Light Amplification Materials Based on Biopolymers Doped with Dye Molecules—Structural Insights from 15N and 13C Solid-State Dynamic Nuclear Polarization
M.V. Höfler, N. Hoinka, T. Schäfer, M. Horn, F. Aussenac, T. Fuhrmann-Lieker, T. Gutmann, Journal of Physical Chemistry C 125 (2021) 21550–21558.
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Journal Article
| English
Author
Höfler, Mark V.;
Hoinka, Nicolai;
Schäfer, Timmy;
Horn, Marilia;
Aussenac, Fabien;
Fuhrmann-Lieker, Thomas;
Gutmann, TorstenLibreCat
Abstract
13C and 15N solid-state nuclear magnetic resonance (NMR) combined with dynamic nuclear polarization (DNP) is used to investigate the structure of dye-doped biopolymer-based materials that can be used in amplified spontaneous emission (ASE) experiments. By comparing calligraphic paper prepared from cellulose and scaffolds prepared from chitosan as substrates, differences in the interactions of the carrier material with the dye molecule Calcofluor White are obtained. These are most probably induced by structural changes of the carrier material due to its interaction with water forming hydrogen bonds. Such structural differences may explain the obtained variation of the emission wavelength of Calcofluor White doped on these substrates in ASE experiments.
Publishing Year
Journal Title
Journal of Physical Chemistry C
Volume
125
Issue
39
Page
21550–21558
ISSN
LibreCat-ID
Cite this
Höfler MV, Hoinka N, Schäfer T, et al. Light Amplification Materials Based on Biopolymers Doped with Dye Molecules—Structural Insights from 15N and 13C Solid-State Dynamic Nuclear Polarization. Journal of Physical Chemistry C. 2021;125(39):21550–21558. doi:10.1021/acs.jpcc.1c06737
Höfler, M. V., Hoinka, N., Schäfer, T., Horn, M., Aussenac, F., Fuhrmann-Lieker, T., & Gutmann, T. (2021). Light Amplification Materials Based on Biopolymers Doped with Dye Molecules—Structural Insights from 15N and 13C Solid-State Dynamic Nuclear Polarization. Journal of Physical Chemistry C, 125(39), 21550–21558. https://doi.org/10.1021/acs.jpcc.1c06737
@article{Höfler_Hoinka_Schäfer_Horn_Aussenac_Fuhrmann-Lieker_Gutmann_2021, title={Light Amplification Materials Based on Biopolymers Doped with Dye Molecules—Structural Insights from 15N and 13C Solid-State Dynamic Nuclear Polarization}, volume={125}, DOI={10.1021/acs.jpcc.1c06737}, number={39}, journal={Journal of Physical Chemistry C}, publisher={American Chemical Society}, author={Höfler, Mark V. and Hoinka, Nicolai and Schäfer, Timmy and Horn, Marilia and Aussenac, Fabien and Fuhrmann-Lieker, Thomas and Gutmann, Torsten}, year={2021}, pages={21550–21558} }
Höfler, Mark V., Nicolai Hoinka, Timmy Schäfer, Marilia Horn, Fabien Aussenac, Thomas Fuhrmann-Lieker, and Torsten Gutmann. “Light Amplification Materials Based on Biopolymers Doped with Dye Molecules—Structural Insights from 15N and 13C Solid-State Dynamic Nuclear Polarization.” Journal of Physical Chemistry C 125, no. 39 (2021): 21550–21558. https://doi.org/10.1021/acs.jpcc.1c06737.
M. V. Höfler et al., “Light Amplification Materials Based on Biopolymers Doped with Dye Molecules—Structural Insights from 15N and 13C Solid-State Dynamic Nuclear Polarization,” Journal of Physical Chemistry C, vol. 125, no. 39, pp. 21550–21558, 2021, doi: 10.1021/acs.jpcc.1c06737.
Höfler, Mark V., et al. “Light Amplification Materials Based on Biopolymers Doped with Dye Molecules—Structural Insights from 15N and 13C Solid-State Dynamic Nuclear Polarization.” Journal of Physical Chemistry C, vol. 125, no. 39, American Chemical Society, 2021, pp. 21550–21558, doi:10.1021/acs.jpcc.1c06737.
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