Exciton-Migration and Three-Pulse Femtosecond Optical Spectroscopies of Photosynthetic Antenna Complexes
T. Meier, W.M. Zhang, V. Chernyak, S. Mukamel, The Journal of Chemical Physics 108 (1998) 7763–7774.
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Author
Meier, TorstenLibreCat 
;
Zhang, W.M.;
Chernyak, V.;
Mukamel, S.
;
Zhang, W.M.;
Chernyak, V.;
Mukamel, S.Department
Abstract
A theory for four-wave-mixing signals from molecular aggregates, which includes effects of two-exciton states, static disorder, and coupling to a phonon bath with an arbitrary spectral density, is developed. The third-order polarization is rigorously partitioned into a coherent and a sequential contribution. The latter is given by a sum of an exciton-hopping and a ground state (bleaching) terms, both expressed using the doorway-window representation. Applications are made to photon-echo and pump-probe spectroscopies of the B850 system of the LH2 antenna in purple bacteria.
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Journal Title
The Journal of chemical physics
Volume
108
Issue
18
Page
7763-7774
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Cite this
Meier T, Zhang WM, Chernyak V, Mukamel S. Exciton-Migration and Three-Pulse Femtosecond Optical Spectroscopies of Photosynthetic Antenna Complexes. The Journal of chemical physics. 1998;108(18):7763-7774. doi:10.1063/1.476212
Meier, T., Zhang, W. M., Chernyak, V., & Mukamel, S. (1998). Exciton-Migration and Three-Pulse Femtosecond Optical Spectroscopies of Photosynthetic Antenna Complexes. The Journal of Chemical Physics, 108(18), 7763–7774. https://doi.org/10.1063/1.476212
@article{Meier_Zhang_Chernyak_Mukamel_1998, title={Exciton-Migration and Three-Pulse Femtosecond Optical Spectroscopies of Photosynthetic Antenna Complexes}, volume={108}, DOI={10.1063/1.476212}, number={18}, journal={The Journal of chemical physics}, publisher={American Institute of Physics}, author={Meier, Torsten and Zhang, W.M. and Chernyak, V. and Mukamel, S.}, year={1998}, pages={7763–7774} }
Meier, Torsten, W.M. Zhang, V. Chernyak, and S. Mukamel. “Exciton-Migration and Three-Pulse Femtosecond Optical Spectroscopies of Photosynthetic Antenna Complexes.” The Journal of Chemical Physics 108, no. 18 (1998): 7763–74. https://doi.org/10.1063/1.476212.
T. Meier, W. M. Zhang, V. Chernyak, and S. Mukamel, “Exciton-Migration and Three-Pulse Femtosecond Optical Spectroscopies of Photosynthetic Antenna Complexes,” The Journal of chemical physics, vol. 108, no. 18, pp. 7763–7774, 1998, doi: 10.1063/1.476212.
Meier, Torsten, et al. “Exciton-Migration and Three-Pulse Femtosecond Optical Spectroscopies of Photosynthetic Antenna Complexes.” The Journal of Chemical Physics, vol. 108, no. 18, American Institute of Physics, 1998, pp. 7763–74, doi:10.1063/1.476212.
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