---
_id: '51136'
abstract:
- lang: eng
  text: "Iron oxide nanoparticles are very interesting for many applications in different
    industrial sectors. A promising\r\nprocess to manufacture these nanoparticles
    is flame spray pyrolysis (FSP). A lack of understanding of the\r\nindividual sub-processes
    in FSP makes it challenging to tailor nanoparticle properties. This work provides\r\ninsights
    into the formation of iron oxide nanoparticles in a turbulent spray flame using
    Large Eddy Simulations\r\n(LES), which are based on a comprehensive model, including
    customized submodels. Highlights are the\r\nadaption of a turbulent combustion
    model and a bivariate hybrid method of moments for modeling nanoparticle\r\ndynamics.
    The work focuses on the SpraySyn burner, which is a standardized laboratory burner
    and was\r\noperated with a precursor-solvent mixture of ethanol and iron(III)
    nitrate nonahydrate. For studying the\r\nrelevance of precursor chemistry, LES
    using an evaporation-limited precursor chemistry model is compared\r\nwith a model
    that includes detailed iron chemistry. A further novelty is the inclusion of adsorption
    in the\r\nsimulation, which defines a third model for comparison. Sufficient validation
    is achieved for the undoped LES\r\nusing experimental data from the literature.
    A strong impact of the detailed iron chemistry and adsorption\r\nis found on the
    precursor consumption and the aggregate and primary particle formation. Comparing
    the\r\nparticle diameters with experimental measurements from the literature and
    data generated for this work is\r\nfound unsuitable to asses the precursor chemistry
    model and revealed an urgent need for future experimental\r\nand numerical research.
    This work serves as a step forward in realizing a reliable model."
citation:
  ama: Fröde F, Grenga T, Pitsch H, et al., eds. <i>Large Eddy Simulation of Iron
    Oxide Formation in a Laboratory Spray Flame</i>. Elsevier; 2023. doi:<a href="https://doi.org/10.1016/j.jaecs.2023.100191">https://doi.org/10.1016/j.jaecs.2023.100191</a>
  apa: Large eddy simulation of iron oxide formation in a laboratory spray flame.
    (2023). In F. Fröde, T. Grenga, H. Pitsch, S. Dupont, R. Kneer, R. Tischendorf,
    O. Massopo, &#38; H.-J. Schmid (Eds.), <i>Applications in Energy and Combustion
    Science</i>. Elsevier. <a href="https://doi.org/10.1016/j.jaecs.2023.100191">https://doi.org/10.1016/j.jaecs.2023.100191</a>
  bibtex: '@book{Fröde_Grenga_Pitsch_Dupont_Kneer_Tischendorf_Massopo_Schmid_2023,
    title={Large eddy simulation of iron oxide formation in a laboratory spray flame},
    DOI={<a href="https://doi.org/10.1016/j.jaecs.2023.100191">https://doi.org/10.1016/j.jaecs.2023.100191</a>},
    journal={Applications in Energy and Combustion Science}, publisher={Elsevier},
    year={2023} }'
  chicago: Fröde, Fabian , Temistocle  Grenga, Heinz  Pitsch, Sophie Dupont, Reinhold
    Kneer, Ricardo Tischendorf, Orlando Massopo, and Hans-Joachim Schmid, eds. <i>Large
    Eddy Simulation of Iron Oxide Formation in a Laboratory Spray Flame</i>. <i>Applications
    in Energy and Combustion Science</i>. Elsevier, 2023. <a href="https://doi.org/10.1016/j.jaecs.2023.100191">https://doi.org/10.1016/j.jaecs.2023.100191</a>.
  ieee: F. Fröde <i>et al.</i>, Eds., <i>Large eddy simulation of iron oxide formation
    in a laboratory spray flame</i>. Elsevier, 2023.
  mla: Fröde, Fabian, et al., editors. “Large Eddy Simulation of Iron Oxide Formation
    in a Laboratory Spray Flame.” <i>Applications in Energy and Combustion Science</i>,
    Elsevier, 2023, doi:<a href="https://doi.org/10.1016/j.jaecs.2023.100191">https://doi.org/10.1016/j.jaecs.2023.100191</a>.
  short: F. Fröde, T. Grenga, H. Pitsch, S. Dupont, R. Kneer, R. Tischendorf, O. Massopo,
    H.-J. Schmid, eds., Large Eddy Simulation of Iron Oxide Formation in a Laboratory
    Spray Flame, Elsevier, 2023.
date_created: 2024-02-05T12:17:35Z
date_updated: 2024-02-05T12:38:43Z
department:
- _id: '150'
doi: https://doi.org/10.1016/j.jaecs.2023.100191
editor:
- first_name: 'Fabian '
  full_name: 'Fröde, Fabian '
  last_name: Fröde
- first_name: 'Temistocle '
  full_name: 'Grenga, Temistocle '
  last_name: Grenga
- first_name: 'Heinz '
  full_name: 'Pitsch, Heinz '
  last_name: Pitsch
- first_name: Sophie
  full_name: Dupont, Sophie
  last_name: Dupont
- first_name: Reinhold
  full_name: Kneer, Reinhold
  last_name: Kneer
- first_name: Ricardo
  full_name: Tischendorf, Ricardo
  id: '67002'
  last_name: Tischendorf
- first_name: Orlando
  full_name: Massopo, Orlando
  id: '98419'
  last_name: Massopo
- first_name: Hans-Joachim
  full_name: Schmid, Hans-Joachim
  id: '464'
  last_name: Schmid
  orcid: 000-0001-8590-1921
has_accepted_license: '1'
keyword:
- Flame spray pyrolysis
- Iron oxide formation
- Large eddy simulation
- Method of moments
- SpraySyn
language:
- iso: eng
main_file_link:
- url: https://www.sciencedirect.com/science/article/pii/S2666352X23000808
publication: Applications in Energy and Combustion Science
publication_status: published
publisher: Elsevier
status: public
title: Large eddy simulation of iron oxide formation in a laboratory spray flame
type: journal_editor
user_id: '98419'
year: '2023'
...