@article{65611,
  abstract     = {{<jats:p>
                    Spins confined in optically active quantum dot molecules (QDMs) can be used for the deterministic generation of photonic graph states with tailored entanglement structures. Their usefulness for the generation of such nonclassical states of light is determined by orbital and spin decoherence mechanisms, particularly phonon-mediated processes dominant at energy scales up to a few millielectronvolts. Here, we directly measure the spectral function of orbital phonon relaxation between the energy states of the neutral exciton in a QDM and benchmark our findings against microscopic
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                    theory. Our results reveal pronounced resonances and antiresonances in the phonon-relaxation rates, ranging from tens of
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                    up to tens of
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                    . Comparison with a kinetic model reveals the voltage (energy) dependent phonon coupling strength and fully explains the interplay between phonon-assisted relaxation and radiative recombination. The resonances and antiresonances enable further tunability of the exciton lifetime which can be leveraged to increase the lifetime of energetically unfavorable charge configurations needed for realizing efficient spin-photon interfaces and multidimensional cluster states.
                  </jats:p>}},
  author       = {{Lienhart, Michelle and Gawarecki, Krzysztof and Stöcker, Markus and Bopp, Frederik and Cullip, Charlotte and Akhlaq, Nadeem and Thalacker, Christopher and Schall, Johannes and Rodt, Sven and Ludwig, Arne and Reuter, Dirk and Reitzenstein, Stephan and Müller, Kai and Machnikowski, Paweł and Finley, Jonathan J.}},
  issn         = {{2469-9950}},
  journal      = {{Physical Review B}},
  number       = {{23}},
  publisher    = {{American Physical Society (APS)}},
  title        = {{{Resonant and antiresonant exciton-phonon coupling in quantum dot molecules}}},
  doi          = {{10.1103/xc25-1tph}},
  volume       = {{112}},
  year         = {{2025}},
}

