{"publication_status":"published","date_updated":"2022-01-06T06:50:22Z","page":"821-825","citation":{"ieee":"C. W. Nicholson <i>et al.</i>, “Beyond the molecular movie: Dynamics of bands and bonds during a photoinduced phase transition,” <i>Science</i>, pp. 821–825, 2018.","bibtex":"@article{Nicholson_Lücke_Schmidt_Puppin_Rettig_Ernstorfer_Wolf_2018, title={Beyond the molecular movie: Dynamics of bands and bonds during a photoinduced phase transition}, DOI={<a href=\"https://doi.org/10.1126/science.aar4183\">10.1126/science.aar4183</a>}, journal={Science}, author={Nicholson, C. W. and Lücke, A. and Schmidt, Wolf Gero and Puppin, M. and Rettig, L. and Ernstorfer, R. and Wolf, M.}, year={2018}, pages={821–825} }","mla":"Nicholson, C. W., et al. “Beyond the Molecular Movie: Dynamics of Bands and Bonds during a Photoinduced Phase Transition.” <i>Science</i>, 2018, pp. 821–25, doi:<a href=\"https://doi.org/10.1126/science.aar4183\">10.1126/science.aar4183</a>.","chicago":"Nicholson, C. W., A. Lücke, Wolf Gero Schmidt, M. Puppin, L. Rettig, R. Ernstorfer, and M. Wolf. “Beyond the Molecular Movie: Dynamics of Bands and Bonds during a Photoinduced Phase Transition.” <i>Science</i>, 2018, 821–25. <a href=\"https://doi.org/10.1126/science.aar4183\">https://doi.org/10.1126/science.aar4183</a>.","apa":"Nicholson, C. W., Lücke, A., Schmidt, W. G., Puppin, M., Rettig, L., Ernstorfer, R., &#38; Wolf, M. (2018). Beyond the molecular movie: Dynamics of bands and bonds during a photoinduced phase transition. <i>Science</i>, 821–825. <a href=\"https://doi.org/10.1126/science.aar4183\">https://doi.org/10.1126/science.aar4183</a>","ama":"Nicholson CW, Lücke A, Schmidt WG, et al. Beyond the molecular movie: Dynamics of bands and bonds during a photoinduced phase transition. <i>Science</i>. 2018:821-825. doi:<a href=\"https://doi.org/10.1126/science.aar4183\">10.1126/science.aar4183</a>","short":"C.W. Nicholson, A. Lücke, W.G. Schmidt, M. Puppin, L. Rettig, R. Ernstorfer, M. Wolf, Science (2018) 821–825."},"year":"2018","publication_identifier":{"issn":["0036-8075","1095-9203"]},"language":[{"iso":"eng"}],"status":"public","_id":"10013","doi":"10.1126/science.aar4183","publication":"Science","date_created":"2019-05-29T06:46:27Z","department":[{"_id":"15"}],"author":[{"full_name":"Nicholson, C. W.","last_name":"Nicholson","first_name":"C. W."},{"first_name":"A.","last_name":"Lücke","full_name":"Lücke, A."},{"orcid":"0000-0002-2717-5076","last_name":"Schmidt","full_name":"Schmidt, Wolf Gero","first_name":"Wolf Gero","id":"468"},{"full_name":"Puppin, M.","last_name":"Puppin","first_name":"M."},{"first_name":"L.","full_name":"Rettig, L.","last_name":"Rettig"},{"last_name":"Ernstorfer","full_name":"Ernstorfer, R.","first_name":"R."},{"first_name":"M.","last_name":"Wolf","full_name":"Wolf, M."}],"title":"Beyond the molecular movie: Dynamics of bands and bonds during a photoinduced phase transition","type":"journal_article","project":[{"_id":"52","name":"Computing Resources Provided by the Paderborn Center for Parallel Computing"},{"name":"TRR 142","_id":"53"},{"_id":"55","name":"TRR 142 - Project Area B"},{"name":"TRR 142 - Subproject B4","_id":"69"}],"user_id":"16199","abstract":[{"text":"<jats:p>Ultrafast nonequilibrium dynamics offer a route to study the microscopic interactions that govern macroscopic behavior. In particular, photoinduced phase transitions (PIPTs) in solids provide a test case for how forces, and the resulting atomic motion along a reaction coordinate, originate from a nonequilibrium population of excited electronic states. Using femtosecond photoemission, we obtain access to the transient electronic structure during an ultrafast PIPT in a model system: indium nanowires on a silicon(111) surface. We uncover a detailed reaction pathway, allowing a direct comparison with the dynamics predicted by ab initio simulations. This further reveals the crucial role played by localized photoholes in shaping the potential energy landscape and enables a combined momentum- and real-space description of PIPTs, including the ultrafast formation of chemical bonds.</jats:p>","lang":"eng"}]}