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Valaei, International Journal of Quality &#38; Reliability Management 38 (2021) 116–146.","chicago":"Tavana, Madjid, Akram Shaabani, and Naser Valaei. “An Integrated Fuzzy Framework for Analyzing Barriers to the Implementation of Continuous Improvement in Manufacturing.” <i>International Journal of Quality &#38; Reliability Management</i> 38, no. 1 (2021): 116–46. <a href=\"https://doi.org/10.1108/ijqrm-06-2019-0196\">https://doi.org/10.1108/ijqrm-06-2019-0196</a>.","mla":"Tavana, Madjid, et al. “An Integrated Fuzzy Framework for Analyzing Barriers to the Implementation of Continuous Improvement in Manufacturing.” <i>International Journal of Quality &#38; Reliability Management</i>, vol. 38, no. 1, Emerald, 2021, pp. 116–46, doi:<a href=\"https://doi.org/10.1108/ijqrm-06-2019-0196\">10.1108/ijqrm-06-2019-0196</a>.","bibtex":"@article{Tavana_Shaabani_Valaei_2021, title={An integrated fuzzy framework for analyzing barriers to the implementation of continuous improvement in manufacturing}, volume={38}, DOI={<a href=\"https://doi.org/10.1108/ijqrm-06-2019-0196\">10.1108/ijqrm-06-2019-0196</a>}, number={1}, journal={International Journal of Quality &#38; Reliability Management}, publisher={Emerald}, author={Tavana, Madjid and Shaabani, Akram and Valaei, Naser}, year={2021}, pages={116–146} }","ama":"Tavana M, Shaabani A, Valaei N. An integrated fuzzy framework for analyzing barriers to the implementation of continuous improvement in manufacturing. <i>International Journal of Quality &#38; Reliability Management</i>. 2021;38(1):116-146. doi:<a href=\"https://doi.org/10.1108/ijqrm-06-2019-0196\">10.1108/ijqrm-06-2019-0196</a>"},"status":"public","page":"116-146","_id":"53862","publisher":"Emerald","user_id":"51811","volume":38,"issue":"1","publication":"International Journal of Quality & Reliability Management","date_created":"2024-05-04T14:06:10Z","type":"journal_article","department":[{"_id":"277"}],"title":"An integrated fuzzy framework for analyzing barriers to the implementation of continuous improvement in manufacturing","year":"2021","author":[{"id":"31858","first_name":"Madjid","last_name":"Tavana","full_name":"Tavana, Madjid"},{"full_name":"Shaabani, Akram","last_name":"Shaabani","first_name":"Akram"},{"full_name":"Valaei, Naser","last_name":"Valaei","first_name":"Naser"}],"publication_identifier":{"issn":["0265-671X"]},"date_updated":"2024-05-04T15:13:24Z","publication_status":"published","intvolume":"        38","language":[{"iso":"eng"}],"doi":"10.1108/ijqrm-06-2019-0196"},{"citation":{"bibtex":"@article{Soares_Tortorella_Bouzon_Tavana_2021, title={A fuzzy maturity-based method for lean supply chain management assessment}, volume={12}, DOI={<a href=\"https://doi.org/10.1108/ijlss-08-2020-0123\">10.1108/ijlss-08-2020-0123</a>}, number={5}, journal={International Journal of Lean Six Sigma}, publisher={Emerald}, author={Soares, Gabriela Pereira and Tortorella, Guilherme and Bouzon, Marina and Tavana, Madjid}, year={2021}, pages={1017–1045} }","ama":"Soares GP, Tortorella G, Bouzon M, Tavana M. A fuzzy maturity-based method for lean supply chain management assessment. <i>International Journal of Lean Six Sigma</i>. 