[{"date_created":"2024-03-08T06:27:10Z","publisher":"The Electrochemical Society","title":"Electrochemical Removal of HF from Carbonate-based LiPF6-containing Li-ion Battery Electrolytes","quality_controlled":"1","year":"2024","language":[{"iso":"eng"}],"keyword":["Materials Chemistry","Electrochemistry","Surfaces","Coatings and Films","Condensed Matter Physics","Renewable Energy","Sustainability and the Environment","Electronic","Optical and Magnetic Materials"],"publication":"Journal of The Electrochemical Society","abstract":[{"text":"Due to the hydrolytic instability of LiPF6 in carbonate-based solvents, HF is a typical impurity in Li-ion battery electrolytes. HF significantly influences the performance of Li-ion batteries, for example by impacting the formation of the solid electrolyte interphase at the anode and by affecting transition metal dissolution at the cathode. Additionally, HF complicates studying fundamental interfacial electrochemistry of Li-ion battery electrolytes, such as direct anion reduction, because it is electrocatalytically relatively unstable, resulting in LiF passivation layers. Methods to selectively remove ppm levels of HF from LiPF6-containing carbonate-based electrolytes are limited. We introduce and benchmark a simple yet efficient electrochemical in situ method to selectively remove ppm amounts of HF from LiPF6-containing carbonate-based electrolytes. The basic idea is the application of a suitable potential to a high surface-area metallic electrode upon which only HF reacts (electrocatalytically) while all other electrolyte components are unaffected under the respective conditions.","lang":"eng"}],"volume":171,"author":[{"full_name":"Ge, Xiaokun","last_name":"Ge","first_name":"Xiaokun"},{"first_name":"Marten","full_name":"Huck, Marten","last_name":"Huck"},{"first_name":"Andreas","full_name":"Kuhlmann, Andreas","last_name":"Kuhlmann"},{"first_name":"Michael","last_name":"Tiemann","orcid":"0000-0003-1711-2722","id":"23547","full_name":"Tiemann, Michael"},{"first_name":"Christian","last_name":"Weinberger","id":"11848","full_name":"Weinberger, Christian"},{"full_name":"Xu, Xiaodan","last_name":"Xu","first_name":"Xiaodan"},{"first_name":"Zhenyu","last_name":"Zhao","full_name":"Zhao, Zhenyu"},{"first_name":"Hans-Georg","last_name":"Steinrueck","full_name":"Steinrueck, Hans-Georg"}],"date_updated":"2024-03-25T17:01:09Z","oa":"1","doi":"10.1149/1945-7111/ad30d3","main_file_link":[{"url":"https://dx.doi.org/10.1149/1945-7111/ad30d3","open_access":"1"}],"publication_identifier":{"issn":["0013-4651","1945-7111"]},"publication_status":"published","page":"030552","intvolume":"       171","citation":{"apa":"Ge, X., Huck, M., Kuhlmann, A., Tiemann, M., Weinberger, C., Xu, X., Zhao, Z., &#38; Steinrueck, H.-G. (2024). Electrochemical Removal of HF from Carbonate-based LiPF6-containing Li-ion Battery Electrolytes. <i>Journal of The Electrochemical Society</i>, <i>171</i>, 030552. <a href=\"https://doi.org/10.1149/1945-7111/ad30d3\">https://doi.org/10.1149/1945-7111/ad30d3</a>","short":"X. Ge, M. Huck, A. Kuhlmann, M. Tiemann, C. Weinberger, X. Xu, Z. Zhao, H.-G. Steinrueck, Journal of The Electrochemical Society 171 (2024) 030552.","bibtex":"@article{Ge_Huck_Kuhlmann_Tiemann_Weinberger_Xu_Zhao_Steinrueck_2024, title={Electrochemical Removal of HF from Carbonate-based LiPF6-containing Li-ion Battery Electrolytes}, volume={171}, DOI={<a href=\"https://doi.org/10.1149/1945-7111/ad30d3\">10.1149/1945-7111/ad30d3</a>}, journal={Journal of The Electrochemical Society}, publisher={The Electrochemical Society}, author={Ge, Xiaokun and Huck, Marten and Kuhlmann, Andreas and Tiemann, Michael and Weinberger, Christian and Xu, Xiaodan and Zhao, Zhenyu and Steinrueck, Hans-Georg}, year={2024}, pages={030552} }","mla":"Ge, Xiaokun, et al. “Electrochemical Removal of HF from Carbonate-Based LiPF6-Containing Li-Ion Battery Electrolytes.” <i>Journal of The Electrochemical Society</i>, vol. 171, The Electrochemical Society, 2024, p. 030552, doi:<a href=\"https://doi.org/10.1149/1945-7111/ad30d3\">10.1149/1945-7111/ad30d3</a>.","ieee":"X. Ge <i>et al.</i>, “Electrochemical Removal of HF from Carbonate-based LiPF6-containing Li-ion Battery Electrolytes,” <i>Journal of The Electrochemical Society</i>, vol. 171, p. 030552, 2024, doi: <a href=\"https://doi.org/10.1149/1945-7111/ad30d3\">10.1149/1945-7111/ad30d3</a>.","chicago":"Ge, Xiaokun, Marten Huck, Andreas Kuhlmann, Michael Tiemann, Christian Weinberger, Xiaodan Xu, Zhenyu Zhao, and Hans-Georg Steinrueck. “Electrochemical Removal of HF from Carbonate-Based LiPF6-Containing Li-Ion Battery Electrolytes.” <i>Journal of The Electrochemical Society</i> 171 (2024): 030552. <a href=\"https://doi.org/10.1149/1945-7111/ad30d3\">https://doi.org/10.1149/1945-7111/ad30d3</a>.","ama":"Ge X, Huck M, Kuhlmann A, et al. Electrochemical Removal of HF from Carbonate-based LiPF6-containing Li-ion Battery Electrolytes. <i>Journal of The Electrochemical Society</i>. 2024;171:030552. doi:<a href=\"https://doi.org/10.1149/1945-7111/ad30d3\">10.1149/1945-7111/ad30d3</a>"},"department":[{"_id":"35"},{"_id":"2"},{"_id":"307"}],"user_id":"23547","_id":"52372","article_type":"original","type":"journal_article","status":"public"},{"user_id":"89054","department":[{"_id":"35"},{"_id":"306"}],"_id":"40981","language":[{"iso":"eng"}],"article_number":"010526","keyword":["Materials Chemistry","Electrochemistry","Surfaces","Coatings and Films","Condensed Matter Physics","Renewable Energy","Sustainability and the Environment","Electronic","Optical and Magnetic Materials"],"type":"journal_article","publication":"Journal of The Electrochemical Society","status":"public","abstract":[{"lang":"eng","text":"Room temperature sodium-sulfur (RT Na-S) batteries are considered potential candidates for stationary power storage applications due to their low cost, broad active material availability and low toxicity. Challenges, such as high volume expansion of the S-cathode upon discharge, low electronic conductivity of S as active material and herewith limited rate capability as well as the shuttling of polysulfides (PSs) as intermediates often impede the cycle stability and practical application of Na-S batteries. Sulfurized poly(acrylonitrile) (SPAN) inherently inhibits the shuttling of PSs and shows compatibility with carbonate-based electrolytes, however, its exact redox mechanism remained unclear to date. Herein, we implement a commercially available and simple electrolyte into the Na-SPAN cell chemistry and demonstrate its high rate and cycle stability. Through the application of in situ techniques utilizing electronic impedance spectroscopy (EIS) and X-ray absorption spectroscopy (XAS) at different depths of charge and discharge, an insight into SPAN’s redox chemistry is obtained."