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Grundmeier, Journal of Raman Spectroscopy 52 (2021) 1237–1245.","ieee":"S. Knust et al., “In situ backside Raman spectroscopy of zinc oxide nanorods in an atmospheric‐pressure dielectric barrier discharge plasma,” Journal of Raman Spectroscopy, vol. 52, no. 7, pp. 1237–1245, 2021, doi: 10.1002/jrs.6123.","chicago":"Knust, Steffen, Lukas Ruhm, Andreas Kuhlmann, Dennis Meinderink, Julius Bürger, Jörg Lindner, Maria Teresa de los Arcos de Pedro, and Guido Grundmeier. “In Situ Backside Raman Spectroscopy of Zinc Oxide Nanorods in an Atmospheric‐pressure Dielectric Barrier Discharge Plasma.” Journal of Raman Spectroscopy 52, no. 7 (2021): 1237–45. https://doi.org/10.1002/jrs.6123.","apa":"Knust, S., Ruhm, L., Kuhlmann, A., Meinderink, D., Bürger, J., Lindner, J., de los Arcos de Pedro, M. T., & Grundmeier, G. (2021). In situ backside Raman spectroscopy of zinc oxide nanorods in an atmospheric‐pressure dielectric barrier discharge plasma. Journal of Raman Spectroscopy, 52(7), 1237–1245. https://doi.org/10.1002/jrs.6123","ama":"Knust S, Ruhm L, Kuhlmann A, et al. In situ backside Raman spectroscopy of zinc oxide nanorods in an atmospheric‐pressure dielectric barrier discharge plasma. Journal of Raman Spectroscopy. 2021;52(7):1237-1245. doi:10.1002/jrs.6123","mla":"Knust, Steffen, et al. “In Situ Backside Raman Spectroscopy of Zinc Oxide Nanorods in an Atmospheric‐pressure Dielectric Barrier Discharge Plasma.” Journal of Raman Spectroscopy, vol. 52, no. 7, Wiley, 2021, pp. 1237–45, doi:10.1002/jrs.6123.","bibtex":"@article{Knust_Ruhm_Kuhlmann_Meinderink_Bürger_Lindner_de los Arcos de Pedro_Grundmeier_2021, title={In situ backside Raman spectroscopy of zinc oxide nanorods in an atmospheric‐pressure dielectric barrier discharge plasma}, volume={52}, DOI={10.1002/jrs.6123}, number={7}, journal={Journal of Raman Spectroscopy}, publisher={Wiley}, author={Knust, Steffen and Ruhm, Lukas and Kuhlmann, Andreas and Meinderink, Dennis and Bürger, Julius and Lindner, Jörg and de los Arcos de Pedro, Maria Teresa and Grundmeier, Guido}, year={2021}, pages={1237–1245} }"},"user_id":"77496","publication":"Journal of Raman Spectroscopy","keyword":["Spectroscopy","General Materials Science"],"publisher":"Wiley","author":[{"first_name":"Steffen","full_name":"Knust, Steffen","last_name":"Knust"},{"last_name":"Ruhm","first_name":"Lukas","full_name":"Ruhm, Lukas"},{"first_name":"Andreas","full_name":"Kuhlmann, Andreas","last_name":"Kuhlmann"},{"id":"32378","last_name":"Meinderink","orcid":"0000-0002-2755-6514","full_name":"Meinderink, Dennis","first_name":"Dennis"},{"last_name":"Bürger","id":"46952","first_name":"Julius","full_name":"Bürger, Julius"},{"id":"20797","last_name":"Lindner","full_name":"Lindner, Jörg","first_name":"Jörg"},{"first_name":"Maria Teresa","full_name":"de los Arcos de Pedro, Maria Teresa","last_name":"de los Arcos de Pedro","id":"54556"},{"last_name":"Grundmeier","id":"194","first_name":"Guido","full_name":"Grundmeier, Guido"}],"date_created":"2022-11-15T14:08:53Z","status":"public","volume":52},{"language":[{"iso":"eng"}],"date_updated":"2023-01-10T12:11:57Z","doi":"10.3390/nano10010141","department":[{"_id":"15"},{"_id":"230"}],"publication_status":"published","publication_identifier":{"issn":["2079-4991"]},"title":"Characterisation of the PS-PMMA Interfaces in Microphase Separated Block Copolymer Thin Films by Analytical (S)TEM","citation":{"ieee":"J. Bürger, V. Kunnathully, D. Kool, J. Lindner, and K. Brassat, “Characterisation of the PS-PMMA Interfaces in Microphase Separated Block Copolymer Thin Films by Analytical (S)TEM,” Nanomaterials, vol. 10, no. 1, Art. no. 141, 2020, doi: 10.3390/nano10010141.","short":"J. Bürger, V. Kunnathully, D. Kool, J. Lindner, K. Brassat, Nanomaterials 10 (2020).","mla":"Bürger, Julius, et al. “Characterisation of the PS-PMMA Interfaces in Microphase Separated Block Copolymer Thin Films by Analytical (S)TEM.” Nanomaterials, vol. 10, no. 1, 141, MDPI AG, 2020, doi:10.3390/nano10010141.","bibtex":"@article{Bürger_Kunnathully_Kool_Lindner_Brassat_2020, title={Characterisation of the PS-PMMA Interfaces in Microphase Separated Block Copolymer Thin Films by Analytical (S)TEM}, volume={10}, DOI={10.3390/nano10010141}, number={1141}, journal={Nanomaterials}, publisher={MDPI AG}, author={Bürger, Julius and Kunnathully, Vinay and Kool, Daniel and Lindner, Jörg and Brassat, Katharina}, year={2020} }","ama":"Bürger J, Kunnathully V, Kool D, Lindner J, Brassat K. Characterisation of the PS-PMMA Interfaces in Microphase Separated Block Copolymer Thin Films by Analytical (S)TEM. Nanomaterials. 2020;10(1). doi:10.3390/nano10010141","apa":"Bürger, J., Kunnathully, V., Kool, D., Lindner, J., & Brassat, K. (2020). Characterisation of the PS-PMMA Interfaces in Microphase Separated Block Copolymer Thin Films by Analytical (S)TEM. Nanomaterials, 10(1), Article 141. https://doi.org/10.3390/nano10010141","chicago":"Bürger, Julius, Vinay Kunnathully, Daniel Kool, Jörg Lindner, and Katharina Brassat. “Characterisation of the PS-PMMA Interfaces in Microphase Separated Block Copolymer Thin Films by Analytical (S)TEM.” Nanomaterials 10, no. 1 (2020). https://doi.org/10.3390/nano10010141."