2021;12(5):1017-1045. doi:<a href=\"https://doi.org/10.1108/ijlss-08-2020-0123\">10.1108/ijlss-08-2020-0123</a>","mla":"Soares, Gabriela Pereira, et al. “A Fuzzy Maturity-Based Method for Lean Supply Chain Management Assessment.” <i>International Journal of Lean Six Sigma</i>, vol. 12, no. 5, Emerald, 2021, pp. 1017–45, doi:<a href=\"https://doi.org/10.1108/ijlss-08-2020-0123\">10.1108/ijlss-08-2020-0123</a>.","chicago":"Soares, Gabriela Pereira, Guilherme Tortorella, Marina Bouzon, and Madjid Tavana. “A Fuzzy Maturity-Based Method for Lean Supply Chain Management Assessment.” <i>International Journal of Lean Six Sigma</i> 12, no. 5 (2021): 1017–45. <a href=\"https://doi.org/10.1108/ijlss-08-2020-0123\">https://doi.org/10.1108/ijlss-08-2020-0123</a>.","short":"G.P. Soares, G. Tortorella, M. Bouzon, M. Tavana, International Journal of Lean Six Sigma 12 (2021) 1017–1045.","ieee":"G. P. Soares, G. Tortorella, M. Bouzon, and M. Tavana, “A fuzzy maturity-based method for lean supply chain management assessment,” <i>International Journal of Lean Six Sigma</i>, vol. 12, no. 5, pp. 1017–1045, 2021, doi: <a href=\"https://doi.org/10.1108/ijlss-08-2020-0123\">10.1108/ijlss-08-2020-0123</a>.","apa":"Soares, G. P., Tortorella, G., Bouzon, M., &#38; Tavana, M. (2021). A fuzzy maturity-based method for lean supply chain management assessment. <i>International Journal of Lean Six Sigma</i>, <i>12</i>(5), 1017–1045. <a href=\"https://doi.org/10.1108/ijlss-08-2020-0123\">https://doi.org/10.1108/ijlss-08-2020-0123</a>"},"status":"public","volume":12,"user_id":"51811","publisher":"Emerald","_id":"53883","page":"1017-1045","publication":"International Journal of Lean Six Sigma","issue":"5","department":[{"_id":"277"}],"type":"journal_article","date_created":"2024-05-04T14:50:31Z","intvolume":"        12","date_updated":"2024-05-04T15:13:17Z","publication_status":"published","author":[{"first_name":"Gabriela Pereira","last_name":"Soares","full_name":"Soares, Gabriela Pereira"},{"last_name":"Tortorella","first_name":"Guilherme","full_name":"Tortorella, Guilherme"},{"last_name":"Bouzon","first_name":"Marina","full_name":"Bouzon, Marina"},{"full_name":"Tavana, Madjid","first_name":"Madjid","last_name":"Tavana","id":"31858"}],"publication_identifier":{"issn":["2040-4166","2040-4166"]},"title":"A fuzzy maturity-based method for lean supply chain management assessment","year":"2021","doi":"10.1108/ijlss-08-2020-0123","language":[{"iso":"eng"}]},{"title":"A robust cross-efficiency data envelopment analysis model with undesirable outputs","status":"public","year":"2021","publication_identifier":{"issn":["0957-4174"]},"author":[{"id":"31858","first_name":"Madjid","last_name":"Tavana","full_name":"Tavana, Madjid"},{"first_name":"Mehdi","last_name":"Toloo","full_name":"Toloo, Mehdi"},{"full_name":"Aghayi, Nazila","first_name":"Nazila","last_name":"Aghayi"},{"full_name":"Arabmaldar, Aliasghar","last_name":"Arabmaldar","first_name":"Aliasghar"}],"date_updated":"2024-05-04T15:13:27Z","publication_status":"published","intvolume":"       167","article_number":"114117","_id":"53861","publisher":"Elsevier BV","language":[{"iso":"eng"}],"doi":"10.1016/j.eswa.2020.114117","user_id":"51811","volume":167,"publication":"Expert Systems with