}],"date_created":"2023-01-30T16:08:15Z","author":[{"first_name":"Julian","full_name":"Kappler, Julian","last_name":"Kappler"},{"orcid":"0000-0002-0999-9995","last_name":"Tonbul","full_name":"Tonbul, Güldeniz","id":"89054","first_name":"Güldeniz"},{"first_name":"Roland","last_name":"Schoch","orcid":"0000-0003-2061-7289","full_name":"Schoch, Roland","id":"48467"},{"first_name":"Saravanakumar","last_name":"Murugan","full_name":"Murugan, Saravanakumar"},{"last_name":"Nowakowski","orcid":"0000-0002-3734-7011","id":"78878","full_name":"Nowakowski, Michał","first_name":"Michał"},{"last_name":"Lange","full_name":"Lange, Pia Lena","first_name":"Pia Lena"},{"full_name":"Klostermann, Sina Vanessa","last_name":"Klostermann","first_name":"Sina Vanessa"},{"orcid":"0000-0002-9294-6076","last_name":"Bauer","id":"47241","full_name":"Bauer, Matthias","first_name":"Matthias"},{"last_name":"Schleid","full_name":"Schleid, Thomas","first_name":"Thomas"},{"first_name":"Johannes","last_name":"Kästner","full_name":"Kästner, Johannes"},{"last_name":"Buchmeiser","full_name":"Buchmeiser, Michael Rudolf","first_name":"Michael Rudolf"}],"volume":170,"date_updated":"2023-05-03T08:27:13Z","publisher":"The Electrochemical Society","doi":"10.1149/1945-7111/acb2fa","title":"Understanding the Redox Mechanism of Sulfurized Poly(acrylonitrile) as Highly Rate and Cycle Stable Cathode Material for Sodium-Sulfur Batteries","issue":"1","publication_status":"published","publication_identifier":{"issn":["0013-4651","1945-7111"]},"citation":{"apa":"Kappler, J., Tonbul, G., Schoch, R., Murugan, S., Nowakowski, M., Lange, P. L., Klostermann, S. V., Bauer, M., Schleid, T., Kästner, J., &#38; Buchmeiser, M. R. (2023). Understanding the Redox Mechanism of Sulfurized Poly(acrylonitrile) as Highly Rate and Cycle Stable Cathode Material for Sodium-Sulfur Batteries. <i>Journal of The Electrochemical Society</i>, <i>170</i>(1), Article 010526. <a href=\"https://doi.org/10.1149/1945-7111/acb2fa\">https://doi.org/10.1149/1945-7111/acb2fa</a>","bibtex":"@article{Kappler_Tonbul_Schoch_Murugan_Nowakowski_Lange_Klostermann_Bauer_Schleid_Kästner_et al._2023, title={Understanding the Redox Mechanism of Sulfurized Poly(acrylonitrile) as Highly Rate and Cycle Stable Cathode Material for Sodium-Sulfur Batteries}, volume={170}, DOI={<a href=\"https://doi.org/10.1149/1945-7111/acb2fa\">10.1149/1945-7111/acb2fa</a>}, number={1010526}, journal={Journal of The Electrochemical Society}, publisher={The Electrochemical Society}, author={Kappler, Julian and Tonbul, Güldeniz and Schoch, Roland and Murugan, Saravanakumar and Nowakowski, Michał and Lange, Pia Lena and Klostermann, Sina Vanessa and Bauer, Matthias and Schleid, Thomas and Kästner, Johannes and et al.}, year={2023} }","mla":"Kappler, Julian, et al. “Understanding the Redox Mechanism of Sulfurized Poly(Acrylonitrile) as Highly Rate and Cycle Stable Cathode Material for Sodium-Sulfur Batteries.” <i>Journal of The Electrochemical Society</i>, vol. 170, no. 1, 010526, The Electrochemical Society, 2023, doi:<a href=\"https://doi.org/10.1149/1945-7111/acb2fa\">10.1149/1945-7111/acb2fa</a>.","short":"J. Kappler, G. Tonbul, R. Schoch, S. Murugan, M. Nowakowski, P.L. Lange, S.V. Klostermann, M. Bauer, T. Schleid, J. Kästner, M.R. Buchmeiser, Journal of The Electrochemical Society 170 (2023).","ama":"Kappler J, Tonbul G, Schoch R, et al. Understanding the Redox Mechanism of Sulfurized Poly(acrylonitrile) as Highly Rate and Cycle Stable Cathode Material for Sodium-Sulfur Batteries. <i>Journal of The Electrochemical Society</i>. 2023;170(1). doi:<a href=\"https://doi.org/10.1149/1945-7111/acb2fa\">10.1149/1945-7111/acb2fa</a>","chicago":"Kappler, Julian, Güldeniz Tonbul, Roland Schoch, Saravanakumar Murugan, Michał Nowakowski, Pia Lena Lange, Sina Vanessa Klostermann, et al. “Understanding the Redox Mechanism of Sulfurized Poly(Acrylonitrile) as Highly Rate and Cycle Stable Cathode Material for Sodium-Sulfur Batteries.” <i>Journal of The Electrochemical Society</i> 170, no. 1 (2023). <a href=\"https://doi.org/10.1149/1945-7111/acb2fa\">https://doi.org/10.1149/1945-7111/acb2fa</a>.","ieee":"J. Kappler <i>et al.</i>, “Understanding the Redox Mechanism of Sulfurized Poly(acrylonitrile) as Highly Rate and Cycle Stable Cathode Material for Sodium-Sulfur Batteries,” <i>Journal of The Electrochemical Society</i>, vol. 170, no. 1, Art. no. 010526, 2023, doi: <a href=\"https://doi.org/10.1149/1945-7111/acb2fa\">10.1149/1945-7111/acb2fa</a>."