},"year":"2020","type":"journal_article","_id":"34092","intvolume":" 10","article_number":"141","issue":"1","author":[{"full_name":"Bürger, Julius","first_name":"Julius","id":"46952","last_name":"Bürger"},{"last_name":"Kunnathully","first_name":"Vinay","full_name":"Kunnathully, Vinay"},{"first_name":"Daniel","full_name":"Kool, Daniel","last_name":"Kool","id":"44586"},{"last_name":"Lindner","id":"20797","first_name":"Jörg","full_name":"Lindner, Jörg"},{"last_name":"Brassat","id":"11305","first_name":"Katharina","full_name":"Brassat, Katharina"}],"publisher":"MDPI AG","publication":"Nanomaterials","keyword":["General Materials Science","General Chemical Engineering"],"volume":10,"status":"public","date_created":"2022-11-15T14:20:33Z","abstract":[{"lang":"eng","text":"Block copolymer (BCP) self-assembly is a promising tool for next generation lithography as microphase separated polymer domains in thin films can act as templates for surface nanopatterning with sub-20 nm features. The replicated patterns can, however, only be as precise as their templates. Thus, the investigation of the morphology of polymer domains is of great importance. Commonly used analytical techniques (neutron scattering, scanning force microscopy) either lack spatial information or nanoscale resolution. Using advanced analytical (scanning) transmission electron microscopy ((S)TEM), we provide real space information on polymer domain morphology and interfaces between polystyrene (PS) and polymethylmethacrylate (PMMA) in cylinder- and lamellae-forming BCPs at highest resolution. This allows us to correlate the internal structure of polymer domains with line edge roughnesses, interface widths and domain sizes. STEM is employed for high-resolution imaging, electron energy loss spectroscopy and energy filtered TEM (EFTEM) spectroscopic imaging for material identification and EFTEM thickness mapping for visualisation of material densities at defects. The volume fraction of non-phase separated polymer species can be analysed by EFTEM. These methods give new insights into the morphology of polymer domains the exact knowledge of which will allow to improve pattern quality for nanolithography."}],"user_id":"77496"},{"date_updated":"2023-01-10T12:12:40Z","doi":"10.1016/j.ultramic.2020.113118","language":[{"iso":"eng"}],"title":"Influence of lens aberrations, specimen thickness and tilt on differential phase contrast STEM images","department":[{"_id":"15"},{"_id":"230"}],"publication_identifier":{"issn":["0304-3991"]},"publication_status":"published","intvolume":" 219","_id":"34088","article_number":"113118","year":"2020","type":"journal_article","citation":{"ama":"Bürger J, Riedl T, Lindner J. Influence of lens aberrations, specimen thickness and tilt on differential phase contrast STEM images. Ultramicroscopy. 2020;219. doi:10.1016/j.ultramic.2020.113118","apa":"Bürger, J., Riedl, T., & Lindner, J. (2020). Influence of lens aberrations, specimen thickness and tilt on differential phase contrast STEM images. Ultramicroscopy, 219, Article 113118. https://doi.org/10.1016/j.ultramic.2020.113118","chicago":"Bürger, Julius, Thomas Riedl, and Jörg Lindner. “Influence of Lens Aberrations, Specimen Thickness and Tilt on Differential Phase Contrast STEM Images.” Ultramicroscopy 219 (2020). https://doi.org/10.1016/j.ultramic.2020.113118.","mla":"Bürger, Julius, et al. “Influence of Lens Aberrations, Specimen Thickness and Tilt on Differential Phase Contrast STEM Images.” Ultramicroscopy, vol. 219, 113118, Elsevier BV, 2020, doi:10.1016/j.ultramic.2020.113118.","bibtex":"@article{Bürger_Riedl_Lindner_2020, title={Influence of lens aberrations, specimen thickness and tilt on differential phase contrast STEM images}, volume={219}, DOI={10.1016/j.ultramic.2020.113118}, number={113118}, journal={Ultramicroscopy}, publisher={Elsevier BV}, author={Bürger, Julius and Riedl, Thomas and Lindner, Jörg}, year={2020} }","short":"J. Bürger, T. Riedl, J. Lindner, Ultramicroscopy 219 (2020).","ieee":"J. Bürger, T. Riedl, and J. Lindner, “Influence of lens aberrations, specimen thickness and tilt on differential phase contrast STEM images,” Ultramicroscopy, vol. 219, Art. no. 113118, 2020, doi: 10.1016/j.ultramic.2020.113118."},"user_id":"77496","publication":"Ultramicroscopy","keyword":["Instrumentation","Atomic and Molecular Physics","and Optics","Electronic","Optical and Magnetic Materials"],"publisher":"Elsevier BV","author":[{"id":"46952","last_name":"Bürger","full_name":"Bürger, Julius","first_name":"Julius"},{"full_name":"Riedl, Thomas","first_name":"Thomas","id":"36950","last_name":"Riedl"},{"last_name":"Lindner","id":"20797","first_name":"Jörg","full_name":"Lindner, Jörg"}],"date_created":"2022-11-15T14:15:16Z","status":"public","volume":219},{"page":"095701","year":"2020","citation":{"ieee":"K. Engelkemeier et al., “Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties,” Nanotechnology, vol. 31, p. 095701, 2020, doi: 10.1088/1361-6528/ab55bc.","short":"K. Engelkemeier, J. Lindner, J. Bürger, K. Vaupel, M. Hartmann, M. Tiemann, K.