Applications","citation":{"mla":"Tavana, Madjid, et al. “A Robust Cross-Efficiency Data Envelopment Analysis Model with Undesirable Outputs.” <i>Expert Systems with Applications</i>, vol. 167, 114117, Elsevier BV, 2021, doi:<a href=\"https://doi.org/10.1016/j.eswa.2020.114117\">10.1016/j.eswa.2020.114117</a>.","bibtex":"@article{Tavana_Toloo_Aghayi_Arabmaldar_2021, title={A robust cross-efficiency data envelopment analysis model with undesirable outputs}, volume={167}, DOI={<a href=\"https://doi.org/10.1016/j.eswa.2020.114117\">10.1016/j.eswa.2020.114117</a>}, number={114117}, journal={Expert Systems with Applications}, publisher={Elsevier BV}, author={Tavana, Madjid and Toloo, Mehdi and Aghayi, Nazila and Arabmaldar, Aliasghar}, year={2021} }","ama":"Tavana M, Toloo M, Aghayi N, Arabmaldar A. A robust cross-efficiency data envelopment analysis model with undesirable outputs. <i>Expert Systems with Applications</i>. 2021;167. doi:<a href=\"https://doi.org/10.1016/j.eswa.2020.114117\">10.1016/j.eswa.2020.114117</a>","ieee":"M. Tavana, M. Toloo, N. Aghayi, and A. Arabmaldar, “A robust cross-efficiency data envelopment analysis model with undesirable outputs,” <i>Expert Systems with Applications</i>, vol. 167, Art. no. 114117, 2021, doi: <a href=\"https://doi.org/10.1016/j.eswa.2020.114117\">10.1016/j.eswa.2020.114117</a>.","apa":"Tavana, M., Toloo, M., Aghayi, N., &#38; Arabmaldar, A. (2021). A robust cross-efficiency data envelopment analysis model with undesirable outputs. <i>Expert Systems with Applications</i>, <i>167</i>, Article 114117. <a href=\"https://doi.org/10.1016/j.eswa.2020.114117\">https://doi.org/10.1016/j.eswa.2020.114117</a>","short":"M. Tavana, M. Toloo, N. Aghayi, A. Arabmaldar, Expert Systems with Applications 167 (2021).","chicago":"Tavana, Madjid, Mehdi Toloo, Nazila Aghayi, and Aliasghar Arabmaldar. “A Robust Cross-Efficiency Data Envelopment Analysis Model with Undesirable Outputs.” <i>Expert Systems with Applications</i> 167 (2021). <a href=\"https://doi.org/10.1016/j.eswa.2020.114117\">https://doi.org/10.1016/j.eswa.2020.114117</a>."},"date_created":"2024-05-04T14:02:10Z","type":"journal_article","department":[{"_id":"277"}]},{"status":"public","_id":"53882","publisher":"Emerald","page":"1041-1062","volume":29,"user_id":"51811","citation":{"chicago":"Mancini, Daniela, Rosa Lombardi, and Madjid Tavana. “Four Research Pathways for Understanding the Role of Smart Technologies in Accounting.” <i>Meditari Accountancy Research</i> 29, no. 5 (2021): 1041–62. <a href=\"https://doi.org/10.1108/medar-03-2021-1258\">https://doi.org/10.1108/medar-03-2021-1258</a>.","short":"D. Mancini, R. Lombardi, M. Tavana, Meditari Accountancy Research 29 (2021) 1041–1062.","apa":"Mancini, D., Lombardi, R., &#38; Tavana, M. (2021). Four research pathways for understanding the role of smart technologies in accounting. <i>Meditari Accountancy Research</i>, <i>29</i>(5), 1041–1062. <a href=\"https://doi.org/10.1108/medar-03-2021-1258\">https://doi.org/10.1108/medar-03-2021-1258</a>","ieee":"D. Mancini, R. Lombardi, and M. Tavana, “Four research pathways for understanding the role of smart technologies in accounting,” <i>Meditari Accountancy Research</i>, vol. 29, no. 5, pp. 1041–1062, 2021, doi: <a href=\"https://doi.org/10.1108/medar-03-2021-1258\">10.1108/medar-03-2021-1258</a>.","ama":"Mancini D, Lombardi R, Tavana M. Four research pathways for understanding the role of smart technologies in accounting. <i>Meditari Accountancy Research</i>. 