},"intvolume":"       170","year":"2023"},{"language":[{"iso":"eng"}],"keyword":["Materials Chemistry","Electrochemistry","Surfaces","Coatings and Films","Condensed Matter Physics","Renewable Energy","Sustainability and the Environment","Electronic","Optical and Magnetic Materials"],"user_id":"84268","department":[{"_id":"633"}],"_id":"30920","status":"public","abstract":[{"lang":"eng","text":"<jats:title>Abstract</jats:title>\r\n               <jats:p>Batteries capable of extreme fast-charging (XFC) are a necessity for the deployment of electric vehicles. Material properties of electrodes and electrolytes along with cell parameters such as stack pressure and temperature have coupled, synergistic, and sometimes deleterious effects on fast-charging performance. We develop a new experimental testbed that allows precise and conformal application of electrode stack pressure. We focus on cell capacity degradation using single-layer pouch cells with graphite anodes, LiNi0.5Mn0.3Co0.2O2 (NMC532) cathodes, and carbonate-based electrolyte. In the tested range (10 – 125 psi), cells cycled at higher pressure show higher capacity and less capacity fading. Additionally, Li plating decreases with increasing pressure as observed with scanning electron microscopy (SEM) and optical imaging. While the loss of Li inventory from Li plating is the largest contributor to capacity fade, electrochemical and SEM examination of the NMC cathodes after XFC experiments show increased secondary particle damage at lower pressure. We infer that the better performance at higher pressure is due to more homogenous reactions of active materials across the electrode and less polarization through the electrode thickness. Our study emphasizes the importance of electrode stack pressure in XFC batteries and highlights its subtle role in cell conditions.</jats:p>"}],"type":"journal_article","publication":"Journal of The Electrochemical Society","doi":"10.1149/1945-7111/ac653f","title":"Conformal Pressure and Fast-Charging Li-Ion Batteries","author":[{"full_name":"Cao, Chuntian","last_name":"Cao","first_name":"Chuntian"},{"first_name":"Hans-Georg","full_name":"Steinrück, Hans-Georg","id":"84268","last_name":"Steinrück","orcid":"0000-0001-6373-0877"},{"first_name":"Partha P","last_name":"Paul","full_name":"Paul, Partha P"},{"first_name":"Alison R.","full_name":"Dunlop, Alison R.","last_name":"Dunlop"},{"first_name":"Stephen E.","last_name":"Trask","full_name":"Trask, Stephen E."},{"first_name":"Andrew","full_name":"Jansen, Andrew","last_name":"Jansen"},{"first_name":"Robert M","last_name":"Kasse","full_name":"Kasse, Robert M"},{"first_name":"Vivek","last_name":"Thampy","full_name":"Thampy, Vivek"},{"last_name":"Yusuf","full_name":"Yusuf, Maha","first_name":"Maha"},{"first_name":"Johanna","full_name":"Nelson Weker, Johanna","last_name":"Nelson Weker"},{"full_name":"Shyam, Badri","last_name":"Shyam","first_name":"Badri"},{"last_name":"Subbaraman","full_name":"Subbaraman, Ram","first_name":"Ram"},{"last_name":"Davis","full_name":"Davis, Kelly","first_name":"Kelly"},{"first_name":"Christina M","full_name":"Johnston, Christina M","last_name":"Johnston"},{"first_name":"Christopher J","last_name":"Takacs","full_name":"Takacs, Christopher J"},{"full_name":"Toney, Michael","last_name":"Toney","first_name":"Michael"}],"date_created":"2022-04-20T06:37:40Z","volume":169,"date_updated":"2022-04-20T06:38:37Z","publisher":"The Electrochemical Society","citation":{"ieee":"C. Cao <i>et al.</i>, “Conformal Pressure and Fast-Charging Li-Ion Batteries,” <i>Journal of The Electrochemical Society</i>, vol. 169, p. 040540, 2022, doi: <a href=\"https://doi.org/10.1149/1945-7111/ac653f\">10.1149/1945-7111/ac653f</a>.","chicago":"Cao, Chuntian, Hans-Georg Steinrück, Partha P Paul, Alison R. Dunlop, Stephen E. Trask, Andrew Jansen, Robert M Kasse, et al. “Conformal Pressure and Fast-Charging Li-Ion Batteries.” <i>Journal of The Electrochemical Society</i> 169 (2022): 040540. <a href=\"https://doi.org/10.1149/1945-7111/ac653f\">https://doi.org/10.1149/1945-7111/ac653f</a>.","ama":"Cao C, Steinrück H-G, Paul PP, et al. Conformal Pressure and Fast-Charging Li-Ion Batteries. <i>Journal of The Electrochemical Society</i>. 2022;169:040540. doi:<a href=\"https://doi.org/10.1149/1945-7111/ac653f\">10.1149/1945-7111/ac653f</a>","apa":"Cao, C., Steinrück, H.-G., Paul, P. P., Dunlop, A. R., Trask, S. E., Jansen, A., Kasse, R. M., Thampy, V., Yusuf, M., Nelson Weker, J., Shyam, B., Subbaraman, R., Davis, K., Johnston, C. M., Takacs, C. J., &#38; Toney, M. (2022). Conformal Pressure and Fast-Charging Li-Ion Batteries. <i>Journal of The Electrochemical Society</i>, <i>169</i>, 040540. <a href=\"https://doi.org/10.1149/1945-7111/ac653f\">https://doi.org/10.1149/1945-7111/ac653f</a>","bibtex":"@article{Cao_Steinrück_Paul_Dunlop_Trask_Jansen_Kasse_Thampy_Yusuf_Nelson Weker_et al._2022, title={Conformal Pressure and Fast-Charging Li-Ion Batteries}, volume={169}, DOI={<a href=\"https://doi.org/10.1149/1945-7111/ac653f\">10.1149/1945-7111/ac653f</a>}, journal={Journal of The Electrochemical Society}, publisher={The Electrochemical Society}, author={Cao, Chuntian and Steinrück, Hans-Georg and Paul, Partha P and Dunlop, Alison R. and Trask, Stephen E. and Jansen, Andrew and Kasse, Robert M and Thampy, Vivek and Yusuf, Maha and Nelson Weker, Johanna and et al.}, year={2022}, pages={040540} }","mla":"Cao, Chuntian, et al. “Conformal Pressure and Fast-Charging Li-Ion Batteries.” <i>Journal of The Electrochemical Society</i>, vol. 169, The Electrochemical Society, 2022, p. 040540, doi:<a href=\"https://doi.org/10.1149/1945-7111/ac653f\">10.1149/1945-7111/ac653f</a>.","short":"C. Cao, H.-G. Steinrück, P.P. Paul, A.R. Dunlop, S.E. Trask, A. Jansen, R.M. Kasse, V. Thampy, M. Yusuf, J. Nelson Weker, B. Shyam, R. Subbaraman, K. Davis, C.M. Johnston, C.J. Takacs, M. Toney, Journal of The Electrochemical Society 169 (2022) 040540."},"intvolume":"       169","page":"040540","year":"2022","publication_status":"published","publication_identifier":{"issn":["0013-4651","1945-7111"]}},{"user_id":"48864","department":[{"_id":"302"}],"_id":"32432","language":[{"iso":"eng"}],"keyword":["Electrochemistry","Spectroscopy","Surfaces and Interfaces","Condensed Matter Physics","General Materials Science"],"type":"journal_article","publication":"Langmuir","status":"public","date_created":"2022-07-27T07:45:51Z","author":[{"last_name":"Yang","full_name":"Yang, Yu","first_name":"Yu"},{"full_name":"Huang, Jingyuan","last_name":"Huang","first_name":"Jingyuan"},{"first_name":"Daniel","full_name":"Dornbusch, Daniel","last_name":"Dornbusch"},{"last_name":"Grundmeier","id":"194","full_name":"Grundmeier, Guido","first_name":"Guido"},{"full_name":"Fahmy, Karim","last_name":"Fahmy","first_name":"Karim"},{"full_name":"Keller, Adrian","id":"48864","last_name":"Keller","orcid":"0000-0001-7139-3110","first_name":"Adrian"},{"full_name":"Cheung, David L.","last_name":"Cheung","first_name":"David L."