-P. Hoyer, M. Schaper, Nanotechnology 31 (2020) 095701.","mla":"Engelkemeier, Katja, et al. “Nano-Architectural Complexity of Zinc Oxide Nanowall Hollow Microspheres and Their Structural Properties.” Nanotechnology, vol. 31, 2020, p. 095701, doi:10.1088/1361-6528/ab55bc.","bibtex":"@article{Engelkemeier_Lindner_Bürger_Vaupel_Hartmann_Tiemann_Hoyer_Schaper_2020, title={Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties}, volume={31}, DOI={10.1088/1361-6528/ab55bc}, journal={Nanotechnology}, author={Engelkemeier, Katja and Lindner, Jörg and Bürger, Julius and Vaupel, Kathrin and Hartmann, Marc and Tiemann, Michael and Hoyer, Kay-Peter and Schaper, Mirko}, year={2020}, pages={095701} }","chicago":"Engelkemeier, Katja, Jörg Lindner, Julius Bürger, Kathrin Vaupel, Marc Hartmann, Michael Tiemann, Kay-Peter Hoyer, and Mirko Schaper. “Nano-Architectural Complexity of Zinc Oxide Nanowall Hollow Microspheres and Their Structural Properties.” Nanotechnology 31 (2020): 095701. https://doi.org/10.1088/1361-6528/ab55bc.","ama":"Engelkemeier K, Lindner J, Bürger J, et al. Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties. Nanotechnology. 2020;31:095701. doi:10.1088/1361-6528/ab55bc","apa":"Engelkemeier, K., Lindner, J., Bürger, J., Vaupel, K., Hartmann, M., Tiemann, M., Hoyer, K.-P., & Schaper, M. (2020). Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties. Nanotechnology, 31, 095701. https://doi.org/10.1088/1361-6528/ab55bc"},"type":"journal_article","_id":"24100","intvolume":" 31","publication":"Nanotechnology","author":[{"full_name":"Engelkemeier, Katja","first_name":"Katja","id":"21743","last_name":"Engelkemeier"},{"first_name":"Jörg","full_name":"Lindner, Jörg","last_name":"Lindner","id":"20797"},{"full_name":"Bürger, Julius","first_name":"Julius","id":"46952","last_name":"Bürger"},{"last_name":"Vaupel","full_name":"Vaupel, Kathrin","first_name":"Kathrin"},{"first_name":"Marc","full_name":"Hartmann, Marc","last_name":"Hartmann"},{"orcid":"0000-0003-1711-2722","full_name":"Tiemann, Michael","first_name":"Michael","id":"23547","last_name":"Tiemann"},{"full_name":"Hoyer, Kay-Peter","first_name":"Kay-Peter","id":"48411","last_name":"Hoyer"},{"first_name":"Mirko","full_name":"Schaper, Mirko","last_name":"Schaper","id":"43720"}],"quality_controlled":"1","volume":31,"date_created":"2021-09-10T06:49:55Z","status":"public","abstract":[{"lang":"eng","text":"Zinc oxide (ZnO) hollow spheres with defined morphology and micro-/nanostructure are prepared by a hydrothermal synthesis approach. The materials possess fine-leaved structures at their particle surface (nanowall hollow micro spheres). Morphology control is achieved by citric acid used as an additive in variable relative quantities during the synthesis. The structure formation is studied by various time-dependent ex situ methods, such as scanning electron microscopy, x-ray diffraction, and Raman spectroscopy. The fine-leaved surface structure is characterized by high-resolution transmission electron microscopy techniques (HRTEM, STEM), using a high-angle annular dark field detector, as well as by differential phase contrast analysis. In-depth structural characterization of the nanowalls by drop-by-drop ex situ FE-SEM analysis provides insight into possible structure formation mechanisms. Further investigation addresses the thermal stability of the particle morphology and the enhancement of the surface-to-volume ratio by heat treatment (examined by N2 physisorption)."}],"article_type":"original","user_id":"43720","language":[{"iso":"eng"}],"date_updated":"2023-06-01T14:29:58Z","doi":"10.1088/1361-6528/ab55bc","department":[{"_id":"9"},{"_id":"158"},{"_id":"301"},{"_id":"286"},{"_id":"35"},{"_id":"307"},{"_id":"2"}],"publication_status":"published","publication_identifier":{"issn":["0957-4484","1361-6528"]},"title":"Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties"},{"language":[{"iso":"eng"}],"year":"2019","type":"journal_article","citation":{"chicago":"Meinderink, Dennis, Karlo J.R. Nolkemper, Julius Bürger, Alejandro G. Orive, Jörg K.N. Lindner, and Guido Grundmeier. “Spray Coating of Poly(Acrylic Acid)/ZnO Tetrapod Adhesion Promoting Nanocomposite Films for Polymer Laminates.” Surface and Coatings Technology, 2019, 112–22. https://doi.org/10.1016/j.surfcoat.2019.06.083.","ama":"Meinderink D, Nolkemper KJR, Bürger J, Orive AG, Lindner JKN, Grundmeier G. Spray coating of poly(acrylic acid)/ZnO tetrapod adhesion promoting nanocomposite films for polymer laminates. Surface and Coatings Technology. 2019:112-122. doi:10.1016/j.surfcoat.2019.06.083","apa":"Meinderink, D., Nolkemper, K. J. R., Bürger, J., Orive, A. G., Lindner, J. K. N., & Grundmeier, G. (2019). Spray coating of poly(acrylic acid)/ZnO tetrapod adhesion promoting nanocomposite films for polymer laminates. Surface and Coatings Technology, 112–122. https://doi.org/10.1016/j.surfcoat.2019.06.083","mla":"Meinderink, Dennis, et al. “Spray Coating of Poly(Acrylic Acid)/ZnO Tetrapod Adhesion Promoting Nanocomposite Films for Polymer Laminates.” Surface and Coatings Technology, 2019, pp. 112–22, doi:10.1016/j.surfcoat.2019.06.083.","bibtex":"@article{Meinderink_Nolkemper_Bürger_Orive_Lindner_Grundmeier_2019, title={Spray coating of poly(acrylic acid)/ZnO tetrapod adhesion promoting nanocomposite films for polymer laminates}, DOI={10.1016/j.surfcoat.2019.06.083}, journal={Surface and Coatings Technology}, author={Meinderink, Dennis and Nolkemper, Karlo J.R. and Bürger, Julius and Orive, Alejandro G. and Lindner, Jörg K.N. and Grundmeier, Guido}, year={2019}, pages={112–122} }","short":"D. Meinderink, K.J.R. Nolkemper, J. Bürger, A.G. Orive, J.K.N. Lindner, G. Grundmeier, Surface and Coatings Technology (2019) 112–122.","ieee":"D. Meinderink, K. J. R. Nolkemper, J. Bürger, A. G. Orive, J. K. N. Lindner, and G. Grundmeier, “Spray coating of poly(acrylic acid)/ZnO tetrapod adhesion promoting nanocomposite films for polymer laminates,” Surface and Coatings Technology, pp. 112–122, 2019."