2021;29(5):1041-1062. doi:<a href=\"https://doi.org/10.1108/medar-03-2021-1258\">10.1108/medar-03-2021-1258</a>","bibtex":"@article{Mancini_Lombardi_Tavana_2021, title={Four research pathways for understanding the role of smart technologies in accounting}, volume={29}, DOI={<a href=\"https://doi.org/10.1108/medar-03-2021-1258\">10.1108/medar-03-2021-1258</a>}, number={5}, journal={Meditari Accountancy Research}, publisher={Emerald}, author={Mancini, Daniela and Lombardi, Rosa and Tavana, Madjid}, year={2021}, pages={1041–1062} }","mla":"Mancini, Daniela, et al. “Four Research Pathways for Understanding the Role of Smart Technologies in Accounting.” <i>Meditari Accountancy Research</i>, vol. 29, no. 5, Emerald, 2021, pp. 1041–62, doi:<a href=\"https://doi.org/10.1108/medar-03-2021-1258\">10.1108/medar-03-2021-1258</a>."},"publication_identifier":{"issn":["2049-372X","2049-372X"]},"author":[{"first_name":"Daniela","last_name":"Mancini","full_name":"Mancini, Daniela"},{"last_name":"Lombardi","first_name":"Rosa","full_name":"Lombardi, Rosa"},{"first_name":"Madjid","last_name":"Tavana","full_name":"Tavana, Madjid","id":"31858"}],"title":"Four research pathways for understanding the role of smart technologies in accounting","year":"2021","intvolume":"        29","publication_status":"published","date_updated":"2024-05-04T15:13:15Z","language":[{"iso":"eng"}],"doi":"10.1108/medar-03-2021-1258","publication":"Meditari Accountancy Research","issue":"5","date_created":"2024-05-04T14:49:28Z","department":[{"_id":"277"}],"type":"journal_article"},{"department":[{"_id":"277"}],"type":"journal_article","date_created":"2024-05-06T14:44:27Z","citation":{"ieee":"M. Tavana, M. Izadikhah, M. Toloo, and R. Roostaee, “A new non-radial directional distance model for data envelopment analysis problems with negative and flexible measures,” <i>Omega</i>, vol. 102, Art. no. 102355, 2021, doi: <a href=\"https://doi.org/10.1016/j.omega.2020.102355\">10.1016/j.omega.2020.102355</a>.","apa":"Tavana, M., Izadikhah, M., Toloo, M., &#38; Roostaee, R. (2021). A new non-radial directional distance model for data envelopment analysis problems with negative and flexible measures. <i>Omega</i>, <i>102</i>, Article 102355. <a href=\"https://doi.org/10.1016/j.omega.2020.102355\">https://doi.org/10.1016/j.omega.2020.102355</a>","short":"M. Tavana, M. Izadikhah, M. Toloo, R. Roostaee, Omega 102 (2021).","chicago":"Tavana, Madjid, Mohammad Izadikhah, Mehdi Toloo, and Razieh Roostaee. “A New Non-Radial Directional Distance Model for Data Envelopment Analysis Problems with Negative and Flexible Measures.” <i>Omega</i> 102 (2021). <a href=\"https://doi.org/10.1016/j.omega.2020.102355\">https://doi.org/10.1016/j.omega.2020.102355</a>.","mla":"Tavana, Madjid, et al. “A New Non-Radial Directional Distance Model for Data Envelopment Analysis Problems with Negative and Flexible Measures.” <i>Omega</i>, vol. 102, 102355, Elsevier BV, 2021, doi:<a