@article{52372, abstract = {{Due to the hydrolytic instability of LiPF6 in carbonate-based solvents, HF is a typical impurity in Li-ion battery electrolytes. HF significantly influences the performance of Li-ion batteries, for example by impacting the formation of the solid electrolyte interphase at the anode and by affecting transition metal dissolution at the cathode. Additionally, HF complicates studying fundamental interfacial electrochemistry of Li-ion battery electrolytes, such as direct anion reduction, because it is electrocatalytically relatively unstable, resulting in LiF passivation layers. Methods to selectively remove ppm levels of HF from LiPF6-containing carbonate-based electrolytes are limited. We introduce and benchmark a simple yet efficient electrochemical in situ method to selectively remove ppm amounts of HF from LiPF6-containing carbonate-based electrolytes. The basic idea is the application of a suitable potential to a high surface-area metallic electrode upon which only HF reacts (electrocatalytically) while all other electrolyte components are unaffected under the respective conditions.}}, author = {{Ge, Xiaokun and Huck, Marten and Kuhlmann, Andreas and Tiemann, Michael and Weinberger, Christian and Xu, Xiaodan and Zhao, Zhenyu and Steinrueck, Hans-Georg}}, issn = {{0013-4651}}, journal = {{Journal of The Electrochemical Society}}, keywords = {{Materials Chemistry, Electrochemistry, Surfaces, Coatings and Films, Condensed Matter Physics, Renewable Energy, Sustainability and the Environment, Electronic, Optical and Magnetic Materials}}, pages = {{030552}}, publisher = {{The Electrochemical Society}}, title = {{{Electrochemical Removal of HF from Carbonate-based LiPF6-containing Li-ion Battery Electrolytes}}}, doi = {{10.1149/1945-7111/ad30d3}}, volume = {{171}}, year = {{2024}}, } @article{52958, author = {{Boeddeker, Christoph and Subramanian, Aswin Shanmugam and Wichern, Gordon and Haeb-Umbach, Reinhold and Le Roux, Jonathan}}, issn = {{2329-9290}}, journal = {{IEEE/ACM Transactions on Audio, Speech, and Language Processing}}, keywords = {{Electrical and Electronic Engineering, Acoustics and Ultrasonics, Computer Science (miscellaneous), Computational Mathematics}}, pages = {{1185--1197}}, publisher = {{Institute of Electrical and Electronics Engineers (IEEE)}}, title = {{{TS-SEP: Joint Diarization and Separation Conditioned on Estimated Speaker Embeddings}}}, doi = {{10.1109/taslp.2024.3350887}}, volume = {{32}}, year = {{2024}}, } @inproceedings{53069, author = {{Banh, Ngoc Chi and Scharlau, Ingrid}}, location = {{Regensburg}}, title = {{{Effects of task difficulty on visual processing speed}}}, year = {{2024}}, } @book{34544, abstract = {{Tax evasion, tax avoidance and tax resistance are widespread phenomena in political, economic, social and fiscal history from antiquity through medieval, early modern and modern times. Histories of Tax Evasion, Avoidance and Resistance shows how different groups and individuals around the globe have succeeded or failed in not paying their due taxes, whether in kind or in cash, on their properties or on their crops. It analyses how, throughout history, wealthy and poor taxpayers have tried to avoid or reduce their tax burden by negotiating with tax authorities, through practices of legal or illegal tax evasion, by filing lawsuits, seeking armed resistance or by migration, and how state authorities have dealt with such acts of claim making, defiance, open resistance or elusion. It fills an important research gap in tax history, addressing questions of tax morale and fairness, and how social and political inequality was negotiated through taxation. It gives rich insights into the development of citizen-state relationships throughout the course of history. The book comprises case studies from Ancient Athens, Roman Egypt, Medieval Europe, Early Modern Mexico, the Ottoman Empire, Nigeria under British colonial rule, the United Kingdom of the early 20th century, Greece during the Second World War, as well as West Germany, Switzerland, Sweden and the United States in the 20th century, including transnational entanglements in the world of late-modern offshore finance and taxation. The authors are experts in fiscal, economic, financial, legal, social and/or cultural history. The book is intended for students, researchers and scholars of economic and financial history, social and world history and political economy. The Open Access version of this book, available at www.taylorfrancis.com, has been made available under a Creative Commons Attribution-Share Alike 4.0 license.