},"page":"112-122","date_updated":"2022-01-06T06:55:38Z","_id":"22687","doi":"10.1016/j.surfcoat.2019.06.083","author":[{"last_name":"Meinderink","id":"32378","first_name":"Dennis","full_name":"Meinderink, Dennis","orcid":"0000-0002-2755-6514"},{"first_name":"Karlo J.R.","full_name":"Nolkemper, Karlo J.R.","last_name":"Nolkemper"},{"first_name":"Julius","full_name":"Bürger, Julius","last_name":"Bürger","id":"46952"},{"full_name":"Orive, Alejandro G.","first_name":"Alejandro G.","last_name":"Orive"},{"last_name":"Lindner","full_name":"Lindner, Jörg K.N.","first_name":"Jörg K.N."},{"id":"194","last_name":"Grundmeier","full_name":"Grundmeier, Guido","first_name":"Guido"}],"department":[{"_id":"302"}],"publication":"Surface and Coatings Technology","status":"public","date_created":"2021-07-09T12:14:03Z","publication_status":"published","publication_identifier":{"issn":["0257-8972"]},"user_id":"32378","title":"Spray coating of poly(acrylic acid)/ZnO tetrapod adhesion promoting nanocomposite films for polymer laminates"},{"author":[{"last_name":"Engelkemeier","id":"21743","first_name":"Katja","full_name":"Engelkemeier, Katja"},{"full_name":"Lindner, Jörg K N","first_name":"Jörg K N","last_name":"Lindner"},{"full_name":"Bürger, Julius","first_name":"Julius","id":"46952","last_name":"Bürger"},{"last_name":"Vaupel","full_name":"Vaupel, Kathrin","first_name":"Kathrin"},{"first_name":"Marc","full_name":"Hartmann, Marc","last_name":"Hartmann"},{"id":"23547","last_name":"Tiemann","orcid":"0000-0003-1711-2722","full_name":"Tiemann, Michael","first_name":"Michael"},{"first_name":"Kay-Peter","full_name":"Hoyer, Kay-Peter","last_name":"Hoyer","id":"48411"},{"full_name":"Schaper, Mirko","first_name":"Mirko","id":"43720","last_name":"Schaper"}],"publisher":"IOP Publishing","quality_controlled":"1","publication":"Nanotechnology","keyword":["Electrical and Electronic Engineering","Mechanical Engineering","Mechanics of Materials","General Materials Science","General Chemistry","Bioengineering"],"status":"public","date_created":"2023-02-02T14:44:47Z","volume":31,"user_id":"43720","type":"journal_article","year":"2019","citation":{"short":"K. Engelkemeier, J.K.N. Lindner, J. Bürger, K. Vaupel, M. Hartmann, M. Tiemann, K.-P. Hoyer, M. Schaper, Nanotechnology 31 (2019).","ieee":"K. Engelkemeier et al., “Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties,” Nanotechnology, vol. 31, no. 9, Art. no. 095701, 2019, doi: 10.1088/1361-6528/ab55bc.","chicago":"Engelkemeier, Katja, Jörg K N Lindner, Julius Bürger, Kathrin Vaupel, Marc Hartmann, Michael Tiemann, Kay-Peter Hoyer, and Mirko Schaper. “Nano-Architectural Complexity of Zinc Oxide Nanowall Hollow Microspheres and Their Structural Properties.” Nanotechnology 31, no. 9 (2019). https://doi.org/10.1088/1361-6528/ab55bc.","ama":"Engelkemeier K, Lindner JKN, Bürger J, et al. Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties. Nanotechnology. 2019;31(9). doi:10.1088/1361-6528/ab55bc","apa":"Engelkemeier, K., Lindner, J. K. N., Bürger, J., Vaupel, K., Hartmann, M., Tiemann, M., Hoyer, K.-P., & Schaper, M. (2019). Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties. Nanotechnology, 31(9), Article 095701. https://doi.org/10.1088/1361-6528/ab55bc","bibtex":"@article{Engelkemeier_Lindner_Bürger_Vaupel_Hartmann_Tiemann_Hoyer_Schaper_2019, title={Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties}, volume={31}, DOI={10.1088/1361-6528/ab55bc}, number={9095701}, journal={Nanotechnology}, publisher={IOP Publishing}, author={Engelkemeier, Katja and Lindner, Jörg K N and Bürger, Julius and Vaupel, Kathrin and Hartmann, Marc and Tiemann, Michael and Hoyer, Kay-Peter and Schaper, Mirko}, year={2019} }","mla":"Engelkemeier, Katja, et al. “Nano-Architectural Complexity of Zinc Oxide Nanowall Hollow Microspheres and Their Structural Properties.” Nanotechnology, vol. 31, no. 9, 095701, IOP Publishing, 2019, doi:10.1088/1361-6528/ab55bc."},"_id":"41524","intvolume":" 31","issue":"9","article_number":"095701","department":[{"_id":"9"},{"_id":"158"}],"publication_status":"published","publication_identifier":{"issn":["0957-4484","1361-6528"]},"title":"Nano-architectural complexity of zinc oxide nanowall hollow microspheres and their structural properties","language":[{"iso":"eng"}],"date_updated":"2023-06-01T14:27:50Z","doi":"10.1088/1361-6528/ab55bc"},{"publication_status":"published","publication_identifier":{"issn":["0743-7463","1520-5827"]},"department":[{"_id":"286"},{"_id":"15"},{"_id":"2"}],"title":"On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays","language":[{"iso":"eng"}],"doi":"10.1021/acs.langmuir.8b00793","date_updated":"2022-01-06T06:59:54Z","date_created":"2018-08-15T12:33:42Z","has_accepted_license":"1","status":"public","publication":"Langmuir","file_date_updated":"2018-08-15T12:44:51Z","author":[{"first_name":"Katharina","full_name":"Brassat, Katharina","last_name":"Brassat","id":"11305"},{"first_name":"Saminathan","full_name":"Ramakrishnan, Saminathan","last_name":"Ramakrishnan"},{"id":"46952","last_name":"Bürger","full_name":"Bürger, Julius","first_name":"Julius"},{"full_name":"Hanke, Marcel","first_name":"Marcel","last_name":"Hanke"},{"last_name":"Doostdar","full_name":"Doostdar, Mahnaz","first_name":"Mahnaz"},{"last_name":"Lindner","id":"20797","first_name":"Jörg","full_name":"Lindner, Jörg"},{"last_name":"Grundmeier","full_name":"Grundmeier, Guido","first_name":"Guido"},{"full_name":"Keller, Adrian","first_name":"Adrian","last_name":"Keller"}],"publisher":"American