---
_id: '59992'
abstract:
- lang: eng
  text: <jats:p>The immobilization of DNA origami nanostructures on solid surfaces
    is an important prerequisite for their application in many biosensors. So far,
    DNA origami immobilization has been investigated in detail only...</jats:p>
author:
- first_name: Xiaodan
  full_name: Xu, Xiaodan
  last_name: Xu
- first_name: Sandra Alicja
  full_name: Golebiowska, Sandra Alicja
  id: '69524'
  last_name: Golebiowska
- first_name: Teresa
  full_name: de los Arcos, Teresa
  last_name: de los Arcos
- first_name: Guido
  full_name: Grundmeier, Guido
  id: '194'
  last_name: Grundmeier
- first_name: Adrian
  full_name: Keller, Adrian
  id: '48864'
  last_name: Keller
  orcid: 0000-0001-7139-3110
citation:
  ama: Xu X, Golebiowska SA, de los Arcos T, Grundmeier G, Keller A. DNA origami adsorption
    at single-crystalline TiO2 surfaces. <i>RSC Applied Interfaces</i>. Published
    online 2025. doi:<a href="https://doi.org/10.1039/d5lf00109a">10.1039/d5lf00109a</a>
  apa: Xu, X., Golebiowska, S. A., de los Arcos, T., Grundmeier, G., &#38; Keller,
    A. (2025). DNA origami adsorption at single-crystalline TiO2 surfaces. <i>RSC
    Applied Interfaces</i>. <a href="https://doi.org/10.1039/d5lf00109a">https://doi.org/10.1039/d5lf00109a</a>
  bibtex: '@article{Xu_Golebiowska_de los Arcos_Grundmeier_Keller_2025, title={DNA
    origami adsorption at single-crystalline TiO2 surfaces}, DOI={<a href="https://doi.org/10.1039/d5lf00109a">10.1039/d5lf00109a</a>},
    journal={RSC Applied Interfaces}, publisher={Royal Society of Chemistry (RSC)},
    author={Xu, Xiaodan and Golebiowska, Sandra Alicja and de los Arcos, Teresa and
    Grundmeier, Guido and Keller, Adrian}, year={2025} }'
  chicago: Xu, Xiaodan, Sandra Alicja Golebiowska, Teresa de los Arcos, Guido Grundmeier,
    and Adrian Keller. “DNA Origami Adsorption at Single-Crystalline TiO2 Surfaces.”
    <i>RSC Applied Interfaces</i>, 2025. <a href="https://doi.org/10.1039/d5lf00109a">https://doi.org/10.1039/d5lf00109a</a>.
  ieee: 'X. Xu, S. A. Golebiowska, T. de los Arcos, G. Grundmeier, and A. Keller,
    “DNA origami adsorption at single-crystalline TiO2 surfaces,” <i>RSC Applied Interfaces</i>,
    2025, doi: <a href="https://doi.org/10.1039/d5lf00109a">10.1039/d5lf00109a</a>.'
  mla: Xu, Xiaodan, et al. “DNA Origami Adsorption at Single-Crystalline TiO2 Surfaces.”
    <i>RSC Applied Interfaces</i>, Royal Society of Chemistry (RSC), 2025, doi:<a
    href="https://doi.org/10.1039/d5lf00109a">10.1039/d5lf00109a</a>.
  short: X. Xu, S.A. Golebiowska, T. de los Arcos, G. Grundmeier, A. Keller, RSC Applied
    Interfaces (2025).
date_created: 2025-05-19T09:30:44Z
date_updated: 2025-05-19T09:32:05Z
department:
- _id: '302'
doi: 10.1039/d5lf00109a
language:
- iso: eng
publication: RSC Applied Interfaces
publication_identifier:
  issn:
  - 2755-3701
publication_status: published
publisher: Royal Society of Chemistry (RSC)
status: public
title: DNA origami adsorption at single-crystalline TiO2 surfaces
type: journal_article
user_id: '48864'
year: '2025'
...