}}, author = {{Schönhärl, Korinna and Hürlimann, Gisela and Rohde, Dorothea}}, isbn = {{9781003333197}}, keywords = {{Tax History, Financial History}}, publisher = {{Routledge}}, title = {{{Histories of Tax Evasion, Avoidance and Resistance}}}, doi = {{10.4324/9781003333197}}, year = {{2023}}, } @inbook{34546, abstract = {{Jean Bodin's list on how the absolutist monarchical state could raise its revenue ranked taxation only in seventh place. From a modern legal perspective, taxes are compulsory transfers of resources that households and enterprises pay to one or several government bodies without receiving an individual, specific benefit in return. Historians have dealt with not paying taxes in various contexts, such as analysing tax resistance and tax resistance movements in history. Tax law is best understood as an outcome of long-term, often conflictual, negotiations and as an expression of specific political mentalities and ideologies. As a consequence, tax law and sometimes even the tax juridical system have a strongly politicised character. Loopholes in tax legislation that enable or facilitate avoidance or evasion can thus be regarded as a result of the interest-driven politics of parliamentary majorities, as the success of concerted lobby pressure.}}, author = {{Schönhärl, Korinna and Hürlimann, Gisela and Rohde, Dorothea}}, booktitle = {{Histories of Tax Evasion, Avoidance and Resistance }}, editor = {{Schönhärl, Korinna and Hürlimann, Gisela and Rohde, Dorothea}}, pages = {{1--15}}, publisher = {{Routledge}}, title = {{{ The Ability and Intention of Not Paying Taxes in History. Some Introductory Observations}}}, doi = {{10.4324/9781003333197}}, year = {{2023}}, } @inbook{34547, abstract = {{As a case study, this chapter examines two tax education films that were produced 11 years apart in the USA and Western Germany during and after World War II: “The New Spirit” and “Putzke wants to know”. In contrast to America's most popular cartoon character 11 years earlier, Erwin Putzke is in a terrible mood at the beginning of the short film “Putzke wants to know”. The family father and electrician with a workshop of his own is annoyed and upset by the duty of filling in his tax return, grumbling at his wife and daughter and even at their budgie. The film's tax morale message is conveyed to its audience against the backdrop of a sober post-war reality characterised by allied occupation and the Allies' say in West German tax policies during a period of laborious economic build-up after a lost war.}}, author = {{Schönhärl, Korinna}}, booktitle = {{Histories of Tax Evasion, Avoidance and Resistance}}, editor = {{Schönhärl, Korinna and Hürlimann, Gisela and Rohde, Dorothea}}, pages = {{154--167}}, publisher = {{Routledge}}, title = {{{ How to Create a Taxpaying Spirit. A Transnational Examination of an US American and a Western German Tax Education Film in and after World War II}}}, doi = {{10.4324/9781003333197}}, year = {{2023}}, } @article{21199, abstract = {{As in almost every other branch of science, the major advances in data science and machine learning have also resulted in significant improvements regarding the modeling and simulation of nonlinear dynamical systems. It is nowadays possible to make accurate medium to long-term predictions of highly complex systems such as the weather, the dynamics within a nuclear fusion reactor, of disease models or the stock market in a very efficient manner. In many cases, predictive methods are advertised to ultimately be useful for control, as the control of high-dimensional nonlinear systems is an engineering grand challenge with huge potential in areas such as clean and efficient energy production, or the development of advanced medical devices. However, the question of how to use a predictive model for control is often left unanswered due to the associated challenges, namely a significantly higher system complexity, the requirement of much larger data sets and an increased and often problem-specific modeling effort. To solve these issues, we present a universal framework (which we call QuaSiModO: Quantization-Simulation-Modeling-Optimization) to transform arbitrary predictive models into control systems and use them for feedback control. The advantages of our approach are a linear increase in data requirements with respect to the control dimension, performance guarantees that rely exclusively on the accuracy of the predictive model, and only little prior knowledge requirements in control theory to solve complex control problems. In particular the latter point is of key importance to enable a large number of researchers and practitioners to exploit the ever increasing capabilities of predictive models for control in a straight-forward and systematic fashion.