Chemical Society (ACS)","file":[{"file_name":"On_the_adsorption_of_DNA_origami_nanostructures_in_nanohole_arrays_2018.pdf","date_created":"2018-08-15T12:44:51Z","access_level":"closed","file_id":"3913","creator":"hclaudia","file_size":1778532,"success":1,"relation":"main_file","date_updated":"2018-08-15T12:44:51Z","content_type":"application/pdf"}],"ddc":["530"],"user_id":"55706","abstract":[{"text":"DNA origami nanostructures are versatile substrates for the controlled arrangement of molecular\r\ncapture sites with nanometer precision and thus have many promising applications in singlemolecule\r\nbioanalysis. Here, we investigate the adsorption of DNA origami nanostructures in\r\nnanohole arrays which represent an important class of biosensors and may benefit from the\r\nincorporation of DNA origami-based molecular probes. Nanoholes with well-defined diameter\r\nthat enable the adsorption of single DNA origami triangles are fabricated in Au films on Siwafers by nanosphere lithography. The efficiency of directed DNA origami adsorption on the\r\nexposed SiO2 areas at the bottoms of the nanoholes is evaluated in dependence of various\r\nparameters, i.e., Mg2+ and DNA origami concentrations, buffer strength, adsorption time, and\r\nnanohole diameter. We observe that the buffer strength has a surprisingly strong effect on DNA\r\norigami adsorption in the nanoholes and that multiple DNA origami triangles with 120 nm edge\r\nlength can adsorb in nanoholes as small as 120 nm in diameter. We attribute the latter\r\nobservation to the low lateral mobility of once adsorbed DNA origami on the SiO2 surface, in\r\ncombination with parasitic adsorption to the Au film. While parasitic adsorption can be\r\nsuppressed by modifying the Au film with a hydrophobic self-assembled monolayer, the limited\r\nsurface mobility of the adsorbed DNA origami still leads to poor localization accuracy in the\r\nnanoholes and results in many DNA origami crossing the boundary to the Au film even under\r\noptimized conditions. We discuss possible ways to minimize this effect by varying the\r\ncomposition of the adsorption buffer, employing different fabrication conditions, or using other\r\nsubstrate materials for nanohole array fabrication.","lang":"eng"}],"article_type":"original","citation":{"short":"K. Brassat, S. Ramakrishnan, J. Bürger, M. Hanke, M. Doostdar, J. Lindner, G. Grundmeier, A. Keller, Langmuir (2018).","ieee":"K. Brassat et al., “On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays,” Langmuir, 2018.","ama":"Brassat K, Ramakrishnan S, Bürger J, et al. On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays. Langmuir. 2018. doi:10.1021/acs.langmuir.8b00793","apa":"Brassat, K., Ramakrishnan, S., Bürger, J., Hanke, M., Doostdar, M., Lindner, J., … Keller, A. (2018). On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays. Langmuir. https://doi.org/10.1021/acs.langmuir.8b00793","chicago":"Brassat, Katharina, Saminathan Ramakrishnan, Julius Bürger, Marcel Hanke, Mahnaz Doostdar, Jörg Lindner, Guido Grundmeier, and Adrian Keller. “On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays.” Langmuir, 2018. https://doi.org/10.1021/acs.langmuir.8b00793.","mla":"Brassat, Katharina, et al. “On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays.” Langmuir, American Chemical Society (ACS), 2018, doi:10.1021/acs.langmuir.8b00793.","bibtex":"@article{Brassat_Ramakrishnan_Bürger_Hanke_Doostdar_Lindner_Grundmeier_Keller_2018, title={On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays}, DOI={10.1021/acs.langmuir.8b00793}, journal={Langmuir}, publisher={American Chemical Society (ACS)}, author={Brassat, Katharina and Ramakrishnan, Saminathan and Bürger, Julius and Hanke, Marcel and Doostdar, Mahnaz and Lindner, Jörg and Grundmeier, Guido and Keller, Adrian}, year={2018} }"},"type":"journal_article","year":"2018","_id":"3912"},{"citation":{"short":"K. Brassat, S. Ramakrishnan, J. Bürger, M. Hanke, M. Doostdar, J. Lindner, G. Grundmeier, A. Keller, Langmuir 34 (2018) 14757–14765.","ieee":"K. Brassat et al., “On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays,” Langmuir, vol. 34, pp. 14757–14765, 2018.","chicago":"Brassat, Katharina, Saminathan Ramakrishnan, Julius Bürger, Marcel Hanke, Mahnaz Doostdar, Jörg Lindner, Guido Grundmeier, and Adrian Keller. “On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays.” Langmuir 34 (2018): 14757–65. https://doi.org/10.1021/acs.langmuir.8b00793.","ama":"Brassat K, Ramakrishnan S, Bürger J, et al. On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays. Langmuir. 2018;34:14757-14765. doi:10.1021/acs.langmuir.8b00793","apa":"Brassat, K., Ramakrishnan, S., Bürger, J., Hanke, M., Doostdar, M., Lindner, J., … Keller, A. (2018). On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays. Langmuir, 34, 14757–14765. https://doi.org/10.1021/acs.langmuir.8b00793","bibtex":"@article{Brassat_Ramakrishnan_Bürger_Hanke_Doostdar_Lindner_Grundmeier_Keller_2018, title={On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays}, volume={34}, DOI={10.1021/acs.langmuir.8b00793}, journal={Langmuir}, author={Brassat, Katharina and Ramakrishnan, Saminathan and Bürger, Julius and Hanke, Marcel and Doostdar, Mahnaz and Lindner, Jörg and Grundmeier, Guido and Keller, Adrian}, year={2018}, pages={14757–14765} }","mla":"Brassat, Katharina, et al. “On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays.” Langmuir, vol. 34, 2018, pp. 14757–65, doi:10.1021/acs.langmuir.8b00793."