{"title":"New and Facile Preparation Method for Highly Active Iron Oxide Catalysts for CO Oxidation","year":"2024","publication_status":"published","type":"journal_article","language":[{"iso":"eng"}],"user_id":"48467","article_type":"original","abstract":[{"lang":"eng","text":"This work presents a new and facile route for the preparation of iron oxide-based catalysts supported on alumina, which enables the targeted synthesis of catalysts with an increased amount of isolated tetrahedrally coordinated iron centers compared to a conventional impregnation procedure, and therefore leads to an increase in activity for CO oxidation reaction. By a multi-step impregnation–calcination protocol, the catalysts were synthesized with iron loadings of between 1 and 10 wt%, and their catalytic activity was then compared with a 10 wt% loaded catalyst prepared by conventional single impregnation. With a loading of 8 wt%, the presented catalysts showed an improved catalytic activity regarding light-off and full conversion temperatures compared to this reference. Through the application of several analytical methods (PXRD, PDF, DRUVS, SEM, XAFS), the improved catalytic activity can be correlated with an increased amount of isolated iron centers and a significantly reduced fraction of agglomerates or particles."}],"intvolume":" 14","_id":"54969","date_updated":"2024-07-02T07:14:37Z","status":"public","date_created":"2024-07-02T07:10:14Z","publication_identifier":{"issn":["2073-4344"]},"issue":"7","volume":14,"article_number":"416","author":[{"last_name":"Schlicher","full_name":"Schlicher, Steffen","first_name":"Steffen"},{"last_name":"Schoch","full_name":"Schoch, Roland","first_name":"Roland","orcid":"0000-0003-2061-7289","id":"48467"},{"full_name":"Prinz, Nils","last_name":"Prinz","first_name":"Nils"},{"first_name":"Mirijam","full_name":"Zobel, Mirijam","last_name":"Zobel"},{"id":"47241","orcid":"0000-0002-9294-6076","first_name":"Matthias","last_name":"Bauer","full_name":"Bauer, Matthias"}],"department":[{"_id":"306"}],"publisher":"MDPI AG","citation":{"short":"S. Schlicher, R. Schoch, N. Prinz, M. Zobel, M. Bauer, Catalysts 14 (2024).","ama":"Schlicher S, Schoch R, Prinz N, Zobel M, Bauer M. New and Facile Preparation Method for Highly Active Iron Oxide Catalysts for CO Oxidation. Catalysts. 2024;14(7). doi:10.3390/catal14070416","ieee":"S. Schlicher, R. Schoch, N. Prinz, M. Zobel, and M. Bauer, “New and Facile Preparation Method for Highly Active Iron Oxide Catalysts for CO Oxidation,” Catalysts, vol. 14, no. 7, Art. no. 416, 2024, doi: 10.3390/catal14070416.","chicago":"Schlicher, Steffen, Roland Schoch, Nils Prinz, Mirijam Zobel, and Matthias Bauer. “New and Facile Preparation Method for Highly Active Iron Oxide Catalysts for CO Oxidation.” Catalysts 14, no. 7 (2024). https://doi.org/10.3390/catal14070416.","apa":"Schlicher, S., Schoch, R., Prinz, N., Zobel, M., & Bauer, M. (2024). New and Facile Preparation Method for Highly Active Iron Oxide Catalysts for CO Oxidation. Catalysts, 14(7), Article 416. https://doi.org/10.3390/catal14070416","bibtex":"@article{Schlicher_Schoch_Prinz_Zobel_Bauer_2024, title={New and Facile Preparation Method for Highly Active Iron Oxide Catalysts for CO Oxidation}, volume={14}, DOI={10.3390/catal14070416}, number={7416}, journal={Catalysts}, publisher={MDPI AG}, author={Schlicher, Steffen and Schoch, Roland and Prinz, Nils and Zobel, Mirijam and Bauer, Matthias}, year={2024} }","mla":"Schlicher, Steffen, et al. “New and Facile Preparation Method for Highly Active Iron Oxide Catalysts for CO Oxidation.” Catalysts, vol. 14, no. 7, 416, MDPI AG, 2024, doi:10.3390/catal14070416."},"publication":"Catalysts","doi":"10.3390/catal14070416"}