}],"volume":38,"publisher":"American Chemical Society (ACS)","date_updated":"2022-08-08T06:39:04Z","doi":"10.1021/acs.langmuir.2c01016","title":"Effect of Surface Hydrophobicity on the Adsorption of a Pilus-Derived Adhesin-like Peptide","publication_status":"published","publication_identifier":{"issn":["0743-7463","1520-5827"]},"citation":{"ama":"Yang Y, Huang J, Dornbusch D, et al. Effect of Surface Hydrophobicity on the Adsorption of a Pilus-Derived Adhesin-like Peptide. <i>Langmuir</i>. 2022;38:9257–9265. doi:<a href=\"https://doi.org/10.1021/acs.langmuir.2c01016\">10.1021/acs.langmuir.2c01016</a>","ieee":"Y. Yang <i>et al.</i>, “Effect of Surface Hydrophobicity on the Adsorption of a Pilus-Derived Adhesin-like Peptide,” <i>Langmuir</i>, vol. 38, pp. 9257–9265, 2022, doi: <a href=\"https://doi.org/10.1021/acs.langmuir.2c01016\">10.1021/acs.langmuir.2c01016</a>.","chicago":"Yang, Yu, Jingyuan Huang, Daniel Dornbusch, Guido Grundmeier, Karim Fahmy, Adrian Keller, and David L. Cheung. “Effect of Surface Hydrophobicity on the Adsorption of a Pilus-Derived Adhesin-like Peptide.” <i>Langmuir</i> 38 (2022): 9257–9265. <a href=\"https://doi.org/10.1021/acs.langmuir.2c01016\">https://doi.org/10.1021/acs.langmuir.2c01016</a>.","mla":"Yang, Yu, et al. “Effect of Surface Hydrophobicity on the Adsorption of a Pilus-Derived Adhesin-like Peptide.” <i>Langmuir</i>, vol. 38, American Chemical Society (ACS), 2022, pp. 9257–9265, doi:<a href=\"https://doi.org/10.1021/acs.langmuir.2c01016\">10.1021/acs.langmuir.2c01016</a>.","bibtex":"@article{Yang_Huang_Dornbusch_Grundmeier_Fahmy_Keller_Cheung_2022, title={Effect of Surface Hydrophobicity on the Adsorption of a Pilus-Derived Adhesin-like Peptide}, volume={38}, DOI={<a href=\"https://doi.org/10.1021/acs.langmuir.2c01016\">10.1021/acs.langmuir.2c01016</a>}, journal={Langmuir}, publisher={American Chemical Society (ACS)}, author={Yang, Yu and Huang, Jingyuan and Dornbusch, Daniel and Grundmeier, Guido and Fahmy, Karim and Keller, Adrian and Cheung, David L.}, year={2022}, pages={9257–9265} }","short":"Y. Yang, J. Huang, D. Dornbusch, G. Grundmeier, K. Fahmy, A. Keller, D.L. Cheung, Langmuir 38 (2022) 9257–9265.","apa":"Yang, Y., Huang, J., Dornbusch, D., Grundmeier, G., Fahmy, K., Keller, A., &#38; Cheung, D. L. (2022). Effect of Surface Hydrophobicity on the Adsorption of a Pilus-Derived Adhesin-like Peptide. <i>Langmuir</i>, <i>38</i>, 9257–9265. <a href=\"https://doi.org/10.1021/acs.langmuir.2c01016\">https://doi.org/10.1021/acs.langmuir.2c01016</a>"},"intvolume":"        38","page":"9257–9265","year":"2022"},{"doi":"10.1021/acsaem.2c00806","title":"Combined Effects of Uniform Applied Pressure and Electrolyte Additives in Lithium-Metal Batteries","author":[{"full_name":"Kasse, Robert M.","last_name":"Kasse","first_name":"Robert M."},{"last_name":"Geise","full_name":"Geise, Natalie R.","first_name":"Natalie R."},{"first_name":"Elias","full_name":"Sebti, Elias","last_name":"Sebti"},{"first_name":"Kipil","full_name":"Lim, Kipil","last_name":"Lim"},{"last_name":"Takacs","full_name":"Takacs, Christopher J.","first_name":"Christopher J."},{"last_name":"Cao","full_name":"Cao, Chuntian","first_name":"Chuntian"},{"orcid":"0000-0001-6373-0877","last_name":"Steinrück","full_name":"Steinrück, Hans-Georg","id":"84268","first_name":"Hans-Georg"},{"first_name":"Michael F.","full_name":"Toney, Michael F.","last_name":"Toney"}],"date_created":"2022-08-09T19:57:18Z","volume":5,"publisher":"American Chemical Society (ACS)","date_updated":"2022-08-09T19:57:44Z","citation":{"ieee":"R. M. Kasse <i>et al.</i>, “Combined Effects of Uniform Applied Pressure and Electrolyte Additives in Lithium-Metal Batteries,” <i>ACS Applied Energy Materials</i>, vol. 5, no. 7, pp. 8273–8281, 2022, doi: <a href=\"https://doi.org/10.1021/acsaem.2c00806\">10.1021/acsaem.2c00806</a>.","chicago":"Kasse, Robert M., Natalie R. Geise, Elias Sebti, Kipil Lim, Christopher J. Takacs, Chuntian Cao, Hans-Georg Steinrück, and Michael F. Toney. “Combined Effects of Uniform Applied Pressure and Electrolyte Additives in Lithium-Metal Batteries.” <i>ACS Applied Energy Materials</i> 5, no. 7 (2022): 8273–81. <a href=\"https://doi.org/10.1021/acsaem.2c00806\">https://doi.org/10.1021/acsaem.2c00806</a>.","ama":"Kasse RM, Geise NR, Sebti E, et al. Combined Effects of Uniform Applied Pressure and Electrolyte Additives in Lithium-Metal Batteries. <i>ACS Applied Energy Materials</i>. 2022;5(7):8273-8281. doi:<a href=\"https://doi.org/10.1021/acsaem.2c00806\">10.1021/acsaem.2c00806</a>","short":"R.M. Kasse, N.R. Geise, E. Sebti, K. Lim, C.J. Takacs, C. Cao, H.-G. Steinrück, M.F. Toney, ACS Applied Energy Materials 5 (2022) 8273–8281.","mla":"Kasse, Robert M., et al. “Combined Effects of Uniform Applied Pressure and Electrolyte Additives in Lithium-Metal Batteries.” <i>ACS Applied Energy Materials</i>, vol. 5, no. 7, American Chemical Society (ACS), 2022, pp. 8273–81, doi:<a href=\"https://doi.org/10.1021/acsaem.2c00806\">10.1021/acsaem.2c00806</a>.","bibtex":"@article{Kasse_Geise_Sebti_Lim_Takacs_Cao_Steinrück_Toney_2022, title={Combined Effects of Uniform Applied Pressure and Electrolyte Additives in Lithium-Metal Batteries}, volume={5}, DOI={<a href=\"https://doi.org/10.1021/acsaem.2c00806\">10.1021/acsaem.2c00806</a>}, number={7}, journal={ACS Applied Energy Materials}, publisher={American Chemical Society (ACS)}, author={Kasse, Robert M. and Geise, Natalie R. and Sebti, Elias and Lim, Kipil and Takacs, Christopher J. and Cao, Chuntian and Steinrück, Hans-Georg and Toney, Michael F.