},"type":"journal_article","year":"2018","page":"14757-14765","language":[{"iso":"eng"}],"doi":"10.1021/acs.langmuir.8b00793","date_updated":"2022-01-06T06:55:38Z","_id":"22664","intvolume":" 34","volume":34,"publication_status":"published","publication_identifier":{"issn":["0743-7463","1520-5827"]},"status":"public","date_created":"2021-07-08T12:23:44Z","author":[{"first_name":"Katharina","full_name":"Brassat, Katharina","last_name":"Brassat","id":"11305"},{"full_name":"Ramakrishnan, Saminathan","first_name":"Saminathan","last_name":"Ramakrishnan"},{"full_name":"Bürger, Julius","first_name":"Julius","id":"46952","last_name":"Bürger"},{"last_name":"Hanke","first_name":"Marcel","full_name":"Hanke, Marcel"},{"last_name":"Doostdar","first_name":"Mahnaz","full_name":"Doostdar, Mahnaz"},{"first_name":"Jörg","full_name":"Lindner, Jörg","last_name":"Lindner","id":"20797"},{"id":"194","last_name":"Grundmeier","full_name":"Grundmeier, Guido","first_name":"Guido"},{"last_name":"Keller","id":"48864","first_name":"Adrian","full_name":"Keller, Adrian","orcid":"0000-0001-7139-3110"}],"department":[{"_id":"302"},{"_id":"286"}],"publication":"Langmuir","title":"On the Adsorption of DNA Origami Nanostructures in Nanohole Arrays","user_id":"48864"},{"author":[{"full_name":"Riedl, Thomas","first_name":"Thomas","id":"36950","last_name":"Riedl"},{"full_name":"Bürger, Julius","first_name":"Julius","id":"46952","last_name":"Bürger"},{"last_name":"Kunnathully","full_name":"Kunnathully, Vinay ","first_name":"Vinay "},{"full_name":"Wiegand, Marie","first_name":"Marie","last_name":"Wiegand"},{"full_name":"Duschik, K.","first_name":"K.","last_name":"Duschik"},{"last_name":"Ramermann","first_name":"D. ","full_name":"Ramermann, D. "},{"last_name":"Ennen","first_name":"I. ","full_name":"Ennen, I. "},{"first_name":"Y. ","full_name":"Hertle, Y. ","last_name":"Hertle"},{"first_name":"Mirko","full_name":"Schaper, Mirko","last_name":"Schaper"},{"last_name":"Hellweg","full_name":"Hellweg, T. ","first_name":"T. "},{"first_name":"A.","full_name":"Hütten, A.","last_name":"Hütten"},{"full_name":"Lindner, Jörg","first_name":"Jörg","id":"20797","last_name":"Lindner"}],"department":[{"_id":"15"},{"_id":"286"}],"status":"public","date_created":"2018-09-18T11:53:03Z","user_id":"55706","title":"Nanostructure Research using Transmission Electron Microscopy at the new OWL Analytic Centre","year":"2018","type":"conference","citation":{"short":"T. Riedl, J. Bürger, V. Kunnathully, M. Wiegand, K. Duschik, D. Ramermann, I. Ennen, Y. Hertle, M. Schaper, T. Hellweg, A. Hütten, J. Lindner, in: 2018.","ieee":"T. Riedl et al., “Nanostructure Research using Transmission Electron Microscopy at the new OWL Analytic Centre,” presented at the 8th NRW Nano Conference, Dortmund (Germany), 2018.","chicago":"Riedl, Thomas, Julius Bürger, Vinay Kunnathully, Marie Wiegand, K. Duschik, D. Ramermann, I. Ennen, et al. “Nanostructure Research Using Transmission Electron Microscopy at the New OWL Analytic Centre,” 2018.","apa":"Riedl, T., Bürger, J., Kunnathully, V., Wiegand, M., Duschik, K., Ramermann, D., … Lindner, J. (2018). Nanostructure Research using Transmission Electron Microscopy at the new OWL Analytic Centre. Presented at the 8th NRW Nano Conference, Dortmund (Germany).","ama":"Riedl T, Bürger J, Kunnathully V, et al. Nanostructure Research using Transmission Electron Microscopy at the new OWL Analytic Centre. In: ; 2018.","mla":"Riedl, Thomas, et al. Nanostructure Research Using Transmission Electron Microscopy at the New OWL Analytic Centre. 2018.","bibtex":"@inproceedings{Riedl_Bürger_Kunnathully_Wiegand_Duschik_Ramermann_Ennen_Hertle_Schaper_Hellweg_et al._2018, title={Nanostructure Research using Transmission Electron Microscopy at the new OWL Analytic Centre}, author={Riedl, Thomas and Bürger, Julius and Kunnathully, Vinay and Wiegand, Marie and Duschik, K. and Ramermann, D. and Ennen, I. and Hertle, Y. and Schaper, Mirko and Hellweg, T. and et al.}, year={2018} }"},"_id":"4447","date_updated":"2022-01-06T07:01:04Z","conference":{"end_date":"2018-11-22","name":"8th NRW Nano Conference","start_date":"2018-11-21","location":"Dortmund (Germany)"}},{"user_id":"55706","ddc":["530"],"abstract":[{"lang":"eng","text":"Bottom-up patterning techniques allow for the creation of surfaces with ordered arrays of nanoscale features\r\non large areas. Two bottom-up techniques suitable for the formation of regular nanopatterns on\r\ndifferent length scales are nanosphere lithography (NSL) and block copolymer (BCP) lithography. In this\r\npaper it is shown that NSL and BCP lithography can be combined to easily design hierarchically nanopatterned\r\nsurfaces of different materials. Nanosphere lithography is used for the pre-patterning of\r\nsurfaces with antidots, i.e. hexagonally arranged cylindrical holes in thin films of Au, Pt and TiO2 on SiO2,\r\nproviding a periodic chemical and topographical contrast on the surface suitable for templating in subsequent\r\nBCP lithography. PS-b-PMMA BCP is used