href=\"https://doi.org/10.1016/j.omega.2020.102355\">10.1016/j.omega.2020.102355</a>.","bibtex":"@article{Tavana_Izadikhah_Toloo_Roostaee_2021, title={A new non-radial directional distance model for data envelopment analysis problems with negative and flexible measures}, volume={102}, DOI={<a href=\"https://doi.org/10.1016/j.omega.2020.102355\">10.1016/j.omega.2020.102355</a>}, number={102355}, journal={Omega}, publisher={Elsevier BV}, author={Tavana, Madjid and Izadikhah, Mohammad and Toloo, Mehdi and Roostaee, Razieh}, year={2021} }","ama":"Tavana M, Izadikhah M, Toloo M, Roostaee R. A new non-radial directional distance model for data envelopment analysis problems with negative and flexible measures. <i>Omega</i>. 2021;102. doi:<a href=\"https://doi.org/10.1016/j.omega.2020.102355\">10.1016/j.omega.2020.102355</a>"},"publication":"Omega","volume":102,"user_id":"51811","doi":"10.1016/j.omega.2020.102355","_id":"53964","publisher":"Elsevier BV","language":[{"iso":"eng"}],"article_number":"102355","intvolume":"       102","publication_status":"published","date_updated":"2024-05-06T14:46:28Z","publication_identifier":{"issn":["0305-0483"]},"author":[{"id":"31858","last_name":"Tavana","first_name":"Madjid","full_name":"Tavana, Madjid"},{"last_name":"Izadikhah","first_name":"Mohammad","full_name":"Izadikhah, Mohammad"},{"last_name":"Toloo","first_name":"Mehdi","full_name":"Toloo, Mehdi"},{"first_name":"Razieh","last_name":"Roostaee","full_name":"Roostaee, Razieh"}],"title":"A new non-radial directional distance model for data envelopment analysis problems with negative and flexible measures","status":"public","year":"2021"},{"doi":"10.1021/acscatal.1c03057","language":[{"iso":"eng"}],"article_type":"original","intvolume":"        11","publication_status":"published","date_updated":"2024-05-07T11:44:19Z","author":[{"last_name":"Ziegler","first_name":"Felix","full_name":"Ziegler, Felix"},{"last_name":"Kraus","first_name":"Hamzeh","full_name":"Kraus, Hamzeh"},{"first_name":"Mathis J.","last_name":"Benedikter","full_name":"Benedikter, Mathis J."},{"full_name":"Wang, Dongren","last_name":"Wang","first_name":"Dongren"},{"last_name":"Bruckner","first_name":"Johanna R.","full_name":"Bruckner, Johanna R."},{"id":"78878","first_name":"Michał","last_name":"Nowakowski","orcid":"0000-0002-3734-7011","full_name":"Nowakowski, Michał"},{"last_name":"Weißer","first_name":"Kilian","full_name":"Weißer, Kilian"},{"full_name":"Solodenko, Helena","last_name":"Solodenko","first_name":"Helena"},{"full_name":"Schmitz, Guido","first_name":"Guido","last_name":"Schmitz"},{"last_name":"Bauer","orcid":"0000-0002-9294-6076","first_name":"Matthias","full_name":"Bauer, Matthias","id":"47241"},{"last_name":"Hansen","first_name":"Niels","full_name":"Hansen, Niels"},{"last_name":"Buchmeiser","first_name":"Michael R.","full_name":"Buchmeiser, Michael R."