Tambornino, S. Hohloch, Angewandte Chemie International Edition
60 (2021) 9534–9539.
date_created: 2023-01-30T17:00:21Z
date_updated: 2023-01-31T08:06:50Z
department:
- _id: '35'
- _id: '306'
doi: 10.1002/anie.202100559
intvolume: ' 60'
issue: '17'
keyword:
- General Chemistry
- Catalysis
language:
- iso: eng
page: 9534-9539
publication: Angewandte Chemie International Edition
publication_identifier:
issn:
- 1433-7851
- 1521-3773
publication_status: published
publisher: Wiley
status: public
title: η 3 ‐Coordination and Functionalization of
the 2‐Phosphaethynthiolate Anion at Lanthanum(III)**
type: journal_article
user_id: '48467'
volume: 60
year: '2021'
...