in the second self-assembly step to form hexagonally\r\narranged nanopores with sub-20 nm diameter within the antidots upon microphase separation. To\r\nachieve this the microphase separation of BCP on planar surfaces is studied, too, and it is demonstrated\r\nfor the first time that vertical BCP nanopores can be formed on TiO2, Au and Pt films without using any\r\nneutralization layers. To explain this the influence of surface energy, polarity and roughness on the microphase\r\nseparation is investigated and discussed along with the wetting state of BCP on NSL-pre-patterned\r\nsurfaces. The presented novel route for the creation of advanced hierarchical nanopatterns is easily applicable\r\non large-area surfaces of different materials. This flexibility makes it suitable for a broad range of\r\napplications, from the morphological design of biocompatible surfaces for life science to complex\r\npre-patterns for nanoparticle placement in semiconductor technology."}],"article_type":"original","date_created":"2018-08-16T12:59:02Z","status":"public","has_accepted_license":"1","volume":10,"file":[{"file_id":"3922","creator":"hclaudia","file_size":3875099,"relation":"main_file","success":1,"content_type":"application/pdf","date_updated":"2018-08-16T12:59:56Z","date_created":"2018-08-16T12:59:56Z","file_name":"Hierarchical_nanopores_by_block_copolymer_lithography_on_surfaces_of_different_materials_pre-patterned_by_nanosphere_lithography_2018.pdf","access_level":"closed"}],"publication":"Nanoscale","file_date_updated":"2018-08-16T12:59:56Z","publisher":"Royal Society of Chemistry (RSC)","author":[{"id":"11305","last_name":"Brassat","full_name":"Brassat, Katharina","first_name":"Katharina"},{"first_name":"Daniel","full_name":"Kool, Daniel","last_name":"Kool","id":"44586"},{"full_name":"Bürger, Julius","first_name":"Julius","id":"46952","last_name":"Bürger"},{"first_name":"Jörg","full_name":"Lindner, Jörg","last_name":"Lindner","id":"20797"}],"issue":"21","_id":"3921","intvolume":" 10","page":"10005-10017","type":"journal_article","year":"2018","citation":{"ieee":"K. Brassat, D. Kool, J. Bürger, and J. Lindner, “Hierarchical nanopores formed by block copolymer lithography on the surfaces of different materials pre-patterned by nanosphere lithography,” Nanoscale, vol. 10, no. 21, pp. 10005–10017, 2018.","short":"K. Brassat, D. Kool, J. Bürger, J. Lindner, Nanoscale 10 (2018) 10005–10017.","mla":"Brassat, Katharina, et al. “Hierarchical Nanopores Formed by Block Copolymer Lithography on the Surfaces of Different Materials Pre-Patterned by Nanosphere Lithography.” Nanoscale, vol. 10, no. 21, Royal Society of Chemistry (RSC), 2018, pp. 10005–17, doi:10.1039/c8nr01397g.","bibtex":"@article{Brassat_Kool_Bürger_Lindner_2018, title={Hierarchical nanopores formed by block copolymer lithography on the surfaces of different materials pre-patterned by nanosphere lithography}, volume={10}, DOI={10.1039/c8nr01397g}, number={21}, journal={Nanoscale}, publisher={Royal Society of Chemistry (RSC)}, author={Brassat, Katharina and Kool, Daniel and Bürger, Julius and Lindner, Jörg}, year={2018}, pages={10005–10017} }","chicago":"Brassat, Katharina, Daniel Kool, Julius Bürger, and Jörg Lindner. “Hierarchical Nanopores Formed by Block Copolymer Lithography on the Surfaces of Different Materials Pre-Patterned by Nanosphere Lithography.” Nanoscale 10, no. 21 (2018): 10005–17. https://doi.org/10.1039/c8nr01397g.","ama":"Brassat K, Kool D, Bürger J, Lindner J. Hierarchical nanopores formed by block copolymer lithography on the surfaces of different materials pre-patterned by nanosphere lithography. Nanoscale. 2018;10(21):10005-10017. doi:10.1039/c8nr01397g","apa":"Brassat, K., Kool, D., Bürger, J., & Lindner, J. (2018). Hierarchical nanopores formed by block copolymer lithography on the surfaces of different materials pre-patterned by nanosphere lithography. Nanoscale, 10(21), 10005–10017. https://doi.org/10.1039/c8nr01397g"},"title":"Hierarchical nanopores formed by block copolymer lithography on the surfaces of different materials pre-patterned by nanosphere lithography","publication_identifier":{"issn":["2040-3364","2040-3372"]},"publication_status":"published","department":[{"_id":"286"},{"_id":"15"}],"doi":"10.1039/c8nr01397g","date_updated":"2022-01-06T06:59:55Z","language":[{"iso":"eng"}]},{"title":"Micro- and nanopatterned surfaces with tailored chemical and topographical contrast by self-assembly techniques","user_id":"55706","status":"public","date_created":"2018-08-20T13:24:15Z","author":[{"id":"11305","last_name":"Brassat","full_name":"Brassat, Katharina","first_name":"Katharina"},{"first_name":"Daniel","full_name":"Kool, Daniel","last_name":"Kool","id":"44586"},{"full_name":"Bürger, Julius","first_name":"Julius","id":"46952","last_name":"Bürger"},{"id":"20797","last_name":"Lindner","full_name":"Lindner, Jörg","first_name":"Jörg"}],"department":[{"_id":"286"},{"_id":"15"}],"date_updated":"2022-01-06T06:59:59Z","_id":"3952","conference":{"end_date":"2017-09-21","name":"E-MRS Fall Meeting 2017","start_date":"2017-09-18","location":"Warsaw (Poland)"},"citation":{"apa":"Brassat, K., Kool, D., Bürger, J., & Lindner, J. (2017). Micro- and nanopatterned surfaces with tailored chemical and topographical contrast by self-assembly techniques. Presented at the E-MRS Fall Meeting 2017, Warsaw (Poland).","ama":"Brassat K, Kool D, Bürger J, Lindner J. Micro- and nanopatterned surfaces with tailored chemical and topographical contrast by self-assembly techniques. In: ; 2017.","chicago":"Brassat, Katharina, Daniel Kool, Julius Bürger, and Jörg Lindner. “Micro- and Nanopatterned Surfaces with Tailored Chemical and Topographical Contrast by Self-Assembly Techniques,” 2017.","bibtex":"@inproceedings{Brassat_Kool_Bürger_Lindner_2017, title={Micro- and nanopatterned surfaces with tailored chemical and topographical contrast by self-assembly techniques}, author={Brassat, Katharina and Kool, Daniel and Bürger, Julius and Lindner, Jörg}, year={2017} }","mla":"Brassat, Katharina, et al. Micro- and Nanopatterned Surfaces with Tailored Chemical and Topographical Contrast by Self-Assembly Techniques. 