{"title":"Hydrogen bond dynamics of interfacial water molecules revealed from two-dimensional vibrational sum-frequency generation spectroscopy","article_number":"2456","language":[{"iso":"eng"}],"date_updated":"2022-10-10T08:12:16Z","publication_status":"published","user_id":"71051","publisher":"Springer Science and Business Media LLC","citation":{"apa":"Ojha, D., &#38; Kühne, T. (2021). Hydrogen bond dynamics of interfacial water molecules revealed from two-dimensional vibrational sum-frequency generation spectroscopy. <i>Scientific Reports</i>, <i>11</i>(1), Article 2456. <a href=\"https://doi.org/10.1038/s41598-021-81635-4\">https://doi.org/10.1038/s41598-021-81635-4</a>","ieee":"D. Ojha and T. Kühne, “Hydrogen bond dynamics of interfacial water molecules revealed from two-dimensional vibrational sum-frequency generation spectroscopy,” <i>Scientific Reports</i>, vol. 11, no. 1, Art. no. 2456, 2021, doi: <a href=\"https://doi.org/10.1038/s41598-021-81635-4\">10.1038/s41598-021-81635-4</a>.","mla":"Ojha, Deepak, and Thomas Kühne. “Hydrogen Bond Dynamics of Interfacial Water Molecules Revealed from Two-Dimensional Vibrational Sum-Frequency Generation Spectroscopy.” <i>Scientific Reports</i>, vol. 11, no. 1, 2456, Springer Science and Business Media LLC, 2021, doi:<a href=\"https://doi.org/10.1038/s41598-021-81635-4\">10.1038/s41598-021-81635-4</a>.","ama":"Ojha D, Kühne T. Hydrogen bond dynamics of interfacial water molecules revealed from two-dimensional vibrational sum-frequency generation spectroscopy. <i>Scientific Reports</i>. 2021;11(1). doi:<a href=\"https://doi.org/10.1038/s41598-021-81635-4\">10.1038/s41598-021-81635-4</a>","bibtex":"@article{Ojha_Kühne_2021, title={Hydrogen bond dynamics of interfacial water molecules revealed from two-dimensional vibrational sum-frequency generation spectroscopy}, volume={11}, DOI={<a href=\"https://doi.org/10.1038/s41598-021-81635-4\">10.1038/s41598-021-81635-4</a>}, number={12456}, journal={Scientific Reports}, publisher={Springer Science and Business Media LLC}, author={Ojha, Deepak and Kühne, Thomas}, year={2021} }","chicago":"Ojha, Deepak, and Thomas Kühne. “Hydrogen Bond Dynamics of Interfacial Water Molecules Revealed from Two-Dimensional Vibrational Sum-Frequency Generation Spectroscopy.” <i>Scientific Reports</i> 11, no. 1 (2021). <a href=\"https://doi.org/10.1038/s41598-021-81635-4\">https://doi.org/10.1038/s41598-021-81635-4</a>.","short":"D. Ojha, T. Kühne, Scientific Reports 11 (2021)."},"department":[{"_id":"613"}],"date_created":"2022-10-10T08:12:00Z","issue":"1","publication":"Scientific Reports","type":"journal_article","year":"2021","publication_identifier":{"issn":["2045-2322"]},"_id":"33645","intvolume":"        11","author":[{"first_name":"Deepak","last_name":"Ojha","full_name":"Ojha, Deepak"},{"last_name":"Kühne","full_name":"Kühne, Thomas","first_name":"Thomas","id":"49079"}],"status":"public","doi":"10.1038/s41598-021-81635-4","abstract":[{"lang":"eng","text":"<jats:title>Abstract</jats:title><jats:p>Vibrational sum-frequency generation (vSFG) spectroscopy allows the study of the structure and dynamics of interfacial systems. In the present work, we provide a simple recipe, based on a narrowband IR pump and broadband vSFG probe technique, to computationally obtain the two-dimensional vSFG spectrum of water molecules at the air–water interface. Using this technique, to study the time-dependent spectral evolution of hydrogen-bonded and free water molecules, we demonstrate that at the interface, the vibrational spectral dynamics of the free OH bond is faster than that of the bonded OH mode.</jats:p>"}],"volume":11,"keyword":["Multidisciplinary"]}