}}, author = {{Peitz, Sebastian and Bieker, Katharina}}, journal = {{Automatica}}, publisher = {{Elsevier}}, title = {{{On the Universal Transformation of Data-Driven Models to Control Systems}}}, doi = {{10.1016/j.automatica.2022.110840}}, volume = {{149}}, year = {{2023}}, } @article{35831, abstract = {{Videografien eigenen Unterrichts sind ein mögliches methodisches Werkzeug zur Förderung der professionellen Kompetenz angehender Lehrkräfte, das allerdings innerhalb der Lehramtsausbildung noch nicht breit implementiert ist. Ein möglicher Grund hierfür könnte neben organisatorischen Herausforderungen auch in einer geringen Akzeptanz von Eigenvideografien durch Lehramtsstudierende liegen. Um besser abschätzen zu können, mit welchen Voraussetzungen affektiv-emotionaler Art bei einer breiteren Implementierung im Lehramtsstudium gerechnet werden kann, wurden N = 938 Lehramtsstudierende im Masterstudium an der Universität Paderborn zu ihren Emotionen und Bereitschaften zur Arbeit mit Eigenvideografien befragt. Dabei wurde auch erfasst, wie sich diese je nach bestehenden Erfahrungen zur Arbeit mit Videografien unterscheiden. In den Ergebnissen zeigen sich kaum affektiv-emotionale Reaktionen zur Eigenvideografie, und wenn, vor allem Gefühle der Unsicherheit. Zu beachten ist, dass zwar bei gut der Hälfte der Studierenden eine eher hohe generelle Bereitschaft zur Eigenvideografie besteht, eine konkrete Intention bzw. eine konkrete Volition zur Videografie aber geringer ist. Die ca. 10 % der Studierenden mit Eigenvideografieerfahrung im Studium zeigen erwartungsgemäß höhere Bereitschaften, aber unerwartet keine signifikant positiveren Emotionen. Insgesamt verdeutlichen die Ergebnisse, dass bzgl. der Akzeptanz der Studierenden ein höheres Potenzial zur Implementation von Eigenvideografien im Studium vorliegt, als aktuell ausgeschöpft wird.}}, author = {{Vogelsang, Christoph and Pollmeier, Pascal and Gockeln, Theresa and Rogge, Tim}}, journal = {{Zeitschrift für Bildungsforschung}}, keywords = {{Lehrerbildung, Videografie, Praxissemester, Emotionen, Akzeptanz}}, publisher = {{Springer}}, title = {{{Zu unangenehm, zu viel Aufwand oder keine Möglichkeit? – Emotionen und Bereitschaft von Lehramtsstudierenden zur Videografie eigenen Unterrichts}}}, doi = {{10.1007/s35834-022-00378-y}}, year = {{2023}}, } @article{36800, abstract = {{Abstract. The miniaturisation of components leads to new demands on measurement systems. One of these is the resolution. As a volumetric analysis method and method of non-destructive testing, industrial X-ray computed tomography (XCT) has the ability to measure geometrical features and their corresponding dimensions without destroying them and can therefore be used for quality assurance. However, the concept of resolution is not trivial for XCT and has not yet been finally clarified. In particular, the interface structural resolution, the detectability of two surfaces facing each other after surface segmentation, faces a lack of a test specimen, a corresponding measurand and a reliable method. Simulation-based XCT investigations of a method to determine this type of resolution are presented in this article using the geometry of a test specimen that contains several radially arranged holes of the same size. The borehole diameters correspond to the distance between the holes to investigate the resolvability of surfaces and interfaces. The evaluation is based on mean and extreme values of grey value profiles between the individual boreholes of the reconstructed volume. It is shown that the geometrical detectability of the test specimen surface and interface can be extended by a reasonable choice of the threshold value for surface segmentation within a defined interval. With regard to the resolving capability, a distinction is made between assured detectability and possible detectability, as well as the threshold value used when using the ISO50 threshold for surface segmentation and measurement chain completion. }}, author = {{Busch, Matthias and Hausotte, Tino}}, issn = {{2194-878X}}, journal = {{Journal of Sensors and Sensor Systems}}, keywords = {{Electrical and Electronic Engineering, Instrumentation}}, number = {{1}}, pages = {{1--8}}, publisher = {{Copernicus GmbH}}, title = {{{Simulation-based investigation of the metrological interface structural resolution capability of X-ray computed tomography scanners}}}, doi = {{10.5194/jsss-12-1-2023}}, volume = {{12}}, year = {{2023}}, } @inproceedings{35426, author = {{Richter, Cedric and Haltermann, Jan Frederik and Jakobs, Marie-Christine and Pauck, Felix and Schott, Stefan and Wehrheim, Heike}}, booktitle = {{37th IEEE/ACM International Conference on Automated Software Engineering}}, publisher = {{ACM}}, title = {{{Are Neural Bug Detectors Comparable to Software Developers on Variable Misuse Bugs?}}}, doi = {{10.1145/3551349.3561156}}, year = {{2023}}, }