}, year={2022}, pages={8273–8281} }","apa":"Kasse, R. M., Geise, N. R., Sebti, E., Lim, K., Takacs, C. J., Cao, C., Steinrück, H.-G., &#38; Toney, M. F. (2022). Combined Effects of Uniform Applied Pressure and Electrolyte Additives in Lithium-Metal Batteries. <i>ACS Applied Energy Materials</i>, <i>5</i>(7), 8273–8281. <a href=\"https://doi.org/10.1021/acsaem.2c00806\">https://doi.org/10.1021/acsaem.2c00806</a>"},"page":"8273-8281","intvolume":"         5","year":"2022","issue":"7","publication_status":"published","publication_identifier":{"issn":["2574-0962","2574-0962"]},"language":[{"iso":"eng"}],"keyword":["Electrical and Electronic Engineering","Materials Chemistry","Electrochemistry","Energy Engineering and Power Technology","Chemical Engineering (miscellaneous)"],"user_id":"84268","department":[{"_id":"633"}],"_id":"32764","status":"public","type":"journal_article","publication":"ACS Applied Energy Materials"},{"issue":"20","publication_identifier":{"issn":["1616-301X","1616-3028"]},"publication_status":"published","intvolume":"        32","citation":{"bibtex":"@article{Khazaei_Ranjbar_Kang_Liang_Khaledialidusti_Bae_Raebiger_Wang_Han_Mizoguchi_et al._2022, title={Electronic Structures of Group III–V Element Haeckelite Compounds: A Novel Family of Semiconductors, Dirac Semimetals, and Topological Insulators}, volume={32}, DOI={<a href=\"https://doi.org/10.1002/adfm.202110930\">10.1002/adfm.202110930</a>}, number={202110930}, journal={Advanced Functional Materials}, publisher={Wiley}, author={Khazaei, Mohammad and Ranjbar, Ahmad and Kang, Yoon‐Gu and Liang, Yunye and Khaledialidusti, Rasoul and Bae, Soungmin and Raebiger, Hannes and Wang, Vei and Han, Myung Joon and Mizoguchi, Hiroshi and et al.}, year={2022} }","mla":"Khazaei, Mohammad, et al. “Electronic Structures of Group III–V Element Haeckelite Compounds: A Novel Family of Semiconductors, Dirac Semimetals, and Topological Insulators.” <i>Advanced Functional Materials</i>, vol. 32, no. 20, 2110930, Wiley, 2022, doi:<a href=\"https://doi.org/10.1002/adfm.202110930\">10.1002/adfm.202110930</a>.","short":"M. Khazaei, A. Ranjbar, Y. Kang, Y. Liang, R. Khaledialidusti, S. Bae, H. Raebiger, V. Wang, M.J. Han, H. Mizoguchi, M.S. Bahramy, T. Kühne, R.V. Belosludov, K. Ohno, H. Hosono, Advanced Functional Materials 32 (2022).","apa":"Khazaei, M., Ranjbar, A., Kang, Y., Liang, Y., Khaledialidusti, R., Bae, S., Raebiger, H., Wang, V., Han, M. J., Mizoguchi, H., Bahramy, M. S., Kühne, T., Belosludov, R. V., Ohno, K., &#38; Hosono, H. (2022). Electronic Structures of Group III–V Element Haeckelite Compounds: A Novel Family of Semiconductors, Dirac Semimetals, and Topological Insulators. <i>Advanced Functional Materials</i>, <i>32</i>(20), Article 2110930. <a href=\"https://doi.org/10.1002/adfm.202110930\">https://doi.org/10.1002/adfm.202110930</a>","ieee":"M. Khazaei <i>et al.</i>, “Electronic Structures of Group III–V Element Haeckelite Compounds: A Novel Family of Semiconductors, Dirac Semimetals, and Topological Insulators,” <i>Advanced Functional Materials</i>, vol. 32, no. 20, Art. no. 2110930, 2022, doi: <a href=\"https://doi.org/10.1002/adfm.202110930\">10.1002/adfm.202110930</a>.","chicago":"Khazaei, Mohammad, Ahmad Ranjbar, Yoon‐Gu Kang, Yunye Liang, Rasoul Khaledialidusti, Soungmin Bae, Hannes Raebiger, et al. “Electronic Structures of Group III–V Element Haeckelite Compounds: A Novel Family of Semiconductors, Dirac Semimetals, and Topological Insulators.” <i>Advanced Functional Materials</i> 32, no. 20 (2022). <a href=\"https://doi.org/10.1002/adfm.202110930\">https://doi.org/10.1002/adfm.202110930</a>.","ama":"Khazaei M, Ranjbar A, Kang Y, et al. Electronic Structures of Group III–V Element Haeckelite Compounds: A Novel Family of Semiconductors, Dirac Semimetals, and Topological Insulators. <i>Advanced Functional Materials</i>. 2022;32(20). doi:<a href=\"https://doi.org/10.1002/adfm.202110930\">10.1002/adfm.202110930</a>"},"year":"2022","volume":32,"date_created":"2022-10-11T08:15:11Z","author":[{"first_name":"Mohammad","full_name":"Khazaei, Mohammad","last_name":"Khazaei"},{"first_name":"Ahmad","last_name":"Ranjbar","full_name":"Ranjbar, Ahmad"},{"last_name":"Kang","full_name":"Kang, Yoon‐Gu","first_name":"Yoon‐Gu"},{"last_name":"Liang","full_name":"Liang, Yunye","first_name":"Yunye"},{"last_name":"Khaledialidusti","full_name":"Khaledialidusti, Rasoul","first_name":"Rasoul"},{"first_name":"Soungmin","last_name":"Bae","full_name":"Bae, Soungmin"},{"first_name":"Hannes","full_name":"Raebiger, Hannes","last_name":"Raebiger"},{"full_name":"Wang, Vei","last_name":"Wang","first_name":"Vei"},{"first_name":"Myung Joon","last_name":"Han","full_name":"Han, Myung Joon"},{"first_name":"Hiroshi","last_name":"Mizoguchi","full_name":"Mizoguchi, Hiroshi"},{"full_name":"Bahramy, Mohammad S.","last_name":"Bahramy","first_name":"Mohammad S."},{"last_name":"Kühne","id":"49079","full_name":"Kühne, Thomas","first_name":"Thomas"},{"first_name":"Rodion V.","full_name":"Belosludov, Rodion V.","last_name":"Belosludov"},{"first_name":"Kaoru","last_name":"Ohno","full_name":"Ohno, Kaoru"},{"first_name":"Hideo","last_name":"Hosono","full_name":"Hosono, Hideo"}],"date_updated":"2022-10-11T08:15:28Z","publisher":"Wiley","doi":"10.1002/adfm.202110930","title":"Electronic Structures of Group III–V Element Haeckelite Compounds: A Novel Family of Semiconductors, Dirac Semimetals, and Topological Insulators","publication":"Advanced Functional Materials","type":"journal_article","status":"public","department":[{"_id":"613"}],"user_id":"71051","_id":"33682","language":[{"iso":"eng"}],"keyword":["Electrochemistry","Condensed Matter Physics","Biomaterials","Electronic","Optical and Magnetic