Multidimensional ultrafast spectroscopy special feature: polarization-dependent optical 2d fourier transform spectroscopy of semiconductors
T. Meier, T. Zhang, I. Kuznetsova, X. Li, R.P. Mirin, P. Thomas, S.T. Cundiff, Proceedings of the National Academy of Sciences 104 (2007) 14227–14232.
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Author
Meier, TorstenLibreCat 
;
Zhang, Tianhao;
Kuznetsova, Irina;
Li, Xiaoqin;
Mirin, R. P.;
Thomas, Peter;
Cundiff, S.T.
;
Zhang, Tianhao;
Kuznetsova, Irina;
Li, Xiaoqin;
Mirin, R. P.;
Thomas, Peter;
Cundiff, S.T.Department
Abstract
Optical 2D Fourier transform spectroscopy (2DFTS) provides insight into the many-body interactions in direct gap semiconductors by separating the contributions to the coherent nonlinear optical response. We demonstrate these features of optical 2DFTS by studying the heavy-hole and light-hole excitonic resonances in a gallium arsenide quantum well at low temperature. Varying the polarization of the incident beams exploits selection rules to achieve further separation. Calculations using a full many-body theory agree well with experimental results and unambiguously demonstrate the dominance of many-body physics.
Publishing Year
Journal Title
Proceedings of the National Academy of Sciences
Volume
104
Issue
36
Page
14227-14232
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Cite this
Meier T, Zhang T, Kuznetsova I, et al. Multidimensional ultrafast spectroscopy special feature: polarization-dependent optical 2d fourier transform spectroscopy of semiconductors. Proceedings of the National Academy of Sciences. 2007;104(36):14227-14232. doi:10.1073/pnas.0701273104
Meier, T., Zhang, T., Kuznetsova, I., Li, X., Mirin, R. P., Thomas, P., & Cundiff, S. T. (2007). Multidimensional ultrafast spectroscopy special feature: polarization-dependent optical 2d fourier transform spectroscopy of semiconductors. Proceedings of the National Academy of Sciences, 104(36), 14227–14232. https://doi.org/10.1073/pnas.0701273104
@article{Meier_Zhang_Kuznetsova_Li_Mirin_Thomas_Cundiff_2007, title={Multidimensional ultrafast spectroscopy special feature: polarization-dependent optical 2d fourier transform spectroscopy of semiconductors}, volume={104}, DOI={10.1073/pnas.0701273104}, number={36}, journal={Proceedings of the National Academy of Sciences}, author={Meier, Torsten and Zhang, Tianhao and Kuznetsova, Irina and Li, Xiaoqin and Mirin, R. P. and Thomas, Peter and Cundiff, S.T.}, year={2007}, pages={14227–14232} }
Meier, Torsten, Tianhao Zhang, Irina Kuznetsova, Xiaoqin Li, R. P. Mirin, Peter Thomas, and S.T. Cundiff. “Multidimensional Ultrafast Spectroscopy Special Feature: Polarization-Dependent Optical 2d Fourier Transform Spectroscopy of Semiconductors.” Proceedings of the National Academy of Sciences 104, no. 36 (2007): 14227–32. https://doi.org/10.1073/pnas.0701273104.
T. Meier et al., “Multidimensional ultrafast spectroscopy special feature: polarization-dependent optical 2d fourier transform spectroscopy of semiconductors,” Proceedings of the National Academy of Sciences, vol. 104, no. 36, pp. 14227–14232, 2007, doi: 10.1073/pnas.0701273104.
Meier, Torsten, et al. “Multidimensional Ultrafast Spectroscopy Special Feature: Polarization-Dependent Optical 2d Fourier Transform Spectroscopy of Semiconductors.” Proceedings of the National Academy of Sciences, vol. 104, no. 36, 2007, pp. 14227–32, doi:10.1073/pnas.0701273104.
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