---
_id: '60913'
abstract:
- lang: eng
  text: <jats:title>ABSTRACT</jats:title><jats:p>Spin‐coated polylactide (PLA) thin
    films were exposed to nitrogen plasma for varying time intervals. The progressive
    etching of the PLA film in direct contact with the nitrogen plasma was monitored
    in situ using polarization modulated infrared reflection absorption spectroscopy
    (PM‐IRRAS). No appreciative changes in composition were seen with PM‐IRRAS, indicating
    that the etching did not significantly affect the bulk composition. Atomic force
    microscopy characterization of the plasma‐etched films showed that the PLA films
    are homogeneously etched. Subsequent ex situ XPS analysis of the treated surface
    revealed the presence of C‐N bonds in the surface‐near region that could be associated
    with amino and/or amide surface species. PLA films were also alternatively exposed
    to nitrogen ion beams produced by an electron‐cyclotron‐resonance (ECR) plasma
    source and were investigated in vacuo by XPS. This treatment revealed the partial
    substitution of surface oxygen species by nitrogen, resulting in a similar surface
    modification as in the plasma case. The comparison of XPS data and water contact
    angle studies suggest that the activated surfaces show a reorientation of macromolecular
    fragments in the surface‐near region depending on the polarity of the phase with
    which they are in contact. Under ultra‐high vacuum (UHV) conditions, the surface
    tends to lower its surface energy, while in contact with the aqueous phase, subsurface
    polar groups orientate outwards, which enables the formation of hydrogen bonds.</jats:p>
author:
- first_name: Sandra Alicja
  full_name: Golebiowska, Sandra Alicja
  id: '69524'
  last_name: Golebiowska
  orcid: 0009-0001-1261-9455
- first_name: Markus
  full_name: Voigt, Markus
  id: '15182'
  last_name: Voigt
- first_name: Teresa
  full_name: de los Arcos, Teresa
  last_name: de los Arcos
- first_name: Guido
  full_name: Grundmeier, Guido
  id: '194'
  last_name: Grundmeier
citation:
  ama: Golebiowska SA, Voigt M, de los Arcos T, Grundmeier G. In Situ PM‐IRRAS and
    XPS Analysis of Nitrogen Plasma Surface Modification of Polylactide Thin Films.
    <i>Surface and Interface Analysis</i>. 2025;57(7):499-509. doi:<a href="https://doi.org/10.1002/sia.7406">10.1002/sia.7406</a>
  apa: Golebiowska, S. A., Voigt, M., de los Arcos, T., &#38; Grundmeier, G. (2025).
    In Situ PM‐IRRAS and XPS Analysis of Nitrogen Plasma Surface Modification of Polylactide
    Thin Films. <i>Surface and Interface Analysis</i>, <i>57</i>(7), 499–509. <a href="https://doi.org/10.1002/sia.7406">https://doi.org/10.1002/sia.7406</a>
  bibtex: '@article{Golebiowska_Voigt_de los Arcos_Grundmeier_2025, title={In Situ
    PM‐IRRAS and XPS Analysis of Nitrogen Plasma Surface Modification of Polylactide
    Thin Films}, volume={57}, DOI={<a href="https://doi.org/10.1002/sia.7406">10.1002/sia.7406</a>},
    number={7}, journal={Surface and Interface Analysis}, publisher={Wiley}, author={Golebiowska,
    Sandra Alicja and Voigt, Markus and de los Arcos, Teresa and Grundmeier, Guido},
    year={2025}, pages={499–509} }'
  chicago: 'Golebiowska, Sandra Alicja, Markus Voigt, Teresa de los Arcos, and Guido
    Grundmeier. “In Situ PM‐IRRAS and XPS Analysis of Nitrogen Plasma Surface Modification
    of Polylactide Thin Films.” <i>Surface and Interface Analysis</i> 57, no. 7 (2025):
    499–509. <a href="https://doi.org/10.1002/sia.7406">https://doi.org/10.1002/sia.7406</a>.'
  ieee: 'S. A. Golebiowska, M. Voigt, T. de los Arcos, and G. Grundmeier, “In Situ
    PM‐IRRAS and XPS Analysis of Nitrogen Plasma Surface Modification of Polylactide
    Thin Films,” <i>Surface and Interface Analysis</i>, vol. 57, no. 7, pp. 499–509,
    2025, doi: <a href="https://doi.org/10.1002/sia.7406">10.1002/sia.7406</a>.'
  mla: Golebiowska, Sandra Alicja, et al. “In Situ PM‐IRRAS and XPS Analysis of Nitrogen
    Plasma Surface Modification of Polylactide Thin Films.” <i>Surface and Interface
    Analysis</i>, vol. 57, no. 7, Wiley, 2025, pp. 499–509, doi:<a href="https://doi.org/10.1002/sia.7406">10.1002/sia.7406</a>.
  short: S.A. Golebiowska, M. Voigt, T. de los Arcos, G. Grundmeier, Surface and Interface
    Analysis 57 (2025) 499–509.
date_created: 2025-08-11T11:45:55Z
date_updated: 2025-12-08T08:13:24Z
department:
- _id: '302'
doi: 10.1002/sia.7406
intvolume: '        57'
issue: '7'
language:
- iso: eng
page: 499-509
project:
- _id: '52'
  name: Computing Resources Provided by the Paderborn Center for Parallel Computing
publication: Surface and Interface Analysis
publication_identifier:
  issn:
  - 0142-2421
  - 1096-9918
publication_status: published
publisher: Wiley
status: public
title: In Situ PM‐IRRAS and XPS Analysis of Nitrogen Plasma Surface Modification of
  Polylactide Thin Films
type: journal_article
user_id: '69524'
volume: 57
year: '2025'
...