Materials"],"article_number":"2110930"},{"date_updated":"2023-01-31T08:00:11Z","volume":38,"author":[{"first_name":"Yanyue","full_name":"Feng, Yanyue","last_name":"Feng"},{"last_name":"Schaefer","full_name":"Schaefer, Andreas","first_name":"Andreas"},{"last_name":"Hellman","full_name":"Hellman, Anders","first_name":"Anders"},{"last_name":"Di","full_name":"Di, Mengqiao","first_name":"Mengqiao"},{"full_name":"Härelind, Hanna","last_name":"Härelind","first_name":"Hanna"},{"first_name":"Matthias","last_name":"Bauer","orcid":"0000-0002-9294-6076","full_name":"Bauer, Matthias","id":"47241"},{"full_name":"Carlsson, Per-Anders","last_name":"Carlsson","first_name":"Per-Anders"}],"doi":"10.1021/acs.langmuir.2c01834","publication_identifier":{"issn":["0743-7463","1520-5827"]},"publication_status":"published","intvolume":"        38","page":"12859-12870","citation":{"bibtex":"@article{Feng_Schaefer_Hellman_Di_Härelind_Bauer_Carlsson_2022, title={Synthesis and Characterization of Catalytically Active Au Core─Pd Shell Nanoparticles Supported on Alumina}, volume={38}, DOI={<a href=\"https://doi.org/10.1021/acs.langmuir.2c01834\">10.1021/acs.langmuir.2c01834</a>}, number={42}, journal={Langmuir}, publisher={American Chemical Society (ACS)}, author={Feng, Yanyue and Schaefer, Andreas and Hellman, Anders and Di, Mengqiao and Härelind, Hanna and Bauer, Matthias and Carlsson, Per-Anders}, year={2022}, pages={12859–12870} }","mla":"Feng, Yanyue, et al. “Synthesis and Characterization of Catalytically Active Au Core─Pd Shell Nanoparticles Supported on Alumina.” <i>Langmuir</i>, vol. 38, no. 42, American Chemical Society (ACS), 2022, pp. 12859–70, doi:<a href=\"https://doi.org/10.1021/acs.langmuir.2c01834\">10.1021/acs.langmuir.2c01834</a>.","short":"Y. Feng, A. Schaefer, A. Hellman, M. Di, H. Härelind, M. Bauer, P.-A. Carlsson, Langmuir 38 (2022) 12859–12870.","apa":"Feng, Y., Schaefer, A., Hellman, A., Di, M., Härelind, H., Bauer, M., &#38; Carlsson, P.-A. (2022). Synthesis and Characterization of Catalytically Active Au Core─Pd Shell Nanoparticles Supported on Alumina. <i>Langmuir</i>, <i>38</i>(42), 12859–12870. <a href=\"https://doi.org/10.1021/acs.langmuir.2c01834\">https://doi.org/10.1021/acs.langmuir.2c01834</a>","ama":"Feng Y, Schaefer A, Hellman A, et al. Synthesis and Characterization of Catalytically Active Au Core─Pd Shell Nanoparticles Supported on Alumina. <i>Langmuir</i>. 2022;38(42):12859-12870. doi:<a href=\"https://doi.org/10.1021/acs.langmuir.2c01834\">10.1021/acs.langmuir.2c01834</a>","ieee":"Y. Feng <i>et al.</i>, “Synthesis and Characterization of Catalytically Active Au Core─Pd Shell Nanoparticles Supported on Alumina,” <i>Langmuir</i>, vol. 38, no. 42, pp. 12859–12870, 2022, doi: <a href=\"https://doi.org/10.1021/acs.langmuir.2c01834\">10.1021/acs.langmuir.2c01834</a>.","chicago":"Feng, Yanyue, Andreas Schaefer, Anders Hellman, Mengqiao Di, Hanna Härelind, Matthias Bauer, and Per-Anders Carlsson. “Synthesis and Characterization of Catalytically Active Au Core─Pd Shell Nanoparticles Supported on Alumina.” <i>Langmuir</i> 38, no. 42 (2022): 12859–70. <a href=\"https://doi.org/10.1021/acs.langmuir.2c01834\">https://doi.org/10.1021/acs.langmuir.2c01834</a>."},"_id":"40984","department":[{"_id":"35"},{"_id":"306"}],"user_id":"48467","type":"journal_article","status":"public","publisher":"American Chemical Society (ACS)","date_created":"2023-01-30T16:22:57Z","title":"Synthesis and Characterization of Catalytically Active Au Core─Pd Shell Nanoparticles Supported on Alumina","issue":"42","year":"2022","keyword":["Electrochemistry","Spectroscopy","Surfaces and Interfaces","Condensed Matter Physics","General Materials Science"],"language":[{"iso":"eng"}],"publication":"Langmuir","abstract":[{"lang":"eng","text":"A two-step seeded-growth method was refined to synthesize Au@Pd core@shell nanoparticles with thin Pd shells, which were then deposited onto alumina to obtain a supported Au@Pd/Al2O3 catalyst active for prototypical CO oxidation. By the strict control of temperature and Pd/Au molar ratio and the use of l-ascorbic acid for making both Au cores and Pd shells, a 1.5 nm Pd layer is formed around the Au core, as evidenced by transmission electron microscopy and energy-dispersive spectroscopy. The core@shell structure and the Pd shell remain intact upon deposition onto alumina and after being used for CO oxidation, as revealed by additional X-ray diffraction and X-ray photoemission spectroscopy before and after the reaction. The Pd shell surface was characterized with in situ infrared (IR) spectroscopy using CO as a chemical probe during CO adsorption–desorption. The IR bands for CO ad-species on the Pd shell suggest that the shell exposes mostly low-index surfaces, likely Pd(111) as the majority facet. Generally, the IR bands are blue-shifted as compared to conventional Pd/alumina catalysts, which may be due to the different support materials for Pd, Au versus Al2O3, and/or less strain of the Pd shell. Frequencies obtained from density functional calculations suggest the latter to be significant. Further, the catalytic CO oxidation ignition-extinction processes were followed by in situ IR, which shows the common CO poisoning and kinetic behavior associated with competitive adsorption of CO and O2 that is typically observed for noble metal catalysts."