}],"publication_identifier":{"issn":["2155-5435","2155-5435"]},"year":"2021","title":"Confinement Effects for Efficient Macrocyclization Reactions with Supported Cationic Molybdenum Imido Alkylidene <i>N</i>-Heterocyclic Carbene Complexes","department":[{"_id":"35"},{"_id":"306"}],"type":"journal_article","keyword":["Catalysis","General Chemistry"],"date_created":"2023-01-30T16:49:07Z","abstract":[{"text":"For entropic reasons, the synthesis of macrocycles via olefin ring-closing metathesis (RCM) is impeded by competing acyclic diene metathesis (ADMET) oligomerization. With cationic molybdenum imido alkylidene N-heterocyclic carbene (NHC) complexes confined in tailored ordered mesoporous silica, RCM can be run with macrocyclization selectivities up to 98% and high substrate concentrations up to 0.1 M. Molecular dynamics simulations show that the high conversions are a direct result of the proximity between the surface-bound catalyst, proven by extended X-ray absorption spectroscopy, and the surface-located substrates. Back-diffusion of the macrocycles decreases with decreasing pore diameter of the silica and is responsible for the high macrocyclization efficiency. Also, Z-selectivity increases with decreasing pore diameter and increasing Tolman electronic parameter of the NHC. Running reactions at different concentrations allows for identifying the optimum substrate concentration for each material and substrate combination.","lang":"eng"}],"issue":"18","publication":"ACS Catalysis","volume":11,"user_id":"48467","_id":"41001","publisher":"American Chemical Society (ACS)","page":"11570-11578","status":"public","citation":{"mla":"Ziegler, Felix, et al. “Confinement Effects for Efficient Macrocyclization Reactions with Supported Cationic Molybdenum Imido Alkylidene <i>N</i>-Heterocyclic Carbene Complexes.” <i>ACS Catalysis</i>, vol. 11, no. 18, American Chemical Society (ACS), 2021, pp. 11570–78, doi:<a href=\"https://doi.org/10.1021/acscatal.1c03057\">10.1021/acscatal.1c03057</a>.","bibtex":"@article{Ziegler_Kraus_Benedikter_Wang_Bruckner_Nowakowski_Weißer_Solodenko_Schmitz_Bauer_et al._2021, title={Confinement Effects for Efficient Macrocyclization Reactions with Supported Cationic Molybdenum Imido Alkylidene <i>N</i>-Heterocyclic Carbene Complexes}, volume={11}, DOI={<a href=\"https://doi.org/10.1021/acscatal.1c03057\">10.1021/acscatal.1c03057</a>}, number={18}, journal={ACS Catalysis}, publisher={American Chemical Society (ACS)}, author={Ziegler, Felix and Kraus, Hamzeh and Benedikter, Mathis J. and Wang, Dongren and Bruckner, Johanna R. and Nowakowski, Michał and Weißer, Kilian and Solodenko, Helena and Schmitz, Guido and Bauer, Matthias and et al.}, year={2021}, pages={11570–11578} }","ama":"Ziegler F, Kraus H, Benedikter MJ, et al. Confinement Effects for Efficient Macrocyclization Reactions with Supported Cationic Molybdenum Imido Alkylidene <i>N</i>-Heterocyclic Carbene Complexes. <i>ACS Catalysis</i>. 2021;11(18):11570-11578. doi:<a href=\"https://doi.org/10.1021/acscatal.1c03057\">10.1021/acscatal.1c03057</a>","ieee":"F. Ziegler <i>et al.</i>, “Confinement Effects for Efficient Macrocyclization Reactions with Supported Cationic Molybdenum Imido Alkylidene <i>N</i>-Heterocyclic Carbene Complexes,” <i>ACS Catalysis</i>, vol. 11, no. 18, pp. 11570–11578, 2021, doi: <a href=\"https://doi.org/10.1021/acscatal.1c03057\">10.1021/acscatal.1c03057</a>.","apa":"Ziegler, F., Kraus, H., Benedikter, M. J., Wang, D., Bruckner, J. R., Nowakowski, M., Weißer, K., Solodenko, H., Schmitz, G., Bauer, M., Hansen, N., &#38; Buchmeiser, M. R. (2021). Confinement Effects for Efficient Macrocyclization Reactions with Supported Cationic Molybdenum Imido