2017.","short":"K. Brassat, D. Kool, J. Bürger, J. Lindner, in: 2017.","ieee":"K. Brassat, D. Kool, J. Bürger, and J. Lindner, “Micro- and nanopatterned surfaces with tailored chemical and topographical contrast by self-assembly techniques,” presented at the E-MRS Fall Meeting 2017, Warsaw (Poland), 2017."},"type":"conference","year":"2017"},{"ddc":["530"],"user_id":"14931","article_type":"original","abstract":[{"text":"Switchable two dimensional liquid crystal diffraction gratings are promising can-\r\ndidates in beam steering devices, multiplexers and holographic displays. For these areas of applications a high degree of integration in optical systems is much sought-after. In the context of diffraction gratings this means that the angle of diffraction should be rather high, which typically poses a problem as the fabrication of small grating periods is challenging. In this paper, we propose the use of nanosphere lithography (NSL) for the fabrication of two-dimensionally\r\nstructured electrodes with a periodicity of a few micrometers. NSL is based on the self-assembly of micro- or nanometer sized spheres into monolayers. It allows for easy substrate structuring on wafer scale. The manufactured electrode is combined with a liquid crystalline polymer-stabilized blue phase, which facilitates sub-millisecond electrical switching of the diffraction efficiency at adiffractionangle of 21.4°.","lang":"eng"}],"volume":25,"status":"public","has_accepted_license":"1","date_created":"2018-08-21T12:04:28Z","author":[{"first_name":"M.","full_name":"Wahle, M.","last_name":"Wahle"},{"last_name":"Brassat","id":"11305","first_name":"Katharina","full_name":"Brassat, Katharina"},{"full_name":"Ebel, J.","first_name":"J.","last_name":"Ebel"},{"id":"46952","last_name":"Bürger","full_name":"Bürger, Julius","first_name":"Julius"},{"last_name":"Lindner","id":"20797","first_name":"Jörg","full_name":"Lindner, Jörg"},{"last_name":"Kitzerow","id":"254","first_name":"Heinz-Siegfried","full_name":"Kitzerow, Heinz-Siegfried"}],"publication":"Optics Express 25","file_date_updated":"2018-08-21T12:02:06Z","file":[{"file_size":4327427,"file_id":"3998","creator":"hclaudia","content_type":"application/pdf","date_updated":"2018-08-21T12:02:06Z","relation":"main_file","success":1,"date_created":"2018-08-21T12:02:06Z","file_name":"Two-dimensional switchable blue phase gratings manufactured by nanosphere lithography.pdf","access_level":"closed"}],"issue":"19","intvolume":" 25","_id":"3997","year":"2017","type":"journal_article","citation":{"ama":"Wahle M, Brassat K, Ebel J, Bürger J, Lindner J, Kitzerow H-S. Two-dimensional switchable blue phase gratings manufactured by nanosphere lithography. Optics Express 25. 2017;25(19):22608-22619. doi:10.1364/OE.25.022607","apa":"Wahle, M., Brassat, K., Ebel, J., Bürger, J., Lindner, J., & Kitzerow, H.-S. (2017). Two-dimensional switchable blue phase gratings manufactured by nanosphere lithography. Optics Express 25, 25(19), 22608–22619. https://doi.org/10.1364/OE.25.022607","chicago":"Wahle, M., Katharina Brassat, J. Ebel, Julius Bürger, Jörg Lindner, and Heinz-Siegfried Kitzerow. “Two-Dimensional Switchable Blue Phase Gratings Manufactured by Nanosphere Lithography.” Optics Express 25 25, no. 19 (2017): 22608–19. https://doi.org/10.1364/OE.25.022607.","bibtex":"@article{Wahle_Brassat_Ebel_Bürger_Lindner_Kitzerow_2017, title={Two-dimensional switchable blue phase gratings manufactured by nanosphere lithography}, volume={25}, DOI={10.1364/OE.25.022607}, number={19}, journal={Optics Express 25}, author={Wahle, M. and Brassat, Katharina and Ebel, J. and Bürger, Julius and Lindner, Jörg and Kitzerow, Heinz-Siegfried}, year={2017}, pages={22608–22619} }","mla":"Wahle, M., et al. “Two-Dimensional Switchable Blue Phase Gratings Manufactured by Nanosphere Lithography.” Optics Express 25, vol. 25, no. 19, 2017, pp. 22608–19, doi:10.1364/OE.25.022607.","short":"M. Wahle, K. Brassat, J. Ebel, J. Bürger, J. Lindner, H.-S. Kitzerow, Optics Express 25 25 (2017) 22608–22619.","ieee":"M. Wahle, K. Brassat, J. Ebel, J. Bürger, J. Lindner, and H.-S. Kitzerow, “Two-dimensional switchable blue phase gratings manufactured by nanosphere lithography,” Optics Express 25, vol. 25, no. 19, pp. 22608–22619, 2017, doi: 10.1364/OE.25.022607."},"page":"22608-22619","title":"Two-dimensional switchable blue phase gratings manufactured by nanosphere lithography","publication_status":"published","department":[{"_id":"2"},{"_id":"286"},{"_id":"230"},{"_id":"15"},{"_id":"313"}],"doi":"10.1364/OE.25.022607","date_updated":"2023-01-10T13:16:11Z","language":[{"iso":"eng"}]}]