}]},{"title":"PtRu nanoparticles supported on noble carbons for ethanol electrooxidation","doi":"10.1016/j.jechem.2021.07.004","date_updated":"2023-01-27T16:36:12Z","publisher":"Elsevier BV","volume":66,"author":[{"first_name":"Alberto","full_name":"Rodríguez-Gómez, Alberto","last_name":"Rodríguez-Gómez"},{"last_name":"Lepre","full_name":"Lepre, Enrico","first_name":"Enrico"},{"last_name":"Sánchez-Silva","full_name":"Sánchez-Silva, Luz","first_name":"Luz"},{"last_name":"Lopez Salas","orcid":"https://orcid.org/0000-0002-8438-9548","id":"98120","full_name":"Lopez Salas, Nieves","first_name":"Nieves"},{"first_name":"Ana Raquel","full_name":"de la Osa, Ana Raquel","last_name":"de la Osa"}],"date_created":"2023-01-27T16:20:02Z","year":"2021","page":"168-180","intvolume":"        66","citation":{"bibtex":"@article{Rodríguez-Gómez_Lepre_Sánchez-Silva_Lopez Salas_de la Osa_2021, title={PtRu nanoparticles supported on noble carbons for ethanol electrooxidation}, volume={66}, DOI={<a href=\"https://doi.org/10.1016/j.jechem.2021.07.004\">10.1016/j.jechem.2021.07.004</a>}, journal={Journal of Energy Chemistry}, publisher={Elsevier BV}, author={Rodríguez-Gómez, Alberto and Lepre, Enrico and Sánchez-Silva, Luz and Lopez Salas, Nieves and de la Osa, Ana Raquel}, year={2021}, pages={168–180} }","short":"A. Rodríguez-Gómez, E. Lepre, L. Sánchez-Silva, N. Lopez Salas, A.R. de la Osa, Journal of Energy Chemistry 66 (2021) 168–180.","mla":"Rodríguez-Gómez, Alberto, et al. “PtRu Nanoparticles Supported on Noble Carbons for Ethanol Electrooxidation.” <i>Journal of Energy Chemistry</i>, vol. 66, Elsevier BV, 2021, pp. 168–80, doi:<a href=\"https://doi.org/10.1016/j.jechem.2021.07.004\">10.1016/j.jechem.2021.07.004</a>.","apa":"Rodríguez-Gómez, A., Lepre, E., Sánchez-Silva, L., Lopez Salas, N., &#38; de la Osa, A. R. (2021). PtRu nanoparticles supported on noble carbons for ethanol electrooxidation. <i>Journal of Energy Chemistry</i>, <i>66</i>, 168–180. <a href=\"https://doi.org/10.1016/j.jechem.2021.07.004\">https://doi.org/10.1016/j.jechem.2021.07.004</a>","ama":"Rodríguez-Gómez A, Lepre E, Sánchez-Silva L, Lopez Salas N, de la Osa AR. PtRu nanoparticles supported on noble carbons for ethanol electrooxidation. <i>Journal of Energy Chemistry</i>. 2021;66:168-180. doi:<a href=\"https://doi.org/10.1016/j.jechem.2021.07.004\">10.1016/j.jechem.2021.07.004</a>","chicago":"Rodríguez-Gómez, Alberto, Enrico Lepre, Luz Sánchez-Silva, Nieves Lopez Salas, and Ana Raquel de la Osa. “PtRu Nanoparticles Supported on Noble Carbons for Ethanol Electrooxidation.” <i>Journal of Energy Chemistry</i> 66 (2021): 168–80. <a href=\"https://doi.org/10.1016/j.jechem.2021.07.004\">https://doi.org/10.1016/j.jechem.2021.07.004</a>.","ieee":"A. Rodríguez-Gómez, E. Lepre, L. Sánchez-Silva, N. Lopez Salas, and A. R. de la Osa, “PtRu nanoparticles supported on noble carbons for ethanol electrooxidation,” <i>Journal of Energy Chemistry</i>, vol. 66, pp. 168–180, 2021, doi: <a href=\"https://doi.org/10.1016/j.jechem.2021.07.004\">10.1016/j.jechem.2021.07.004</a>."},"publication_identifier":{"issn":["2095-4956"]},"publication_status":"published","keyword":["Electrochemistry","Energy (miscellaneous)","Energy Engineering and Power Technology","Fuel Technology"],"language":[{"iso":"eng"}],"_id":"40566","user_id":"98120","status":"public","publication":"Journal of Energy Chemistry","type":"journal_article"},{"type":"journal_article","status":"public","_id":"62806","department":[{"_id":"985"}],"user_id":"116779","article_type":"original","article_number":"e202112679","extern":"1","publication_identifier":{"issn":["1433-7851","1521-3773"]},"publication_status":"published","intvolume":"        61","citation":{"short":"M. Azimzadeh Sani, N.G. Pavlopoulos, S. Pezzotti, A. Serva, P. Cignoni, J. Linnemann, M. Salanne, M. Gaigeot, K. Tschulik, Angewandte Chemie International Edition 61 (2021).","bibtex":"@article{Azimzadeh Sani_Pavlopoulos_Pezzotti_Serva_Cignoni_Linnemann_Salanne_Gaigeot_Tschulik_2021, title={Unexpectedly High Capacitance of the Metal Nanoparticle/Water Interface: Molecular‐Level Insights into the Electrical Double Layer}, volume={61}, DOI={<a href=\"https://doi.org/10.1002/anie.202112679\">10.1002/anie.202112679</a>}, number={5e202112679}, journal={Angewandte Chemie International Edition}, publisher={Wiley}, author={Azimzadeh Sani, Mahnaz and Pavlopoulos, Nicholas G. and Pezzotti, Simone and Serva, Alessandra and Cignoni, Paolo and Linnemann, Julia and Salanne, Mathieu and Gaigeot, Marie‐Pierre and Tschulik, Kristina}, year={2021} }","mla":"Azimzadeh Sani, Mahnaz, et al. “Unexpectedly High Capacitance of the Metal Nanoparticle/Water Interface: Molecular‐Level Insights into the Electrical Double Layer.” <i>Angewandte Chemie International Edition</i>, vol. 61, no. 5, e202112679, Wiley, 2021, doi:<a href=\"https://doi.org/10.1002/anie.202112679\">10.1002/anie.202112679</a>.","apa":"Azimzadeh Sani, M., Pavlopoulos, N. G., Pezzotti, S., Serva, A., Cignoni, P., Linnemann, J., Salanne, M., Gaigeot, M., &#38; Tschulik, K. (2021). Unexpectedly High Capacitance of the Metal Nanoparticle/Water Interface: Molecular‐Level Insights into the Electrical Double Layer. <i>Angewandte Chemie International Edition</i>, <i>61</i>(5), Article e202112679. <a href=\"https://doi.org/10.1002/anie.202112679\">https://doi.org/10.1002/anie.202112679</a>","chicago":"Azimzadeh Sani, Mahnaz, Nicholas G. Pavlopoulos, Simone Pezzotti, Alessandra Serva, Paolo Cignoni, Julia Linnemann, Mathieu Salanne, Marie‐Pierre Gaigeot, and Kristina Tschulik. “Unexpectedly High Capacitance of the Metal Nanoparticle/Water Interface: Molecular‐Level Insights into the Electrical Double Layer.” <i>Angewandte Chemie International Edition</i> 61, no. 5 (2021). <a href=\"https://doi.org/10.1002/anie.202112679\">https://doi.org/10.1002/anie.202112679</a>.","ieee":"M. Azimzadeh Sani <i>et al.</i>, “Unexpectedly High Capacitance of the Metal Nanoparticle/Water Interface: Molecular‐Level Insights into the Electrical Double Layer,” <i>Angewandte Chemie International Edition</i>, vol. 61, no. 5, Art. no. e202112679, 2021, doi: <a href=\"https://doi.org/10.1002/anie.202112679\">10.1002/anie.202112679</a>.","ama":"Azimzadeh Sani M, Pavlopoulos NG, Pezzotti S, et al. Unexpectedly High Capacitance of the Metal Nanoparticle/Water Interface: Molecular‐Level Insights into the Electrical Double Layer. <i>Angewandte Chemie International Edition</i>. 2021;61(5). doi:<a href=\"https://doi.org/10.1002/anie.202112679\">10.1002/anie.202112679</a>"},"oa":"1","date_updated":"2025-12-03T16:31:54Z","volume":61,"author":[{"first_name":"Mahnaz","last_name":"Azimzadeh Sani","full_name":"Azimzadeh Sani, Mahnaz"},{"full_name":"Pavlopoulos, Nicholas G.","last_name":"Pavlopoulos","first_name":"Nicholas G."