Alkylidene <i>N</i>-Heterocyclic Carbene Complexes. <i>ACS Catalysis</i>, <i>11</i>(18), 11570–11578. <a href=\"https://doi.org/10.1021/acscatal.1c03057\">https://doi.org/10.1021/acscatal.1c03057</a>","short":"F. Ziegler, H. Kraus, M.J. Benedikter, D. Wang, J.R. Bruckner, M. Nowakowski, K. Weißer, H. Solodenko, G. Schmitz, M. Bauer, N. Hansen, M.R. Buchmeiser, ACS Catalysis 11 (2021) 11570–11578.","chicago":"Ziegler, Felix, Hamzeh Kraus, Mathis J. Benedikter, Dongren Wang, Johanna R. Bruckner, Michał Nowakowski, Kilian Weißer, et al. “Confinement Effects for Efficient Macrocyclization Reactions with Supported Cationic Molybdenum Imido Alkylidene <i>N</i>-Heterocyclic Carbene Complexes.” <i>ACS Catalysis</i> 11, no. 18 (2021): 11570–78. <a href=\"https://doi.org/10.1021/acscatal.1c03057\">https://doi.org/10.1021/acscatal.1c03057</a>."}},{"language":[{"iso":"eng"}],"doi":"10.1002/chem.202103099","publication_identifier":{"issn":["0947-6539","1521-3765"]},"author":[{"full_name":"Panyam, Pradeep K. R.","last_name":"Panyam","first_name":"Pradeep K. R."},{"last_name":"Atwi","first_name":"Boshra","full_name":"Atwi, Boshra"},{"full_name":"Ziegler, Felix","first_name":"Felix","last_name":"Ziegler"},{"last_name":"Frey","first_name":"Wolfgang","full_name":"Frey, Wolfgang"},{"id":"78878","first_name":"Michał","last_name":"Nowakowski","orcid":"0000-0002-3734-7011","full_name":"Nowakowski, Michał"},{"id":"47241","full_name":"Bauer, Matthias","orcid":"0000-0002-9294-6076","last_name":"Bauer","first_name":"Matthias"},{"last_name":"Buchmeiser","first_name":"Michael R.","full_name":"Buchmeiser, Michael R."}],"title":"Rh(I)/(III)‐N‐Heterocyclic Carbene Complexes: Effect of Steric Confinement Upon Immobilization on Regio‐ and Stereoselectivity in the Hydrosilylation of Alkynes","year":"2021","article_type":"original","intvolume":"        27","publication_status":"published","date_updated":"2024-05-07T11:43:40Z","date_created":"2023-01-30T16:48:41Z","department":[{"_id":"35"},{"_id":"306"}],"keyword":["General Chemistry","Catalysis","Organic Chemistry"],"type":"journal_article","publication":"Chemistry – A European Journal","issue":"68","abstract":[{"text":"Rh(I) NHC and Rh(III) Cp* NHC complexes (Cp*=pentamethylcyclopentadienyl, NHC=N-heterocyclic carbene=pyrid-2-ylimidazol-2-ylidene (Py−Im), thiophen-2-ylimidazol-2-ylidene) are presented. Selected catalysts were selectively immobilized inside the mesopores of SBA-15 with average pore diameters of 5.0 and 6.2 nm. Together with their homogenous progenitors, the immobilized catalysts were used in the hydrosilylation of terminal alkynes. For aromatic alkynes, both the neutral and cationic Rh(I) complexes showed excellent reactivity with exclusive formation of the β(E)-isomer. For aliphatic alkynes, however, selectivity of the Rh(I) complexes was low. By contrast, the neutral and cationic Rh(III) Cp* NHC complexes proved to be highly regio- and stereoselective catalysts, allowing for the formation of the thermodynamically less stable β-(Z)-vinylsilane isomers at room temperature. Notably, the SBA-15 immobilized Rh(I) catalysts, in which the pore walls provide an additional confinement, showed excellent β-(Z)-selectivity in the hydrosilylation of aliphatic