},{"first_name":"Simone","last_name":"Pezzotti","full_name":"Pezzotti, Simone"},{"first_name":"Alessandra","full_name":"Serva, Alessandra","last_name":"Serva"},{"last_name":"Cignoni","full_name":"Cignoni, Paolo","first_name":"Paolo"},{"orcid":"0000-0001-6883-5424","last_name":"Linnemann","id":"116779","full_name":"Linnemann, Julia","first_name":"Julia"},{"full_name":"Salanne, Mathieu","last_name":"Salanne","first_name":"Mathieu"},{"last_name":"Gaigeot","full_name":"Gaigeot, Marie‐Pierre","first_name":"Marie‐Pierre"},{"first_name":"Kristina","last_name":"Tschulik","full_name":"Tschulik, Kristina"}],"doi":"10.1002/anie.202112679","main_file_link":[{"open_access":"1"}],"publication":"Angewandte Chemie International Edition","abstract":[{"lang":"eng","text":"The electrical double‐layer plays a key role in important interfacial electrochemical processes from catalysis to energy storage and corrosion. Therefore, understanding its structure is crucial for the progress of sustainable technologies. We extract new physico‐chemical information on the capacitance and structure of the electrical double‐layer of platinum and gold nanoparticles at the molecular level, employing single nanoparticle electrochemistry. The charge storage ability of the solid/liquid interface is larger by one order‐of‐magnitude than predicted by the traditional mean‐field models of the double‐layer such as the Gouy–Chapman–Stern model. Performing molecular dynamics simulations, we investigate the possible relationship between the measured high capacitance and adsorption strength of the water adlayer formed at the metal surface. These insights may launch the active tuning of solid–solvent and solvent–solvent interactions as an innovative design strategy to transform energy technologies towards superior performance and sustainability."}],"keyword":["single-entity electrochemistry","electrical double layer","supercapacitor","nanoparticles"],"language":[{"iso":"eng"}],"quality_controlled":"1","issue":"5","year":"2021","publisher":"Wiley","date_created":"2025-12-03T15:39:25Z","title":"Unexpectedly High Capacitance of the Metal Nanoparticle/Water Interface: Molecular‐Level Insights into the Electrical Double Layer"},{"publication":"International Journal of Molecular Sciences","abstract":[{"text":"Single-entity electrochemistry allows for assessing electrocatalytic activities of individual material entities such as nanoparticles (NPs). Thus, it becomes possible to consider intrinsic electrochemical properties of nanocatalysts when researching how activity relates to physical and structural material properties. Conversely, conventional electrochemical techniques provide a normalized sum current referring to a huge ensemble of NPs constituting, along with additives (e.g., binders), a complete catalyst-coated electrode. Accordingly, recording electrocatalytic responses of single NPs avoids interferences of ensemble effects and reduces the complexity of electrocatalytic processes, thus enabling detailed description and modelling. Herein, we present insights into the oxygen evolution catalysis at individual cubic Co3O4 NPs impacting microelectrodes of different support materials. Simulating diffusion at supported nanocubes, measured step current signals can be analyzed, providing edge lengths, corresponding size distributions, and interference-free turnover frequencies. The provided nano-impact investigation of (electro-)catalyst-support effects contradicts assumptions on a low number of highly active sites.","lang":"eng"}],"language":[{"iso":"eng"}],"keyword":["electrocatalysis","oxygen evolution reaction","cobalt spinel","single-entity electrochemistry"],"issue":"23","quality_controlled":"1","year":"2021","date_created":"2025-12-03T15:35:52Z","publisher":"MDPI AG","title":"Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects","type":"journal_article","status":"public","user_id":"116779","department":[{"_id":"985"}],"_id":"62805","extern":"1","article_number":"13137","article_type":"original","publication_status":"published","publication_identifier":{"issn":["1422-0067"]},"citation":{"apa":"Liu, Z., Corva, M., Amin, H. M. A., Blanc, N., Linnemann, J., &#38; Tschulik, K. (2021). Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects. <i>International Journal of Molecular Sciences</i>, <i>22</i>(23), Article 13137. <a href=\"https://doi.org/10.3390/ijms222313137\">https://doi.org/10.3390/ijms222313137</a>","bibtex":"@article{Liu_Corva_Amin_Blanc_Linnemann_Tschulik_2021, title={Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects}, volume={22}, DOI={<a href=\"https://doi.org/10.3390/ijms222313137\">10.3390/ijms222313137</a>}, number={2313137}, journal={International Journal of Molecular Sciences}, publisher={MDPI AG}, author={Liu, Zhibin and Corva, Manuel and Amin, Hatem M. A. and Blanc, Niclas and Linnemann, Julia and Tschulik, Kristina}, year={2021} }","short":"Z. Liu, M. Corva, H.M.A. Amin, N. Blanc, J. Linnemann, K. Tschulik, International Journal of Molecular Sciences 22 (2021).","mla":"Liu, Zhibin, et al. “Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects.” <i>International Journal of Molecular Sciences</i>, vol. 22, no. 23, 13137, MDPI AG, 2021, doi:<a href=\"https://doi.org/10.3390/ijms222313137\">10.3390/ijms222313137</a>.","ieee":"Z. Liu, M. Corva, H. M. A. Amin, N. Blanc, J. Linnemann, and K. Tschulik, “Single Co<sub>3</sub>O<sub>4</sub> Nanocubes Electrocatalyzing the Oxygen Evolution Reaction: Nano-Impact Insights into Intrinsic Activity and Support Effects,” <i>International Journal of Molecular Sciences</i>, vol. 22, no. 23, Art. no. 13137, 2021, doi: <a href=\"https://doi.org/10.3390/ijms222313137\">10.3390/ijms222313137</a>.","chicago":"Liu, Zhibin, Manuel Corva, Hatem M. A. 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