alkynes, too. Also, in the case of 4-aminophenylacetylene, selective formation of the β(Z)-isomer was observed with a neutral SBA-15 supported Rh(III) Cp* NHC complex but not with its homogenous counterpart. These are the first examples of high β(Z)-selectivity in the hydrosilylation of alkynes by confinement generated upon immobilization inside mesoporous silica.","lang":"eng"}],"_id":"40999","publisher":"Wiley","page":"17220-17229","volume":27,"user_id":"48467","status":"public","citation":{"ieee":"P. K. R. Panyam <i>et al.</i>, “Rh(I)/(III)‐N‐Heterocyclic Carbene Complexes: Effect of Steric Confinement Upon Immobilization on Regio‐ and Stereoselectivity in the Hydrosilylation of Alkynes,” <i>Chemistry – A European Journal</i>, vol. 27, no. 68, pp. 17220–17229, 2021, doi: <a href=\"https://doi.org/10.1002/chem.202103099\">10.1002/chem.202103099</a>.","apa":"Panyam, P. K. R., Atwi, B., Ziegler, F., Frey, W., Nowakowski, M., Bauer, M., &#38; Buchmeiser, M. R. (2021). Rh(I)/(III)‐N‐Heterocyclic Carbene Complexes: Effect of Steric Confinement Upon Immobilization on Regio‐ and Stereoselectivity in the Hydrosilylation of Alkynes. <i>Chemistry – A European Journal</i>, <i>27</i>(68), 17220–17229. <a href=\"https://doi.org/10.1002/chem.202103099\">https://doi.org/10.1002/chem.202103099</a>","short":"P.K.R. Panyam, B. Atwi, F. Ziegler, W. Frey, M. Nowakowski, M. Bauer, M.R. Buchmeiser, Chemistry – A European Journal 27 (2021) 17220–17229.","chicago":"Panyam, Pradeep K. R., Boshra Atwi, Felix Ziegler, Wolfgang Frey, Michał Nowakowski, Matthias Bauer, and Michael R. Buchmeiser. “Rh(I)/(III)‐N‐Heterocyclic Carbene Complexes: Effect of Steric Confinement Upon Immobilization on Regio‐ and Stereoselectivity in the Hydrosilylation of Alkynes.” <i>Chemistry – A European Journal</i> 27, no. 68 (2021): 17220–29. <a href=\"https://doi.org/10.1002/chem.202103099\">https://doi.org/10.1002/chem.202103099</a>.","mla":"Panyam, Pradeep K. R., et al. “Rh(I)/(III)‐N‐Heterocyclic Carbene Complexes: Effect of Steric Confinement Upon Immobilization on Regio‐ and Stereoselectivity in the Hydrosilylation of Alkynes.” <i>Chemistry – A European Journal</i>, vol. 27, no. 68, Wiley, 2021, pp. 17220–29, doi:<a href=\"https://doi.org/10.1002/chem.202103099\">10.1002/chem.202103099</a>.","bibtex":"@article{Panyam_Atwi_Ziegler_Frey_Nowakowski_Bauer_Buchmeiser_2021, title={Rh(I)/(III)‐N‐Heterocyclic Carbene Complexes: Effect of Steric Confinement Upon Immobilization on Regio‐ and Stereoselectivity in the Hydrosilylation of Alkynes}, volume={27}, DOI={<a href=\"https://doi.org/10.1002/chem.202103099\">10.1002/chem.202103099</a>}, number={68}, journal={Chemistry – A European Journal}, publisher={Wiley}, author={Panyam, Pradeep K. R. and Atwi, Boshra and Ziegler, Felix and Frey, Wolfgang and Nowakowski, Michał and Bauer, Matthias and Buchmeiser, Michael R.}, year={2021}, pages={17220–17229} }","ama":"Panyam PKR, Atwi B, Ziegler F, et al. Rh(I)/(III)‐N‐Heterocyclic Carbene Complexes: Effect of Steric Confinement Upon Immobilization on Regio‐ and Stereoselectivity in the Hydrosilylation of Alkynes. <i>Chemistry – A European Journal</i>. 2021;27(68):17220-17229. doi:<a href=\"https://doi.org/10.1002/chem.202103099\">10.1002/chem.202103099</a>"}}]